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| 1 | Fermented soybean meal improves the growth performance, nutrient digestibility, and microbial flora in piglets显示文摘In order to increase nutritive values of soybean meal(SBM), 3 species of microbes were used to ferment SBM. Through a 3 x 3 orthogonal design and parameter measurements of soybean peptide and antinutritional factor contents in the fermented soybean meal(FSBM), it was estimated that the best microbial proportion of Bacillus subtilis, Hansenula anomala and Lactobacillus casei was 2:1:2 for SBM fermentation(P < 0.05). The further piglet feeding experiment showed that 10% FSBM substitute for SBM had no significant effect on growth performance of suckling piglets(d 7-28)(P> 0.05). However, newlyweaned piglets(d 28-38) fed 10% FSBM and different levels of plasma protein obtained higher average daily gain(ADG) and feed conversion ratio(FCR), compared with those without FSBM but with 6% plasma protein(P < 0.05). Piglets(d 38-68) fed diets supplemented with FSBM and soybean protein concentrate(SBPC) at 3.75% and 7.5% respectively increased nutrient digestibility,fecal enzyme activity and lactic acid bacteria counts, and decreased fecal Escherichia coli counts(P < 0.05), compared with the control. These data indicated that FSBM had positive effects on nutrient digestibility and fecal microflora for piglets. | Lin Yuan Juan Chang Qingqiang Yin Min Lu Yuanran Di Ping Wang Zhixiang Wang Erzhu Wang Fushan Lu | 2017 | Animal Nutrition2017，，1： | 31 |
| 2 | AMPK activation by peri-sciatic nerve administration of ozone attenuates CCl-induced neuropathic pain in rats显示文摘 | Lijuan Lu Cailong Pan Lu Chen Liang Hu Chaoyu Wang Yuan Han Yanjing Yang Zhixiang Cheng Wen-Tao Liu | 2017 | Journal of Molecular Cell Biology2017，9，2： | 14 |
| 3 | Simulation of hydrological processes of mountainous watersheds in inland river basins: taking the Heihe Mainstream River as an example显示文摘The hydrological processes of mountainous watersheds in inland river basins are complicated.It is absolutely significant to quantify mountainous runoff for social,economic and ecological purposes.This paper takes the mountainous watershed of the Heihe Mainstream River as a study area to simulate the hydrological processes of mountainous watersheds in inland river basins by using the soil and water assessment tool(SWAT)model.SWAT simulation results show that both the Nash–Sutcliffe efficiency and the determination coefficient values of the calibration period(January 1995 to December 2002)and validation period(January 2002 to December 2009)are higher than 0.90,and the percent bias is controlled within±5%,indicating that the simulation results are satisfactory.According to the SWAT performance,we discussed the yearly and monthly variation trends of the mountainous runoff and the runoff components.The results show that from 1996 to 2009,an indistinctive rising trend was observed for the yearly mountainous runoff,which is mainly recharged by lateral flow,and followed by shallow groundwater runoff and surface runoff.The monthly variation demonstrates that the mountainous runoff decreases slightly from May to July,contrary to other months.The mountainous runoff is mainly recharged by shallow groundwater runoff in January,February,and from October to December,by surface runoff in March and April,and by lateral flow from May to September. | ZhenLiang YIN HongLang XIAO SongBing ZOU Rui ZHU ZhiXiang LU YongChao LAN YongPing SHEN | 2014 | Journal of Arid Land2014，6，1： | 7 |
| 4 | Ternary Organic Solar Cells Based on Two Non-fullerene Acceptors with Complimentary Absorption and Balanced Crystallinity显示文摘Summary of main observation and conclusion The ternary blend structure has been demonstrated as an effective approach to increase the power conversion efficiency of organic solar cells.An effective approach to enhance the power conversion efficiency of ternary solar cells is based on two non-fullerene acceptors with complimentary absorption range and balanced crystallinity.In this work,we have introduced a high crystallinity small-molecule acceptor,named C8IDTT-4CI with appropriate alkyl side chains into a low crystalline blend of conjugated polymer donor PBDT-TPD and fused-ring electron acceptor ITIC-4F.A ternary device based on the blend PBDT-TPD:1TIC-4F:C81DTT-4CI exhibits a best power conversion efficiency of 9.51%with a simultaneous improvement of the short-circuit current density to 18.76 mA-cm^-2 and the fill factor up to 67.53%.The absorption onset for C8IDTT-4CI is located at 900 nm,so that the well complementary light absorption is beneficial to the photocurrent.In addition,the existence of high crystallinity C8IDTT-4CI in the ternary device is found helpful to modulate crystallinity,improve heterojunction morphologies and stacking structure,therefore to realize higher charge mobility and better performance. | Lan Xie Chen Yang Ruimin Zhou Zhen Wang Jianqi Zhang Kun Lu Zhixiang Wei | 2020 | Chinese Journal of Chemistry2020，38，9： | 7 |
| 5 | Fluorination-substitution effect on all-small-molecule organic solar cells显示文摘Due to the strong crystallinity and anisotropy of small molecules, matched molecular photoelectric properties and morphologies between small molecules and non-fullerene acceptors are especially important in all-small-molecule organic solar cells(OSCs).Introducing fluorine atoms has been proved as an effective strategy to achieve a high device performance through tuning molecular energy levels, absorption and assembly properties. Herein, we designed a novel benzodithiophene-based small molecule donor BDTF-CA with deep highest occupied molecular orbital(HOMO) energy level. All-small-molecule OSCs were fabricated by combing non-fullerene acceptor IDIC with different fluorine-atom numbers. Two or four fluorine atoms were introduced to the end-capped acceptor of IDIC, which are named as IDIC-2 F and IDIC-4 F, respectively. With the increase of fluorination from IDIC to IDIC-4 F, the open circuit voltage(Voc) of the devices decreased, while hole and electron mobilities of the active layers increased by one order of magnitude. Contributed to the most balanced Voc, short-circuit current(Jsc) and fill factor(FF), the device based on BDTF-CA/IDIC-2 F achieved the highest power conversion efficiency of 9.11%. | Qiong Wu Dan Deng Jianqi Zhang Wenjun Zou Yang Yang Zhen Wang Huan Li Ruimin Zhou Kun Lu Zhixiang Wei | 2019 | Science China Chemistry2019，62，7： | 3 |
| 6 | Combining chlorination and sulfuration strategies for high-performance all-small-molecule organic solar cells显示文摘Three small-molecule donors based on dithieno [2,3-d:2’,3 ’-d’]-benzo[1,2-b:4,5-b’] dithiophene(DTBDT)unit were designed and synthesized by side chain regulation with chlorinated or/and sulfurated substitutions(namely ZR1,ZR1-Cl,and ZR1-S-Cl respectively),along with a crystalline non-fullerene acceptor IDIC-4 Cl with a chlorinated 1,1-dicyanomethylene-3-indanone(IC) end group.Energy levels,molar extinction coefficients and crystallinities of three donor molecules can be effectively altered by combining chlorination and sulfuration strategies.Especially,the ZR1-S-Cl exhibited the best absorption ability,lowest higher occupied molecular orbital(HOMO) energy level and highest crystallinity among three donors,resulting in the corresponding all-small-molecule organic solar cells to produce a high power conversion efficiency(PCE) of 12.05% with IDIC-4 Cl as an acceptor. | Ruimin Zhou Chen Yang Wenjun Zou Muhammad Abdullah Adil Huan Li Min Lv Ziyun Huang Menglan Lv Jianqi Zhang Kun Lu Zhixiang Wei | 2021 | Journal of Energy Chemistry2021，30，1： | 3 |
| 7 | Driving Force and Ecosystem Service Values Estimation in the Extreme Arid Region from 1975 to 2015:A Case Study of Alxa League,China显示文摘The research on ecosystem service values(ESVs)estimation in arid region is weak.We took the Alxa League of China’s Inner Mongolia Autonomous Region,an extreme arid region,as an example and constructed an equivalent coefficient method to assess its ESVs from 1975 to 2015,by determining the standard unit of ESVs and the basic equivalent of the value of different ecosystem services per unit area based on the regional characteristics,literature research,expert knowledge and land use data.The results show that the ESVs first decreased from 83170.4 million yuan(RMB)in 1975 to 82337.8 million yuan(RMB)in 2000 and then increased to84033.6 million yuan(RMB)in 2015,and the ESV of sparse grassland and desert account for about 33%and 29%of the total ESVs,respectively.Among the four service types,the regulating services,support services,supply services and cultural services account for66.5%,22.8%,6.0%and 4.7%,respectively.The changes of ESVs in Alxa League are determined by the socio-economic development and ecological changes.This study provides a new method to estimate the ESVs in arid region by integrating existing methods and regional characteristics,such as the cost of water for arid ecosystems. | XIE Jiali LU Zhixiang XIAO Shengchun YAN Changzhen | 2021 | Chinese Geographical Science2021，31，6： | 3 |
| 8 | The heterogeneity of hydrometeorological changes during the period of 1961-2016 in the source region of the Yellow River, China显示文摘Runoff in the source region of a river makes up most of water resources in the whole basin in arid and semi-arid areas. It is very important for water resources management to timely master the latest dynamic changes of the runoff and quantitatively reveal its main driving factors. This paper aims to discover the variation heterogeneity of runoff and the impacts of climatic factors on this runoff in the source region of the Yellow River(SRYR) in China from 1961 to 2016. We divided SRYR into four sub-regions, and analyzed changes of their contributions to total runoff in SRYR. We also revealed the impacts of precipitation, temperature and potential evapotranspiration on runoff in each sub-region by constructing the regression relationships between them at multiple temporal scales. The changes of runoff in the four sub-regions and their contributions to the total runoff were not exactly consistent. The climatic variables’ changes also have heterogeneity, and runoff was mainly affected by precipitation compared to influences of temperature or potential evapotranspiration. Their impacts on runoff have spatiotemporal heterogeneity and can be reflected by very significant-linear regression equations.It provided a simple method to predict headwater runoff for better water management in the whole basin. | ZhiXiang Lu Qi Feng SongBing Zou JiaLi Xie ZhenLiang Yin Fang Li | 2020 | Research in Cold and Arid Regions2020，12，2： | 3 |
| 9 | Self-assembly of conjugated polymers for anisotropic nanostructures显示文摘As their potential applications in various electronic devices increase, the preparation of anisotropic conjugated polymer nanostructures are highly desirable. This paper presents a review of the literature and our recent results on the self-assembly of one-, two- and three-dimensional anisotropic nanostructures using conjugated polymers as building blocks, including the formation of one-dimensional (1D) nanofibers and nanotubes, two-dimensional (2D) nanoribbons and nanosheets, and three-dimensional (3D) superstructures. The mechanisms guiding the formation of various nanostructures are analyzed by a cooperative effect of - stacking interaction and other noncovalent interactions. | YU Zai LU Kun WEI ZhiXiang | 2012 | Science China Chemistry2012，55，11： | 3 |
| 10 | A-π-D-π-A small-molecule donors with different end alkyl chains obtain different morphologies in organic solar cells显示文摘For bulk-heterojunction organic solar cells, the morphology of the blend films highly influence the exciton dissociation and charge transport process. In this work, two novel A-π-D-π-A(A represents the acceptor unit and D represents the donor unit) backbone structure small molecular electron donors based on two dimensional conjugated naphtho[1,2-b:5,6-b']dithiophene(NDT) with different end alkyl chains, named as NDT-3T-EH and NDT-3T-O, have been designed and synthesized. The photovoltaic property of NDT-3T-O-based device is better than that of the NDT-3T-EH and the best efficiency reaches 7.06%, and the photovoltaic property of NDT-3T-EH reaches 6.11%. The difference in the performance should be attributed to the different morphology and phase separation resulted from the different crystallinity and aggregation ability of two donors. The results demonstrate that the optimized end alkyl chains can be used to design A-π-D-π-A backbone structure small molecular electron donors for smallmolecule organic solar cells. | Yanan Shi Chen Yang Huan Li Lixuan Liu Ruimin Zhou Wenjun Zou Zhen Wang Qiong Wu Dan Deng Jianqi Zhang Kun Lu Zhixiang Wei | 2019 | Chinese Chemical Letters2019，30，4： | 3 |
| 11 | Surgical Management and Prognostic Factors of Hilar Cholangiocarcinoma: Experience with 115 Cases in China显示文摘 | Liu Yubin PhD Fang Chihua PhD Jian Zhixiang MM Ou Jinrui BA Liu Zixian BA Zheng Jianghua BA Lin Ye MD Jin Haosheng MD Lu Chaomin PhD | 2008 | Annals of Surgical Oncology2008，，8： | 2 |
| 12 | Connecting Calcium-Based Nanomaterials and Cancer:From Diagnosis to Therapy显示文摘As the indispensable second cellular messenger,calcium signaling is involved in the regulation of almost all physiological processes by activating specific target proteins.The importance of calcium ions(Ca^(2+))makes its“Janus nature”strictly regulated by its concentration.Abnormal regulation of calcium signals may cause some diseases;however,artificial regulation of calcium homeostasis in local lesions may also play a therapeutic role.“Calcium overload,”for example,is characterized by excessive enrichment of intracellular Ca^(2+),which irreversibly switches calcium signaling from“positive regulation”to“reverse destruction,”leading to cell death.However,this undesirable death could be defined as“calcicoptosis”to offer a novel approach for cancer treatment.Indeed,Ca^(2+)is involved in various cancer diagnostic and therapeutic events,including calcium overload-induced calcium homeostasis disorder,calcium channels dysregulation,mitochondrial dysfunction,calcium-associated immunoregulation,cell/vascular/tumor calcification,and calcification-mediated CT imaging.In paral-lel,the development of multifunctional calcium-based nanomaterials(e.g.,calcium phosphate,calcium carbonate,calcium peroxide,and hydroxyapatite)is becoming abundantly available.This review will highlight the latest insights of the calcium-based nanomaterials,explain their application,and provide novel perspective.Identifying and characterizing new patterns of calcium-dependent signaling and exploiting the disease element linkage offer additional translational opportunities for cancer theranostics. | Shuang Bai Yulu Lan Shiying Fu Hongwei Cheng Zhixiang Lu Gang Liu | 2022 | Nano-Micro Letters2022，14，9： | 2 |
| 13 | Elicitor hydrophobin Hyd1 interacts with Ubiquilin1-like to induce maize systemic resistance显示文摘Trichoderma harzianum is a plant-beneficial fungus that secretes small cysteine-rich proteins that induce plant defense responses;however, the molecular mechanism involved in this induction is largely unknown.Here, we report that the class Ⅱ hydrophobin Th Hyd1 acts as an elicitor of induced systemic resistance(ISR) in plants. Immunogold labeling and immunofluorescence revealed Th Hyd1 localized on maize(Zea mays) root cell plasma membranes. To identify host plant protein interactors of Hyd1, we screened a maize B73 root c DNA library. Th Hyd1 interacted directly with ubiquilin1-like(UBL). Furthermore, the N-terminal fragment of UBL was primarily responsible for binding with Hyd1 and the eight-cysteine amino acid of Hyd1 participated in the protein-protein interactions. Hyd1 from T. harzianum(Thhyd1) and ubl from maize were co-expressed in Arabidopsis thaliana, they synergistically promoted plant resistance against Botrytis cinerea. RNA-sequencing analysis of global gene expression in maize leaves 24 h after spraying with Curvularia lunata spore suspension showed that Thhyd1-induced systemic resistance was primarily associated with brassinosteroid signaling, likely mediated through BAK1. Jasmonate/ethylene(JA/ET)signaling was also involved to some extent in this response. Our results suggest that the Hyd1-UBL axis might play a key role in inducing systemic resistance as a result of Trichoderma-plant interactions. | Chuanjin Yu Kai Dou Shaoqing Wang Qiong Wu Mi Ni Tailong Zhang Zhixiang Lu Jun Tang Jie Chen | 2020 | Journal of Integrative Plant Biology2020，62，4： | 1 |
| 14 | Evaluation of groundwater sustainability based on groundwater age simulation in the Zhangye Basin of Heihe River watershed, northwestern China显示文摘Water resources, as the primary limiting factor, constrain the economic and social development in arid inland areas. The Zhangye Basin is a representative area of inland river basins, which is located in the middle parts of the Heihe River watershed, northwestern China. Facing with the huge water shortage, people exploited ground- water at a large scale in recent years. The reducing recharge from surface water and over-exploitation of ground- water led to the decline of groundwater levels and threatened the sustainability of water resources. This study con- structed a conceptual and numerical groundwater flow model and calibrated the model based on the observed wells. A solute transport model was built using MT3DMS to calculate the groundwater age distribution in the Zhangye Basin. The simulated result shows that the youngest groundwater is distributed near the most upstream areas in the model domain, which is less than 1,000 a, older groundwater is distributed in deeper parts of the aquifer and near the discharge outlets, ranging from 6,000 a to over 20,000 a. Spatial variation of groundwater ages in the middle area indicates the recharge diversity between unconfined and confined aquifer. Groundwater age can serve as an indicator to evaluate groundwater's renewal capacity and sustainability. The formation of groundwater resources in the lower stream area would spend 10,000 a or even more than 20,000 a, so exploitation of groundwater in these areas should be restrained. | Heng WEI HongLang XIAO ZhenLiang YIN ZhiXiang LU | 2014 | Journal of Arid Land2014，6，3： | 1 |
| 15 | Triggering the biocontrol of Botrytis cinerea by Trichoderma harzianum through inhibition of pathogenicity and virulence related proteins显示文摘This study reports a strain of Trichoderma harzianum CCTCC-SBW0162 with potential to enhance biocontrol activity against gray mold pathogen, Botrytis cinerea, and with a pivotal role in tomato(Solanum esculentum) plant growth enhancement. A total of 254 Trichoderma isolates were screened by in vitro antagonistic assay. Of these, 10 were selected for greenhouse experiments based on their greater inhibition of B. cinerea.The in vitro antagonistic assay and greenhouse experiments indicated that T. harzianum CCTCC-SBW0162 gave the highest inhibition rate(90.6%) and disease reduction(80.7%). Also, to study the possible mechanism associated with antifungal activity of CCTCC-SBW0162 against B. cinerea, molecular docking was used to assess the interactions between CCTCC-SBW0162-derived metabolites, and pathogencity and virulence related proteins of B. cinerea. The molecular docking results indicated that the combination of harzianopyridone,harzianolide and anthraquinone C derived from CCTCCSBW0162 could synergistically improve antifungal activity against B. cinerea through the inhibition/modification of pathogenicity and virulence related proteins.However, this computerized modeling work emphasized the need for further study in the laboratory to confirm the effect T. harzianum-derived metabolites against the proteins of B. cinerea and their interactions. | Kandasamy SARAVANAKUMAR Zhixiang LU Hai XIA Meng WANG Jianan SUN Shaoqing WANG Qiang-qiang WANG Yaqian LI Jie CHEN | 2018 | Frontiers of Agricultural Science and Engineering2018，5，2： | 1 |
| 16 | Seven new 3,4-dihydro-furanocoumarin derivatives from Angelica dahurica显示文摘Objective:To study the chemical constituents of the roots of Angelica dahurica,a well-known Chinese herbal medicine named Baizhi in Chinese.Methods:Compounds were separated by various chromatographies,and the structures of new compounds were elucidated based on the analysis of their spectroscopic and spectrometric data(1D,2D NMR,HRESI MS,IR,and UV).The absolute configurations of new compounds were determined by the calculated electronic circular dichroism and chemical derivatization.The inhibitory activities of all isolates against nitric oxide(NO)production were evaluated using lipopolysaccharide-activated RAW 264.7macrophage cells.Results:Seven new 3,4-dihydro-furanocoumarin derivatives(1a/1b,2a/2b,3a/3b,4)together with a known furanocoumarin(5)were isolated from the roots of A.dahurica.The new compounds included three pairs of enantiomers,(4S,2’’R)-angelicadin A(1a)/(4R,2’’S)-angelicadin A(1b),(4S,2’’S)-angelicadin A(2a)/(4R,2’’R)-angelicadin A(2b),and(4S,2’’S)-secoangelicadin A(3a)/(4R,2’’R)-secoangelicadin A(3b),together with(4R,2’’R)-secoangelicadin A methyl ester(4).The known xanthotoxol(5)inhibited the NO production with the half-maximal inhibitory concentration(IC50)value of(32.8±0.8)μmol/L,but all the new compounds showed no inhibitory activities at the concentration of100μmol/L.Conclusion:This is the first report of the discovery of 3,4-dihydro-furanocoumarins from A.dahurica.The results are not only meaningful for the understanding of the chemical constituents of A.dahurica,but also enrich the reservoir of natural products. | Yang Wang Fanyu Shi Zihan Lu Mingliang Zhang Zekun Zhang Fangfang Jia Beibei Zhang Lishan Ouyang Zhixiang Zhu Shepo Shi | 2023 | Chinese Herbal Medicines2023，15，3： | 1 |
| 17 | In situ performance and stability tests of large-area flexible polymer solar cells in the 35-km stratospheric environment显示文摘Flexible organic solar cells(FOSCs)are one of the most promising power sources for aerospace aircraft due to their atractive advantages with high power-per-weight ratio and excellent mechanical flexibility.Understanding the performance and stability of high-performance FOSCs is essential for the further development of FOSCs for aerospace applications.In this paper,after systematic investigations on the performance of the state-of-the-art high-performance solar cells under thermal cycle and intensive UV irradiation conditions,in situ performance and stability tests of the solar cells in the 35 km stratospheric environment were carried out through a high-altitude balloon uploading.The encapsulated FOSCs with an area of 0.64 cm^(2)gave the highest power density of 15.26 mW/cm^(2)and an efficiency over 11%,corresponding to a power-per-weight ratio of over 3.32 k W/kg.More importantly,the cells showed stable power output during the 3-h continuous flight at 35 km and only 10%performance decay after return to the lab,suggesting promising stability of the FOSCs in the stratospheric environment. | Zihan Xu Guoning Xu Qun Luo Yunfei Han Yu Tang Ying Miao Yongxiang Li Jian Qin Jingbo Guo Wusong Zha Chao Gong Kun Lu Jianqi Zhang Zhixiang Wei Rong Cai Yanchu Yang Zhaojie Li Chang-Qi Ma | 2023 | National Science Review2023，10，4： | 0 |
| 18 | The role of central ion in chiral recognition by taking phenylalanine as an example显示文摘Chiral recognition of phenylalanine(Phe) was achieved in the gas phase by electrospray ionization Q-TOF tandem mass spectrometry.In this method,two central ions,i.e.proton and divalent copper,were used and chiral crown ether,(+)-2,3,11,12-tetracarboxylic acid-18-crown-6(18-C-6-TCA),was used as a chiral host.Dimeric complexes were readily formed by electrospray ionization of a methanol/water(50/50,V/V) solution containing central ions,Phe and 18-C-6-TCA.The dimeric complex included proton-bound(18-C-6-TCA)(Phe)H+ and copper-bound deprotonated [Cu2+(18-C-6-TCA)(Phe)-H]+ ions were mass selected and then collided with Ar in the CID experiments.The chiral recognition capability of these complexes was evaluated using the relative abundance of daughter ion to parent ion.A higher degree of chiral recognition ability was observed with Cu2+ compared to that of H+.Different central ions exhibited distinctive dissociation pathways and unique chiral recognition characteristics.The chiral recognition mechanism was also discussed in detail with the help of the structure of copper-bound complex predicted by theoretical calculation. | YU Qing CAO Jie LU Gang WANG ZhiXiang | 2009 | Science China Chemistry2009，52，8： | 0 |
| 19 | Single-bond-linked oligomeric donors for high performance organic solar cells显示文摘The effective design and synthesis of novel small-molecule donors(SMDs) is extremely essential for the in-depth study of the scientific problems of bulk heterojunction morphology and the improvement of photovoltaic performance in organic solar cells(OSCs). Importantly, developing a series of donors with different conjugated central donor(D) units is a remarkable strategy to obtain high-performance donors. Herein, two acceptor-donor-donor-acceptor(A-D-D-A) type oligomeric donors 2DTBDT and2DTBDT-2T with two dithieno[2,3-d:2,3-d’]benzo[1,2-b:4,5-b’]dithiophene(DTBDT) as D units, without and with bithiophene as the π bridge respectively are designed and synthesized successfully. The central linked-DTBDT unit can provide a larger conjugated plane and promote π electron delocalization, which can effectively improve π-π interactions between donors and regulate the crystallinity. And we found that the π bridge provided 2DTBDT-2T with 12.31% efficiency that is already a high efficiency in OSCs,whereas 2DTBDT with merely 3.63% efficiency, both with 2,2-((2Z,2 Z)-((12,13-bis(2-ethylhexyl)-3,9-diundecyl-12,13-dihydro-[1,2,5]thiadiazolo[3,4-e]thieno[2,'3 ’:4,5 ]thieno[2,3 :4,5]pyrrolo[3,2-g]thieno-[2,3 :4,5]thieno[3,2-b]indole,10-diyl)bis(methanylylidene))bis(5,6-difluoro-3-oxo-2,3-dihydro-1H-indene-2,1-diylidene)) dimalononitrile(Y6) as the acceptor. We conjecture that the main reason for the different device performance may be ascribed to the different molecular stacking orientation of the oligomeric donors and morphology features of the donors:Y6 blend films. Compared to the predominant face-on orientation of the 2DTBDT neat film, the 2DTBDT-2T neat film performed a preferential edge-on orientation, which obtained a smoother surface, stronger crystallinity and more uniform phase separation in the 2DTBDT-2T:Y6 blend films with nanofiber structure, which delivered higher and more balanced carrier mobilities, the more efficient exciton dissociation and reduced biomolecule recombination, therefore obtaining better power conversion efficiencies(PCEs). We speculate that the transformation of molecular stacking orientation of oligomeric donors is possibly due to that π bridge extended and twisted the molecular structure of 2DTDBT-2T, resulting in an edge-on orientation relative to the substrate. These findings demonstrate that the single-bond-linked donor strategy is an alternative method to design the donors towards high-performance OSCs. | Min Lv Yi Tang Dingding Qiu Wenjun Zou Ruimin Zhou Lixuan Liu Ziyun Huang Jianqi Zhang Kun Lu Zhixiang Wei | 2023 | Chinese Chemical Letters2023，34，2： | 0 |
| 20 | Investigation on interfacial and electrical properties of Ge MOS capacitor with different NH_3-plasma treatment procedure显示文摘The effects of different NH_3-plasma treatment procedures on interfacial and electrical properties of Ge MOS capacitors with stacked gate dielectric of HfTiON/TaON were investigated.The NH3-plasma treatment was performed at different steps during fabrication of the stacked gate dielectric,i.e.before or after interlayer(TaON)deposition,or after deposition of high-k dielectric(HfTiON).It was found that the excellent interface quality with an interface-state density of 4.79×10^(11) eV^(-1) cm^(-2) and low gate leakage current(3.43 × 10^(-5) A/cm^2 at V_g = 1 V)could be achieved for the sample with NH_3-plasma treatment directly on the Ge surface before TaON deposition.The involved mechanisms are attributed to the fact that the NH_3-plasma can directly react with the Ge surface to form more Ge-N bonds,i.e.more GeO_xN_y,which effectively blocks the inter-diffusion of elements and suppresses the formation of unstable GeO_x interfacial layer,and also passivates oxygen vacancies and dangling bonds near/at the interface due to more N incorporation and decomposed H atoms from the NH_3-plasma. | Xiaoyu Liu Jingping Xu Lu Liu Zhixiang Cheng Yong Huang Jingkang Gong | 2017 | Journal of Semiconductors2017，38，8： | 0 |
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