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| 1 | Genetic Mechanism of Dolomitization in Fengcheng Formation in the Wu-Xia area of Junggar Basin,China显示文摘The dolomitic rocks of the Fengcheng Formation are considered to be formed under special geologic conditions,and are significant hydrocarbon reservoir rocks in the Wu-Xia area in the Junggar Basin.Analyses of petrologic characteristics and stable isotope composition indicate that the dolomitizing host rock is volcanic and the dolomitizing fluids probably consists of brine from shore-shallow lakes with great evaporation and salinity in the Fengcheng Formation,which have formed under arid climatic conditions,as well as residual Mg-rich seawater from the underlying Jiamuhe Formation and Carboniferous.Dust tuff in the area has significant plagioclase content.Anorthite and labradorite hydrolysis by CO2 can be coupled with calcite precipitation.Late Mg-rich brine percolated and replaced calcite formed in the early time,which lead to precipitate dolostones with different occurrences,such as graniphyric,random bedded or lumpy.The diagenetic dolostones with different occurrences resulting from particular formation conditions occurred in different tectonic settings.The dolomitizing fluid has been driven by the thermal convection flow generated by volcanic eruptions.At the same time,the overthrusts of the Wu-Xia growth fault have speeded up the flow of deep Mg-rich water upwards,and induced the water to quickly penetrate and horizontally migrate in the strata.Fracture is the major and the most important reservoir space in dolomitic reservoir of the Fengcheng Formation.Fracture and fault plays a decisive role in controlling the formation of dolostone and the distribution of favorable reservoirs.The deliverability of oil and gas is determined by the development and match relations of dissolved pores and fractures to a certain degree. | ZHU Shifa ZHU Xiaomin NIU Huapeng HAN Xuefang ZHANG Yueqian YOU Xincai | 2012 | Acta Geologica Sinica(English Edition)2012，86，2： | 12 |
| 2 | Multiple Dolomitization and Fluid Flow Events in the Precambrian Dengying Formation of Sichuan Basin, Southwestern China显示文摘The Precambrian Dengying Formation is a set of large-scale, extensively dolomitized, carbonate reservoirs occurring within the Sichuan Basin. Petrographic and geochemical studies reveal dolomitization was a direct result of precipitation by chemically distinct fluids occurring at different times and at different intensities. Based on this evidence, dolomitization and multiple fluid flow events are analyzed, and three types of fluid evolution models are proposed. Results of analysis show that Precambrian Dengying Formation carbonates were deposited in a restricted peritidal environment(630–542 Ma). A high temperature and high Mg^(2+) concentration seawater was a direct result of dolomitization for the micrite matrix, and for fibrous aragonite in primary pores. Geochemical evidence shows low δ^(18)O values of micritic dolomite varying from-1.29‰ to-4.52‰ PDB, abundant light rare earth elements(REEs), and low dolomite order degrees. Microbes and meteoric water significantly altered dolomite original chemical signatures, resulting in algal micritic dolomite and the fine-grained, granular, dolosparite dolomite having very negative δ^(18)O values. Finely crystalline cement dolomite(536.3–280 Ma) and coarsely crystalline cement dolomite have a higher crystallization degree and higher order degree. The diagenetic sequence and fluid inclusion evidence imply a linear correlation between their burial depth and homogenization temperatures, which closely resemble the temperature of generated hydrocarbon. Compared with finely crystalline dolomite, precipitation of coarsely crystalline dolomite was more affected by restricted basinal fluids. In addition, there is a trend toward a more negative δ^(18)O value, higher salinity, higher Fe and Mn concentrations, REE-rich. Two periods of hydrothermal fluids are identified, as the exceptionally high temperatures as opposed to the temperatures of burial history, in addition to the presence of high salinity fluid inclusions. The early hydrothermal fluid flow event was characterized by hot magnesium-and silicon-rich fluids, as demonstrated by the recrystallized matrix dolomite that is intimately associated with flint, opal, and microcrystalline quartz in intergranular or intercrystalline pores. This event was likely the result of a seafloor hydrothermal chimney eruption during Episode I of the Tongwan Movement(536.3±5.5 Ma). In contrast, later hydrothermal fluids, which caused precipitation of saddle dolomite, were characterized by high salinity(15–16.05 wt% NaCl equivalent) and homogenization temperatures(250 to 265°C), δ^(18)O values that were more enriched, and REE signatures. Geochemical data and the paragenetic sequence indicate that this hydrothermal fluid was related to extensive Permian large igneous province activity(360–280 Ma). This study demonstrates the presence of complicated dolomitization processes occurring during various paleoclimates, tectonic cycles, and basinal fluids flow; results are a useful reference for these dolomitized Precambrian carbonates reservoirs. | PENG Bo LI Zongxing LI Guorong LIU Chenglin ZHU Shifa ZHANG Wang ZUO Yinhui GUO Yingchun WEI Xiaojie | 2018 | Acta Geologica Sinica(English Edition)2018，92，1： | 5 |
| 3 | Chelating agents role on phase formation and surface morphology of single orthorhombic YMn_2O_5 nanorods via modified polyacrylamide gel route显示文摘YMn2O5nanorods were synthesized through a modified polyacrylamide gel route.The synthesis strategy in this work is based on a sol-gel process using a polyacrylamide gel method in which oxalic acid,citric acid or tartaric acid is employed as the chelating agent.In the gel routes,oxalic acid was used as a carboxyl chelating agent,while citric acid or tartaric acid was a carboxyl and hydroxyl chelating agent.The as-prepared samples were characterized by means of techniques such as X-ray powder diffraction(XRD)measurement,thermogravimetric analysis(TG),differential scanning calorimetry analysis(DSC),Fourier transform infrared spectroscopy(FTIR),X-ray photoelectron spectroscopy(XPS),thermal expansion measurement and field-emission scanning electron microscopy(SEM)investigations.It was found that oxalic acid is the best chelating agent with Y(NO3)3·6H2O and Mn(CH3COO)2·4H2O as precursors to prepare a single orthorhombic YMn2O5nanorods at 1000°C.Scanning electron microscope observation shows that the morphology of YMn2O5powders is significantly dependent on the chelating agent.The peaks(single orthorhombic YMn2O5nanorods)at 642,600,573,546,521,493,486,468,448 and 400cm?1were observed from FTIR spectra.The phase,surface morphology and chelation mechanisms of YMn2O5samples have been discussed on the basis of the experimental results. | WANG ShiFa ZHANG ChuanFei SUN GuangAi CHEN Bo XIANG Xia DING QingPing ZU XiaoTao | 2014 | Science China Chemistry2014，57，3： | 4 |
| 4 | Identification of abnormal conditions in high-dimensional chemical process based on feature selection and deep learning显示文摘Identification of abnormal conditions is essential in the chemical process.With the rapid development of artificial intelligence technology,deep learning has attracted a lot of attention as a promising fault identification method in chemical process recently.In the high-dimensional data identification using deep neural networks,problems such as insufficient data and missing data,measurement noise,redundant variables,and high coupling of data are often encountered.To tackle these problems,a feature based deep belief networks(DBN)method is proposed in this paper.First,a generative adversarial network(GAN)is used to reconstruct the random and non-random missing data of chemical process.Second,the feature variables are selected by Spearman’s rank correlation coefficient(SRCC)from high-dimensional data to eliminate the noise and redundant variables and,as a consequence,compress data dimension of chemical process.Finally,the feature filtered data is deeply abstracted,learned and tuned by DBN for multi-case fault identification.The application in the Tennessee Eastman(TE)process demonstrates the fast convergence and high accuracy of this proposal in identifying abnormal conditions for chemical process,compared with the traditional fault identification algorithms. | Wende Tian Zijian Liu Lening Li Shifa Zhang Chuankun Li | 2020 | Chinese Journal of Chemical Engineering2020，28，7： | 3 |
| 5 | Selective growth of wide band gap atomically thin Sb2O3 inorganic molecular crystal on WS2显示文摘Heterostructures combined by different individual two-dimensional(2D)materials are essential building blocks to realize unique electronic,optoelectronic properties and multifunctional applications.To date,the direct growth of 2D/2D atomic van der Waals heterostructures(vdWHs)have been extensively investigated.However,the heterostructures from 2D inorganic molecular crystals and atomic crystals have been rarely reported.Here we report two-step direct epitaxial growth of the inorganic molecular-atomic Sb2O3/WS2 vdWHs.The thickness of Sb2O3 nanosheets on WS2 nanosheets can be tuned by variable growth temperatures.Oriented growth behavior of Sb2O3 on WS2 was determined through statistics.Optical images,Raman spectra,Raman mappings and selected-area electron diffraction(SAED),etc.,reveal that Sb2O3/WS2 heterostructures are vertically stacked with high crystal quality.Electrical transport measurements demonstrate that the heterotransistors based on the heterostructures possess high current on/off ratio of 5 × 10^5,obvious gate-tunable and current rectification output characteristics.Optoelectronic characterizations show that the heterostructures have a clear photoresponse with high responsivity of 16.4 AW.The growth of vdWHs from 2D inorganic molecular-atomic crystals may open up new opportunities in 2D functional electronics and optoelectronics. | Guangzhuang Sun Bo Li Shifa Wang Zhengwei Zhang Jia Li Xidong Duan Xiangfeng Duan | 2019 | Nano Research2019，12，11： | 2 |
| 6 | Immune enhancement of Taishan Robinia pseudoacacia polysaccharide on recombinant Proteus mirabilis OmpA in chickens显示文摘 | Yongbing Zhang Shifa Yang Xue Zhao | 2014 | International Immunopharmacology2014，22，1： | 1 |
| 7 | SJES14110700453116显示文摘 | Yongbing Zhang Shifa Yang Xue Zhao Ya Yang Bing Li Fujie Zhu Ruiliang Zhu | 2014 | International Immunopharmacology2014，，1： | 1 |
| 8 | Characterizing the urban spatial structure using taxi trip big data and implications for urban planning显示文摘Urban spatial structure is an important feature for assessing the effects of urban planning.Quantifying an urban spatial structure cannot only help in identifying the problems with current planning but also provide a basic reference for future adjustments.Evaluation of spatial structure is a difficult task for planners and researchers and this has been usually carried out by comparing different land use structures.However,these methods cannot efficiently reflect the influence of human activities.With the wide application of big data,analyzing data on human travel behavior has increasingly been carried out to reveal the relationship between urban spatial structure and urban planning.In this study,we constructed a human-activity space network using the taxi trip big data.Clustering at different scales revealed the hierarchy and redundancy of the spatial structure for assessing the appropriateness and shortcomings of urban planning.This method was applied to a case study based on one-month taxi trip data of Dongguan City.Existing urban spatial structures at different scales were retrieved and utilized to assess the effectiveness of the master plan designed for 2000 to 2015 and 2008 to 2020,which can help identify the limitations and improvements in the spatial structure designed in these two versions of the master plan.We also evaluated the potential effect of the master plan designed for 2016 to 2035 by providing a reference for reconstructing and optimizing future urban spatial structure.The analysis demonstrated that the taxi trip data are important big data on social spatial perception,and taxi data should be used for evaluating spatial structures in future urban planning. | Haibo LI Xiaocong XU Xia LI Shifa MA Honghui ZHANG | 2021 | Frontiers of Earth Science2021，15，1： | 1 |
| 9 | Unconventional Petroleum Sedimentology:A Key to Understanding Unconventional Hydrocarbon Accumulation显示文摘The commercial exploitation of unconventional petroleum resources(e.g.,shale oil/gas and tight oil/gas)has drastically changed the global energy structure within the past two decades.Sweet-spot intervals(areas),the most prolific unconventional hydrocarbon resources,generally consist of extraordinarily high organic matter(EHOM)deposits or closely associated sandstones/carbonate rocks.The formation of sweet-spot intervals(areas)is fundamentally controlled by their depositional and subsequent diagenetic settings,which result from the coupled sedimentation of global or regional geological events,such as tectonic activity,sea level(lake level)fluctuations,climate change,bottom water anoxia,volcanic activity,biotic mass extinction or radiation,and gravity flows during a certain geological period.Black shales with EHOM content and their associated high-quality reservoir rocks deposited by the coupling of major geological events provide not only a prerequisite for massive hydrocarbon generation but also abundant hydrocarbon storage space.The Ordovician-Silurian Wufeng-Longmaxi shale of the Sichuan Basin,Devonian Marcellus shale of the Appalachian Basin,Devonian-Carboniferous Bakken Formation of the Williston Basin,and Triassic Yanchang Formation of the Ordos Basin are four typical unconventional hydrocarbon systems selected as case studies herein.In each case,the formation of sweet-spot intervals for unconventional hydrocarbon resources was controlled by the coupled sedimentation of different global or regional geological events,collectively resulting in a favorable environment for the production,preservation,and accumulation of organic matter,as well as for the generation,migration,accumulation,and exploitation of hydrocarbons.Unconventional petroleum sedimentology,which focuses on coupled sedimentation during dramatic environmental changes driven by major geological events,is key to improve the understanding of the formation and distribution of sweet-spot intervals(areas)in unconventional petroleum systems. | Caineng Zou Zhen Qiu Jiaqiang Zhang Zhiyang Li Hengye Wei Bei Liu Jianhua Zhao Tian Yang Shifa Zhu Huifei Tao Fengyuan Zhang Yuman Wang Qin Zhang Wen Liu Hanlin Liu Ziqing Feng Dan Liu Jinliang Gao Rong Liu Yifan Li | 2022 | Engineering2022，，11： | 1 |
| 10 | A novel flavonol-based colorimetric and turn-on fluorescent probe for rapid determination of hydrazine in real water samples and its bioimaging in vivo and in vitro显示文摘Hydrazine is extremely toxic and causes severe harm to human body.Herein,a novel fluorescent probe 4-oxo-2-styryl-4H-chromen-3-yl thiophene-2-carboxylate(FHT)was synthesized for detecting hydrazine by using natural cinnamaldehyde as starting material.This probe exhibited significantly enhanced fluorescence response towards hydrazine over various common metal ions,anions,and amine compounds.The detection limit of probe FHT for hydrazine was as low as 0.14μmol·L^(-1),significantly lower than that of the threshold value of 0.312μmoi·L^(-1),imposed by the Environmental Protection Agency.Moreover,the proposed probe was able to detect hydrazine within wide pH(5-10)and linear detection ranges(0-110μmol·L^(-1)).This probe was employed for determining trace hydrazine in different environmental water samples.The probe FHT-loaded filter paper strips werea able to conveniently detect hydrazine of low concentration through distinct naked-eye and fluorescent color changes.Importantly,the probe FHT with low cytotoxicitywas successfullyapplied to visualize hydrazine in living Hela cells and zebrafish. | Ahui Qin Yan Zhang Shuai Gong Mingxin Li Yu Gao Xu Xu Jie Song Zhonglong Wang Shifa Wang | 2023 | Frontiers of Chemical Science and Engineering2023，17，1： | 1 |
| 11 | Simulation and Analysis of the Electrical Feedback System during the Process of Imaging in Scanning Probe Microscope显示文摘 | ZHANG Kun PAN Shi WU Shifa | 2006 | Chinese Journal of Electronics2006，15，3： | 0 |
| 12 | YBa_(2)Cu_(3)O_(7-x) Superconducting Thin Films Grown on CaNdA1O_(4)(100) Substrates显示文摘We report the fabrication of high temperature superconducting YBa_(2)Cu_(3)O_(7-x) thin films on CaNdA1O_(4)(100) substrate by pulsed laser deposition.Films have excellent features.X-ray diffraction patterns show that thin films are epitaxial with c-axis orientation normal to the surface of su bstrate.The four-terminal measurements indicate the zero resistance temperature of 92.1 K,and transition width of 0.7K,the critical current density of 3×10^(6)A/cm^(2)at 77K and under zero magnetic field. | XU Shifa ZHOU Yueliang LÜHuibin CUI Dafu CHEN Zhenghao YANG Guozhen TIAN Yongjun LIU Junzheng LI Lin CHANG Yingchuan HOU Desen FAN Hui ZHANG Zuren | 1994 | Chinese Physics Letters1994，11，5： | 0 |
| 13 | Shale Lithofacies and Sedimentary Environment of the Third Member,Shahejie Formation,Zhanhua Sag,Eastern China显示文摘Researches into shale lithofacies,their sedimentary environments and relationship benefit understanding both of sedimentary cycle division and unconventional hydrocarbon exploration in lacustrine basins.Based on a 100~300-m-thick dark shale,mudstone and limestone encountered in the lower third member of the Eocene Shahejie Formation(Es3l member)in Zhanhua Sag,Bohai Bay Basin,eastern China,routine core analysis,thin sectioning,scanning electron microscopy(SEM),mineralogical and geochemical measurements were used to understand detailed facies characterization and paleoclimate in the member.This Es3l shale sediment includes three sedimentary cycles(C3,C2 and C1),from bottom to top,with complex sedimentary characters and spatial distribution.In terms of the composition,texture,bedding and thickness,six lithofacies are recognized in this succession.Some geochemical parameters,such as trace elements(Sr/Ba,Na/Al,V/Ni,V/(V+Ni),U/Th),carbon and oxygen isotopes(δ^(18)O,δ^(13)C),and total organic carbon content(TOC)indicate that the shales were deposited in a deep to semi-deep lake,with the water column being salty,stratified,enclosed and reductive.During cycles C3 and C2 of the middle-lower sections,the climate was arid,and the water was salty and stratified.Laminated and laminar mudstone-limestone was deposited with moderate organic matter(average TOC 1.8%)and good reservoir quality(average porosity 6.5%),which can be regarded as favorable reservoir.During the C1 cycle,a large amount of organic matter was input from outside the basin and this led to high productivity with a more humid climate.Massive calcareous mudstone was deposited,and this is characterized by high TOC(average 3.6%)and moderate porosity(average 4%),and provides favorable source rocks. | ZHU Xiaomin ZHANG Meizhou ZHU Shifa DONG Yanlei LI Chao BI Yuequan MA Lichi | 2022 | Acta Geologica Sinica(English Edition)2022，96，3： | 0 |
| 14 | Abnormal thermal conductivity enhancement in covalently bonded bilayer borophene allotrope显示文摘Thermal conductivity of two-dimensional(2D)materials has gained prominence due to the attractive applications in thermal management and thermoelectric devices.In this work,we present a new member of bilayer 2D boron allotropes,denoted as bilayerβ12 borophene,and study the thermal transport properties by solving phonon Boltzmann transport equation based on density functional theory.Based on quantitative chemical bonding analysis,we identify large degrees of covalent bonding of the interlayer interaction.In comparison to its monolayer counterpart,the bilayer exhibits much higher in-plane thermal conductivity despite the lower phonon group velocity and buckling structure,inferring a new physical mechanism.The thermal conductivity(κ)of bilayerβ_(12)borophene at 300 K is 140.5(86.3)W·m^(-1)·K^(-1)along armchair(zigzag)direction,andκ_(armchair)is about 52.7%higher than that of monolayerβ12 borophene.The abnormal enhancement is attributed to the suppressed phonon scattering possibility and elongation of phonon lifetime.More interesting,after forming bilayerβ12 borophene through interlayer covalent bonding,the dominated phonon branch to thermal conductivity changes to transverse acoustic phonons from out-of-plane flexural acoustic(ZA)phonons in the monolayer borophene.Our study elucidates the rich thermal transport characteristics in bilayer covalently bonded 2D materials,and injects fresh insights into the phonon engineering of 2D borophene relevant for emergent thermal management applications. | Yan Yin Yanxiao Hu Shichang Li Guangqian Ding Shifa Wang Dengfeng Li Gang Zhang | 2022 | Nano Research2022，15，4： | 0 |
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