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| 1 | Recoverable Mn~Ⅲ (salen) supported on diamine modified zirconium poly(styrene-isopropenyl phosphonate)-phosphate as an efficient catalyst for epoxidation of unfunctionalized olefins显示文摘Chiral Mn Ⅲ (salen) (Jacobsen's catalyst) was axially immobilized onto a new type of organic polymer-inorganic hybrid materialzirconium poly(styrene-isopropenyl phosphonate)-phosphate(ZPS-IPPA) with different linkage lengths and evaluated as catalysts for the epoxidation of unfunctionalized olefins. The results demonstrated that the prepared catalysts exhibited moderate to good activity and enantioselectivity in the asymmetric epoxidation of unfunctionalized olefins. Furthermore, the immobilized catalysts were relatively stable and could be conveniently separated from the reaction system by simple precipitation in hexane. Moreover, higher enantioselectivity was obtained with catalyst 2c than that of homogeneous counterpart catalyzed even after eight times. The excellent recycling of the catalyst was attributed to its structure feature of ZPS-IPPA which is different from either pure polystyrene or pure zirconium phosphates. | ZOU XiaoChuan CHEN ShaoCheng REN YanRong SHI KaiYun LI Jun FU XiangKai | 2012 | Science China Chemistry2012，55，11： | 3 |
| 2 | Genetic diversity of the wild Asian lotus (Nelumbo nucifera) from Northern China显示文摘Asian lotus(Nelumbo nucifera Gaertn.)is an aquatic plant with ornamental,cultural,economic,and ecological values.China has abundant germplasm resources of Asian lotus.However,in many areas,the wild Asian lotuses have been destroyed and the germplasms is now facing extinction.In addition,the knowledge of the genetic diversity of the wild Asian lotus in China is poor.To identify and protect the germplasms of Chinese wild Asian lotus,eleven genomic-SSR primers,three EST-SSR primers,and three chloroplast DNA primers were used to investigate the genetic diversity among 69 samples of wild Asian lotus from 25 locations in northern China.The genetic diversity of 27 samples of wild Asian lotus from southern China and other countries,the ancient Asian lotus,Asian lotus cultivars from China,and Asian-American hybrids was also compared.The genetic diversity of the wild Asian lotus from northern China was characterized as medium,and themean values of observed heterozygosity(Ho)and expected heterozygosity(He)were 0.087 and 0.552,respectively.Based on a UPGMA dendrogram and STRUCTURE analysis,the wild Asian lotus samples in northern China were divided into three groups.The wild Asian lotus samples from northern China contained 16 haplotypes.The Nei’s genetic distance between the wild Asian lotus samples from the Songhua River basin and the Liao River basin in northeastern China was relatively small,and these germplasms might be relatively primitive compared to those from other regions.This study provides essential information regarding the genetic diversity of the wild Asian lotus resources in northern China,and provides a basis for further analysis of population-level genetic evolution through high-throughput sequencing. | Yanrong Fu Fengluan Liu Shuo Li Daike Tian Li Dong Yuchu Chen Yan Su | 2021 | Horticultural Plant Journal2021，7，5： | 3 |
| 3 | Study on the Treatment of Acid Mine Drainage Containing Fe^(2+) and Mn^(2+) Using Modified Spontaneous Combustion Gangue显示文摘The high concentrations of Fe^(2+) and Mn^(2+) in acid mine drainage make it difficult and expensive to treat.It is urgent that we find a cheap and efficient adsorption material to treat Fe^(2+) and Mn^(2+).As a solid waste in mining areas,coal gangue occupies a large area and pollutes the surrounding environment during the stacking process.Developing a method of resource utilization is thus a research hotspot.In this study,we modified spontaneous combustion gangue using NaOH,NaCl,and HCl by chemically modifying the minerals.We determined the optimal conditions for treating Fe^(2+) and Mn^(2+) in acid mine drainage with spontaneous combustion gangue and modified coal gangue using the single factor test method.Based on results of the static test,two dynamic test columns,column No.1(spontaneous combustion gangue)and column No.2(NaOH modified spontaneous combustion gangue),were constructed,and the repair effects of acid mine drainage were compared and analyzed using dynamic experiments.The results show that overall,NaOH modified spontaneous combustion gangue is the most efficient at removing the Fe^(2+) and Mn^(2+) in acid mine drainage.The optimal conditions for NaOH modification are an NaOH concentration of 3 mol/L,a liquid to solid ratio of 2 L/kg,and a modification time of 8 h.The overall efficiency of column No.2 at removing Fe^(2+) and Mn^(2+) from acid mine drainage is better than that of column No.1.Among them,the average removal efficiency of Fe^(2+)and Mn^(2+) from acid mine drainage in column No.2 were 97.73%and 44.82%,respectively.The above results show that NaOH modified spontaneous combustion gangue is a good adsorbent,which has application potential in wastewater remediation,as it can achieve the purpose of“treating dust with waste”. | Xuying Guo Saiou Fu Junzhen Di Yanrong Dong Guoliang Jiang | 2021 | Journal of Renewable Materials2021，9，3： | 2 |
| 4 | The characteristics of Na + , K + and free proline distribution in several drought-resistant plants of the Alxa Desert, China显示文摘 | Suomin Wang Changgui Wan Yanrong Wang Hua Chen Zhiyu Zhou Hua Fu Ronald E Sosebee | 2003 | Journal of Arid Environments2003，，3： | 2 |
| 5 | Quantification and simulation of particle kinematics and local strains in granular materials using X-ray tomography imaging and discrete-element method 显示文摘 | Fu Yanrong Wang Linbing Tumay Mehmet T | 2008 | Journal of Engineering Mechanics2008，134，2： | 1 |
| 6 | The characteristics of Na + , K + and free proline distribution in several drought-resistant plants of the Alxa Desert, China显示文摘 | Suomin Wang Changgui Wan Yanrong Wang Hua Chen Zhiyu Zhou Hua Fu Ronald E Sosebee | 2003 | Journal of Arid Environments2003，，3： | 1 |
| 7 | Observation of Refractive Index Line Shape in Ultrafast XUV Transient Absorption Spectroscopy显示文摘Ultrafast extreme ultraviolet (XUV) transient absorption spectroscopy measures the time- and frequencydependent light losses after light–matter interactions. In the linear region, the matter response to an XUV light field is usually determined by the complex refractive index ̃n. The absorption signal is directly related to the imaginary part of ̃n, namely, the absorption index. The real part of ̃n refers to the real refractive index, which describes the chromatic dispersion of an optical material. However, the real refractive index information is usually not available in conventional absorption experiments. Here, we investigate the refractive index line shape in ultrafast XUV transient absorption spectroscopy by using a scheme that the XUV pulse traverses the target gas jet off-center. The jet has a density gradient in the direction perpendicular to the gas injection direction, which induces deflection on the XUV radiation. Our experimental and theoretical results show that the shape of the frequency-dependent XUV deflection spectra reproduces the refractive index line profile. A typical dispersive refractive index line shape is measured for a single-peak absorption;an additional shoulder structure appears for a doublet absorption.Moreover, the refractive index line shape is controlled by introducing a later-arrived near-infrared pulse to modify the phase of the XUV free induction decay, resulting in different XUV deflection spectra. The results promote our understanding of matter-induced absorption and deflection in ultrafast XUV spectroscopy. | Mingze Sun Zixiang Jiang Yong Fu Yanrong Jiang Hongtao Hu Chunyuan Bai Zhongyao Yue Jiaming Jiang Hongqiang Xie Cheng Jin Ruxin Li P.B.Corkum D.M.Vileneuvere Ppeng Peng | 2023 | Ultrafast Science2023，3，4： | 0 |
| 8 | Treatment of Agate Dyeing Wastewater Using an Immobilized Gel Mixture with Nano-Fe_(3)O_(4) Sulfate-Reducing Bacteria显示文摘To solve the problems of high Cr^(6+),Cr^(3+),SO_(4)^(2-)and H+concentrations,pollution and processing costs associated with agate dyeing industrial drainage,we prepared an immobilized gel mixture for the treatment of such drainage on the basis of microbial immobilization technology.The immobilized gel mixture was composed of sulfate-reducing bacteria(SRB),corn cob,and nano-Fe_(3)O_(4)(nFe_(3)O_(4)).We used a single-factor experiment to determine the optimal dose of each matrix component.We analyzed the mechanism underlying the treatment of agate dyeing wastewater with an immobilized gel mixture by X-ray diffraction and scanning electron microscopy detection.The results of the single-factor test showed that the best treatment was obtained under the following conditions for each matrix component:SRB mass percentage of 30%,nFe_(3)O_(4) dose of 3%,and corn cob mesh size of 100 and dose of 3%.On this basis,we conducted an L9(34)orthogonal experiment to determine the optimal proportion of each matrix component.The results showed that the best treatment was obtained when the gel mixture met the following conditions:SRB mass percentage of 40%,nFe_(3)O_(4) dose of 4%,and corn cob dose of 1%and mesh size of 100.Accordingly,the SO_(4)^(2-),Cr^(6+)and Cr^(3+)removal rates from the agate dyeing drainage were 70.54%,84.75%,and 73.80%,respectively;the total Fe and chemical oxygen demand releases were 1.086 mg·L^(-1)and 1104 mg·L^(-1),respectively;and the pH was 6.27.The gel mixture had the best treatment effect on agate dyeing wastewater under this composition ratio. | Xuying Guo Guoliang Jiang Saiou Fu Zhiyong Hu Junzhen Di Yanrong Dong Ying Li | 2021 | Journal of Renewable Materials2021，9，11： | 0 |
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