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| 1 | Graphene: a promising 2D material for electrochemical energy storage显示文摘Graphene, with unique two-dimensional form and numerous appealing properties, promises to remarkably increase the energy density and power density of electrochemical energy storage devices(EESDs),ranging from the popular lithium ion batteries and supercapacitors to next-generation high-energy batteries. Here, we review the recent advances of the state-of-the-art graphene-based materials for EESDs,including lithium ion batteries, supercapacitors, micro-supercapacitors, high-energy lithium-air and lithium-sulfur batteries, and discuss the importance of the pore, doping, assembly, hybridization and functionalization of different nano-architectures in improving electrochemical performance. The major roles of graphene are highlighted as(1) a superior active material,(2) ultrathin 2D flexible support,and(3) an inactive yet electrically conductive additive. Furthermore, we address the enormous potential of graphene for constructing new-concept emerging graphene-enabled EESDs with multiple functionalities of lightweight, ultra-flexibility, thinness, and novel cell configurations. Finally, future perspectives and challenges of graphene-based EESDs are briefly discussed. | Yanfeng Dong Zhong-Shuai Wu Wencai Ren Hui-Ming Cheng Xinhe Bao | 2017 | Science Bulletin2017，62，10： | 22 |
| 2 | Recent progress in methane dehydroaromatization: From laboratory curiosities to promising technology显示文摘Direct conversion of methane to benzene or other valuable chemicals is a very promising process for the efficient application of natural gas. Compared with conversion processes that require oxidants, non-oxidative direct conversion is more attractive due to high selectivity to the target product. In this paper, an alternative route for methane dehydrogenation and selective conversion to benzene and hydrogen without the participation of oxygen is discussed. A brief review of the catalysts used in methane dehydroaromatization (MDA) is first given, followed by our current understanding of the location and the active phase of Mo species, the reaction mechanism, the mechanism of carbonaceous deposit and the deactivation of Mo/zeolite catalysts are systematically discussed. Ways to improve the catalytic activity and stability are described in detail based on catalyst and reaction as well as reactor design. Future prospects for methane dehydroaromatization process are also presented. | Shuqi Ma Xiaoguang Guo Lingxiao Zhao Susannah Scott Xinhe Bao | 2013 | Journal of Energy Chemistry2013，22，1： | 17 |
| 3 | Nitrogen doped carbon catalyzing acetylene conversion to vinyl chloride显示文摘Commercial production of vinyl chloride from acetylene relies on the use of HgCl2as the catalyst, which has caused severe environmental problem and threats to human health because of its toxicity. Therefore, it is vital to explore alternative catalysts without mercury. We report here that N-doped carbon can catalyze directly transformation of acetylene to vinyl chloride. Particularly, N-doped high surface area mesoporous carbon exhibits a rather high activity with the acetylene conversion reaching 77% and vinyl chloride selectivity above 98% at a space velocity of 1.0 mL min-1 g-1and 200 ℃. It delivers a stable performance within a test period of 100 h and no obvious deactivation is observed,demonstrating potentials to substitute the notoriously toxic mercuric chloride catalyst. | Xingyun Li Xiulian Pan Xinhe Bao | 2014 | Journal of Energy Chemistry2014，23，2： | 11 |
| 4 | Enhanced aromatic selectivity by the sheet-like ZSM-5 in syngas conversion显示文摘Aromatics are important basic chemicals. However, direct conversion of syngas via the conventional Fischer-Tropsch synthesis produces little aromatics. We presented herein that a bifunctional composite of ZSM-5 in combination with Zn Cr Oxcatalyzes syngas conversion to aromatics. Particularly, ZSM-5 crystals with a sheet-like morphology can enhance significantly the aromatization activity. The lower length ratio of the b/a axes of the crystals, the more aromatics form but without influencing the selectivity of small molecules such as CH4 and C2–C4. Since the acid properties and the Al chemical environment were not altered while the morphology changed, the enhanced aromatic selectivity is likely attributed to the favored diffusion of aromatics in these sheet-like crystals. | Junhao Yang Ke Gong Dengyun Miao Feng Jiao Xiulian Pan Xiangju Meng Fengshou Xiao Xinhe Bao | 2019 | Journal of Energy Chemistry2019，28，8： | 10 |
| 5 | Understanding nano effects in catalysis显示文摘Catalysis, as a key and enabling technology, plays an increasingly important role in ields ranging from energy, environment and agriculture to health care. Rational design and synthesis of highly eicient catalysts has become the ultimate goal of catalysis research. hanks to the rapid development of nanoscience and nanotechnology, and in particular a theoretical understanding of the tuning of electronic structure in nanoscale systems, this element of design is becoming possible via precise control of nanoparticles' composition, morphology, structure and electronic states. At the same time, it is important to develop tools for in situ characterization of nanocatalysts under realistic reaction conditions, and for monitoring the dynamics of catalysis with high spatial, temporal and energy resolution. In this review, we discuss coninement efects in nanocatalysis, a concept that our group has put forward and developed over several years. Taking the conined catalytic systems of carbon nanotubes, metal-conined nano-oxides and 2D layered nanocatalysts as examples, we summarize and analyze the fundamental concepts, the research methods and some of the key scientiic issues involved in nanocatalysis. Moreover, we present a perspective on the challenges and opportunities in future research on nanocatalysis from the aspects of:(1) controlled synthesis of nanocatalysts and rational design of catalytically active centers;(2) in situ characterization of nanocatalysts and dynamics of catalytic processes;(3) computational chemistry with a complexity approximating that of experiments; and (4) scale-up and commercialization of nanocatalysts. | Fan Yang Dehui Deng Xiulian Pan Qiang Fu Xinhe Bao | 2015 | National Science Review2015，2，2： | 9 |
| 6 | Architecture of PtFe/C catalyst with high activity and durability for oxygen reduction reaction显示文摘PtFe/C 催化剂被列在后面由的受精和高温度的减小综合了酸沥滤。X 光检查衍射, X 光检查光电子光谱学和在边光谱学描述附近原子的 X 光检查揭示那磅 < 潜水艇 class= “ a-plus-plus ” > 3 Fe 合金形成发生在高温度的减小和那不稳定的 Fe 种期间被溶解进酸溶液。在到表面并且强壮的 O-Fe 结合的从核心区域的 Fe 集中的差别可以驾驶 Fe 的外面的散开到高度弄皱的磅骨骼,并且高度结果驱散表面 FeO <潜水艇class=“ a-plus-plus ”> x 在酸的媒介是稳定的,导致磅的构造<潜水艇class=“ a-plus-plus ”> 3 Fe@Pt-FeO <潜水艇class=“ a-plus-plus ”> x 建筑学。是准备了 PtFe/C 催化剂与 Pt/C 催化剂相比为氧减小反应表明一项更高的活动和可比较的耐久性,它可能在 PtFe/C 催化剂由于表面和表面下的 Fe 种类的合作效果。 | Jiayuan Li Guoxiong Wang Jing Wang Shu Miao Mingming Wei Fan Yang Liang Yu Xinhe Bao | 2014 | Nano Research2014，7，10： | 8 |
| 7 | Switchable C02 electroreduction via engineering active phases of Pd nanoparticles显示文摘活跃阶段的工程定期被利用在异构的催化作用调节金属 nanoparticles (NP ) 的选择。然而,在 electrocatalysis 的活跃阶段的理解的缺乏为公司 2 electroreduction 妨碍了有效催化剂的发展。此处,我们报导 Pd NP 的活跃阶段的系统的工程,它被利用为公司 2 electroreduction 选择反应小径。在 situ X光检查吸收光谱学,在稀释的 situ 总计思考红外线的光谱学,并且密度功能的理论计算建议吸附氢的 Pd 的形成出现在混合物上-并且一个钯氢化物核心的阶段(在 0.2 V 上面的+ PdH x @PdH x )(对一个可逆的氢电极)经由 HCOO 便于甲酸盐生产*中间,而阶段 Pd 氢化物核心上的金属性的 Pd 表面的形成( PdH x @主要产品,是甲酸盐或公司,能有选择地与高 Faradaic 效率被生产(>90%) 并且在有可伸缩的申请的 0.05 ~ 0.9 V 的潜在的窗户中的集体活动示范。 | Dunfeng Gao Hu Zhou Fan Cai Dongniu Wang Yongfeng Hu Bei Jiang Wen-Bin Cai Xiaoqi Chen Rui Si Fan Yang Shu Miao Jianguo Wang Guoxiong wang Xinhe Bao | 2017 | Nano Research2017，10，6： | 8 |
| 8 | Direct production of light olefins from syngas over a carbon nanotube confined iron catalyst显示文摘Iron particles confined in carbon nanotube (CNT) channels have been used as a catalyst for the direct conversion of syngas to light olefins.Compared with iron catalysts supported on other materials such as Silica-1,SBA-15 and carbon black,the CNT-confined catalyst exhibits a higher CO conversion and selectivity to the light olefins.This can be attributed to the CNT channels,which provide a unique confinement environment for iron particles. | WANG ChuanFu PAN XiuLian BAO XinHe | 2010 | Chinese Science Bulletin2010，55，12： | 8 |
| 9 | Enhanced hydrogen evolution reaction over molybdenum carbide nanoparticles confined inside single-walled carbon nanotubes显示文摘Carbon nanotubes(CNTs) have shown as unique nanoreactors to tune the catalytic activity of confined nano-catalysts. Here we report that the catalytic performance of molybdenum carbide nanoparticles(MoC_x NPs) for the hydrogen evolution reaction(HER) process can be enhanced by encapsulation within single-walled carbon nanotubes(SWNTs) with a diameter of 1–2 nm. The catalyst with MoC_x NPs located on the interior surface of SWNTs(MoCx@SWNTs) exhibits a lower onset over-potential and a smaller Tafel slope than the one with MoC_x NPs attached on the exterior surface(MoCx/SWNTs). This is likely attributed to the much smaller particle size and the more reduced states of the confined MoC_x NPs, as well as the larger specific surface area of MoCx@SWNTs compared with Mo Cx/SWNTs. In addition, the electronic structure of the confined MoC_x NPs might be modified by the confinement effects of SWNTs, and hence the adsorption free energy of H atoms on the confined MoC_x NPs, which could also contribute to their higher performance. These results suggest that the SWNTs can be further explored for constructing novel catalysts with beneficial catalytic performance. | Tingting Cui Jinhu Dong Xiulian Pan Tie Yu Qiang Fu Xinhe Bao | 2019 | Journal of Energy Chemistry2019，28，1： | 7 |
| 10 | Recent advances of graphene-based materials for high-performance and new-concept supercapacitors显示文摘Supercapacitors, with ultrahigh power density, superior rate capability, long-term cyclability, and exceptional safety, are regarded as one highly competitive candidate of electrochemical energy storage devices,filling the gap between batteries and conventional capacitors. Despite of tremendous effort, elaborated screening of high-performance electrode materials, e.g., graphene, is still intensively required. In this review, we describe the most recent progress in the research and development of graphene-based materials for high-performance and new-concept supercapacitors for the targeted applications in next-generation and smart electronics. First, the design and fabrication of high-performance supercapacitors, including electrical double layer capacitors, pseudocapacitors and hybrid supercapacitors, were summarized in term of the charge storage mechanism. Second, new-concept supercapacitors with multiple functionalities of high-voltage, fiber-shape, microscale and shape-diversity in order to fulfill the requirements of future electronics are reviewed. Accordingly, special emphasis is given to the structure-dependent-performance effects of pores, hybridization, dimensionalities of graphene-based materials on performance of supercapacitors, and tremendous potential of graphene-based planar micro-supercapacitors for the direct seamlessly integration with versatile micro-electronics. Finally, perspectives and challenges of graphene-based supercapacitors are briefly discussed. | Xiaoyu Shi Shuanghao Zheng Zhong-Shuai Wu Xinhe Bao | 2018 | Journal of Energy Chemistry2018，27，1： | 7 |
| 11 | A novel approach to design microwave medium of negative refractive index and simulation verification显示文摘In this paper, a novel approach is presented to synthesize microwave medium of negative refractive index by incorporating metallic wire array with negative effective permittivity into the host media such as ferrimagnet-YIG (yttrium iron garnet) applied by external magnetic field whose permeability is negative. We have designed the composite medium having negative refractive index in C/X band frequencies, analyzed and simulated its electromagnetic (EM) properties by use of EM EDA package based on time-domain finite integration method. The simulation results show that: ① the effective permittivity of the designed metallic wire array is negative in the frequency range from 7.02 GHz to 9.80 GHz; ② the permeability of YIG substrate immersed into an external magnetic field is negative in the frequency range from 5.22 GHz to 8.14 GHz; ③ EM wave can pass through the composite medium synthesized by the above designed metallic wire array and YIG substrate, and ④ the negative refraction behavior occurs on the interface between the composite medium and the normal material with positive refractive index in 7.51―8.13 GHz frequency range, in which the effective permittivity of the metallic wire array and the permeability of YIG substrate are negative simultaneously. The full wave simulation has demonstrated that the effective refractive index of the designed composite medium is indeed negative and ascertained that the proposed approach to design microwave medium with negative refractive index is viable. | CAO YunJian WEN GuangJun WU KaiMin XU XinHe | 2007 | Chinese Science Bulletin2007，52，4： | 6 |
| 12 | Co-electrolysis of CO_2 and H_2O in high-temperature solid oxide electrolysis cells: Recent advance in cathodes显示文摘Co-electrolysis of CO_2 and H_2O using high-temperature solid oxide electrolysis cells(SOECs) into valuable chemicals has attracted great attentions recently due to the high conversion and energy efficiency,which provides opportunities of reducing CO_2 emission, mitigating global warming and storing intermittent renewable energies. A single SOEC typically consists of an ion conducting electrolyte, an anode and a cathode where the co-electrolysis reaction takes place. The high operating temperature and difficult activated carbon-oxygen double-bond of CO_2 put forward strict requirements for SOEC cathode. Great efforts are being devoted to develop suitable cathode materials with high catalytic activity and excellent long-term stability for CO_2/H_2O electro-reduction. The so far cathode material development is the key point of this review and alternative strategies of high-performance cathode material preparation is proposed. Understanding the mechanism of CO_2/H_2O electro-reduction is beneficial to highly active cathode design and optimization. Thus the possible reaction mechanism is also discussed. Especially, a method in combination with electrochemical impedance spectroscopy(EIS) measurement, distribution functions of relaxation times(DRT) calculation, complex nonlinear least square(CNLS) fitting and operando ambient pressure X-ray photoelectron spectroscopy(APXPS) characterization is introduced to correctly disclose the reaction mechanism of CO_2/H_2O co-electrolysis. Finally, different reaction modes of the CO_2/H_2O coelectrolysis in SOECs are summarized to offer new strategies to enhance the CO_2 conversion. Otherwise,developing SOECs operating at 300-600 °C can integrate the electrochemical reduction and the Fischer-Tropsch reaction to convert the CO_2/H_2O into more valuable chemicals, which will be a new research direction in the future. | Xiaomin Zhang Yuefeng Song Guoxiong Wang Xinhe Bao | 2017 | Journal of Energy Chemistry2017，26，5： | 6 |
| 13 | Methane dehydroaromatization with periodic CH_4-H_2 switch:A promising process for aromatics and hydrogen显示文摘Long-term stability test of Mo/HZSM-5-N catalysts(HZSM-5-N stands for nano-sized HZSM-5) in methane dehydroaromatization(MDA)reaction has been performed with periodic CH4-H2 switch at 1033-1073 K for more than 1000 h.During this test,methane conversion ranges from 13% to 16%,and mean yield to aromatics(i.e.benzene and naphthalene) exceeds 10%.N2-physisorption,XRD,NMR and TPO measurements were performed for the used Mo/HZSM-5 catalysts and coke deposition,and the results revealed that the periodic hydrogenation can effectively suppress coke deposition by removing the inert aromatic-type coke,thus ensuring Mo/HZSM-5 partly maintained its activity even in the presence of large amount of coke deposition.The effect of zeolite particle size on the catalytic activity was also explored,and the results showed that the nano-sized zeolite with low diffusion resistance performed better.It is recognized that the size effect was enhanced by reaction time,and it became more remarkable in a long-term MDA reaction even at a low space velocity. | Changyong Sun Guangzong Fang Xiaoguang Guo Yuanli Hu Shuqi Ma Tianhua Yang Jie Han Hao Ma Dali Tan Xinhe Bao | 2015 | Journal of Energy Chemistry2015，24，3： | 6 |
| 14 | Selective conversion of syngas to propane over ZnCrO_x-SSZ-39 OX-ZEO catalysts显示文摘Oxide-Zeolite(OX-ZEO) bifunctional catalyst design concept has been exemplified in several processes to direct conversion syngas to value-added chemicals and fuels such as mixed light olefins, ethylene, aromatics and gasoline.Herein we demonstrate that the product can be steered toward liquefied petroleum gas(LPG) with a selectivity up to 89% in hydrocarbons especially propane selectivity reaching 80% at CO conversion of 63% using ZnCrOx-H-SSZ-39 catalyst.Interestingly, the quantity of the acid sites of SSZ-39 does not influence obviously the hydrocarbon distribution but the strength is crucial for selective formation of propane.This finding provides an alternative route of LPG synthesis from a variety of carbon resources via syngas. | Gen Li Feng Jiao Dengyun Miao Yong Wang Xiulian Pan Toshiyuki Yokoi Xiangju Meng Feng-Shou Xiao Andrei-Nicolae Parvulescu Ulrich Müller Xinhe Bao | 2019 | Journal of Energy Chemistry2019，28，9： | 6 |
| 15 | Intelligent identification of two-dimensional nanostructures by machine-learning optical microscopy显示文摘Two-dimensional (2D)materials and their heterostructures,with wafer-scale synthesis methods and fascinating properties,have attracted significant interest and triggered revolutions in corresponding device applications.However,facile methods to realize accurate,intelligent,and large-area characterizations of these 2D nanostructures are still highly desired.Herein,we report the successful application of machine-learning strategy in the optical identification of 2D nanostructures.The machine-leaming optical identification (MOI)method endows optical microscopy with intelligent insight into the characteristic color information of 2D nanostructures in the optical photograph.The experimental results indicate that the MOI method enables accurate,intelligent,and large-area characterizations of graphene,molybdenum disulfide,and their heterostructures, including identifications of the thickness,existence of impurities,and even stacking order.With the convergence of artificial intelligence and nanoscience,this intelligent identification method can certainly promote fundamental research and wafer-scale device applications of 2D nanostructures. | Xiaoyang Lin Zhizhong Si Wenzhi Fu Jianlei Yang Side Guo Yuan Cao Jin Zhang Xinhe Wang Peng Liu Kaili Jiang Weisheng Zhao | 2018 | Nano Research2018，11，12： | 5 |
| 16 | Scalable fabrication of printed Zn//MnO2 planar micro-batteries with high volumetric energy density and exceptional safety显示文摘The rapid development of printed and microscale electronics imminently requires compatible micro-batteries(MBs)with high performance,applicable scalability,and exceptional safety,but faces great challenges from the ever-reported stacked geometry.Herein the first printed planar prototype of aqueous-based,high-safety Zn//MnO2 MBs,with outstanding performance,aesthetic diversity,flexibility and modularization,is demonstrated,based on interdigital patterns of Zn ink as anode and MnO2 ink as cathode,with high-conducting graphene ink as a metal-free current collector,fabricated by an industrially scalable screen-printing technique.The planar separator-free Zn//MnO2 MBs,tested in neutral aqueous electrolyte,deliver a high volumetric capacity of 19.3 mAh/cm^3(corresponding to 393 mAh/g)at 7.5 mA/cm^3,and notable volumetric energy density of 17.3 mWh/cm^3,outperforming lithium thin-film batteries(≤10 mWh/cm^3).Furthermore,our Zn//MnO2 MBs present long-term cyclability having a high capacity retention of 83.9%after 1300 cycles at 5 C,which is superior to stacked Zn//MnO2 batteries previously reported.Also,Zn//MnO2 planar MBs exhibit exceptional flexibility without observable capacity decay under serious deformation,and remarkably serial and parallel integration of constructing bipolar cells with high voltage and capacity output.Therefore,low-cost,environmentally benign Zn//MnO2 MBs with in-plane geometry possess huge potential as high-energy,safe,scalable and flexible microscale power sources for direction integration with printed electronics. | Xiao Wang Shuanghao Zheng Feng Zhou Jieqiong Qin Xiaoyu Shi Sen Wang Chenglin Sun Xinhe Bao Zhong-Shuai Wu | 2020 | National Science Review2020，7，1： | 5 |
| 17 | Loss of heterozygosity in multistage carcinogenesis of esophageal carcinoma at high-incidence area in Henan Province, China显示文摘AIM: Microsatellites are the repeated DNA sequences scattered widely within the genomes and closely linked with many important genes. This study was designed to characterize the changes of microsatellite DNA loss of heterozygosity (LOH) in esophageal carcinogenesis. METHODS: Allelic deletions in 32 cases of matched precancerous, cancerous and normal tissues were examined by syringe microdissection under an anatomic microscope and microsatellite polymorphism analysis using 15 polymorphic markers on chromosomes 3p, 5q, 6p, 9p, 13q,17p, 17q and 18q.RESULTS: Microsatellite DNA LOH was observed in precancerous and cancerous tissues, except D9S1752. The rate of LOH increased remarkably with the lesions progressed from basal cell hyperplasia (BCH) to squamous cell carcinoma (SCC) (P<0.05). Three markers, D9S171, D13S260 and TP53, showed the highest incidence of LOH (>60%). LOH loci were different in precancerous and cancerous tissues. LOH in D3S1234 and TP53 was the common event in different lesions from the same patients. CONCLUSION: Microsatellite DNA LOH occurs in early stage of human esophageal carcinogenesis, even in BCH. With the lesion progressed, gene instability increases, the accumulation of this change may be one of the important mechanisms driving precancerous lesions to cancer. | Ji-YeAn Zong-MinFan Shan-ShanGao Ze-HaoZhuang Yan-RuQin Ji-LinLi XinHe GeorgeSai-WahTsao Li-DongWang | 2005 | World Journal of Gastroenterology2005，11，14： | 5 |
| 18 | Catalysis under shell: Improved CO oxidation reaction confined in Pt@h-BN core-shell nanoreactors显示文摘Core-shell nanostructures consisting of active metal cores and protective shells often exhibit enhanced catalytic performance, in which reactants can access a small part of the core surfaces through the pores in the shells. In this study, we show that Pt nanoparticles (NPs) can be embedded into few-layer hexagonal boron nitride (h-BN) overlayers, forming Pt@h-BN core-shell nanocatalysts. The h-BN shells not only protect the Pt NPs under harsh conditions but also allow gaseous molecules such as CO and O2 to access a large part of the Pt surfaces through a facile intercalation process. As a result, the Pt@h-BN nanostructures act as nanoreactors, and CO oxidation reactions with improved activity, selectivity, and stability occur at the core-shell interfaces. The confinement effect exerted by the h-BN shells promotes the Pt-catalyzed reactions. Our work suggests that two-dimensional shells can function as robust but flexible covers on nanocatalyst surfaces and tune the surface reactivity. | Mengmeng Sun Qiang Fu Lijun Gao Yanping Zheng Yangyang Li Mingshu Chen Xinhe Bao | 2017 | Nano Research2017，10，4： | 5 |
| 19 | Adaptive sliding mode output tracking control based-FODOB for a class of uncertain fractional-order nonlinear time-delayed systems显示文摘An adaptive sliding mode control(ASMC) method, based on fractional-order disturbance-observer(FODOB), is presented for a class of fractional-order nonlinear time-delay systems(FONTDS) with uncertainties to solve the target output tracking problem.The external disturbances are estimated by FODOB, and the unknown internal perturbations of the system are adaptively estimated by sliding mode control(SMC). Furthermore, Gronwall's inequality approach is used to ensure that the output tracking error is uniformly bounded for FONTDS. Firstly, a fractional-order sliding mode control(FOSMC) based FODOB is proposed for a fractional-order linear time-delay system(FOLTDS). Secondly, combined with adaptive estimation, the ASMC of FONTDS is studied. Finally, a numerical example of FONTDS is used to verify the effectiveness of the proposed methods. | WANG Zhen WANG XinHe XIA JianWei SHEN Hao MENG Bo | 2020 | Science China(Technological Sciences)2020，63，9： | 5 |
| 20 | Fabrication of metal nanoclusters on graphene grown on Ru(0001)显示文摘Monolayer graphene was epitaxially grown on Ru(0001) through exposure of the Ru(0001) to ethylene at room temperature followed by annealing in ultrahigh vacuum at elevated temperatures. The resulting graphene structures were studied by scanning tunneling microscopy (STM), X-ray photoelectron spectroscopy (XPS), and ultraviolet photoelectron spectroscopy (UPS). The graphene/Ru(0001) surface was used as a periodic template for growth of metal nanoclusters. Highly dispersed Pt clusters with well controlled size and spatial distribution were fabricated on the surface. | ZHANG Hui FU Qiang CUI Yi TAN DaLi BAO XinHe | 2009 | Chinese Science Bulletin2009，54，14： | 4 |
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