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115篇 您的检索式:作者名="Zhaoji Li"
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1cMyc-mediated activation of serine biosynthesis pathway is critical for cancer progression under nutrient deprivation conditions显示文摘癌症房间被知道经历新陈代谢的 reprogramming 然而,支撑幸存和快速的增长 oncogenic 损害怎么在各种各样的强调条件下面协调新陈代谢的开关,尚待充分被阐明。这里,我们显示出葡萄糖或夫酸安的那剥夺,为癌症房间的二主要营养来源,被伴随由的戏剧性地激活的丝氨酸生合成小径(SSP ) 提高了 cMyc 表示。我们进一步鉴别那 cMyc 刺激了 SSP 激活由 transcriptionally 多重 SSP 酶的 upregulating 表示。而且,我们证明 cMyc 便于的 SSP 激活导致了提高的谷胱甘肽(GSH ) 生产,房间周期前进和 nucleic 酸合成,它在剥夺营养素的条件下面特别为房间幸存和增长是必要的。我们进一步揭开了那 phosphoserine 磷酸酶( PSPH ), SSP 小径的最后的限制率的酶,在 vitro 并且在 vivo 为 驾驶cMyc 的癌症前进是批评的,并且重要地, PSPH 的异常表示高度在 hepatocellular 与死亡被相关癌( HCC )病人,一般来说建议在这 调整cMyc 的酶,或 SSP 激活之间的一种潜在的原因的关系,并且癌症开发。一起拿,我们的结果表明 cMyc 的那异常表情导致提高的 SSP 激活,新陈代谢的开关的必要部分,在剥夺营养素的条件下面便于癌症前进。Linchong Sun Libing Song Qianfen Wan Gongwei Wu Xinghua Li Yinghui Wang Jin Wang Zhaoji Liu Xiuying Zhong Xiaoping He Shengqi Shen Xin Pan Ailing Li Yulan Wang Ping Gao Huiru Tang Huafeng Zhang 2015Cell Research2015,25,4:33
2Geochronology, geochemistry, and its geological significance of the Permian Mandula mafic rocks in Damaoqi, Inner Mongolia显示文摘The Hujierte-Chaganhadamiao volcanic-plutonic sequence is located in the Mandula area of northern Damaoqi, Inner Mongolia. It contains mainly mafic volcanics, with several ultramafic blocks in its central part and mafic-intermediate intrusions in the east. The zircon U-Pb ages of the gabbro and basalt samples are 278.5±3.0 Ma (MSWD=0.66) and 273.7±1.0 Ma (MSWD=0.36), respectively. These ages constrain the magmatism occurred in the Early Permian. The Mandula Permian mafic rocks are characterized by low abundances of REE and slightly LREE-enriched chondrite-normalized N-MORB-type REE patterns. And these mafic samples have high ( 143 Nd/ 144 Nd) i (0.51262-0.51270), relatively high positive ε Nd (t) (3.4-8.0), and high Mg # (49-54), suggesting derivation from the depleted asthenosphere mantle source. But they also show the enrichment in large ion lithophile elements (LILE, e.g. Rb, Ba and Sr), depletion in high field strength elements (HFSE); distinctly negative Nb, Ta anomalies and slightly negative P, Ti anomalies; high ( 87 Sr/ 86 Sr) i (0.70490-0.70537), low ( 206 Pb/ 204 Pb) i (17.39-17.93). All of these resemble the characteristics of the enriched mantle source or involvement of arc materials in the magma genesis. Furthermore, as shown in the correlation plots of ε Nd (t) vs ( 87 Sr/ 86 Sr) i , ( 206 Pb/ 204 Pb) i vs ( 207 Pb/ 204 Pb) i and ( 208 Pb/ 204 Pb) i , La/Ba La/Nb vs La/Nb, and La/Nb ratio, the magma source could have been experienced the contamination and metasomation from the previous subduction process. And the positive correlation between the selected major oxides and trace elements could be explained by the contamination from continental crust and arc materials during the magmatic emplacement. Combined with the distinct geochemistry features of Mandula mafic samples and many previous researches in the study area, the Early Permian magmatism in Mandula occurred under an extensional rift setting, and a juvenile ocean basin probably had already been formed after further development.CHEN Chen ZHANG ZhiCheng GUO ZhaoJie LI JianFeng FENG ZhiShuo TANG WenHao 2012Science China Earth Sciences2012,55,1:30
3Nature of the Precambrian metamorphic blocks in the eastern segment of Central Tianshan:Constraint from geochronology and Nd isotopic geochemistry显示文摘Granitoid gneisses are widespread in Precambrian metamorphic blocks of eastern segment of the Central Tianshan Tectonic Zone, and they have intrusive contact relationships with their metamorphic sedimentary country rocks of Proterozoic Xingxingxia and Kawabulag groups. Zircon U-Pb ages from a granodioritic gneiss (IW11-1) and a parametamorphic schist (W05-9) are determined at the Weiya area. Euhedral prismatic zircons from the granodioritic gneiss (IW11-1) provide U-Pb isotopic discordia intercept ages of 1218±17 Ma and 426±26 Ma, respectively, and euhedral prismatic zircons from the parametamorphic schist (W05-9) display U-Pb isotopic discordia intercept ages of 1216±74 Ma and 290±15 Ma, respectively. A whole-rock Sm-Nd isotopic isochron is determined in augen granitoid gneiss samples at the Gang- gou-Kumishi area and we obtain the isochron age of 1142±120 Ma, and its ε Nd (t) = -4.3. These geochronological data suggest that these Precambrian metamorphic basement blocks within eastern segment of the Central Tianshan Tectonic Zone can be produced during 1140—1220 Ma, and occur a nearly homochronous metamorphism. Integrated to these geochronological data, Nd depleted mantle model ages (T DM ) and epsilon Nd(t) values of these granitoid gneiss samples indicate that they can derive from mixing in various scales both magmas from mantle and crust sources at a late Mesoproterozoic active continental margin tectonic environment. Similarity in geochronology, Sm-Nd isotopic geochemistry between Weiya-Xingxingxia, Pargangtag and Ganggou-Kumishi areas suggests that they could be a bigger uniform metamorphic basement block, which could be formed by the assembly of the supercontinent Rodinia and be separated by late geological processes.LIU Shuwen,GUO Zhaojie,ZHANG Zhicheng,LI Qiugen & ZHENG Haifei The Key Laboratory of Orogenic Belts and Crustal Evolution,Ministry of Education,China School of Earth and Space Sciences,Peking University,Beijing 100871,China 2004Science China Earth Sciences2004,47,12:26
4Analyzing the Flavor Compounds in Chinese Traditional Fermented Shrimp Pastes by HS-SPME-GC/MS and Electronic Nose显示文摘Shrimp paste is a type of condiments with high nutritional value.However,the flavors of shrimp paste,particularly the non-uniformity flavors,have limited its application in food processing.In order to identify the characteristic flavor compounds in Chinese traditional shrimp pastes,five kinds of typical commercial products were evaluated in this study.The differences in the volatile composition of the five products were investigated.Solid phase micro-extraction method was employed to extract the volatile compounds.GC-MS and electronic nose were applied to identify the compounds,and the data were analyzed using principal component analysis(PCA).A total of 62 volatile compounds were identified,including 8 alcohols,7 aldehydes,3 ketones,7 ethers,7 acids,3 esters,6 hydrocarbons,12 pyrazines,2 phenols,and 7 other compounds.The typical volatile compounds contributing to the flavor of shrimp paste were found as follows:dimethyl disulfide,dimethyl tetrasulfide,dimethyl trisulfide,2,3,5-trimethyl-6-ethyl pyrazine,ethyl-2,5-dimethyl-pyrazine,phenol and indole.Propanoic acid,butanoic acid,furans,and 2-hydroxy-3-pentanone caused unpleasant odors,such as pungent and rancid odors.Principal component analysis showed that the content of volatile compounds varied depending on the processing conditions and shrimp species.These results indicated that the combinations of multiple analysis and identification methods could make up the limitations of a single method,enhance the accuracy of identification,and provide useful information for sensory research and product development.FAN Yan YIN Li-ang XUE Yong LI Zhaojie HOU Hu XUE Changhu 2017Journal of Ocean University of China2017,16,2:25
5Changes in the Contents of ATP and Its Related Breakdown Compounds in Various Tissues of Oyster During Frozen Storage显示文摘The changes in the contents of adenosine 5’-triphosphate (ATP) and its related breakdown compounds were investigated in the adductor muscle, mantle, gill and body trunk of oyster (Crassostrea gigas) during frozen storage at -20℃ and -30℃ and compared with that of the fresh oyster. The investigation was performed using an HPLC system. Different extents of ATP decomposi- tion were found in various tissues frozen at the two temperatures. The K, K’ and A.E.C values were calculated as the chemical fresh- ness indices. Considering the results of sensory evaluation, the A.E.C. value in body trunk at -20℃ and -30℃ could be used as the best freshness index for frozen oyster.WANG Qi XUE Changhu LI Zhaojie FU Xueyan XU Jie XUE Yong 2007Journal of Ocean University of China2007,6,4:13
6Groundwater Flow Simulation and its Application in Groundwater Resource Evaluation in the North China Plain,China显示文摘这研究的目的是为评估北方中国的地下水资源建立 3D 地下水流动建模平凡的。首先,北方中国平原通过 hydrogeological 条件的描述垂直地被划分成三含水土层。地下水模型软件公克被用于当模特儿把模拟的区域划分成 164 排和 148 根线的一个常规网络。这个模型通过适合被验证观察并且模仿的地下水流动在 64 口典型观察井在在观察并且模仿的自记水位计之间的深、浅的层和比较删除。而且,水预算分析也在模拟时期(20022003 ) 期间被执行。确定的地下水流动模型的结果证明平均年度地下水在 1991 ~ 2003 期间北方中国平原再装 256.68 是慭档湩 e ??辸 吗??SHAO Jingli LI Ling CUI Yali ZHANG Zhaoji 2013Acta Geologica Sinica(English Edition)2013,87,1:9
7Heavy mineral assemblage characteristics and the Cenozoic paleogeographic evolution in southwestern Qaidam Basin显示文摘Based on the analysis of heavy mineral assemblages in Cenozoic southwestern Qaidam Basin, we found that different areas have variable heavy mineral assemblage characteristics, which suggested that there were two source areas—the Altyn Mountains and the Qimen Tagh-East Kunlun Mountains. In Ganchaigou-Shizigou-Huatugou(Area A), which was mainly source from the Altyn Mountains, its heavy minerals were mainly composed of zircon, Ti-oxides, and wollastonite in the Paleoceneearly Eocene and mainly of unstable minerals, especially amphibole, in the middle Eocene-Oligene. Since the late OligoceneMiocene, the heavy minerals were still mainly unstable minerals, but the content of epidote increased and the content of amphibole decreased. In Qigequan-Hongliuquan(Area B), which was the mixed source from the Altyn Mountains and the Qimen Tagh-East Kunlun Mountains, its heavy minerals were mainly garnet, epidote, and amphibole. The source of LücaotanDongchaishan-Kunbei(Area C) was mainly from the Qimen Tagh-East Kunlun Mountains, heavy minerals in the sediments in Area C were mainly zircon and Ti-oxides in Paleogene and garnet, epidote, and amphibole in Neogene. In Yuejin-Youshashan(Area D), where the stable minerals and unstable minerals were present simultaneously, the heavy mineral assemblages was controlled by multi-direction source. The variation of heavy mineral assemblages in southwestern Qaidam Basin shows that Altyn Mountains was of low-lying topographic relief in Paleocene-early Eocene, and the rapid uplift of Altyn Mountains started from the middle Eocene. In Paleogene, the Altyn Tagh Fault had a slow strike-slip velocity, but the strike-slip velocity increased greatly since the late Oligocene, leading to a strike-slip displacement above 300 km since Neogene. Meanwhile, the Qimen Tagh-East Kunlun fault zone was under a stable tectonic stage in Paleogene with the Qimen Tagh Mountain being lowlying hills; since the late Oligocene, the fault zone started to activate and the Qimen Tagh Mountain began to uplift rapidly.LI LinLin GUO ZhaoJie GUAN ShuWei ZHOU SuPing WANG MingZhen FANG YaNan ZHANG ChenChen 2015Science China Earth Sciences2015,58,6:6
8Assessment of deep groundwater over-exploitation in the North China Plain显示文摘A series of environmental—geological problems have been caused by over-exploitation of deep groundwater(i.e.,confined aquifer water) in the North China Plain.In order to better understand the status of deep groundwater over-exploitation and the resultant environmental—geological problems on a regional scale,the over-exploitation of groundwater has been assessed by way of the groundwater exploitation potential coefficient(i.e.,the ratio of exploitable amount of deep groundwater to current exploitation), cumulative land subsidence,and long-term average lowering rate of the groundwater table.There is a good correlation among the results calculated by the different methods.On a regional scale,deep groundwater has been over-exploited and there is no further exploitation potential under the current conditions.The groundwater exploitation degree index takes the exploitation in 2003 as the reference for the calculations, so the results mainly reflect the degree of current groundwater exploitation.The results of over-exploitation of deep groundwater obtained by land subsidence data and long-term average rate of depression of the water table mainly reflect environmental—geological problems caused by exploitation of deep groundwater.Jiansheng Shi Zhao Wang Zhaoji Zhang Yuhong Fei Yasong Li Feng'e Zhang Jingsheng Chen Yong Qian 2011Geoscience Frontiers2011,2,4:5
9New Apatite Fission-Track Ages of the Western Kuqa Depression:Implications for the Mesozoic–Cenozoic Tectonic Evolution of South Tianshan,Xinjiang显示文摘The Mesozoic–Cenozoic uplift history of South Tianshan has been reconstructed in many ways using thermochronological analyses for the rocks from the eastern Kuqa Depression. The main difference in the reconstructions concerns the existence and importance of Early Cretaceous and Paleogene tectonic activities, but the existence of a Cenozoic differential uplift in the Kuqa Depression remains enigmatic. Here, we present new apatite fission-track ages obtained for 12 sandstone samples from the well-exposed Early Triassic to Quaternary sequence of the Kapushaliang section in the western Kuqa Depression. The results reveal that there were four pulses of tectonic exhumation, which occurred during the Early Cretaceous(peak ages of 112 and 105 Ma), Late Cretaceous(peak age of 67 Ma), Paleocene–Eocene(peak ages at 60, 53, and 36 Ma), and early Oligocene to late Miocene(central ages spanning 30–11 Ma and peak ages of 23 and 14 Ma), respectively. A review of geochronological and geological evidence from both the western and eastern Kuqa Depression is shown as follows.(1) The major exhumation of South Tians Shan during the Early Cretaceous was possibly associated with docking of the Lhasa block with the southern margin of the Eurasian plate.(2) The Late Cretaceous uplift of the range occurred diachronically due to the far-field effects of the Kohistan-Dras Arc and Lhasa block accretion.(3) The Paleogene uplift in South Tianshan initially corresponded to the far-field effects of the India–Eurasia collision.(4) The rapid exhumation in late Cenozoic was driven by the continuous far-field effects of the collision between India and Eurasia plates. The apatite fission-track ages of 14–11 Ma suggest that late Cenozoic exhumation in the western Kuqa Depression prevailed during the middle to late Miocene, markedly later than the late Oligocene to early Miocene activity in the eastern segment. It can be hypothesized that a possible differential uplift in time occurred in the Kuqa Depression during the late Cenozoic.YANG Wei LI Jianfeng GUO Zhaojie Marc JOLIVET Gloria HEILBRONN 2017Acta Geologica Sinica(English Edition)2017,91,2:4
10Mixed-cation perovskite solar cells in space显示文摘The metal halide perovskite materials demonstrate outstanding performance in photovoltaics because of their excellent optoelectronic properties (1-7)The perovskite solar cells (PSCs) exhibiting outstanding efficiency [8,9], high power-per-weight [10], and excellent radiation resistance[11-13] are considered to be promising for developing the new-generation energy technology for space application.YongGuang Tu GuoNing Xu XiaoYu Yang YiFei Zhang ZhaoJie Li Rui Su DeYing Luo WenQiang Yang Ying Miao Rong Cai LuHua Jiang XiaoWei Du YanChu Yang QianShi Liu Yang Gao Shuai Zhao Wei Huang QiHuang Gong Rui Zhu 2019Science China(Physics,Mechanics & Astronomy)2019,62,7:4
11Carbon quantum dot-induced self-assembly of ultrathin Ni(OH)2 nanosheets: A facile method for fabricating three-dimensional porous hierarchical composite micro-nanostructures with excellent supercapacitor performance显示文摘Significant efforts have been directed towards the preparation and applicationof porous hierarchically structured materials owing to their large surface area,rich active sites, and enhanced mass transport and diffusion. In this study, asimple and cost-effective method for the carbon quantum dot (CQD)-inducedassembly of two-dimensional ultrathin Ni(OH)2 nanosheets into a three-dimensional (3D) porous hierarchical structure was developed. The electrostaticforces between the CQDs and cations drove the self-assembly of the 3DCQDs/Ni(OH)2 hierarchical structures. As a new type of structure-directingagent, the CQDs played dual roles in tuning the morphology of the productsand improving the supercapacitor performance. The multilevel CQDs/Ni(OH)2micro-nanostructures had a large specific surface area and rich porosity. Owingto their unique structures and the conductivity of the CQDs, an optimizedasymmetric supercapacitor using the CQDs/Ni(OH)2 exhibited a maximumspecific capacity of 161.3 F.g-1 and a high energy density of 57.4 Wh·kg^-1 Thisstudy introduces a potential method for the fabrication of many other 3Dhierarchical structures with great potential for applications in various fields.Guijuan Wei Kun Du Xixia Zhao Zhaojie Wang Ming Liu Chuang Li Hui Wang Changhua An Wei Xing 2017Nano Research2017,10,9:4
12Experimental investigation on impact performances of GLARE laminates显示文摘An experimental investigation was carried out on the damage resistance to a concentrated quasi-static indentation force and low-velocity impact of four kinds of glass-reinforced aluminum laminates(GLARE for short). Compared with the experimental results of the CFRP(Carbon Fiber Reinforced Plastics) laminates, the performance of GLARE was determined. By means of concentrated quasi-static indentation force test, typical force–displacement response,the maximum contact force and dent depth were received. Through drop-weight low-velocity impact tests, impact force histories, indentation depths(through a new method) and dissipated energy were obtained. The test results show that the force–displacement response of GLARE 4laminates under the concentrated quasi-static indentation force has an obvious flat roof and the failure is instantaneous, which are different from CFRP laminates. The indention will be visible once the impact happens. C-scan results find that there is no delamination besides the impact area after both the concentrated quasi-static indentation and low-velocity impact. The dissipated energy approximately equals the impact energy.Chen Qi Guan Zhidong Li Zengshan Ji Zhaojie Zhuo Yue 2015Chinese Journal of Aeronautics2015,28,6:3
13Evaluation technology and practice of continental shale oil development in China显示文摘This paper analyzes the differences in geological and development characteristics between continental shale oil in China and marine shale oil in North America, reviews the evaluation methods and technological progress of the continental shale oil development in China, and points out the existing problems and development directions of the continental shale oil development. The research progress of development evaluation technologies such as favorable lithofacies identification, reservoir characterization, mobility evaluation, fracability evaluation, productivity evaluation and geological-mathematical modeling integration are introduced. The efficient exploration and development of continental shale oil in China are faced with many problems, such as weak basic theoretical research, imperfect exploration and development technology system, big gap in engineering technology between China and other countries, and high development cost. Three key research issues must be studied in the future:(1) forming differentiated development technologies of continental shale oil through geological and engineering integrated research;(2) strengthening the application of big data and artificial intelligence to improve the accuracy of development evaluation;(3) tackling enhanced shale oil recovery technology and research effective development method, so as to improve the development effect and benefit.LI Yang ZHAO Qingmin LYU Qi XUE Zhaojie CAO Xiaopeng LIU Zupeng 2022Petroleum Exploration and Development2022,49,5:3
14Effect of enzymatic fish frame protein hydrolysate on freeze-induced denaturation of myofibrillar protein from bighead carp fish (Aristichthys nobilis ) during frozen storage显示文摘薛勇 Xue Changhu Zhang Yongqin Li Zhaojie Gao Ruichang Gao Xin 2006High Technology Letters2006,12,4:2
15Evolution Characteristics and Influence Factors of Deep Groundwater Depression Cone in North China Plain,China——A Case Studyin Cangzhou Region显示文摘The North China Plain(NCP) is one of the global hotspots of groundwater depletion, groundwater is almost the only source of water for agricultural, industrial and drinking water in this region. After long-term's over-exploitation of deep groundwater, there appeared several deep groundwater depression cones, such as Cangzhou cone, Dezhou cone, Hengshui cone, Tianjin cone, etc., in which the Cangzhou cone is one of the typical cones for its special geography and hydrogeology conditions. In this study, the authors intended to analyze the evolution characteristics and influence factors of deep groundwater depression cone in Cangzhou region, especially the No. III aquifer depression cone, which is the main exploitation zone in this region. Analysis of the evolution of the groundwater depression cone of the No. III aquifer group in Cangzhou region showed that this process can be divided into four stages, namely, development, stable development, rapid expansion, and gradual recovery. The shape and evolution characteristics of the depression cone at different stages are described by analyzing the evolution of the-30,-40, and-50 contours of the groundwater table, for example the closed area of water table contour of-50 m has been enlarged from 95 km2 in 1985 to 6 528.5 km2 in 2005. The dominant factors that affect the evolution characteristics at different stages are proposed. The results showed that relatively long dry periods with less precipitation, special geological and hydrogeological conditions, and sharply increased water consumption for industrial and agricultural development are the main factors that cause the formation of deep groundwater depression cones. Meanwhile, an environmental response against groundwater exploitation is presented, and rational solutions are suggested to avert water crisis.Yasong Li Fawang Zhang Zhantao Han Ping Wang Honghan Chen Zhaoji Zhang 2014Journal of Earth Science2014,25,6:2
16Concept and design of super junction devices显示文摘The super junction(SJ) has been recognized as the 'milestone' of the power MOSFET, which is the most important innovation concept of the voltage-sustaining layer(VSL). The basic structure of the SJ is a typical junction-type VSL(J-VSL) with the periodic N and P regions. However, the conventional VSL is a typical resistance-type VSL(R-VSL) with only an N or P region. It is a qualitative change of the VSL from the R-VSL to the JVSL, introducing the bulk depletion to increase the doping concentration and optimize the bulk electric field of the SJ. This paper firstly summarizes the development of the SJ, and then the optimization theory of the SJ is discussed for both the vertical and the lateral devices, including the non-full depletion mode, the minimum specific on-resistance optimization method and the equivalent substrate model. The SJ concept breaks the conventional'silicon limit' relationship of R_(on)∝V_B^(2.5), showing a quasi-linear relationship of R_(on)∝V_B^(1.03).Bo Zhang Wentong Zhang Ming Qiao Zhenya Zhan Zhaoji Li 2018Journal of Semiconductors2018,39,2:2
17Identification of Five Sea Cucumber Species Through PCR-RFLP Analysis显示文摘Sea cucumbers are traditional marine food and Chinese medicine in Asia. The rapid expansion of sea cucumber market has resulted in various problems, such as commercial fraud and mislabeling. Conventionally, sea cucumber species could be distinguished by their morphological and anatomical characteristics; however, their identification becomes difficult when they are processed. The aim of this study was to develop a new convenient method of identifying and distinguishing sea cucumber species. Polymerase chain reaction-restriction fragment length polymorphism(PCR-RFLP) analysis of mitochondrial cytochrome oxidase I gene(COI) was used to identifing five sea cucumber species(Apostichopus japonicus, Cucumaria frondosa, Thelenota ananas, Parastichopus californicus and Actinopyga lecanora). A 692 bp fragment of COI was searched for BamHI, KpnI, PstI, XbaI and Eco31 I restriction sites with DNAMAN 6.0, which were then used to PCR-RFLP analysis. These five sea cucumber species can be discriminated from mixed sea cucumbers. The developed PCR-RFLP assay will facilitate the identification of sea cucumbers, making their source tracing and quality controlling feasible.LV Yingchun ZHENG Rong ZUO Tao WANG Yuming LI Zhaojie XUE Yong XUE Changhu TANG Qingjuan 2014Journal of Ocean University of China2014,13,5:2
18Structural and optical properties of Dy^(3+):YAlO3 phosphors for yellow light-emitting diode applications显示文摘The spectroscopic properties of a series of Dy^(3+)single-doped and Dy^(3+)/Nd^(3+),Dy^(3+)/Tb^(3+),and Dy^(3+)/Tm^(3+)co-doped YAlO_(3)(yttrium aluminum perovskite,YAP)phosphors were investigated and compared through the measurements of optical absorption,emission spectra,and fluorescence decay curves.For the Dy^(3+)ion single-doped samples,the intensity of each absorption band increases with an increment in Dy^(3+)ion doping concentration,and the identified strong absorption peak at 447 nm indicates that Dy^(3+):YAP phosphors are suitable to be pumped by a blue laser diode(LD).For all co-doped samples,absorption peaks of Dy^(3+)ion along with some of the absorption bands of Nd^(3+),Tb^(3+),and Tm^(3+)ions are observed.Under 351 and 447 nm excitation,a prominent emission peak at 572 nm was obtained in all the samples,corresponding to Dy^(3+):^(4)F_(9/2)→^(6)H_(13/2)transition.Here,2 at%Dy^(3+):YAP phosphor exhibits the highest yellow emission intensity under 447 nm pumping.Among the three kinds of Dy^(3+)co-doped phosphors,Dy^(3+)/Tb^(3+):YAP phosphor possesses the dominant yellow emission.The fluorescence decay curves show exponential behaviour and are fitted well.The Commission International de L’Eclairage(CIE)chromaticity coordinates were calculated following the respective emission spectra,and it is found that all the coordinates locate in the yellow region.The energy transfer(ET)processes were investigated and the concentration quenching mechanism was discussed.The obtained results suggest that Dy^(3+)-activated YAP phosphors are good candidates for yellow LED applications.Yingshu Lian Yan Wang Jianfu Li Zhaojie Zhu Zhenyu You Chaoyang Tu Yadong Xu Wanqi Jie 2021Journal of Rare Earths2021,39,8:2
191T@2H-MoSe2 nanosheets directly arrayed on Ti plate: An efficient electrocatalytic electrode for hydrogen evolution reaction显示文摘Jingtong Zhang Yalan Chen Ming Liu Kun Du Yan Zhou Yanpeng Li Zhaojie Wang Jun Zhang 2018Nano Research2018,11,9:2
20An ultrasound-triggered cation chelation and reassembly route to one-dimensional Ni-rich cathode material enabling fast charging and stable cycling of Li-ion batteries显示文摘Ni-rich oxides,LiNixMnyCozO2(NMC),are among leading candidates for cathode materials in Li-ion batteries.However,they are mostly fabricated by coprecipitation approach under complex conditions,which usually produces large secondary particles composed of aggregated primary particles.Undesirable cation mixing and crack propagation upon cycling block ion and electron transport,result in fast capacity fading and poor rate capability.Herein,we present an ultrasound-triggered cation chelation and reassembly route for synthesizing one-dimensional precursor with homogeneous element distribution at the atomic level.This process is accomplished by the synergistic combination of ultrasound and surfactant,which can disperse reactants and remove hydration shells surrounding cations so as to accelerate chelating reaction,and then separate and assemble chelates into one dimensional structure.The whole synthesis time is only 20 min(8.9 min of ultrasonic working time)in an open vessel under natural ambient conditions.One-dimensional LiNi0.6Mn0.2Co0.2O2 has a high reversible capacity(184 mAh·g^−1 at 0.1 C)and long cycling stability(95.1%and 82.4%capacity retention for 100 and 1000 cycles,respectively).The short charging time of 76 s is realized at super high current rate of 20 C,which is very important to improve the competitiveness of electric vehicles relative to fuel vehicles.Our synthetic approach can provide a general strategy for the growth of mixed-metal-EDTA chelate precursors by changing the feeding ratio of Ni2+,Mn2+and Co2+cations in reaction for fabricating NMC cathode materials with other compositions.Yongjian Lai Zhaojie Li Wenxia Zhao Xiaoning Cheng Shuo Xu Xiao Yu Yong Liu 2020Nano Research2020,13,12:2
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