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| 1 | Recent progress of surface coating on cathode materials for high-performance lithium-ion batteries显示文摘Lithium-ion batteries (LIB) have received substantial attention in the last 10 years,as they offer great promise as power sources that can lead to the electric vehicle (EV) revolution in the next 5 years.Since the cathode serves as a key component in LIB,its properties significantly affect the performance of the whole system.Recently,the cathode surface modification based on coating technique has been widely employed to enhance the electrochemical performances by improving the material conductivity,stabilising the physical structure of materials,as well as preventing the reactions between the electrode and electrolyte.In this work,we reviewed the present of a number of promising cathode materials for Li-ion batteries.After that,we summarized the very recent research progress focusing on the surface coating strategies,mainly including the coating materials,the coating technologies,as well as the corresponding working mechanisms for cathodes.At last,the challenges faced and future guidelines for optimizing cathode materials are discussed.In this study,we propose that the structure of cathode is a crucial factor during the selection of coating materials and technologies. | Peiyuan Guan Lu Zhou Zhenlu Yu Yuandong Sun Yunjian Liu Feixiang Wu Yifeng Jiang Dewei Chu | 2020 | Journal of Energy Chemistry2020,29,4: | 28 |
| 2 | Progress of the key materials for organic solar cells显示文摘Organic solar cells have attracted academic and industrial interests due to the advantages like lightweight,flexibility and roll-to-roll fabrication.Nowadays,18%power conversion efficiency has been achieved in the state-of-the-art organic solar cells.The recent rapid progress in organic solar cells relies on the continuously emerging new materials and device fabrication technologies,and the deep understanding on film morphology,molecular packing and device physics.Donor and acceptor materials are the key materials for organic solar cells since they determine the device performance.The past 25 years have witnessed an odyssey in developing high-performance donors and acceptors.In this review,we focus on those star materials and milestone work,and introduce the molecular structure evolution of key materials.These key materials include homopolymer donors,D-A copolymer donors,A-D-A small molecular donors,fullerene acceptors and nonfullerene acceptors.At last,we outlook the challenges and very important directions in key materials development. | Yang Tong Zuo Xiao Xiaoyan Du Chuantian Zuo Yuelong Li Menglan Lv Yongbo Yuan Chenyi Yi Feng Hao Yong Hua Ting Lei Qianqian Lin Kuan Sun Dewei Zhao Chunhui Duan Xiangfeng Shao Wei Li Hin-Lap Yip Zhengguo Xiaol Bin Zhang Qingzhen Bian Yuanhang Cheng Shengjian Liu Ming Cheng Zhiwen Jin Shangfeng Yang Liming Ding | 2020 | Science China Chemistry2020,63,6: | 15 |
| 3 | Two-Stage Transformerless Dual-Buck PV Grid-Connected Inverters with High Efficiency显示文摘A semi-two-stage common-ground-type transformerless dual-buck-based grid-connected inverter is proposed in this paper.The common-ground-type topology can eliminate common mode(CM)leakage current by connecting the negative terminal of the photovoltaic(PV)directly to the neutral point of the grid,which bypasses the PV array’s stray capacitance.The dual-buck-based topology guarantees increased robustness since the dc-link cannot be short-circuited by a shoot-through event.The semi-two-stage topology features multi-level characteristic,which has a lower forward-voltage drop and smaller dv/dt.Compared with the conventional two-stage inverter,the proposed topology achieves higher efficiency and higher reliability.Experimental results of a 1.5kW prototype show that the proposed inverter is able to achieve high efficiency and low leakage currents. | Li Zhang Fengkai Jiang Dewei(David)Xu Kai Sun Yongqiang Hao Tao Zhang | 2018 | Chinese Journal of Electrical Engineering2018,4,2: | 4 |
| 4 | Medical Additive Manufacturing: From a Frontier Technology to the Research and Development of Products显示文摘1.Research and development(R&D)and the challenges of raw materials for medical additive manufacturing Raw materials for medical additive manufacturing have a wide range of commonalities that are also seen in many other fields,making them an important basis in the field of three-dimensional(3D)printing.Problems and challenges related to material types,powder properties,formability,viscoelasticity,and so forth also share common features.For example,many metal materials are used in the field of aviation,while metals,polymers,and inorganic materials are used in the field of biomedicine.The most widely used materials in biomedicine are biocompatible.Various homogeneous and non-homogeneous composites are also available for 3D printing,and impose an additional challenge in additive manufacturing;the use of heterogeneous composites in 3D printing is particularly challenging. | Guixing Qiu Wenjiang Ding Wei Tian Ling Qin Yu Zhao Lianmeng Zhang Jian Lu Daijie Chen Guangyi Yuan Chengtie Wu Bingheng Lu Ruxu Du Jimin Chen Mo Elbestawi Zhongwei Gu Dichen Li Wei Sun Yuanjin Zhao Jie He Dadi Jin Bin Liu Kai Zhang Jianmo Li Kam WLeong Dewei Zhao Dingjun Hao Yingfang Ao Xuliang Deng Huilin Yang ShaoKeh Hsu Yingqi Chen Long Li Jianping Fan Guohui Nie Yun Chen Hui Zeng Wei Chen Yuxiao Lai | 2020 | Engineering2020,6,11: | 1 |
| 5 | Treatment of severe IgA nephropathy:mycophenolate mofetil/prednisone compared to cyclophosphamide/prednisone显示文摘 | Liu X Dewei D Sun S | | 0,,: | 1 |
| 6 | Treatment of severe IgA nephropa- thy: mycophenolate mofetil/prednisone compared to cyelophospha- mide/prednisone显示文摘 | Liu X Dewei D Sun S | 2014 | Int J Clin Pharmacol Ther2014,52,2: | 1 |
| 7 | Comparison of the neuroprotective effects and recovery profiles of isoflurane, sevoflu- rane and desflurane as neurosurgical pre - conditioning on ischemi-a/reperfusion cerebral injury 显示文摘 | Shan Jinghua Sun Lianmei Wang Dewei | 2015 | International Journal of Clinical and Experimental Pathology2015,8,2: | 1 |
| 8 | Orbital-regulated interfacial electronic coupling endows Ni3N with superior catalytic surface for hydrogen evolution reaction显示文摘The interstitial structure and weak Ni-N interaction of Ni3N lead to high unoccupied d orbital energy and unsuitable orbital orientation,which consequently results in weak orbital coupling with H2O and slow water dissociation kinetics for alkaline hydrogen evolution catalysis.Herein,we successfully lower the unoccupied d orbital energy of Ni3N to strengthen the interfacial electronic coupling by employing the strong electron pulling capability of oxygen dopants.The prepared O-Ni3N catalyst delivers an overpotential of 55 mV at 10 mA cm−2,very close to the commercial Pt/C.Refined structural characterization indicates the oxygen incorporation can decrease the electron densities around the Ni sites.Moreover,density functional theory calculation further proves the oxygen incorporation can create more unoccupied orbitals with lower energy and superior orientation for water adsorption and dissociation.The concept of orbital-regulated interfacial electronic coupling could offer a unique approach for the rational design of hydrogen evolution catalysts and beyond. | Yanyan Fang Da Sun Shuwen Niu Jinyan Cai Yipeng Zang Yishang Wu Linqin Zhu Yufang Xie Yun Liu Zixuan Zhu Amirabbas Mosallanezhad Di Niu Zheng Lu Junjie Shi Xiaojing Liu Dewei Rao Gongming Wang Yitai Qian | 2020 | Science China Chemistry2020,63,11: | 1 |
| 9 | Study on Induction of Phytolacca acinosa Roxb. Polyploids with Colchicine显示文摘[Objective] This study aimed to obtain Phytolacca acinosa Roxb. polyploids and provide high-efficiency raw materials for the preparation of biological pesticides. [Method]Terminal bud growing points of Phytolacca acinosa Roxb. seedlings were treated with 0. 1%,0. 2%,0. 3% colchicine and 1% agar solution for 24,48 and 72 h,respectively,while Phytolacca acinosa Roxb. without treatment was adopted as the control. The mutagenic effect of various concentrations of colchicine was calculated. Phytolacca acinosa Roxb. mutants were identified using morphological,anatomical and cytological methods. [Result] Induction with 0. 2% colchicine for 48 h led to the highest mutagenic effect. Compared with the control,leaf width and leaf thickness of mutants were enhanced by 40. 15% and 33. 25%,respectively; vertical and horizontal diameter of stomata of mutants were enhanced by 30. 25% and 60. 82%,respectively; the stomata density of mutants was improved by 150%. Identification of meiotic chromosome of pollen mother cells using compression method showed that the chromosome number of microspore cells of Phytolacca acinosa Roxb. mutants was n = 2x = 36,while that of the control was n = x = 18,indicating that the mutants were tetraploids. [Conclusion] Phytolacca acinosa Roxb. polyploids were induced using the traditional liquid droplet method,which was easy and direct with simple operation and good effect to acquire a large number of polyploid materials within a short time. | Dongye YANG Lizhen ZHANG Jie LIU Dewei SUN | 2013 | Agricultural Biotechnology2013,2,4: | 1 |
| 10 | Treatment of severe Ig A nephropathy:mycophenolatemofetil/prednisone compared to cyclophosphamide/prednisone显示文摘 | Liu X Dewei D Sun shiren | 2014 | Int J Clin Pharmacol Ther2014,2,2: | 1 |
| 11 | Accelerating water dissociation kinetics of Ni3N by tuning interfacial orbital coupling显示文摘The high unoccupied d band energy of Ni_(3)N basically results in weak orbital coupling with water molecule,consequently leading to slow water dissociation kinetics.Herein,we demonstrate Cr doping can downshift the unoccupied d orbitals and strengthen the interfacial orbital coupling to boost the water dissociation kinetics.The prepared Cr-Ni_(3)N/Ni displays an impressive overpotential of 37 mV at 10 mA·cmgeo-2,close to the benchmark Pt/C in 1.0 M KOH solution.Refined structural analysis reveals the Cr dopant exists as the Cr-N_(6)states and the average d band energy of Ni_(3)N is also lowered.Density functional theory calculation further confirms the downshifted d band energy can strengthen the orbital coupling between the unpaired electrons in O 2p and the unoccupied state of Ni 3d,which thus facilitates the water adsorption and dissociation.The work provides a new concept to achieve on-demand functions for hydrogen evolution catalysis and beyond,by regulating the interfacial orbital coupling. | Yishang Wu Yufang Xie Shuwen Niu Yipeng Zang Jinyan Cai Zenan Bian Xuanwei Yin Yanyan Fang Da Sun Di Niu Zheng Lu Amirabbas Mosallanezhad Huijuan Wang Dewei Rao Hongge Pan Gongming Wang | 2021 | Nano Research2021,14,10: | 1 |
| 12 | Cu_(2+1)O/CuO_(x)heterostructures promote the electrosynthesis of C^(2+)products from CO_(2)显示文摘Manipulating the oxidation state of Cu catalysts can significantly affect the selectivity and activity of electrocatalytic carbon dioxide reduction(CO_(2)RR).However,the thermodynamically favorable cathodic reduction to metallic states typically leads to catalytic deactivation.Herein,a defect construction strategy is employed to prepare crystalline/amorphous Cu_(2+1)O/CuO_(x)heterostructures(c/a-CuO_(x))with abundant Cu0 and Cuδ+(0<δ<1)sites for CO_(2)RR.The C^(2+)Faradaic efficiency of the heterostructured Cu catalyst is up to 81.3%,with partial current densities of 406.7 mA·cm−2.Significantly,real-time monitoring of the Cu oxidation state evolution by in-situ Raman spectroscopy confirms the stability of Cuδ+species under long-term high current density operation.Density functional theory(DFT)calculations further reveal that the adjacent Cu0 and Cuδ+sites in heterostructured c/a-CuO_(x)can efficiently reduce the energy barrier of CO coupling for C^(2+)products. | Rongbo Sun Cong Wei Zixiang Huang Shuwen Niu Xiao Han Cai Chen Haoran Wang Jia Song Jun-Dong Yi Geng Wu Dewei Rao Xusheng Zheng Yuen Wu Gongming Wang Xun Hong | 2023 | Nano Research2023,16,4: | 0 |
| 13 | High Temperature-preventing Cultivation Technology of Single-season Middle Rice for High Yield and High Quality in Jianghuai Area显示文摘In recent years,with the global climate change,the frequency and duration of high temperature in summer and autumn have increased,causing high temperature heat damage to summer crops such as rice and maize.From the end of July to early August is the main period of high temperature occurrence,during which the daily average temperature above 30℃is a high probability event,and even the highest temperature is above 38℃,while this period coincides with the booting-blooming-filling stage of the single-season middle rice in Jianghuai,especially the middle-season indica rice,so it often leads to the degradation of rice spikelets,pollen abortion,difficulty in pollen dispersion,and even difficulty in heading,resulting in a serious decline in the seed setting rate and poor filling of grains,which finally affect the yield and quality.Based on the goal of high-yielding high-quality rice cultivation,this paper proposed targeted technical measures for single-season middle rice from the aspects of planting time sequence optimization,selection of high-temperature-resistant varieties,population construction,fertilizer and water management technology,and how to compensate for the occurrence of unexpected disasters to promote plant growth.This study provides technical support for high-yielding high-quality stress-resistant and disaster-reducing rice cultivation technology. | Dewen ZHANG Wei ZHANG Youzun XU Wanlin WANG Dewei TAI Xiaozhong ZHANG Xueyuan SUN | 2022 | Agricultural Biotechnology2022,11,2: | 0 |
| 14 | Unraveling the Effect of Stacking Configurations on Charge Transfer in WS_(2) and Organic Semiconductor Heterojunctions显示文摘Photoinduced interfacial charge transfer plays a critical role in energy conversion involving van der Waals(vdW)heterostructures constructed of inorganic nanostructures and organic materials.However,the effect of molecular stacking configurations on charge transfer dynamics is less understood.In this study,we demonstrated the tunability of interfacial charge separation in a type-Ⅱ heterojunction between monolayer(ML)WS_(2) and an organic semiconducting molecule[2-(3″′,4′-dimethyl-[2,2′:5′,2′:5″,2″′-quaterthiophen]-5-yl)ethan-1-ammonium halide(4Tm)]by rational design of relative stacking configurations.The assembly between ML-WS_(2) and the 4Tm molecule forms a face-to-face stacking when 4Tm molecules are in a selfaggregation state.In contrast,a face-to-edge stacking is observed when 4Tm molecule is incorporated into a 2D organic-inorganic hybrid perovskite lattice.The face-to-face stacking was proved to be more favorable for hole transfer from WS_(2) to 4Tm and led to interlayer excitons(IEs)emission.Transient absorption measurements show that the hole transfer occurs on a time scale of 150 fs.On the other hand,the face-to-edge stacking resulted in much slower hole transfer without formation of IEs.This inefficient hole transfer occurs on a similar time scale as A exciton recombination in WS_(2),leading to the formation of negative trions.These investigations offer important fundamental insights into the charge transfer processes at organic−inorganic interfaces. | Shuchen Zhang Dewei Sun Jiaonan Sun Ke Ma Zitang Wei Jee Yung Park Aidan H.Coffey Chenhui Zhu Letian Dou Libai Huang | 2023 | Precision Chemistry2023,1,7: | 0 |
| 15 | Characterization of tree shrew telomeres and telomerase显示文摘The use of tree shrews as experimental animals for biomedical research is a new practice.Several recent studies suggest that tree shrews are suitable for studying cancers,including breast cancer,glioblastoma,lung cancer,and hepatocellular carcinoma.However,the telomeres and the telomerase of tree shrews have not been studied to date.Here,we characterize telomeres and telomerase in tree shrews.The telomere length of tree shrews is approximately 23 kb,which is longer than that of primates and shorter than that of mice,and it is extended in breast tumor tissues according to Southern blot and flow-fluorescence in situ hybridization(FISH)analyses.Tree shrew spleen,bone marrow,testis,ovary,and uterus show high telomerase activities,which are increased in breast tumor tissues by telomeric repeat amplification protocol assays.The telomere length becomes shorter,and telomerase activity decreases with age.The tree shrew TERT and TERC are more highly similar to primates than to rodents.These findings lay a solid foundation for using tree shrews to study aging and cancers. | Jian Sun Wenjing Liu Yongbo Guo Hailin Zhang Dewei Jiang Ying Luo Rong Liu Ceshi Chen | 2021 | Journal of Genetics and Genomics2021,48,7: | 0 |
| 16 | DNA damage chemotherapeutic drugs suppress basal-like breast cancer growth by down-regulating the transcription of the FOXO1-KLF5 axis显示文摘Most basal-like breast cancers(BLBCs)have a poor prognosis and high crossover with triple-negative breast cancers(TNBCs).However,approximately 50%of TNBC patients develop chemoresistance.^(1) Dexamethasone reportedly induces Krüppel-like factor 5(KLF5)and can cause docetaxel and cisplatin resistance in TNBC.A super-enhancer can maintain the transcription of KLF5. | Qiuxia Cui Jian Sun Jingping Yuan Juanjuan Li Chuanyu Yang Guangshi Du Chengang Zhou Pu Qiu Jidong Gao Yuanqi Zhang Dewei Jiang Ceshi Chen | 2024 | Genes & Diseases2024,11,1: | 0 |