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| 1 | Nanocluster PtNiP supported on graphene as an efficient electrocatalyst for methanol oxidation reaction显示文摘In this study,phosphorus doped graphene supported PtNiP nanocluster electrocatalyst(PtNiP/P-graphene)was successfully prepared via a simple hypophosphite-assisted co-reduction method.The improved anchoring force and increased anchoring sites of graphene support result from phosphorus doping as well as size-confined growth effect of NaH_(2)PO_(2) leads to uniform dispersion of ultrafine PtNiP nanoclusters.Doped P also promotes the removal of CO-like intermediate by adjusting Pt electronic structure combining with alloyed Ni via electronic effects.As a result,the as-prepared PtNiP/P-graphene catalyst with more exposed active sites and optimized electronic structure of Pt alloy shows excellent electrocatalytic performances for methanol oxidation reaction(MOR)both in activity and durability in an acidic medium. | Long Yang Guoqiang Li Rongpeng Ma Shuai Hou Jinfa Chang Mingbo Ruan Wenbin Cai Zhao Jin Weilin Xu Guiling Wang Junjie Ge Changpeng Liu Wei Xing | 2021 | Nano Research2021，14，8： | 4 |
| 2 | Real contribution of formic acid in direct formic acid fuel cell: Investigation of origin and guiding for micro structure design显示文摘 | Weiwei Cai Liang Liang Yuwei Zhang Wei Xing Changpeng Liu | 2013 | International Journal of Hydrogen Energy2013，，1： | 1 |
| 3 | Direct electrochemistry behavior of Cytochrome c on silicon dioxide nanoparticles-modified electrode显示文摘A newfangled direct electrochemistry behavior of Cytochrome c (Cyt c) was found on glassy carbon (GC) electrode modified with the silicon dioxide (SiO2) nanoparticles by physical adsorption. A pair of stable and well-defined redox peaks of Cyt c′ quasi-reversible electrochemical reaction were obtained with a heterogeneous electron transfer rate constant of 1.66×10-3 cm/s and a formal potential of 0.069 V (vs. Ag/AgCl) (0.263 V versus NHE) in 0.1 mol/L pH 6.8 PBS. Both the size and the amount of SiO2 nanoparticles could influence the electron transfer between Cyt c and the electrode. Electrostatic interaction which is between the negative nanoparticle surface and positively charged amino acid residues on the Cyt c surface is of importance for the stability and reproducibility toward the direct electron transfer of Cyt c. It is suggested that the modification of SiO2 nanoparticles proposes a novel approach to realize the direct electrochemistry of proteins. | ZHU Lin SUN DongMei LU TianHong CAI ChenXin LIU ChangPeng XING Wei | 2007 | Science China Chemistry2007，50，3： | 1 |
| 4 | Vector deflection stability control of aero-engine based on linear active disturbance rejection显示文摘Aimed at the problem of instability in engine control caused by vector deflection in experiment of turbofan engines with Axisymmetric Vectoring Exhaust Nozzle(AVEN),a vector deflection stability control method of aero-engine based on Linear Active Disturbance Rejection Control(LADRC)is proposed.Firstly,based on CFD numerical simulation,aerodynamic performance model of AVEN is established,and the aerodynamic load change rule of the nozzle throat area actuator during vector deflection is revealed.Subsequently,the integrated model of AVEN/-turbofan engine is established by Simulink/AMESim co-simulation.Finally,the nozzle throat area control loop based on LADRC is designed.The simulation results show that the integrated model can reflect the influence of vector deflection on the stability of the control system.The accuracy comparison between the fan rotor speed and the test data during vector deflection is larger than 1%,indicating a high degree of confidence.Compared with the conventional PID control,the designed LADRC control loop reduces the speed of the low-pressure rotor during vector deflection by 70%,which effectively improves the control stability of the vector deflection.Meanwhile,the fuel flow ratechange during the vector deflection process is smaller and more economical,which provides an important reference for engineering applications. | Changpeng CAI Yerong PENG Qiangang ZHENG Haibo ZHANG | 2022 | Chinese Journal of Aeronautics2022，35，8： | 0 |
| 5 | Maneuver control at high angle of attack based on real-time optimization of integrated aero-propulsion显示文摘To reduce the propulsion system installation thrust loss under high angle of attack maneuvering,a control method based on real-time optimization of the integrated aeropropulsion is proposed.Firstly,based on data fitting and physical principle,an integrated onboard model of propulsion system is established,which can calculate various performance parameters of the propulsion system in real time,and has high accuracy and real-time performance.Secondly,to improve the compatibility of optimization real-time performance and search accuracy,the online optimization control of aero-propulsion system is realized based on an improved trust region algorithm.Finally,by controlling the auxiliary intake valve,a good match between inlet and engine is realized,which solves the problems of intake flow reducing and total pressure recovery coefficient declining,and improves the installation performance of propulsion system.The simulation results indicate that,compared with the conventional independent engine control,the real-time integrated optimization method reduces the installed thrust loss by 3.61%under the design condition,and 4.58%under the off-design condition.Furthermore,the simulation on HIL(Hardware-In-theLoop)platform verifies the real-time performance of integrated optimization method. | Juan FANG Qiangang ZHENG Changpeng CAI Haibo ZHANG | 2022 | Chinese Journal of Aeronautics2022，35，12： | 0 |
| 6 | Flow control of double bypass variable cycle engine in modal transition显示文摘To study the change mechanism and the control of the variable cycle engine in the process of modal transition,a variable cycle engine model based on component level characteristics is established.The two-dimensional CFD technology is used to simulate the influence of mode selection valve rotation on the engine flow field,which improves the accuracy of the model.Furthermore,the constant flow control plan is proposed in the modal transition process to reduce the engine installed drag.The constant flow control plan adopts the augmentation linear quadratic regulator control method.Simulation results indicate that the control method is able to effectively control the bypass ratio and demand flow of the variable cycle engine,and make the engine transform smoothly,which ensures the stable operation of the engine in modal transition and the constant demand flow of the engine. | Haoying CHEN Changpeng CAI Jiayi LUO Haibo ZHANG | 2022 | Chinese Journal of Aeronautics2022，35，10： | 0 |
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