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| 1 | The FGOALS climate system model as a modeling tool for supporting climate sciences:An overview显示文摘Climate system models are useful tools for understanding the interactions among the components of the climate system and predicting/projecting future climate change. The development of climate models has been a central focus of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences(LASG/IAP) since the establishment of the laboratory in 1985. In China, many pioneering component models and fully coupled models of the climate system have been developed by LASG/IAP. The fully coupled climate system developed in the recent decade is named FGOALS(Flexible Global Ocean-Atmosphere-Land System Model). In this paper, an application-oriented review of the LASG/IAP FGOALS model is presented. The improved model performances are demonstrated in the context of cloud-radiation processes, Asian monsoon, ENSO phenomena, Atlantic Meridional Overturning Circulation(AMOC) and sea ice. The FGOALS model has contributed to both CMIP5(Coupled Model Intercomparison Project-phase 5) and IPCC(Intergovernmental Panel on Climate Change) AR5(the Fifth Assessment Report). The release of FGOALS data has supported the publication of nearly 500 papers around the world. The results of FGOALS are cited ~106 times in the IPCC WG1(Working Group 1) AR5. In addition to the traditional long-term simulations and projections, near-term decadal climate prediction is a new set of CMIP experiment, progress of LAGS/IAP in the development of nearterm decadal prediction system is reviewed. The FGOALS model has supported many Chinese national-level research projects and contributed to the national climate change assessment report. The crucial role of FGOALS as a modeling tool for supporting climate sciences is highlighted by demonstrating the model's performances in the simulation of the evolution of Earth's climate from the past to the future. | TianJun Zhou Bin Wang YongQiang Yu YiMin Liu WeiPeng Zheng LiJuan Li Bo Wu PengFei Lin Zhun Guo WenMin Man Qing Bao AnMin Duan HaiLong Liu XiaoLong Chen Bian He JianDong Li LiWei Zou XiaoCong Wang LiXia Zhang Yong Sun WenXia Zhang | 2018 | Earth and Planetary Physics2018，2，4： | 6 |
| 2 | A single Au nanoparticle anchored inside the porous shell of periodic mesoporous organosilica hollow spheres显示文摘理想的金属催化剂对沥滤或粒子凝块与反应试剂,很多暴露的活跃地点,和高稳定性要求容易的接触。抛锚尽管几乎没报导,在多孔的壳内的一个金属核心可以由于常规支持的金属安排的集成把这些优点合为 core@void@shell 体系结构。然而,完成这由于弱 coreshell 亲密关系是极其困难的。此处,第一次,我们报导一条途径由增加核心壳相互作用克服这挑战。在这方面,我们综合了一个单个 Au 核心是的新奇 Au@void@periodic mesoporous organosilica (PMO ) 在体系结构坚定地在空 PMO 范围的多孔的壳内抛锚了。在之间的非共有原子价相互作用(vinylpyrrolidone )(PVP ) poly,一些 functionalized Au 和 PMO 的乙烷一半向多孔的壳便于 Au 核心的运动在期间 Au@SiO2@PMO 的选择碱的蚀刻。抛锚壳的 Au 核心以与活跃地点的试剂和暴露的接触比在常规 Au@void@PMO 的推迟的核心优异,并且因此为 4-nitrophenol 减小显示出更高催化的效率。这里表明的方法论提供新卓见因为有核心的万用的多功能的 nanostructures 的制造在空壳内抛锚了。 | Ying Yang Wen Zhang Ying Zhang Anmin Zheng Hui Sun Xinsong Li Suyan Liu Pengfang Zhang Xin Zhang | 2015 | Nano Research2015，8，10： | 3 |
| 3 | Identification of miRNomes in Human Liver and Hepatocellular Carcinoma Reveals miR-199a/b-3p as Therapeutic Target for Hepatocellular Carcinoma显示文摘 | Jin Hou Li Lin Weiping Zhou Zhengxin Wang Guoshan Ding Qiongzhu Dong Lunxiu Qin Xiaobing Wu Yuanyuan Zheng Yun Yang Wei Tian Qian Zhang Chunmei Wang Qinghua Zhang Shi-Mei Zhuang Limin Zheng Anmin Liang Wenzhao Tao Xuetao Cao | 2011 | Cancer Cell2011，，2： | 3 |
| 4 | High population and dispersion of pentacoordinated Al~Ⅴ species on the surface of ?ame-made amorphous silica-alumina显示文摘Pentacoordinated Al(Al~Ⅴ)species in silica-alumina are promising to promote the formation of acid sites or act as surface defects for tailoring single-atom catalysts.However,pentahedral coordination(Al~Ⅴ)is rarely observed in conventionally prepared silica-alumina.Here,we show that high population and dispersion of Al~Ⅴ species on the surface of amorphous silica-alumina(ASA)can be achieved by means of flame spray pyrolysis.High resolution TEM/EDX,high magnetic-field NMR and DFT calculations are employed to characterize the structure of as-prepared ASAs.Solid-state ^(27)Al multi-quantum MAS NMR experiments show that most of the Al~Ⅴspecies are formed independently from the alumina phase and are accessible for guest molecules on the surface.Upon water adsorption,these Al~Ⅴ species are transformed to Al~Ⅵ species,structurally similar to surface Al~Ⅳ species,as confirmed by DFT calculations.The outstanding catalytic activity of as-synthesized ASA is demonstrated using the in situ H/D exchange reaction with deuterated benzene as an example.The Al~Ⅴ-rich ASA provides a much lower activation energy(~30 kJ/mol)than that reported for zeolite H-ZSM-5(~60 kJ/mol).The superior catalytic performance is attributed to the high Al~Ⅴcontent promoting the surface active sites in ASA.The knowledge gained on the synthesis of Al~Ⅴ-rich ASAs and the nature of aluminum coordination in these materials could pave the way to more efficient silica-alumina based catalysts. | Zichun Wang Yijiao Jiang Xianfeng Yi Cuifeng Zhou Aditya Rawal James Hook Zongwen Liu Feng Deng Anmin Zheng Michael Hunger Alfons Baiker Jun Huang | 2019 | Science Bulletin2019，64，8： | 2 |
| 5 | Coalfield structure and structural controls on coal in China显示文摘The occurrence of coal-bearing strata in a variety of coal-bearing basins of China is characterized by late tectonic deformation and remarkable spatial and geochronologic differences.The main controlling factors,which determine the tectonic framework of coalfields,include the geodynamic environment,tectonic evolution,deep structures,tectonic stress,and lithologic combination of the coal measures.The Chinese continent has experienced multi-stage tectonic movements since the Late Paleozoic.The spatial and temporal heterogeneity of its continental tectonic evolution,the complexity of its basement properties,and its stratigraphic configurations control the tectonic framework of its coalfields’present complex and orderly patterns.The concept of coal occurrence structural units is proposed in this paper and is defined as the structural zoning of coal occurrence.China’s coalfields are divided into five coal occurrence structural areas,and the structural characteristics of the coalfields in five main coal occurrence areas throughout the country are summarized.Based on the analysis of the relationship between the structure characteristics and occurrence of coal in these coalfields,the coal-controlling structures are divided into six groups:extensional structural styles,compressional structural styles,shearing and rotational structural styles,inverted structural styles,sliding structural styles,and syn-depositional structural styles.In addition,the distribution of coal-controlling structural styles is briefly summarized in this paper. | Daiyong Cao Anmin Wang Shuzheng Ning Huantong Li Aijun Guo Limin Chen Kang Liu Jieqing Tan Zhihong Zheng | 2020 | International Journal of Coal Science & Technology2020，7，2： | 2 |
| 6 | Bronsted/Lewis acid synergy in dealuminated HY zeolite: A combined solid - state NMR and theoretical calculation study 显示文摘 | Li Shenhui Zheng Anmin Su Yongchao | 2007 | J AM Chem Soc2007，129，11： | 1 |
| 7 | Identification of miRNomes in Human Liver and Hepatocellular Carcinoma Reveals miR-199a/b-3p as Therapeutic Target for Hepatocellular Carcinoma显示文摘 | Jin Hou Li Lin Weiping Zhou Zhengxin Wang Guoshan Ding Qiongzhu Dong Lunxiu Qin Xiaobing Wu Yuanyuan Zheng Yun Yang Wei Tian Qian Zhang Chunmei Wang Qinghua Zhang Shi-Mei Zhuang Limin Zheng Anmin Liang Wenzhao Tao Xuetao Cao | 2011 | Cancer Cell2011，，2： | 1 |
| 8 | Bronsted/Lewis acid synergy in dealuminated HY zeolite: a combined solid-state NMR and theoretical calculation study 显示文摘 | Li Shenhui Zheng Anmin | 2007 | J Am Chem Soc2007，129，11： | 1 |
| 9 | Boron environments in B doped and (B, N) codoped TiO2 pho- tocatalysts: a combined solid-state NMR and theoretical calculation study 显示文摘 | FENG Ning Dong ZHENG Anmin WANG Qiang | 2011 | J Phys Chem C2011，115，6： | 1 |
| 10 | Boron environments in B-doped and ( B, N) -codoped TiO2 photo- catalysts: a combined solid-state NMR and theoretical calculation study 显示文摘 | Feng Ningdong Zheng Anmin Wang Qiang | 2011 | J Journal of Physical Chemistry C2011，115，： | 1 |
| 11 | ^31P chemical shift of adsorbed trialkylphosphine oxides for acidity characterization of solid acids catalysts 显示文摘 | ZHENG Anmin HUANG Shingjong CHEN Wenhua | 2008 | J Phys Chem A2008，112，： | 1 |
| 12 | Understanding the high photocatalytic activity of (B, Ag)-co- doped TiO2 under solar-light irradiation with XPS, solid-state NMR, and DFT calculations 显示文摘 | FENG Ningdong WANG Qiang ZHENG Anmin | 2013 | J Am Chem Soc2013，135，4： | 1 |
| 13 | Combined DFT theoretical calculation and solid-state NMR studies of A1 substitution and acid sites in zeolite MCM-22显示文摘 | Anmin Zheng Lei Chen Jun Yang | 2005 | J Phys Chem B2005，109，24： | 1 |
| 14 | Functional groups to modify g-C3N4 for improved photocatalytic activity of hydrogen evolution from water splitting显示文摘Rational modification by functional groups was regarded as one of efficient methods to improve the photocatalytic performance of graphitic carbon nitride(g-C3 N4).Herein,g-C3 N4 with yellow(Y-GCN)and brown(C-GCN)were prepared by using the fresh urea and the urea kept for five years,respectively,for the first time.Experimental results show that the H2 production rate of the C-GCN is 39.06μmol/h,which is about 5 times of the Y-GCN.Meantime,in terms of apparent quantum efficiency(AQ.E)at 420 nm,C-GCN has a value of 6.3%and nearly 7.3 times higher than that of Y-GCN(0.86%).The results of XRD,IR,DRS,and NMR show,different from Y-GCN,a new kind of functional group of—N=CH—was firstly in-situ introduced into the C-GCN,resulting in good visible light absorption,and then markedly improving the photocatalytic performance.DFT calculation also confirms the effect of the—N=CH—group band structure of g-C3N4.Furthermore,XPS results demonstrate that the existence of—N=CH—groups in C-GCN results in tight interaction between C-GCN and Pt nanoparticles,and then improves the charge separation and photocatalytic performance.The present work demonstrates a good example of'defect engineering'to modify the intrinsic molecular structure of g-C3N4 and provides a new avenue to enhance the photocatalytic activity of g-C3N4 via facile and environmental-friendly method. | Fan Yu Laichun Wang Qiuju Xing Dengke Wang Xunheng Jiang Guangchao Li Anmin Zheng Fanrong Ai Jian-Ping Zou | 2020 | Chinese Chemical Letters2020，31，6： | 1 |
| 15 | Relationship between 1H chemical shifts of deuterated pyridinium ions and Bronsted acid strength of solid acids显示文摘 | Anmin Zheng Lei Chen Jun Yang | 2007 | J Phys Chem B2007，111，12： | 1 |
| 16 | Phosphotungstic acid loaded on hydrophilic ionic liquid modified SBA-15 for selective oxidation of alcohols with aqueous H 2 O 2显示文摘 | Rong Tan Cheng Liu Ningdong Feng Jun Xiao Weiguo Zheng Anmin Zheng Donghong Yin | 2012 | Microporous and Mesoporous Materials2012，，： | 1 |
| 17 | Design and synthesis of hydrophobic and stable mesoporous polymeric solid acid with ultra strong acid strength and excellent catalytic activities for biomass transformation显示文摘 | Fujian Liu Anmin Zheng Iman Noshadi Feng-Shou Xiao | 2013 | Applied Catalysis B: Environmental2013，，： | 1 |
| 18 | Theoretical investigation of the effects of the zeolite framework on the stability of carbenium ions显示文摘 | FANG Hanjun ZHENG Anmin XU Jun | 2011 | J Phys ChemC2011，115，15： | 1 |
| 19 | Synthesis and memory characteristics of polyimides containing noncoplanar aryl pendant groups显示文摘 | Yueqin Li Yueying Chu Runchen Fang Shijin Ding Yulong Wang Yingzhong Shen Anmin Zheng | 2011 | Polymer2011，，1： | 1 |
| 20 | Rational construction of multiple hollow silicalite-1 zeolite with enhanced quasi acidity for robust vapor-phase Beckmann rearrangement显示文摘Developing efficient and stable zeolites for vapor-phase Beckmann rearrangement of cyclohexanone oxime is still a great challenge to realizeε-caprolactam(CPL)green production.In this work,the hierarchical porous silicalite-1 zeolites with multiple hollow structure(S-1-M)are explored by in-situ desilication−recrystallization post-treatment of spongy highway-like zeolites(S-1-S),which are synthesized through silanization synthesis of conventional bulky silicalite-1(S-1).Compared to S-1,S-1-M achieves superior catalytic performance,with improving the CPL selectivity from 85.7%to 94.1%and prolonging the catalyst lifetime from 74 to 126 h at a weight hourly space velocity(WHSV)of 6 h^(−1).Comprehensive physiochemical studies demonstrate that the highly dispersed intracrystalline cavities within S-1-M endow greater mass diffusion and better quasi acidity inducing by the enhanced H-bonds among abundant H-bonded silanols,which is cooperatively responsible for its superior catalytic performance. | Peng Zhang Xianfeng Yi Changjiu Xia Xinxin Peng Shuai Zhang Chengxiang Li Anmin Zheng Xiaoxin Zhang Yibin Luo Lifeng Cui Fuhong Yu Xingtian Shu | 2023 | Nano Research2023，16，5： | 1 |
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