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| 1 | Ultrafast epitaxial growth of metre-sized single-crystal graphene on industrial Cu foil显示文摘A foundation of the modern technology that uses single-crystal silicon has been the growth of highquality single-crystal Si ingots with diameters up to 12 inches or larger. For many applications of graphene, large-area high-quality(ideally of single-crystal) material will be enabling. Since the first growth on copper foil a decade ago, inch-sized single-crystal graphene has been achieved. We present here the growth, in 20 min, of a graphene film of(5 ×50) cm^2 dimension with >99% ultra-highly oriented grains.This growth was achieved by:(1) synthesis of metre-sized single-crystal Cu(1 1 1) foil as substrate;(2)epitaxial growth of graphene islands on the Cu(1 1 1) surface;(3) seamless merging of such graphene islands into a graphene film with high single crystallinity and(4) the ultrafast growth of graphene film.These achievements were realized by a temperature-gradient-driven annealing technique to produce single-crystal Cu(1 1 1) from industrial polycrystalline Cu foil and the marvellous effects of a continuous oxygen supply from an adjacent oxide. The as-synthesized graphene film, with very few misoriented grains(if any), has a mobility up to ~23,000 cm^2 V^(-1)s^(-1)at 4 K and room temperature sheet resistance of ~230 Ω/□. It is very likely that this approach can be scaled up to achieve exceptionally large and high-quality graphene films with single crystallinity, and thus realize various industrial-level applications at a low cost. | Xiaozhi Xu Zhihong Zhang Jichen Dong Ding Yi Jingjing Niu Muhong Wu Li Lin Rongkang Yin Mingqiang Li Jingyuan Zhou Shaoxin Wang Junliang Sun Xiaojie Duan Peng Gao Ying Jiang Xiaosong Wu Hailin Peng Rodney S. Ruoff Zhongfan Liu Dapeng Yu Enge Wang Feng Ding Kaihui Liu | 2017 | Science Bulletin2017，62，15： | 40 |
| 2 | Synthesis and exfoliation of isocyanate-treated graphene oxide nanoplatelets显示文摘 | Sasha Stankovich Richard D. Piner SonBinh T. Nguyen Rodney S. Ruoff | 2006 | Carbon2006，，15： | 4 |
| 3 | Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide显示文摘 | Sasha Stankovich Dmitriy A. Dikin Richard D. Piner Kevin A. Kohlhaas Alfred Kleinhammes Yuanyuan Jia Yue Wu SonBinh T. Nguyen Rodney S. Ruoff | 2007 | Carbon2007，，7： | 3 |
| 4 | Outstanding performance of activated graphene based supercapacitors in ionic liquid electrolyte from ?50 to 80<ce:hsp sp='0.25'/>°C显示文摘 | Wan-Yu Tsai Rongying Lin Shanthi Murali Li Li Zhang John K. McDonough Rodney S. Ruoff Pierre-Louis Taberna Yury Gogotsi Patrice Simon | 2013 | Nano Energy2013，，3： | 2 |
| 5 | 兼具高负载量和高性能的碳/硫复合材料的低成本合成显示文摘单质硫能够与锂离子在正极发生多电子反应,使得锂硫电池具有高达2567 W·h·kg^-1的理论能量密度,因而锂硫电池也成为了目前锂离子电池的研究焦点。 | 季恒星 RUOFF Rodney S. | 2016 | 物理化学学报2016，32，3： | 2 |
| 6 | Mechanical and thermal properties of carbon nanotubes显示文摘 | Rodney S. Ruoff Donald C. Lorents | 1995 | Carbon1995，，7： | 2 |
| 7 | Chlorination of Reduced Graphene Oxide Enhances the Dielectric Constant of Reduced Graphene Oxide/Polymer Composites显示文摘 | Jin‐Young Kim Wi Hyoung Lee Ji Won Suk Jeffrey R. Potts Harry Chou Iskandar N. Kholmanov Richard D. Piner Jongho Lee Deji Akinwande Rodney S. Ruoff | 2013 | Mater2013，，16： | 1 |
| 8 | Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide显示文摘 | Sasha Stankovich Dmitriy A. Dikin Richard D. Piner Kevin A. Kohlhaas Alfred Kleinhammes Yuanyuan Jia Yue Wu SonBinh T. Nguyen Rodney S. Ruoff | 2007 | Carbon2007，，7： | 1 |
| 9 | Graphene-based polymer nanocomposites显示文摘 | Jeffrey R. Potts Daniel R. Dreyer Christopher W. Bielawski Rodney S. Ruoff | 2010 | Polymer2010，，1： | 1 |
| 10 | Synthesis and exfoliation of isocyanate-treated graphene oxide nanoplatelets显示文摘 | Sasha Stankovich Richard D. Piner SonBinh T. Nguyen Rodney S. Ruoff | 2006 | Carbon2006，，15： | 1 |
| 11 | Chemical analysis of graphene oxide films after heat and chemical treatments by X-ray photoelectron and Micro-Raman spectroscopy显示文摘 | Dongxing Yang Aruna Velamakanni Gülay Bozoklu Sungjin Park Meryl Stoller Richard D. Piner Sasha Stankovich Inhwa Jung Daniel A. Field Carl A. Ventrice Rodney S. Ruoff | 2008 | Carbon2008，，1： | 1 |
| 12 | Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide显示文摘 | Sasha Stankovich Dmitriy A. Dikin Richard D. Piner Kevin A. Kohlhaas Alfred Kleinhammes Yuanyuan Jia Yue Wu SonBinh T. Nguyen Rodney S. Ruoff | 2007 | Carbon2007，，7： | 1 |
| 13 | Graphene-based polymer nanocomposites显示文摘 | Jeffrey R. Potts Daniel R. Dreyer Christopher W. Bielawski Rodney S. Ruoff | 2010 | Polymer2010，，1： | 1 |
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