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| 1 | Influence of N doping and the functional groups of graphene on a RGO/TiO2 composite photocatalyst显示文摘Reduced graphene oxide(RGO)assisted TiO2 composite photocatalysts have attracted increased attention because of their high photocatalytic performance under both UV-and visible-light irradiation.However,the corresponding properties under the long wavelength irradiation is far from expected.In this study,a series of RGO samples with well-designed N impurity and optimized surface functional groups are prepared and employed during hybridization with TiO2(named N-RGO/TiO2).The coupling between the doped N atoms and surface functional groups is analyzed based on the resulting photocatalytic performances,and the specific mechanism is revealed by the EPR,IR and lifetime of the photoinduced electrons.After comparing the corresponding performances of the RGO/TiO2 and RGO/N-TiO2 specimens,the results show that the surface functional groups of the RGO serve as a precondition to achieveπ-d coupling between the graphene basal plane and TiO2 nanoparticles,while N atoms in the RGO enhance the resulting photoactivity under a long wavelength range(>510 nm).The findings provide a potential approach to promote the photocatalytic properties of graphene-based composite photocatalysts with the low-energy incident photons. | TANG Bo HE YanFeng ZHANG ZhenYu WANG ZhengWei JI Li MA TingTing LI Sen DAI YuanZhe ZHANG GuoLiang | 2020 | Science China(Technological Sciences)2020，63，6： | 3 |
| 2 | Optical properties and chemical bonding characteristics of amorphous SiN: H thin films grown by the plasma enhanced chemical vapor deposition method 显示文摘 | He Yin Wang Yuanzhe Li Wang | 2012 | Journal of Non-Crystalline Solids2012，358，3： | 1 |
| 3 | A thiophene-containing covalent triazine-based framework with ultramicropore for CO2 capture显示文摘In this work, a 2D covalent triazine-based framework was prepared by using 1,3-dicyanobenzo[c]thiophene(DCBT) as monomer to effectively capture CO_2. The resulting CTF-DCBT was characterized by FT-IR, XPS, PXRD, elemental analysis, SEM, TEM, and N_2 adsorption-desorption.The results indicate that CTF-DCBT is partially crystalline and has ultramicropore(6.5 A?) as well as high heteroatom contents(11.24 wt% and 12.61 wt% for N and S, respectively). In addition, the BET surface area and total pore volume of CTF-DCBT are 500 m^2/g and 0.26 cm^3/g, respectively. CTF-DCBT possesses excellent thermal stability(450 °C) and chemical stability towards boiling water, 4 M HCl, and 1 M Na OH.The CO_2 adsorption capacity of CTF-DCBT is 37.8 cm^3/g at 1 bar and 25 °C. After six adsorption-desorption cycles, there is no obvious loss of CO_2 uptake observed. Due to the ultramicropore and high heteroatom contents, CTF-DCBT has high isosteric heats of adsorption for CO_2 and high selectivities of CO_2 over N_2 and CH_4. At 25 °C, the CO_2/N_2 and CO_2/CH_4 selectivities are 112.5 and 10.3, respectively, which are higher than those of most POFs. Breakthrough curves indicate that CTF-DCBT could effectively separate CO_2/N_2 and CO_2/CH_4 mixtures. | Keke Wang Yuanzhe Tang Qin Jiang Youshi Lan Hongliang Huang Dahuan Liu Chongli Zhong | 2017 | Journal of Energy Chemistry2017，26，5： | 1 |
| 4 | Transport Patterns and Potential Sources of Atmospheric Pollution during the ⅩⅩⅣ Olympic Winter Games Period显示文摘The attainment of suitable ambient air quality standards is a matter of great concern for successfully hosting the ⅩⅩⅣ Olympic Winter Games(OWG). Transport patterns and potential sources of pollutants in Zhangjiakou(ZJK) were investigated using pollutant monitoring datasets and a dispersion model. The PM_(2.5) concentration during February in ZJK has increased slightly(28%) from 2018 to 2021, mostly owing to the shift of main potential source regions of west-central Inner Mongolia and Mongolian areas(2015–18) to the North China Plain and northern Shanxi Province(NCPS) after 2018.Using CO as an indicator, the relative contributions of the different regions to the receptor site(ZJK) were evaluated based on the source-receptor-relationship method(SRR) and an emission inventory. We found that the relative contribution of pollutants from NCPS increased from 33% to 68% during 2019–21. Central Inner Mongolia(CIM) also has an important impact on ZJK under unfavorable weather conditions. This study demonstrated that the effect of pollution control measures in the NCPS and CIM should be strengthened to ensure that the air quality meets the standard during the ⅩⅩⅣ OWG. | Yuting ZHANG Xiaole PAN Yu TIAN Hang LIU Xueshun CHEN Baozhu GE Zhe WANG Xiao TANG Shandong LEI Weijie YAO Yuanzhe REN Yongli TIAN Jie LI Pingqing FU Jinyuan XIN Yele SUN Junji CAO Zifa WANG | 2022 | Advances in Atmospheric Sciences2022，39，10： | 1 |
| 5 | A Rat Model of Autologous Oral Mucosal Epithelial Transplantation for Corneal Limbal Stem Cell Failure显示文摘Purpose: To establish an animal model of autologous oral mucosa grafting for limbal stem cell deficiency.Methods: The study was carried from August to October2012. Fourteen SD rats were randomly and evenly allocated to study group A and control group B. Limbal stem cell deficiency was established by alkali burn in the right eye of each rat in both groups. Rats in group A received autologous oral mucosa strip transplantation following the chemical burn. Rats in group B did not receive surgery after the chemical burn.Topical antibiotics and dexamethasone were used in all rats.Corneal clarity, corneal fluorescein staining, oral mucosal graft survival, and complications at postoperative days 1,3,7,14 were observed.Results: The oral mucosa strip graft was detached in one rat in group A. Reepithelialization was observed starting from the graft position and was completed within 14 days in the remaining 6 eyes in group A. However, persistent corneal epithelium defect was observed in all eyes in group B, among which corneal melting and perforation was observed in 2 eyes and corneal opacification with neovascularization was observed in the remaining 5 eyes.Conclusion: Autologous oral mucosa strip grafting for limbal stem cell deficiency can be achieved by a rat model following chemical burn. The fate of the transplanted oral mucosal epithelial cells warrants further study. | Weihua Li Qiaoli Li Wencong Wang Kaijing Li Shiqi Ling Yuanzhe Yang Lingyi Liang | 2014 | Eye Science2014，29，1： | 0 |
| 6 | Study of a water-soluble supramolecular complex of curcumin andβ-cyclodextrin polymer with electrochemical property and potential anti-cancer activity显示文摘As a member of the curcuminoid compound family,curcumin(Cur)has many interesting therapeutic properties.However,its low aqueous solubility and stability have resulted in poor bioavailability and restricted clinical efficacy.Based on size matching,β-cyclodextrin polymer(β-CDP),with its hydrophilic polymer chains and hydrophobic cavities,can form an inclusion complex with Cur.To improve the water solubility and stability of Cur,a simple and eco-friendly grinding method was designed to formβ-CDP inclusion complexes.According to the Boltzmann-Hamel's method and Job's method,the molar ratio of theβ-CD unit inβ-CDP to Cur was determined to be 1:1.The diffusion coefficient and diffusion activation energy of Cur-β-CDP were calculated in an electrochemical study.This supramolecular complex worked well in vitro to inhibit the proliferation of hepatoma carcinoma cells HepG2.Remarkably,this method visibly reduced the undesirable side effects on normal cells,without weakening the anti-cancer activity of the drugs.We expect that the obtained host-guest complex will provide a new approach for delivering natural drug molecules,having low water solubility. | Wang Zhang Ping Xiao Liwei Lin Fang Guo Qingyue Wang Yuanzhe Piao Guowang Diao | 2022 | Chinese Chemical Letters2022，33，8： | 0 |
| 7 | Scientific Advances and Weather Services of the China Meteorological Administration’s National Forecasting Systems during the Beijing 2022 Winter Olympics显示文摘Since the Beijing 2022 Winter Olympics was the first Winter Olympics in history held in continental winter monsoon climate conditions across complex terrain areas,there is a deficiency of relevant research,operational techniques,and experience.This made providing meteorological services for this event particularly challenging.The China Meteorological Administration(CMA)Earth System Modeling and Prediction Centre,achieved breakthroughs in research on short-and medium-term deterministic and ensemble numerical predictions.Several key technologies crucial for precise winter weather services during the Winter Olympics were developed.A comprehensive framework,known as the Operational System for High-Precision Weather Forecasting for the Winter Olympics,was established.Some of these advancements represent the highest level of capabilities currently available in China.The meteorological service provided to the Beijing 2022 Games also exceeded previous Winter Olympic Games in both variety and quality.This included achievements such as the“100-meter level,minute level”downscaled spatiotemporal resolution and forecasts spanning 1 to 15 days.Around 30 new technologies and over 60 kinds of products that align with the requirements of the Winter Olympics Organizing Committee were developed,and many of these techniques have since been integrated into the CMA’s operational national forecasting systems.These accomplishments were facilitated by a dedicated weather forecasting and research initiative,in conjunction with the preexisting real-time operational forecasting systems of the CMA.This program represents one of the five subprograms of the WMO’s high-impact weather forecasting demonstration project(SMART2022),and continues to play an important role in their Regional Association(RA)II Research Development Project(Hangzhou RDP).Therefore,the research accomplishments and meteorological service experiences from this program will be carried forward into forthcoming highimpact weather forecasting activities.This article provides an overview and assessment of this program and the operational national forecasting systems. | Guo DENG Xueshun SHEN Jun DU Jiandong GONG Hua TONG Liantang DENG Zhifang XU Jing CHEN Jian SUN Yong WANG Jiangkai HU Jianjie WANG Mingxuan CHEN Huiling YUAN Yutao ZHANG Hongqi LI Yuanzhe WANG Li GAO Li SHENG Da LI Li LI Hao WANG Ying ZHAO Yinglin LI Zhili LIU Wenhua GUO | 2024 | Advances in Atmospheric Sciences2024，41，5： | 0 |
| 8 | Design Strategy for Vulcanization Accelerator of Diphenylguanidine/Cyclodextrin Inclusion Complex for Natural Rubber Latex Foam with Enhancing Performance显示文摘Vulcanization is an essential process to obtain high-performance rubber products.Diphenylguanidine(DPG)is often used as the secondary accelerator in the vulcanization process of natural rubber(NR)latex.However,DPG would make NR latex emulsion exhibit gelation,resulting in the negative vulcanization efficiency.In addition,exposure to DPG might lead to some physiological diseases during the production process of DPG doped NR latex.Hydroxypropyl-β-cyclodextrin(HP-β-CD)with the hydrophobic interior and hydrophilic exterior has the advantages of good water solubility,high bioavailability,reliable stability,and low toxicity.In this study,the inclusion complex of diphenylguanidine-hydroxypropyl-β-cyclodextrin(DPG-HP-β-CD)is prepared by bali milling with a host-guest molar ratio of 1:1,which has also been applied to the foaming process of NR latex.The mechanical properties of DPG-HP-β-CD inclusion complex/natural rubber latex foam(DPG-HP-β-CD/NRLF)have been significantly improved,including the tensile strength,elongation at break,hardness,compression set,resilience,and antiaging performance.Further,the usage of DPG has been reduced,leading to the reduction of toxicity and environmental hazards. | Wang Zhang Liwei Lin Junqiang Guo Ming Wu Sumin Park Hang Yao Sun Ha Paek Guowang Diao Yuanzhe Piao | 2023 | Research2023，，1： | 0 |
| 9 | Consecutive hybrid mechanism boosting Na+storage performance of dual-confined SnSe2 in N,Se-doping double-walled hollow carbon spheres显示文摘Rationally designed hierarchical structures and heteroatomic doping of carbon are effective strategies to enhance the stability and electrical conductivity of materials.Herein,SnSe_(2)flakes were generated in the double-walled hollow carbon spheres(DWHCSs),in which N and Se atoms were doped in the carbon walls,to construct SnSe_(2)@N,Se-DWHCSs by confined growth and in-situ derivatization.The N and Sedoped DWHCSs can effectively limit the size increase of SnSe_(2),promote ion diffusion kinetics,and buffer volume expansion,which can be proved by electron microscope observation and density functional theory calculation.Consequently,the SnSe_(2)@N,Se-DWHCSs as an anode material for sodium ion batteries(SIBs)demonstrated a distinguished reversible capacity of 322.8 mAh g^(-1)at 5 A g^(-1)after 1000 cycles and a superior rate ability of 235.3 m Ah g^(-1)at an ultrahigh rate of 15 A g^(-1).Furthermore,the structure evolution and electrochemical reaction processes of SnSe2@N,Se-DWHCSs in SIBs were analyzed by exsitu methods,which confirmed the consecutive hybrid mechanism and the phase transition process. | Xiaoyu Wu Zhenshan Yang Lin Xu JianHua Wang Lele Fan Fanjie Kong Qiaofang Shi Yuanzhe Piao Guowang Diao Ming Chen | 2022 | Journal of Energy Chemistry2022，31，11： | 0 |
| 10 | Wearable and stretchable conductive polymer composites for strain sensors:How to design a superior one?显示文摘Wearable and stretchable strain sensors have potential values in the fields of human motion and health monitoring,flexible electronics,and soft robotic skin.The wearable and stretchable strain sensors can be directly attached to human skin,providing visualized detection for human motions and personal healthcare.Conductive polymer composites(CPC)composed of conductive fillers and flexible polymers have the advantages of high stretchability,good flexibility,superior durability,which can be used to prepare flexible strain sensors with large working strain and outstanding sensitivity.This review has put forward a comprehensive summary on the fabrication methods,advanced mechanisms and strain sensing abilities of CPC strain sensors reported in recent years,especially the sensors with superior performance.Finally,the structural design,bionic function,integration technology and further application of CPC strain sensors are prospected. | Liwei Lin Sumin Park Yuri Kim Minjun Bae Jeongyeon Lee Wang Zhang Jiefeng Gao Sun Ha Paek Yuanzhe Piao | 2023 | Nano Materials Science2023，5，4： | 0 |
| 11 | A universal synthesis of N,S,Cl-doped carbon materials directly from dye waste liquid for high performance lithium storage显示文摘The complicated structured dyes produced by the textile industry have become a serious problem in the last few decades,which can be attributed to their stable chemical structures and difficult to degrade.Therefore,in this article,we described a method to fix dye macromolecules by flocculation process and then transform the colloid to N,S,Cl-doped porous carbon materials.This material can effectively improve the capacity and cycle stability of lithium ion batteries,and recycle the dyes in the water.The N,S,Cl-doped porous carbon materials show a superior electrocatalytic performance of 473.5 mAhg^(−1) at the current density of 100 mAg^(−1) after 60 cycles.The present work combines the lithium ion batteries with dyes waste treatment and has a broad prospect for development. | Junshuang Zhou Kuo Wei Lina Tian Zhuoran Hao Ying Bian Yuanzhe Wang Faming Gao | 2021 | Waste Disposal and Sustainable Energy2021，3，2： | 0 |
| 12 | Advanced flexible humidity sensors:structures,techniques,mechanisms and performances显示文摘Flexible humidity sensors are widely used in many fields,such as environmental monitoring,agricultural soil moisture content determination,food quality monitoring and healthcare services.Therefore,it is essential to measure humidity accurately and reliably in different conditions.Flexible materials have been the focusing substrates of humidity sensors because of their rich surface chemical properties and structural designability.In addition,flexible materials have superior ductility for different conditions.In this review,we have summarized several sensing mechanisms,processing techniques,sensing layers and substrates for specific humidity sensing requirements.Aadditionally,we have sorted out some cases of flexible humidity sensors based on different functional materials.We hope this paper can contribute to the development of flexible humidity sensors in the future. | Yuzhe Zhang Yuxi Liu Lifei Lin Man Zhou Wang Zhang Liwei Lin Zhongyu Li Yuanzhe Piao Sun Ha Paek | 2023 | Frontiers of Materials Science2023，17，4： | 0 |
| 13 | Passive imaging through dense scattering media显示文摘Imaging through non-static and optically thick scattering media such as dense fog,heavy smoke,and turbid water is crucial in various applications.However,most existing methods rely on either active and coherent light illumination,or image priors,preventing their application in situations where only passive illumination is possible.In this study we present a universal passive method for imaging through dense scattering media that does not depend on any prior information.Combining the selection of small-angle components out of the incoming information-carrying scattering light and image enhancement algorithm that incorporates timedomain minimum filtering and denoising,we show that the proposed method can dramatically improve the signal-to-interference ratio and contrast of the raw camera image in outfield experiments. | YAOMING BIAN FEI WANG YUANZHE WANG ZHENFENG FU HAISHAN LIU HAIMING YUAN GUOHAI SITU | 2024 | Photonics Research2024，12，1： | 0 |
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