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| 1 | A Novel Hierarchical Porous 3D Structured Vanadium Nitride/Carbon Membranes for High-performance Supercapacitor Negative Electrodes显示文摘Transition-metal nitrides exhibit wide potential windows and good electrochemical performance, but usually experience imbalanced practical applications in the energy storage field due to aggregation, poor circulation stability, and complicated syntheses. In this study, a novel and simple multiphase polymeric strategy was developed to fabricate hybrid vanadium nitride/carbon(VN/C) membranes for supercapacitor negative electrodes, in which VN nanoparticles were uniformly distributed in the hierarchical porous carbon 3D networks. The supercapacitor negative electrode based on VN/C membranes exhibited a high specific capacitance of 392.0 F g^(-1) at 0.5 A g^(-1) and an excellent rate capability with capacitance retention of 50.5% at 30 A g^(-1). For the asymmetric device fabricated using Ni(OH)_2//VN/C membranes, a high energy density of 43.0 Wh kg^(-1) at a power density of800 W kg^(-1) was observed. Moreover, the device also showed good cycling stability of 82.9% at a current density of 1.0 A g^(-1) after 8000 cycles. This work may throw a light on simply the fabrication of other high-performance transition-metal nitridebased supercapacitor or other energy storage devices. | Yage Wu Yunlong Yang Xiaoning Zhao Yongtao Tan Ying Liu Zhen Wang Fen Ran | 2018 | Nano-Micro Letters2018，10，4： | 13 |
| 2 | Effects of three coniferous plantation species on plant-soil feedbacks and soil physical and chemical properties in semiarid mountain ecosystems显示文摘Background:Large-scale afforestation can significantly change the ground cover and soil physicochemical properties,especially the soil fertility maintenance and water conservation functions of artificial forests,which are very important in semi-arid mountain ecosystems.However,how different tree species affect soil nutrients and soil physicochemical properties after afforestation,and which is the best plantation species for improving soil fertility and water conservation functions remain largely unknown.Methods:This study investigated the soil nutrient contents of three different plantations(Larix principis-rupprechtii,Picea crassifolia,Pinus tabuliformis),soils and plant-soil feedbacks,as well as the interactions between soil physicochemical properties.Results:The results revealed that the leaves and litter layers strongly influenced soil nutrient availability through biogeochemical processes:P.tabuliformis had higher organic carbon,ratio of organic carbon to total nitrogen(C:N)and organic carbon to total phosphorus(C:P)in the leaves and litter layers than L.principis-rupprechtii or P.crassifolia,suggesting that higher C:N and C:P hindered litter decomposition.As a result,the L.principis-rupprechtii and P.crassifolia plantation forests significantly improved soil nutrients and clay components,compared with the P.tabuliformis plantation forest.Furthermore,the L.principis-rupprechtii and P.crassifolia plantation forests significantly improved the soil capacity,soil total porosity,and capillary porosity,decreased soil bulk density,and enhanced water storage capacity,compared with the P.tabuliformis plantation forest.The results of this study showed that,the strong link between plants and soil was tightly coupled to C:N and C:P,and there was a close correlation between soil particle size distribution and soil physicochemical properties.Conclusions:Therefore,our results recommend planting the L.principis-rupprechtii and P.crassifolia as the preferred tree species to enhance the soil fertility and water conservation functions,especially in semi-arid regions mountain forest ecosystems. | Chun Han Yongjing Liu Cankun Zhang Yage Li Tairan Zhou Salman Khan Ning Chen Changming Zhao | 2021 | Forest Ecosystems2021，8，1： | 3 |
| 3 | Slip rate of the seismogenic fault of the 2021 Maduo earthquake in western China inferred from GPS observations显示文摘Seismic and field observations indicate that the Mw7.4 Maduo earthquake ruptured the Jiangcuo fault,which is a secondary fault~85 km south of the northern boundary of the Bayan Hor block in western China.The kinematic characteristics of the Jiangcuo fault can shed lights on the seismogenic mechanism of this earthquake.Slip rate is one of the key parameters to describe the kinematic features of a fault,which can also provide quantitative evidences for regional seismic hazard assessments.However,due to lack of effective observations,the slip rate of the Jiangcuo fault has not been studied quantitatively.In this study,we consider the interaction between the Jiangcuo fault and the eastern Kunlun fault,and estimate the slip rates of the two faults using the interseismic GPS observations across the seismogenic region.The inferred results show that the slip rates of the Jiangcuo fault and the Tuosuo Lake segment of the Kunlun fault are 1.2±0.8 and 5.4±0.3 mm a^(-1),respectively.Combining the slip rate with the average slip inferred from the coseismic slip model,the earthquake recurrence interval of the Jiangcuo fault is estimated to be 1800700+3700 years(1100–5500 years).Based on the results derived from previous studies,as well as calculations in this study,we infer that the slip rate of the Kunlun fault may decrease gradually from the Tuosuo Lake segment to the eastern tip.The Jiangcuo fault and its adjacent parallel secondary faults may have absorbed the relative motion of blocks together with the Kunlun fault. | Yage ZHU Faqi DIAO Yuchao FU Chengli LIU Xiong XIONG | 2021 | Science China Earth Sciences2021，64，8： | 3 |
| 4 | Reflection and transmission properties of double submerged rectangular blocks显示文摘An analytic method is used to study the reflection and transmission coefficients of the double submerged rectangular blocks (DSRBs) in oblique waves. The scattering potentials are obtained by means of the eigenfunction expansion method, and expressions for the reflection and transmission coefficients are determined. The boundary element method is employed to verify the correctness of the present analytical method. The DSRBs have better performance than the single submerged rectangular block (SSRB) in certain cases. The reflection and transmission properties of the DSRBs are investigated for some specific cases, and the influences of the geometric parameters are also presented. | HE Zaiming LIU Pengfei YOU Yage FENG Bo | 2007 | Acta Oceanologica Sinica2007，26，2： | 2 |
| 5 | A hyperbranched polymer-based water-resistant adhesive:Durable underwater adhesion and primer for anchoring anti-fouling hydrogel coating显示文摘Direct deployment of gluing and achieving durable robust adhesion in water is challenging due to difficulty in repelling interface water.This work reports a novel hyperbranched polymer-based water-resistant adhesive(HBPBA)based on Michael addition reaction of multi-vinyl monomers with dopamine and 3-aminophenylboronic acid.Upon encountering water,the HBPBA forms coacervates whose hydrophobic chains aggregate to displace interface water,and meanwhile the catechols exposing outwards contribute to underwater adhesion.The HBPBA can strongly glue diverse substrates including PTFE,PE,PET,ceramic,Ti and stainless steel.The HBPBA can maintain stable adhesion in different environments,such as tap water,simulated sea water,PBS,and a wide range of pH solutions(pH 2 to 10)for 3 months,supposedly due to the complexation of catechol with boronic acid.Intriguingly,HBPBA film can be bonded to the titanium surface as a primer,which firmly anchors the antifouling PNAGAPCBAA hydrogel coating through copolymerization of remaining double bonds in HBPBA and NAGA plus CBAA.The PNAGA-PCBAA hydrogel-modified titanium is biocompatible and shows outstanding antifouling ability both in vitro and in vivo.This work proposes a new strategy for creating underwater deployable and water-resistant adhesives that may find promising applications in engineering and biomedical fields. | ZHANG YaHan CUI ChunYan SUN YaGe ZHANG XiaoPing YANG Rong YANG JianHai XIE Fei LIU WenGuang | 2022 | Science China(Technological Sciences)2022，65，1： | 1 |
| 6 | Improving the WRF/urban modeling system in China by developing a national urban dataset显示文摘Accurate modeling of urban climate is essential to predict potential environmental risks in cities.Urban datasets,such as urban land use and urban canopy parameters(UCPs),are key input data for urban climate models and largely affect their performance.However,access to reliable urban datasets is a challenge,especially in fast urbanizing countries.In this study,we developed a high-resolution national urban dataset in China(NUDC)for the WRF/urban modeling system and evaluated its effect on urban climate modeling.Specifically,an optimization method based on building morphology was proposed to classify urban land use types.The key UCPs,including building height and width,street width,surface imperviousness,and anthropogenic heat flux,were calculated for both single-layer Urban Canopy Model(UCM)and multiple-layer Building Energy Parameterization(BEP).The results show that the derived morphological-based urban land use classification could better reflect the urban characteristics,compared to the socioeconomic-function-based classification.The UCPs varied largely in spatial within and across the cities.The integration of the developed urban land use and UCPs datasets significantly improved the representation of urban canopy characteristics,contributing to a more accurate modeling of near-surface air temperature,humidity,and wind in urban areas.The UCM performed better in the modeling of air temperature and humidity,while the BEP performed better in the modeling of wind speed.The newly developed NUDC can advance the study of urban climate and improve the prediction of potential urban environmental risks in China. | Huidong Li Fenghui Yuan Lidu Shen Yage Liu Zhonghua Zheng Xu Zhou | 2022 | Geoscience Frontiers2022，13，4： | 0 |
| 7 | Copper-linked IT MoS2/Cu2O Heterostructure for Efficient Photocatalytic Hydrogen Evolution显示文摘Metallic IT phase molybdenum disulfide(lT MoS2)is an excellent catalyst due to the abundant active sites and good conductivity.However,complex synthesis and unstable nature of IT MoS2 still limit its practical application.Herein,we propose a simple method to trigger the phase transition of MoS2.This phase transition is first predicted by density functional theory(DFT)calculations and then confirmed by Raman spectroscopy and high-resolution transmission electron microscopy(HRTEM).IT MoS2/CU2O heterostructure catalyst is then developed,showing enhanced photocatalytic hydrogen evolution. | YIN Yage WEI Shuting ZHANG Lei GUO Ziwang HUANG Haihua SAl Shiran WU Jiandong XU Yanchao LIU Ying ZHENG Lirong FAN Xiaofeng CUI Xiaogiang | 2020 | Chemical Research in Chinese Universities2020，36，6： | 0 |
| 8 | 3D-printed,bi-layer,biomimetic artificial periosteum for boosting bone regeneration显示文摘Periosteum,a membrane covering the surface of the bone,plays an essential role in maintaining the function of bone tissue—and especially in providing nourishment and vascularization during the bone regeneration process.Currently,most artificial periostea have relatively weak mechanical strength and a rapid degradation rate,and they lack integrated angiogenesis and osteogenesis functions.In this study,a bi-layer,biomimetic,artificial periosteum composed of a methacrylated gelatin–nano-hydroxyapatite(GelMA-nHA)cambium layer and a poly(N-acryloyl 2-lycine)(PACG)-GelMA-Mg^(2+)fibrous layer was fabricated via 3D printing.The GelMA-nHA layer is shown to undertake the function of improving osteogenic differentiation of rat bone marrow mesenchymal stem cells with the sustainable release of Ca^(2+) from nHA nanoparticles.The hydrogen-bonding-strengthened P(ACG-GelMA-L)-Mg^(2+)hydrogel layer serves to protect the inner defect site and prolong degradation time(60 days)to match new bone regeneration.Furthermore,the released magnesium ion exhibits a prominent effect in regulating the polarization phenotype of macrophage cells into theM2 phenotype and thus promotes the angiogenesis of the human umbilical vein endothelial cells in vitro.This bi-layer artificial periosteum was implanted into a critical-sized cranial bone defect in rats,and the 12-week post-operative outcomes demonstrate optimal new bone regeneration. | Yage Sun Ziwei Gao Xiaoping Zhang Ziyang Xu Yahan Zhang Binbin He Rong Yang Qian Zhang Qiang Yang Wenguang Liu | 2022 | Bio-Design and Manufacturing2022，5，3： | 0 |
| 9 | Wet adhesive hydrogel cardiac patch loaded with anti-oxidative,autophagy-regulating molecule capsules and MSCs for restoring infarcted myocardium显示文摘Hydrogel patch-based stem cell transplantation and microenvironment-regulating drug delivery strategy is promising for the treatment of myocardial infarction(MI).However,the low retention of cells and drugs limits their therapeutic efficacies.Here,we propose a prefixed sponge carpet strategy,that is,aldehyde-dextran sponge(ODS)loading anti-oxidative/autophagy-regulating molecular capsules of 2-hydroxy-β-cyclodextrin@resveratrol(HP-β-CD@Res)is first bonded to the rat’s heart via capillary removal of interfacial water from the tissue surface,and the subsequent Schiff base reaction between the aldehyde groups on ODS and amino groups on myocardium tissue.Then,an aqueous biocompatible hydrazided hyaluronic acid(HHA)solution encapsulating mesenchymal stem cells(MSCs)is impregnated into the anchored carpet to form HHA@ODS@HP-β-CD@Res hydrogel in situ via click reaction,thus prolonging the in vivo retention time of therapeutic drug and cells.Importantly,the HHA added to outer surface consumes the remaining aldehydes to contribute to nonsticky top surface,avoiding adhesion to other tissues.The embedded HP-β-CD@Res molecular capsules with antioxidant and autophagy regulation bioactivities can considerably improve cardiac microenvironment,reduce cardiomyocyte apoptosis,and enhance the survival of transplanted MSCs,thereby promoting cardiac repair by facilitating angiogenesis and reducing cardiac fibrosis. | Tengling Wu Xiaoping Zhang Yang Liu Chunyan Cui Yage Sun Wenguang Liu | 2023 | Bioactive Materials2023，，3： | 0 |
| 10 | 3D printedβ-sheet-reinforced natural polymer hydrogel bilayer tissue engineering scaffold显示文摘It remains a significant challenge to fabricate natural polymer(NP)hydrogels with anti-swelling ability and high strengths in the physiological environment.Herein,theβ-sheet-reinforced NP hydrogel is developed by copolymerizing methacrylated gelatin(GelMA)and methacrylated silk fibroin(SFMA)in aqueous solution,followed by ethanol treatment(named GelMA-SFMAAL).Theβ-sheets formed by SFMA can act as a stable physical crosslink to enhance the mechanical properties and prolong the degradation of the GelMA network.Importantly,the chemical crosslinking in the GelMA-SFMA hydrogel prevents excessive aggregation of hydrophobicβ-sheets,thereby avoiding the formation of brittle hydrogel.The obtained GelMA-SFMA-AL hydrogels exhibit considerably enhanced mechanical properties(Young's modulus:0.89–3.68 MPa;tensile strength:0.31–0.96 MPa;toughness:0.09–0.63 MJ/m^(3);compressive modulus:0.78–2.20 MPa;compressive strength:2.65–5.93 MPa)compared with GelMA-SFMA hydrogels(Young's modulus:0.04–0.13 MPa;tensile strength:0.04–0.07 MPa;toughness:0.01–0.02 MJ/m^(3);compressive modulus:0.03–0.09 MPa;compressive strength:0.30–0.64 MPa).A bilayer osteochondral scaffold is constructed via digital light processing(DLP)three-dimensiaonl(3D)printing technology,comprising GelMA-SFMA@diclofenac sodium(DS)-AL as the top layer and GelMA-SFMA@bioactive glass(BG)-AL as the bottom layer.The bilayer hydrogel scaffold is demonstrated to support cell attachment and spreading,and facilitate osteogenic differentiation of rat bone marrow stem cells in vitro.In vivo implantation experiment suggests this bilayer scaffold is promising to be used for osteochondral tissue regeneration. | ZHAO XinRui NIE XiongFeng ZHANG XiaoPing SUN YaGe YANG Rong BIAN XinYu ZHANG Qian WANG HongYing XU ZiYang LIU WenGuang | 2024 | Science China(Technological Sciences)2024，67，4： | 0 |
| 11 | Efficient generation of targeted point mutations in the Brassica oleracea var.botrytis genome via a modified CRISPR/Cas9 system显示文摘In this study,we used the modified CRISPR/Cas9 system to produce targeted point mutations in cauliflower.Acetolactate synthase(ALS)and Centromere-specific histone H3 variant(CENH3)genes were selected as the base-editing targets and hypocotyls of cauliflower were used as explants.For ALS gene,a C-to-T conversion in the Pro182 codon(CCT)can alter the encoded amino acid,likely resulting in herbicide resistance,and a C-to-T mutation in the Leu133 codon(CTT)in the CENH3 gene may produce a haploid inducer.Results indicated that the transformation efficiency was 1.8%–4.5%and the mutation efficiencies for the ALS and CENH3 genes were approximately 22%and 87%,respectively.The ALS mutant cauliflower showed strong herbicide resistance,with possible immediate implications for broadleaf weed control in cauliflower fields. | Guixiang Wang Mei Zong Di Liu Yage Wu Shouwei Tian Shuo Han Ning Guo Mengmeng Duan Liming Miao Fan Liu | 2022 | Horticultural Plant Journal2022，8，4： | 0 |
| 12 | Histone demethylase Kdm5c regulates osteogenesis and bone formation via PI3K/Akt/HIF1α and Wnt/β-catenin signaling pathways显示文摘Fractures have an extraordinarily negative impact on individuals'quality of life and functional status.Nonunion or disability of fracture is a major health issue with important clinical,social,and economic implications.1 Mesenchymal stem cells(MSCs)play an indispensable role in the initiation of the fracture repair process including the formation of a callus which is replaced by new bone.The use of MSCs in the treatment of fractures is very attractive as they can reduce the time of healing and occurrence of nonunion. | Ying Li Lingli Ding Yage Zhang Bingyu Zhou Gene Chi Wai Man Min Wang Jinglan Li Yamei Liu Weiping Lin Haibin Wang Sien Lin Liangliang Xu | 2024 | Genes & Diseases2024，11，1： | 0 |
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