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| 1 | Mass production of 2D materials by intermediate-assisted grinding exfoliation显示文摘The scalable and high-efficiency production of 2D materials is a prerequisite to their commercial use.Currently,only graphene and graphene oxide can be produced on a ton scale,and the inability to produce other 2D materials on such a large scale hinders their technological applications.Here we report a grinding exfoliation method that uses micro-particles as force intermediates to resolve applied compressive forces into a multitude of small shear forces,inducing the highly efficient exfoliation of layer materials.The method;referred to as intermediate-assisted grinding exfoliation(iMAGE);can be used for the large-scale production of many 2D materials.As an example;we have exfoliated bulk h-BN into 2D h-BN with large flake sizes;high quality and structural integrity,with a high exfoliation yield of 67%,a high production rate of 0.3 g h^-1 and a low energy consumption of 3.01 x 106 J g^-1.The production rate and energy consumption are one to two orders of magnitude better than previous results.Besides h-BN,this iMAGE technology has been used to exfoliate various layer materials such as graphite,black phosphorus,transition metal dichalcogenides;and metal oxides;provings universality.Molybdenite concentrate,a natural low-cost and abundant mineral;was used as a demo for the large-scale exfoliation production of 2D M0S2 flakes.Our work indicates the huge potential of the iMAGE method to produce large amounts of various 2D materials;which paves the way for their commercial application. | Chi Zhang Junyang Tan Yikun Pan Xingke Cai Xiaolong Zou Hui-Ming Cheng Bilu Liu | 2020 | National Science Review2020,7,2: | 10 |
| 2 | Thickness-dependent patterning of MoS2 sheets with well-oriented triangular pits by heating in air显示文摘自从 MoS2 表的性质对边结构敏感,有常规边或可控制的形状的 Patterning ultrathin MoS2 层正在呼吁。在这个工作,我们介绍了一种简单、有效、控制得好的技术由简单地在空中加热样品与面向井的等边的三角形的坑蚀刻分层的 MoS2 表。各向异性的氧化蚀刻被包围温度和 MoS2 层的数字极大地影响,坑由此随包围温度和 MoS2 层的数字的增加缩放增加。第一原则的计算被执行了解释三角形的坑的形成机制。这种技术把一条其他的大街提供给设计 MoS2 表的结构。 | Haiqing Zhou Fang Yu Yuanyue Liu Xiaolong Zou Chunxiao Cong Caiyu Qiu Ting Yu Zheng Yan Xiaonan Shen Lianfeng Sun Boris I. Yakobson James M. Tour | 2013 | Nano Research2013,6,10: | 9 |
| 3 | O_(3)oxidation combined with semi-dry method for simultaneous desulfurization and denitrification of sintering/pelletizing flue gas显示文摘With the vigorous development of China's iron and steel industry and the introduction of ultra-low emission policies,the emission of pollutants such as SO_(2)and NO x has received unprecedented attention.Considering the increase of the proportion of semi-dry desulfurization technology in the desulfurization process,several semi-dry desulphurization technologies such as flue gas circulating fluidized bed(CFB),dense flow absorber(DFA)and spray drying absorption(SDA)are briefly summarized.Moreover,a method for simultaneous treatment of SO_(2)and NOx in sintering/pelletizing flue gas by O_(3)oxidation combined with semidry method is introduced.Meantime,the effects of key parameters such as O_(3)/NO molar ratio,Ca SO_(3),SO_(2),reaction temperature,Ca/(S+2 N)molar ratio,droplet size and approach to adiabatic saturation temperature(AAST)on denitrification and desulfurization are analyzed.Furthermore,the reaction mechanism of denitrification and desulfurization is further elucidated.Finally,the advantages and development prospects of the new technology are proposed. | Fagao Liu Maoyu Cai Xiaolong Liu Tingyu Zhu Yang Zou | 2021 | Journal of Environmental Sciences2021,33,6: | 8 |
| 4 | Simultaneous removal of SO2 and NO using a spray dryer absorption(SDA) method combined with O3 oxidation for sintering/pelleting flue gas显示文摘Based on the demand of sintering/pelleting flue gas ultra-low emission,a semi-dry method using a spray dryer absorber (SDA) combined with O3 oxidation was proposed for simultaneous removal of SO2 and NO.Effects of O3 injection site,O3/NO molar ratio,and spray tower temperature on the removal efficiencies were investigated.It was revealed that both desulfurization and denitrification efficiencies could reach to 85%under the conditions of setting O3 injection site inside of tower,O3/NO molar ratio 1.8,spray tower temperature 85°C,Ca/(S+2N) molar ratio 2.5 and slurry flow rate 300 m L/hr.CaSO3/Ca(OH)2 mixture slurry was used as absorbent to simulate operating conditions in iron and steel industry.The result shows that the addition of CaSO3 weakens both removal efficiencies.In addition,the reaction mechanism of simultaneous removal of SO2 and NO using SDA combined with O3 oxidation was proposed. | Maoyu Cai Xiaolong Liu Tingyu Zhu Yang Zou Wenliang Tao Mengkui Tian | 2020 | Journal of Environmental Sciences2020,32,10: | 7 |
| 5 | The FGOALS climate system model as a modeling tool for supporting climate sciences:An overview显示文摘Climate system models are useful tools for understanding the interactions among the components of the climate system and predicting/projecting future climate change. The development of climate models has been a central focus of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics, Institute of Atmospheric Physics, Chinese Academy of Sciences(LASG/IAP) since the establishment of the laboratory in 1985. In China, many pioneering component models and fully coupled models of the climate system have been developed by LASG/IAP. The fully coupled climate system developed in the recent decade is named FGOALS(Flexible Global Ocean-Atmosphere-Land System Model). In this paper, an application-oriented review of the LASG/IAP FGOALS model is presented. The improved model performances are demonstrated in the context of cloud-radiation processes, Asian monsoon, ENSO phenomena, Atlantic Meridional Overturning Circulation(AMOC) and sea ice. The FGOALS model has contributed to both CMIP5(Coupled Model Intercomparison Project-phase 5) and IPCC(Intergovernmental Panel on Climate Change) AR5(the Fifth Assessment Report). The release of FGOALS data has supported the publication of nearly 500 papers around the world. The results of FGOALS are cited ~106 times in the IPCC WG1(Working Group 1) AR5. In addition to the traditional long-term simulations and projections, near-term decadal climate prediction is a new set of CMIP experiment, progress of LAGS/IAP in the development of nearterm decadal prediction system is reviewed. The FGOALS model has supported many Chinese national-level research projects and contributed to the national climate change assessment report. The crucial role of FGOALS as a modeling tool for supporting climate sciences is highlighted by demonstrating the model's performances in the simulation of the evolution of Earth's climate from the past to the future. | TianJun Zhou Bin Wang YongQiang Yu YiMin Liu WeiPeng Zheng LiJuan Li Bo Wu PengFei Lin Zhun Guo WenMin Man Qing Bao AnMin Duan HaiLong Liu XiaoLong Chen Bian He JianDong Li LiWei Zou XiaoCong Wang LiXia Zhang Yong Sun WenXia Zhang | 2018 | Earth and Planetary Physics2018,2,4: | 6 |
| 6 | Toward emerging gallium oxide semiconductors:A roadmap显示文摘Owing to the advantages of ultra-wide bandgap and rich material systems,gallium oxide(Ga_(2)O_(3))has emerged as a highly viable semiconductor material for new researches.This article mainly focuses on the growth processes,material characteristics,and applications of Ga_(2)O_(3).Compared with single crystals and the epitaxial growth of other wide-bandgap semiconductors,large-size and high-quality��-Ga_(2)O_(3) single crystals can be efficiently grown with a low cost,making them highly competitive.Thanks to the availability of high-quality single crystals,epi-taxial films,and rich material systems,high-performance semiconductor devices based on Ga_(2)O_(3) go through a booming development in recent years.The defects and interfaces of Ga_(2)O_(3) are comprehensively analyzed owing to their significant influence on practical applications.In this study,the two most common applications of Ga_(2)O_(3) materials are introduced.The high breakdown electric field,high working temperature,and excellent Baliga’s figure-of-merit of Ga_(2)O_(3) represent an inspiring prospect for power electronic devices.In addition,the excellent absorption in deep-ultraviolet band provides new ideas for optoelectronic detectors and ensures the dramatic progress.Finally,the summary,challenges,and prospects of the Ga_(2)O_(3) materials and devices are presented and discussed. | Yuan Yuan Weibing Hao Wenxiang Mu Zhengpeng Wang Xuanhu Chen Qi Liu Guangwei Xu Chenlu Wang Hong Zhou Yanni Zou Xiaolong Zhao Zhitai Jia Jiandong Ye Jincheng Zhang Shibing Long Xutang Tao Rong Zhang Yue Hao | 2021 | Fundamental Research2021,1,6: | 5 |
| 7 | Group VB transition metal dichalcogenides for oxygen reduction reaction and strain-enhanced activity governed by p-orbital electrons of chalcogen显示文摘Developi ng alter native oxyge n reducti on reactio n (ORR) catalysts to replace precious Pt-based metals with abundant materials is the key challe nge of commercial application of fuel cells. Owing to their various compositi ons and tun able electronic properties, transition metal dichalcogenides (TMDs) have the great potential to realize high-efficiency catalysts for ORR. Here, various 3R-phase dichalcogenides of group VB and VIB transition metals (MX2, M = Nb, Ta, Mo, W;X = S, Se, Te) are investigated for ORR catalysts by using density functional theory calculations. The computed over-potentials of group VB TMDs are much less than those of group VIB TMDs. For group VB TMDs, a volcano-type plot of ORR catalytic activity is established on the adsorption energies of *OH, and NbS2 and TaTe2 exhibit best ORR activity with an oveepotential of 0.54 V. To achieve even better activity, strain engineering is performed to tune ORR catalytic activity, and the minimum over-potential of 0.43 V can be realized. We further dem on strate that the shift of p orbital center of surface chalcoge n elements under strain is responsible for tuning the catalytic activity of TMDs. | Shuyang Zhao Ke Wang Xiaolong Zou Lin Gan Hongda Du Chengjun Xu Feiyu Kang Wenhui Duan Jia Li | 2019 | Nano Research2019,12,4: | 4 |
| 8 | Space-confined growth of monolayer ReSe2 under a graphene layer on Au foils显示文摘Vertical heterostructures based on two-dimensional(2D)materials have attracted widespread interest for their numerous applications in electronic and optoelectronic devices.Herein,we report the direct construct!on of an abnormal graphene/ReSe2 stack on Au foils by a two-step chemical vapor deposition(CVD)strategy.During the second growth stage,mono layer ReSe2 is found to prefere ntially evolve at the irUerface between the first-grown graphene layer and the Au substrate.The unusual stacking behavior is unraveled by in-situ'cutting open'the upper graphene from the defects to expose the lower ReSe2 using scanning tunneling microscopy(STM).From combination of these results with density functional theory calculations,the domain boundaries and edge sites of graphene are proposed to be adsorption sites for Re and Se precursors,further facilitating the growth of ReSe2 at the van der Waals gap of graphene/Au.This work hereby offers an intriguing strategy for obtaining vertical 2D heterostructures featured with an ultra-clean interface and a designed stacking geometry. | Chunyu Xie Shaolong Jiang Xiaolong Zou Yuanwei Sun Liyun Zhao Min Hong Shulin Chen Yahuan Huan Jianping Shi Xiebo Zhou Zhepeng Zhang Pengfei Yang Yuping Shi Porun Liu Qing Zhang Peng Gao Yanfeng Zhang | 2019 | Nano Research2019,12,1: | 4 |
| 9 | Density functional theory(DFT) studies of vanadium-titanium based selective catalytic reduction(SCR) catalysts显示文摘Based on density functional theory(DFT)and basic structure models,the chemical reactions on the surface of vanadium-titanium based selective catalytic reduction(SCR)denitrification catalysts were summarized.Reasonable structural models(non-periodic and periodic structural models)are the basis of density functional calculations.A periodic structure model was more appropriate to represent the catalyst surface,and its theoretical calculation results were more comparable with the experimental results than a nonperiodic model.It is generally believed that the SCR mechanism where NH3 and NO react to produce N2 and H2 O follows an Eley-Rideal type mechanism.NH2 NO was found to be an important intermediate in the SCR reaction,with multiple production routes.Simultaneously,the effects of H2 O,SO2 and metal on SCR catalysts were also summarized. | Ziwei Zhao Erwei Li Yu Qin Xiaolong Liu Yang Zou Heng Wu Tingyu Zhu | 2020 | Journal of Environmental Sciences2020,32,4: | 4 |
| 10 | Effect of methotrexate combined with Sanhuang Yilong decoction on serum and synovial fluid aquaporin levels in rheumatoid arthritis dampness-heat blockage syndrome显示文摘OBJECTIVE:To study the effect of methotrexate(MTX) combined with Sanhuang Yilong decoction(SYD) on aquaporin(AQP) expression,and to explore the role of AQPs in the pathogenesis of rheumatoid arthritis(RA).METHODS:A total of 118 dampness-heat blockage type RA patients who were hospitalized in the General Chengdu Military Hospital between January2014 and December 2016 were selected as subjects in this study(30 patient of these patients with knee joint effusion were assigned to the RA synovial fluid group).For the pre-treatment controlgroups,30 healthy volunteers were recruited as the healthy control group and 30 osteoarthritis(OA) patients with knee joint effusion were included as OA synovial fluid control group.The RA dampnessheat blockage syndrome treatment groups were divided into 45 cases in the combined group and 45 cases in the MTX group.The combined group received MTX combined with SYD treatment while the MTX group received MTX alone.AQP1,AQP2 and AQP3 expressions were detected in the serum and synovial fluid.RESULTS:AQP1 had the highest expression,followed by AQP3,and AQP2.The serum levels of AQP1,AQP2 and AQP3 were all significantly lower than those in the healthy volunteers(P < 0.05),while the synovial fluid AQP1,AQP2 and AQP3 expression in the RA group were comparable to these in the OA groups(P > 0.05).After treatment for2 weeks,serum AQP1,AQP2,AQP3 were significantly increased and erythrocyte sedimentation rate,C-reactive protein,disease activity score of 28 joints were decreased in the combined group(P < 0.05).CONCLUSION:Abnormal expression of AQPs inhibits water metabolism in RA dampness-heat blockage syndrome,so liquid is accumulated at the joint,which may play an important role in the pathogenesis of RA.MTX combined with SYD for the treatment of RA can effectively increase AQP expression. | Liu Defang Yan Jiao Guo Mingyang Luo Yong Yang Mei Yang Min Zou Longfu Li Wan Zhong Xiaolong Liu Tao Hu Yonghe | 2018 | Journal of Traditional Chinese Medicine2018,38,4: | 4 |
| 11 | A Robustness Analysis of CMIP5 Models over the East Asia-Western North Pacific Domain显示文摘 | Tianjun Zhou Xiaolong Chen Bo Wu Zhun Guo Yong Sun Liwei Zou Wenmin Man Lixia Zhang Chao He | 2017 | Engineering2017,3,5: | 4 |
| 12 | High-precision whispering gallery microsensors with ergodic spectra empowered by machine learning显示文摘Whispering gallery mode(WGM)microcavities provide increasing opportunities for precision measurement due to their ultrahigh sensitivity,compact size,and fast response.However,the conventional WGM sensors rely on monitoring the changes of a single mode,and the abundant sensing information in WGM transmission spectra has not been fully utilized.Here,empowered by machine learning(ML),we propose and demonstrate an ergodic spectra sensing method in an optofluidic microcavity for high-precision pressure measurement.The developed ML method realizes the analysis of the full features of optical spectra.The prediction accuracy of 99.97%is obtained with the average error as low as 0.32 kPa in the pressure range of 100 kPa via the training and testing stages.We further achieve the real-time readout of arbitrary unknown pressure within the range of measurement,and a prediction accuracy of 99.51%is obtained.Moreover,we demonstrate that the ergodic spectra sensing accuracy is∼11.5%higher than that of simply extracting resonating modes’wavelength.With the high sensitivity and prediction accuracy,this work opens up a new avenue for integrated intelligent optical sensing. | BING DUAN HANYING ZOU JIN-HUI CHEN CHUN HUI MA XINGYUN ZHAO XIAOLONG ZHENG CHUAN WANG LIANG LIU DAQUAN YANG | 2022 | Photonics Research2022,10,10: | 3 |
| 13 | Diffusion and Regeneration Mechanism of Waste Composite Oils Rejuvenator in Aged Asphalt显示文摘The physical performance of recycled asphalt was used as the main evaluation index to study the optimal range of a self-made rejuvenator.Through the penetration,viscosity and gel permeation chromatography(GPC)tests,the diffusion degree of the rejuvenator under different temperatures and time process was analyzed,and the diffusion efficiency of the rejuvenator was evaluated from the macro and micro perspective.The regeneration mechanism of the rejuvenator in the aged asphalt was also analyzed using the Fourier transform infrared spectroscopy(FTIR),scanning electron microscope(SEM)and chemical composition tests.The research results showed that the optimum rejuvenator content was about 3%.Higher temperature and longer time were beneficial to improving the permeability and diffusion of the rejuvenator.During the aging process,the light components were reduced,and more macromolecular asphaltenes were generated as well as a large number of carbonyl and sulfoxide.After diffusion and regeneration,the light components in the asphalt were supplemented,the wrinkles and gullies of the aged asphalt were almost improved to the surface state of the matrix asphalt. | 李海滨 YANG Fayong ZHANG Fan ZOU Xiaolong ZHAO Guijuan | 2021 | Journal of Wuhan University of Technology(Materials Science)2021,36,5: | 3 |
| 14 | An Improved Image Enhancement Algorithm显示文摘To solve the problems of noise,detail loss and poor contrast in the successive mean quantization transform(SMQT),a new SMQT algorithm based on Otsu algorithm is proposed.In this algorithm,we integrate the optimal threshold selected by the Otsu algorithm into the SMQT algorithm,then obtain the successive mean quantization of the binary tree.By this algorithm,an enhanced image is output with a higher quality.From both subjective visual effect and objective quality evaluation,the experimental results show that the improved algorithm reduces noise,improves contrast and makes the image details more clear. | MA Jing ZOU Chengming JIN Xiaolong | 2017 | Wuhan University Journal of Natural Sciences2017,22,1: | 3 |
| 15 | Experimental study of freak waves due to three-dimensional island terrain in random wave显示文摘An experimental study is carried out for waves passing an isolated reef terrain in a wave tank. A three-dimensional model of a representative and isolated reef terrain in the West Pacific is built. Random wave trains with various periods and wave heights are generated by a wave maker using the improved JONSWAP spectrum. It is observed that there are different kinds of generation processes and waveforms of freak waves. The freak wave factor Hm/Hs (where Hm is the maximum wave height of wave series, and Hs is significant wave height) is analyzed in detail, in terms of the skewness, kurtosis and water depth, as well as the relationship between freak wave height H& and skewness. The freak wave factor Hm/Hs is found to be in positive correlation with the kurtosis, while larger H[x tends to be related with bigger skewness. The rapid variation of water depth, such as slope and seamount, contributes to the occurrence probability of freak waves. | Li Zou Aimin Wang Zhen Wang Yuguo Pei Xiaolong Liu | 2019 | Acta Oceanologica Sinica2019,38,6: | 2 |
| 16 | Improving the mid-infrared energy absorption efficiency by using a dual-band metamaterial absorber显示文摘In this paper, a dual-band mid-infrared metamaterial absorber was proposed to improve the energy absorption efficiency. Up to 99% absorption was obtained at 9.03 and 11.83 μm in the simulation, and each absorption band can be tuned by the dielectric spacing layer, i.e., the dielectric constant and its thickness. The dual-band absorption mechanism was analyzed, and the quite well absorption performance at large incident angles was also presented. The results of this study can be applied in the field of thermal absorbing and solar energy harvesting. | Nan Zhang Peiheng Zhou Shifeng Zou Xiaolong Weng Jianliang Xie Longjiang Deng | 2014 | Progress in Natural Science:Materials International2014,24,2: | 2 |
| 17 | A minimization problem of the risk probability in first passage semi-Markov decision processes with loss rates显示文摘This paper is the first attempt to investigate the risk probability criterion in semi-Markov decision processes with loss rates. The goal is to find an optimal policy with the minimum risk probability that the total loss incurred during a first passage time to some target set exceeds a loss level. First, we establish the optimality equation via a successive approximation technique, and show that the value function is the unique solution to the optimality equation. Second, we give suitable conditions, under which we prove the existence of optimal policies and develop an algorithm for computing ?-optimal policies. Finally, we apply our main results to a business system. | HUANG XiangXiang ZOU XiaoLong GUO XianPing | 2015 | Science China Mathematics2015,58,9: | 2 |
| 18 | First passage Markov decision processes with constraints and varying discount factors显示文摘这份报纸与多限制,州依赖者的折扣因素,和可能无界的费用在可数的州、紧缩的 Borel 行动空格集中于分离时间的 Markov 决定处理的第一个段落(DTMDP ) 的抑制 optimality 问题(警察) 。借助于一条政策的一项所谓的职业措施的性质,我们证明抑制 optimality 问题等价于一(无限维) 职业的集合上的线性编程与一些限制测量,并且因此在合适的条件下面证明一条最佳的政策的存在。用在抑制 optimality 问题和线性编程之间的等价,而且,我们为有限状态和行动的盒子获得一条最佳的政策的一种准确形式。作为一个例子,最后,一个控制排队系统被给说明我们的结果。 | Xiao WU Xiaolong ZOU Xianping GUO | 2015 | Frontiers of Mathematics in China2015,10,4: | 2 |
| 19 | On Derivations of Bounded Hyperlattices显示文摘In this paper we introduce derivations in hyperlatices and derive some basic properties of them. Also, some properties of differential hyperideals and differential hypercongruences are studied. Further we prove that for an injective strong differential hyperlattice(L, d) and for a strongly differential hypercongruence R of(L, d), the quotient hyperlattice(L/R, g) is an injective strongly differential hyperlattice, where g is an injective strong derivation on L/R induced by d. | Juntao WANG Youngbae JUN Xiaolong XIN Yuxi ZOU | 2016 | Journal of Mathematical Research with Applications2016,36,2: | 2 |
| 20 | Identification of Salmonella and Listeria monocytogenes by Near-infrared Spectroscopy and PCA显示文摘Near-infrared spectra of pathogenic bacteria (salmonella and Listeria monocytogenes ) were determined, and the spectral data were analyzed by the projection discriminant analysis based on principal component analysis (PCA). The expected results were obtained. The results showed that salmonella and L. monocytogenes could be distinguished from each other by the near-infrared spectroscopy of the whole cells, cell walls or cytoplasm. | Jiang Chuan Zhang Xiaohong Zou Xiaolong Lu Guangying Liu Yangchun | 2019 | Meteorological and Environmental Research2019,10,4: | 2 |