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| 1 | Effects of dissolved organic matter from sewage sludge on sorption of tetrabromobisphenol A by soils显示文摘Sorption of tetrabromobisphenol A (TBBPA) by soil influences its fate and transport in the environment. The presence of dissolved organic matter (DOM) may complicate the sorption process in soil. The effects of DOM from sewage sludge on TBBPA sorption by three soils were investigated using batch equilibration experiments in the study. DOM was observed to be sorbed on the soils and the isotherms could be fitted by the Langmuir model. The effects of DOM on TBBPA sorption were dependent on the characteristics of soils and the concentrations of DOM present. TBBPA sorption by Henan (HN) soil (sandy loam) and Liaoning (LN) soil (loamy clay) was promoted in the presence of DOM at low concentration ( 90 mg organic carbon (OC)/L), and the sorption was promoted by HN soil and inhibited by LN soil at DOM added concentration of 180 mg OC/L. TBBPA sorption by Guangxi (GX) soil (silt loam) was always inhibited in the presence of DOM. It was also found that the amount of TBBPA sorbed decreased with the increase in the solution pH value in the absence of DOM. The influencing mechanisms of DOM on the sorption of TBBPA by soils were also discussed. | Zhaohai SUN Hongxia YU | 2008 | Journal of Environmental Sciences2008，20，9： | 6 |
| 2 | Nitrated and parent PAHs in the surface water of Lake Taihu,China:Occurrence,distribution,source,and human health risk assessment显示文摘Nitrated polycyclic aromatic hydrocarbons(NPAHs)have toxic potentials that are higher than those of their corresponding parent polycyclic aromatic hydrocarbons(PAHs)and thus have received increasing attention in recent years.In this study,the occurrence,distribution,source,and human health risk assessment of 15 NPAHs and 16 PAHs were investigated in the surface water from 20 sampling sites of Lake Taihu during the dry,normal,and flood seasons of 2018.The PAH concentrations ranged from 255 to 7298 ng/L and the NPAH concentrations ranged from not-detected(ND)to 212 ng/L.Among the target analytes,2-nitrofluorene(2-n Flu)was the predominant NPAH,with a detection frequency ranging from 85%to 90%and a maximum concentration of 56.2 ng/L.The three-ringed and four-ringed NPAHs and PAHs comprised the majority of the detected compounds.In terms of seasonal variation,the highest levels of the NPAHs and PAHs were in the dry season and flood season,respectively.Diagnostic ratio analysis indicated that the prime source of NPAHs was direct combustion,whereas in the case of PAHs the contribution was predominantly from a mixed pattern including pollution from unburned petroleum and petroleum combustion.The human health risk of NPAHs and PAHs was evaluated using a lifetime carcinogenic risk assessment model.The carcinogenic risk level of the targets ranged from 2.09×10^(-7)to 5.75×10^(-5)and some surface water samples posed a potential health risk. | Jijie Kong Yuxuan Dai Mengshu Han Huan He Jiapeng Hu Junyi Zhang Junzhe Shi Qiming Xian Shaogui Yang Cheng Sun | 2021 | Journal of Environmental Sciences2021，33，4： | 6 |
| 3 | Polybrominated diphenyl ethers (PBDEs) in aquatic biota from the lower reach of the Yangtze River, East China显示文摘 | Zishen Gao Jie Xu Qiming Xian Jianfang Feng Xiaohui Chen Hongxia Yu | 2009 | Chemosphere2009，，9： | 1 |
| 4 | Occurrence, partition behavior, source and ecological risk assessment of nitro-PAHs in the sediment and water of Taige Canal, China显示文摘Nitrated polycyclic aromatic hydrocarbons(NPAHs)are widespread organic pollutants that possess carcinogenic and mutagenic properties,so they may pose a risk to the environment and human health.In this study,the concentrations of 15 NPAHs and 16 polycyclic aromatic hydrocarbons(PAHs)in 30 surface water samples and 26 sediment samples were measured in 2018 from the Taige Canal,one of the main rivers flowing into Taihu Lake,China.The total NPAH concentrations in water and sediment ranged from 14.7 to 235 ng/L and 22.9 to 96.5 ng/g dw,respectively.9-nitrophenanthrene(nd–76.3 ng/L)was the dominant compound in surface water,while 2+3-nitrofluoranthene(1.73–18.1 ng/g dw)dominated in sediment.Among PAHs,concentration ranging from 1,097 to 2,981 ng/L and 1,089 to 4,489 ng/g dw in surface water and sediment,respectively.There was a strong positive correlation between the log octanol-water partition coefficient(Kow)and log sediment-water partition coefficient due to hydrophobic interaction.The fugacity fraction value increased with the decrease of log Kow,and chrysene was transferred from water into sediment.The residual NPAHs in surface water and sediment of the Taige Canal have partial correlation.Diesel engine and coal combustion emissions were probably the principal sources of NPAHs in surface water and sediment.The results of ecological risk assessment showed that some NPAHs inwater(e.g,1-nitropyrene and 6-nitrochrysene)and sediment(e.g.,2-nitrobiphenyl,5-nitroacenaphthene,9-nitrophenanthrene and 2+3-nitrofluoranthene)had moderate ecological risks,which should be of concern. | Jijie Kong Tao Ma Xiaoyu Cao Weidi Li Fengxiao Zhu Huan He Cheng Sun Shaogui Yang Shiyin Li Qiming Xian | 2023 | Journal of Environmental Sciences2023，，2： | 1 |
| 5 | Adsorption of copper and lead in aqueous solution onto bentonite modified by 4'-methylbenzo-15-crown- S显示文摘 | Lin Yun Shen Xing Xian Qiming | 2006 | Journal of Hazardous Materials2006，137，2： | 1 |
| 6 | Polybrominated diphenyl ethers (PBDEs) in aquatic biota from the lower reach of the Yangtze River, East China显示文摘 | Zishen Gao Jie Xu Qiming Xian Jianfang Feng Xiaohui Chen Hongxia Yu | 2009 | Chemosphere2009，，9： | 1 |
| 7 | Adsorption of copper and lead in aqueous solution onto bentonite modi fied by 4-methylbenzo-15-crown-5 显示文摘 | Liu Yun Shen Xing Xian Qiming | 2006 | Journal of Haz- ardous Materials2006，137，： | 1 |
| 8 | Molecular simulation-guided and physics-informed mechanistic modeling of multifunctional polymers显示文摘Polymeric materials have a broad range of mechanical and physical properties.They have been widely used in material science,biomedical engineering,chemical engineering,and mechanical engineering.The introduction of active elements into the soft matrix of polymers has enabled much more diversified functionalities of polymeric materials,such as self-healing,electroactive,magnetosensitive,pH-responsive,and many others.To further enable applications of these multifunctional polymers,a mechanistic modeling method is required and of great significance,as it can provide links between materials’micro/nano-structures and their macroscopic mechanical behaviors.Towards this goal,molecular simulation plays an important role in understanding the deformation and evolution of polymer networks under external loads and stimuli.These molecular insights provide physical guidance in the formulation of mechanistic-based continuum models for multifunctional polymers.In this perspective,we present a molecular simulation-guided and physics-informed modeling framework for polymeric materials.Firstly,the physical theory for polymer chains and their networks is briefly introduced.It serves as the foundation for mechanistic-models of polymers,linking their chemistry,physics,and mechanics together.Secondly,the deformation of the polymer network is used to derive the strain energy density functions.Thus,the corresponding continuum models can capture the intrinsic deformation mechanisms of polymer networks.We then highlight several representative examples across multiphysics coupling problems to describe in detail for this proposed framework.Last but not least,we discuss potential challenges and opportunities in the modeling of multifunctional polymers for future research directions. | Guang Chen Weikang Xian Qiming Wang Ying Li | 2021 | Acta Mechanica Sinica2021，37，5： | 1 |
| 9 | Adsorption of copper and lead in aqueous solution onto bentonite modified by 4-methylbenzo-15-crown-5显示文摘 | Liu Yun Shen Xing Xian Qiming | 2006 | Journal of Hazardous Materials2006，137，： | 1 |
| 10 | Levels and distribution of polybrominated diphenyl ethers ( PBDEs ) in the freshwater environment surrounding a PBDE manufacturing plant in China 显示文摘 | XU Jie GAO Zishen XIAN Qiming | 2009 | Environ Pollut2009，157，6： | 1 |
| 11 | Levels and body distribution of polybrominated diphenyl ethers (PBDEs) and hexabromocyclododecanes (HBCDs) in freshwater fishes from the Yangtze River, China显示文摘 | XIAN Qiming RAMU K ISOBE T | 2008 | Chemosphere2008，71，2： | 1 |
| 12 | Isolation andIdentification of antialgal compounds from the Leaves of Vallisneriaspiralis L, by activity-guided fractionation 显示文摘 | XIAN Qiming CHEN Haidong LIU Huili | 2006 | EnvironmentalScience and Pollution Research2006，13，4： | 1 |
| 13 | Adsorption of copper and lead in aqueous solution onto bentonite modified by 4' - methylbenzo - 15 - crown - 5 显示文摘 | Yun Liu Xing Shen Qiming Xian | 2006 | Journal of Hazardous Materi- als2006，137，2： | 1 |
| 14 | Levels and body distribution of polybrominated diphenyl ethers (PBDEs) and hexabromocyclododecanes (HBCDs) in freshwater fishes from the Yangtze River, China显示文摘 | Qiming Xian Karri Ramu Tomohiko Isobe Agus Sudaryanto Xiaohua Liu Zishen Gao Shin Takahashi Hongxia Yu Shinsuke Tanabe | 2007 | Chemosphere2007，，2： | 1 |
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