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| 1 | BODIPY-derived ratiometric fluorescent sensors: pH-regulated aggregation-induced emission and imaging application in cellular acidification triggered by crystalline silica exposure显示文摘Modification of classic fluorophore to possess the emission transitions between aggregation-induced emission(AIE)and intrinsic emission offers reliable approach to the design of ratiometric fluorescent sensors.In this study,a proton acceptor benzimidazole was integrated with BODIPY to form three compounds,BBI-1/2/3,which demonstrated the AIE(~595 nm,I_(agg))in neutral aqueous medium and intrinsic BODIPYemission(~510 nm,I_(int))in acidic medium.All the three showed the ratiometric pH sensing behavior in a dual excitation/dual emission mode,yet BBI-3 displayed still the dual emission ratiometric pH sensing ability.The pH-dependent emission ratio I_(int)/I_(agg)of the three were fully reversible,and no interference was observed from normal abundant chemical species in live cells.Their different p K_a(BBI-1,p K_a4.4;BBI-2,p K_a2.7;BBI-3,p K_a3.6)suggested that the substituents on benzimidazole moiety were essential to govern their functioning pH range.The ratiometric imaging of BBI-1 in A549 cells provided an effective intracellular pH(pH_i)calibration formula corresponding to emission ratio of I_(int)/I_(agg).Ratiometric pH_iimaging in A549 cells upon small particle exposure confirmed the particle-induced cellular acidification with this formula.Both particle size and the chemical nature of the particle contribute to the observed acidification effect.The synchronization of lysosome disruption to cellular acidification in A549 cells upon crystalline silica exposure was directly observed for the first time with BBI-1,showing the potential application of BBI-1 in the study of silicosis and other related diseases.This study demonstrated that endowing fluorophore with AIE/intrinsic emission transition could be a promising strategy for ratiometric sensor design. | Yang Bai Danyang Liu Zhong Han Yuncong Chen Zhongyan Chen Yang Jiao Weijiang He Zijian Guo | 2018 | Science China Chemistry2018，61，11： | 4 |
| 2 | Validation results of NmF2 and hmF2 derived from ionospheric density profiles of GNOS on FY-3C satellite显示文摘The first Global Navigation Satellite System Occultation Sounder(GNOS) which is compatible of both Bei Dou System(BDS)and Global Positioning System(GPS) was successfully launched into orbit onboard the Feng Yun 3 C satellite(FY-3 C) on September 23, 2013, and it has already gathered a large amount of ionosphere radio occultation(RO) data so far. However, the detailed analysis and validation of GPS ionosphere RO data have not been done up to now. Therefore, this paper discusses the configuration of the FY-3 C GNOS, the methods and results of GPS ionosphere occultation processment, the quality analysis of the GPS ionosphere RO products, and the precision consistency between the GNOS GPS ionosphere RO product and ionosonde data. The peak electron density(Nm F2) correlation coefficient is 0.97, the corresponding standard deviation is 16.08%. The peak value altitude(hm F2) correlation coefficient is 0.89, and the corresponding standard deviation is 23.79 km. The in-orbit operation of GNOS provides a basis data set for the monitoring, forecasting and research of ionosphere's space weather. | YANG GuangLin SUN YueQiang BAI WeiHua ZHANG XiaoXin LIU CongLiang MENG XiangGuang BI YanMeng WANG DongWei ZHAO DanYang | 2018 | Science China(Technological Sciences)2018，61，9： | 2 |
| 3 | The C_(6)D_(6)detector system on the Back-n beam line of CSNS显示文摘Introduction The neutron capture cross sections are very important in the field of nuclear device design and basic physics research.Hydrogen-free liquid scintillator such as C_(6)D_(6)detectors are widely used in the neutron capture cross-sectional measurements for the low neutron sensitivity and fast time response.The Back-n white neutron source at China Spallation Neutron Source is the first spallation white neutron source in China,and it is suitable for neutron capture cross-sectional measurement.Materials and methods A C_(6)D_(6)detector system was built in the Back-n experimental station.The pulse height weighting technique was used to determine the system’s detection efficiency.The response to gamma rays of the C_(6)D_(6)detector was measured,and the energy resolution function was determined.Monte Carlo simulation with Geant4 code was carried out to get the weighting function of this C_(6)D_(6)detector system.Additionally,the systematic uncertainty of the weighting function was also determined.Conclusion According to the experimental and simulation results,this C_(6)D_(6)detector system can be used to measure neutron capture cross section. | Jie Ren Xichao Ruan Jie Bao Guangyuan Luan Wei Jiang Qi An Huaiyong Bai Ping Cao Qiping Chen Yonghao Chen Pinjing Cheng Zengqi Cui Ruirui Fan Changqing Feng Minhao Gu Fengqin Guo Changcai Han Zijie Han Guozhu He Yongcheng He Yuefeng He Hanxiong Huang Weiling Huang Xiru Huang Xiaolu Ji Xuyang Ji Haoyu Jiang Hantao Jing Ling Kang Mingtao Kang Bo Li Lun Li Qiang Li Xiao Li Yang Li Yang Li Rong Liu Shubin Liu Xingyan Liu Yinglin Ma Changjun Ning Binbin Qi Zhaohui Song Hong Sun Xiaoyang Sun Zhijia Sun Zhixin Tan Hongqing Tang Jingyu Tang Pengcheng Wang Qi Wang Taofeng Wang Yanfeng Wang Zhaohui Wang Zheng Wang Jie Wen Zhongwei Wen Qingbiao Wu Xiaoguang Wu Xuan Wu Likun Xie Yiwei Yang Han Yi Li Yu Tao Yu Yongji Yu Guohui Zhang Jing Zhang Linhao Zhang Liying Zhang Qingmin Zhang Qiwei Zhang Xianpeng Zhang Yuliang Zhang Zhiyong Zhang Yingtan Zhao Liang Zhou Zuying Zhou Danyang Zhu Kejun Zhu Peng Zhu | 2019 | Radiation Detection Technology and Methods2019，3，3： | 1 |
| 4 | 2-22 Elastic Scattering Studies of Light Proton-rich显示文摘The elastic scattering is an important probe to study the properties of a nucleus. An accurate measurement ofthe elastic scattering differential cross section is very important to determine the optical potential parameters andthe so-called one quarter angle (q1=4). Also, the optical potential parameters of stable nuclei and unstable nucleiare found to be different. 8B, the binding energy of the last proton is only 0.137 MeV, is a well-known protonhalonucleus even there are still some arguments. Many investigations have been done for 8B by measuring thetotal reaction cross sections, breakup cross section and inelastic scattering differential cross section. However, theexperimental data of elastic scattering of 8B and other light proton-rich nuclei on heavy target are few. Therefore, aseries of experiments have been carried out for such nuclei at the Radioactive Ion Beam Line in Lanzhou (RIBLL). | Wang Jiansong Yang Yanyun Wang Qi Pang Danyang Ma Junbing Huang Meirong Ma Peng Jin Shilun Han Jianlong Bai Zhen Ma Weihu Zhou Yuanjie Chen Jie Jin Lei Chen Jiangbo Hu Qiang R. Wada S. Mukherjee | 2014 | IMP & HIRFL Annual Report2014，，1： | 0 |
| 5 | Enhanced monopole transition strength from the cluster decay of ^(13)C显示文摘The inelastic excitations and cluster decay of ^(13)C have been measured using the reaction,9Be(^(13)C, ^(13)C* →~9Be + α)~9Be. We observe strong excitation to the 14.3-MeV(1/2-) resonant state from the cluster-decay channel, leading to an enhanced monopole matrix element of(6.3 ± 0.6) fm^2. This large cluster-related monopole strength is a clear indication of the cluster-structure domination of this state and is consistent with the recent prediction of the orthogonality condition model(OCM). It would be interesting to further explore the three-center molecular rotational band that is initiated from the observed band-head. | Jun Feng YanLin Ye Biao Yang ChengJian Lin HuiMin Jia DanYang Pang ZhiHuan Li JianLing Lou QiTe Li XiaoFei Yang Jing Li HongLiang Zang Qiang Liu Wei Jiang ChenGuang Li Yang Liu ZhiQiang Chen HongYi Wu ChunGuang Wang Wei Liu Xiang Wang JingJing Li DiWen Luo Ying Jiang ShiWei Bai JinYan Xu NanRu Ma LiJie Sun DongXi Wang | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，1： | 0 |
| 6 | Impact of Big Events on Urban Renewal Based on Urban Catalyst Theory: A Case Study of 2016 Rio Summer Olympics and 2010 Shanghai World Expo显示文摘With the acceleration of the process of economic globalization and information synchronization, every major event is accompanied by the simultaneous renewal of the city. In the era of urban development, the launch of major events is also for the renewal and development of the city. 2016 Rio Summer Olympics and 2010 Shanghai World Expo are taken as the research objects. Through the analysis of urban renewal from the perspective of the role of big event catalyst, it is verified that the big event catalyst has a positive impact on urban renewal, transportation, industrial transformation and other aspects. Moreover, it tries to combine the theory of urban catalyst to analyze its inspiration for the Beijing Winter Olympic Games, hoping to play a catalytic role in accelerating the urban renewal and transformation of Beijing and the reorganization of urban structure. | BAI Mei ZHOU Yang TAO Danyang | 2022 | Journal of Landscape Research2022，14，6： | 0 |
| 7 | Melatonin biosynthesis pathways in nature and its production in engineered microorganisms显示文摘Melatonin is a biogenic amine that can be found in plants,animals and microorganism.The metabolic pathway of melatonin is different in various organisms,and biosynthetic endogenous melatonin acts as a molecular signal and antioxidant protection against external stress.Microbial synthesis pathways of melatonin are similar to those of animals but different from those of plants.At present,the method of using microorganism fermentation to produce melatonin is gradually prevailing,and exploring the biosynthetic pathway of melatonin to modify microorganism is becoming the mainstream,which has more advantages than traditional chemical synthesis.Here,we review recent advances in the synthesis,optimization of melatonin pathway.L-tryptophan is one of the two crucial precursors for the synthesis of melatonin,which can be produced through a four-step reaction.Enzymes involved in melatonin synthesis have low specificity and catalytic efficiency.Site-directed mutation,directed evolution or promotion of cofactor synthesis can enhance enzyme activity and increase the metabolic flow to promote microbial melatonin production.On the whole,the status and bottleneck of melatonin biosynthesis can be improved to a higher level,providing an effective reference for future microbial modification. | Xiaotong Xie Dongqin Ding Danyang Bai Yaru Zhu Wei Sun Yumei Sun Dawei Zhang | 2022 | Synthetic and Systems Biotechnology2022，7，1： | 0 |
| 8 | Experimental Study of the Elastic Scattering and Breakup Reactions of Proton Drip-line Nucleus^(8)B on^(208)Pb at energies around Four Times of Coulomb Barrier显示文摘First measurement of the angular distribution of breakup reaction for^(8)B on a^(208)Pb target at an energy around four times of Coulomb barrier was carried out at the National Laboratory of Heavy Ion Research of Institute of Modern Physics. | Wang Kang Yang Yanyun Duan Fangfang Pang Danyang Wang Jiansong Gao Zhihao Ma Peng Xu Shiwei Liu Xingquan Ma Junbing Bai Zhen Hu Qiang Jin Shuya Sun Zhiyu | 2019 | IMP & HIRFL Annual Report2019，，1： | 0 |
| 9 | Experimental Study of the Elastic Scattering of^(10)Be on^(208)Pb at the Energy around Three Times of the Coulomb Barrier显示文摘Elastic scattering is the simplest nuclear process and has been widely used to investigate the structure of the interacting nuclei[1,2]. | Duan Fangfang Yang Yanyun Pang Danyang Hu Bitao Wang Jiansong Wang Kang Yang Guo Valdir Guimaraes Ma Peng Xu Shiwei Liu Xingquan Ma Junbing Bai Zhen Hu Qiang Shu Jinya Sun Xinxin Yao Jiasheng Qi Hangkai Sun Zhiyu | 2019 | IMP & HIRFL Annual Report2019，，1： | 0 |
| 10 | A first comprehensive evaluation of China's GNSS-R airborne campaign: part II—river remote sensing显示文摘The Global Navigation Satellite System Reflectometry(GNSS-R) has been proven to be a powerful technique for retrieving geophysical parameters of ocean and land. Airborne GNSS-R is an important experimental platform, because it is not only needed as validation for spaceborne application, but also possesses the advantages to be capable of remote sensing of small and medium scale targets, such as rivers and lakes. This paper presents an overview of China's airborne GNSS-R campaign conducted on May 30, 2014, in Henan. The campaign has two objectives, i.e.:(1) to examine the capability of a GNSS-R payload developed by National Space Science Center,Chinese Academy of Sciences(NSSC, CAS) for airborneobservations and(2) to study the algorithms for soil moisture and river remote sensing, including altimetry and flow velocity measurement. A previous paper has presented results of soil moisture retrieval as part I, and in this paper,initial results of the Yellow River remote sensing are presented as part II. This paper presents the river altimetry results and explores a new potential application of GNSS-R technology, which is used to detect the flow velocity of the river. The river surface height results observed by code delay altimetry method were consistent with the height results of GPS dual-frequency differential positioning altimetry. The GNSS-R altimetry results showed that decimeter level heights were achieved in 1-min sliding average. Comparing with in situ measurements, the GNSSR flow velocity result was reasonable; the error was about0.027 m/s, which indicated the validity and feasibility of using GNSS-R technique to detect river flow velocity. | Weihua Bai Junming Xia Wei Wan Limin Zhao Yueqiang Sun Xiangguang Meng Congliang Liu Hua Chen Qifei Du Dongwei Wang Danyang Zhao Xianyi Wang Cheng Cheng | 2015 | Science Bulletin2015，60，17： | 0 |
| 11 | Suppressing byproduct formation for high selective CO_(2) reduction over optimized Ni/TiO_(2) based catalysts显示文摘One of the challenges for catalytic CO_(2)reduction is to control product selectivity,and new findings that can modify selectivity would be transformative.Herein,two kinds of TiO_(2)(homemade and commercial)with the same crystal phase but different surface properties are chosen as supports to prepare Ni-based catalysts for CO_(2)reduction,which show distinctly different product selectivity for CO_(2)reduction to CH_(4) or CO,as well as the CO_(2)conversion.The catalysts based on the homemade TiO_(2)support are highly selective for CH_(4) formation,while the latter ones are about 100%selective for CO formation under the same reaction conditions.In addition,the former ones are much active(more than 3 times)than the latter ones.We found that the collaborative contribution of Ti^(3+)and Ni^(2+)species and the electronic metal-support interactions effect maybe the main driving force behind for determining the product selectivity.Methane is almost exclusively produced over the catalysts with abundant Ti^(3+)and Ni^(2+)species and greater electronic metal-support interaction,otherwise,it will give priority to CO generation.The addition of CeO_(2)can reduce the Ni particle size and improve the dispersion of Ni nanoparticles,as well as create more Ti^(3+)species,contributing to the enhancement of CO_(2)conversion,but shows a negligible effect on product selectivity.Furthermore,the in situ DRIFT experiments and kinetic experiments indicate that the CO route is probably involved in the CO_(2)reduction process over the homemade Ni-CeO_(2)/TiO_(2)-CO catalyst with abundant Ti^(3+)and Ni^(2+)species and a strong electronic transform effect. | Danyang Li Ruidong Xu Roong Jien Wong Xing Zhu Dong Tian Lei Jiang Qingjie Guo Hongcun Bai Linan Huang Wen Liu Hua Wang Kongzhai Li | 2022 | Journal of Energy Chemistry2022，31，9： | 0 |
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