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| 1 | Rapid growth of a large-scale(600 mm aperture) KDP crystal and its optical quality显示文摘Potassium dihydrogen phosphate(KDP) single crystals are the only nonlinear crystals currently used for electro-optic switches and frequency converters in inertial confinement fusion research, due to their large dimension and exclusive physical properties. Based on the traditional solution-growth process, large bulk KDP crystals, usually with sizes up to600 × 600 mm2 so as to make a frequency doubler for the facility requirement loading highly flux of power laser, can be grown in standard Holden-type crystallizers, without spontaneous nucleation and visible defects, one to two orders of magnitude faster than by conventional methods. Pure water and KDP raw material with a few ion impurities such as Fe,Cr, and Al(less than 0.1 ppm) were used. The rapid-growth method includes extreme conditions such as temperature range from 60 to 35℃ , overcooling up to 5℃ , growth rates exceeding 10 mm/day, and crystal size up to 600 mm. The optical parameters of KDP crystals were determined. The optical properties of crystals determined indicate that they are of favorable quality for application in the facility. | Guohui Li Guozong Zheng Yingkun Qi Peixiu Yin En Tang Fei Li Jing Xu Taiming Lei Xiuqin Lin Min Zhang Junye Lu Jinbo Ma Youping He Yuangen Yao | 2014 | High Power Laser Science and Engineering2014，2，1： | 3 |
| 2 | Identification of Histoplasma causing an unexplained disease cluster in Matthews Ridge, Guyana显示文摘Here,we report the identification of Histoplasma causing an unexplained disease cluster in Matthews Ridge,Guyana.In March 2019,14 employees of Chongqing Bosai Mining Company,China,working in a manganese mining of Guyana,had unexplained fever,and two of them died.We obtained lung and brain tissues as well as the blood samples from the two deceased cases(patient No.1 and 2),and bronchoscopy lavages and cerebrospinal fluid samples from one severe case(patient No.3),respectively.All samples were tested by pathological examination,high-throughput sequencing,and real-time PCR.Pathological detection showed the presence of spore-like structures in the lung tissue of patient No.1,indicating a fungal infection in this patient.Nanopore sequencing identified the existing of H.capsulatum in the lung tissue sample within 13 h.Next-generation sequencing identified specific fragments of H.capsulatum in all of the samples tested(lung,brain and blood serum from the deceased cases,and plasma from the severe case).Real-time PCR assays did not reveal any viral infection related to transmission from bat feces.We conclude that H.capsulatum was the causative pathogen of this disease cluster based on epidemiologic,clinical,pathological and nucleic acid evidence. | Ji Wang Weimin Zhou Hua Ling Xiaoping Dong Yi Zhang Jiandong Li Yong Zhang Jingdong Song William J.Liu Yang Li Ruiqing Zhang Wei Zhen Kun Cai Shuangli Zhu Dongyan Wang Jinbo Xiao Yigang Tong Wenli Liu Lihua Song Wei Wu Yang Liu Xiang Zhao Ruihuan Wang Sheng Ye Jing Wang Roujian Lu Baoying Huang Fei Ye Wenwen Lei Rongbao Gao Qi Shi Cao Chen Jun Han Wenbo Xu George F.Gao Xuejun Ma Guizhen Wu | 2019 | Biosafety and Health2019，1，3： | 3 |
| 3 | Ultra-deep desulfurization of diesel by selective oxidation with [C 18 H 37 N(CH 3 ) 3 ] 4 [H 2 NaPW 10 O 36 ] catalyst assembled in emulsion droplets显示文摘 | Hongying Lü Jinbo Gao Zongxuan Jiang Fei Jing Yongxing Yang Gang Wang Can Li | 2006 | Journal of Catalysis2006，，2： | 1 |
| 4 | pH - responsive PolysaccharideMicrocapsules through Covalent Bonding Assembly 显示文摘 | Yi Jia Jinbo Fei Yue Cui | 2011 | ChemicalCommunications2011，47，4： | 1 |
| 5 | Controlled fabrication of polyaniline spherical and cubic shells with hierarchical nanostructures 显示文摘 | Fei Jinbo Cui Yue Yan Xuehai | 2009 | ACS Nano2009，3，11： | 1 |
| 6 | Deep desulfurization from fuel oil via selective oxidation using an amphiphilic peroxotungsten catalyst assembled in emulsion droplets显示文摘 | Jinbo Gao Shouguo Wang Zongxuan Jiang Hongying Lu Yongxing Yang Fei Jing Can Li | 2006 | Journal of Molecular Catalysis A Chemical2006，，1： | 1 |
| 7 | Selective Oxidations on Recoverable Catalysts Assembled in Emulsions显示文摘 | Can Li Jinbo Gao Zongxuan Jiang Shouguo Wang Hongying Lu Yongxing Yang Fei Jing | 2005 | Topics in Catalysis (-)2005，，12： | 1 |
| 8 | Ultra-deep desulfurization of diesel by selective oxidation with [C 18 H 37 N(CH 3 ) 3 ] 4 [H 2 NaPW 10 O 36 ] catalyst assembled in emulsion droplets显示文摘 | Hongying Lü Jinbo Gao Zongxuan Jiang Fei Jing Yongxing Yang Gang Wang Can Li | 2006 | Journal of Catalysis2006，，2： | 1 |
| 9 | Controlled Preparation of MnO2 Hierarchical Hollow Nanostructures and Their Application in Water Treatment显示文摘 | Fei Jinbo Cui Yue Yan Xuehai | 2008 | Advanced Materials2008，20，： | 1 |
| 10 | Mutation and inhibition studies of mevalonate 5-diphosphate decarboxylase显示文摘 | Qiu Yongge Gao Jinbo Guo Fei | 2007 | Bioorganic & Medicinal Chemistry Letters2007，17，22： | 1 |
| 11 | Selective Oxidations on Recoverable Catalysts Assembled in Emulsions显示文摘 | Can Li Jinbo Gao Zongxuan Jiang Shouguo Wang Hongying Lu Yongxing Yang Fei Jing | 2005 | Topics in Catalysis (-)2005，，1： | 1 |
| 12 | Large-scale preparation of 3D self-assembled iron hydroxide and oxide hierarchical nanostructures and their applications for water treatment显示文摘 | Jinbo Fei Yue Cui Jie Zhao | 2011 | J Mater Chem2011，21，11： | 1 |
| 13 | Design spherical particles of potassium peroxymonosulfate compound salt with high stability and good powder properties via an agglomeration-dissolution mechanism显示文摘With the outbreak of COVID-19,disinfection protection has become a necessary measure to prevent infection.As a new type of disinfectant,potassium peroxymonosulfate compound salt(PMS)has the advantages of good bactericidal effect,non-toxicity,high safety and stability.However,the current PMS products with irregular particle shapes lead to poor flowability,high hygroscopicity,poor stability of reactive oxygen species(ROS)and serious caking problems.In this work,an agglomeration-dissolution mechanism was designed to prepare spherical PMS particles with large size(>300μm)and high sphericity(up to 90%),effectively addressing the above problems.Shaping(dissolution and abrasion)is the key to improving sphericity,which is mainly controlled by the design of the heating mode,residence time and stirring rate.Compared with the irregular PMS particles,the large spherical particles present better flowability(angle of repose decreased by 35.80%,Carr's index decreased by 64.29%,Hausner's ratio decreased by 19.14%),lower hygroscopicity(decreased by 38.0%),lower caking ratio(decreased by 84.50%),and higher stability(the monthly loss of ROS was reduced by 61.68%).The agglomeration-dissolution mechanism demonstrates the crystallization,agglomeration,dissolution and abrasion process of inorganic salt crystals,providing an opportunity to prepare high-end inorganic crystal materials with high-quality morphologies. | Shanshan Feng Changyou Yu Shilin Guo Jinbo Ouyang Fei Yin Xiaodong Zhang Yongjian Zhang Mingyang Chen Dandan Han Junbo Gong Jingkang Wang | 2023 | Particuology2023，，9： | 0 |
| 14 | Free radical fluoroalkylation of terminal alkenes and alkynes with iododifluoromethanesulfonamides显示文摘Free radical fluoroalkylation of terminal alkenes and alkynes with iododifluoromethanesulfonamides has been successfully achieved.It was found that both the catalytic amount of sodium dithionite (Na2S2O4) and the stoichiometric amount of triethylborane (Et3B)/air can efficiently initiate the current free-radical atom transfer reaction. | ZHU JieMing,WANG Fei & HU JinBo CAS Key Laboratory of Organofluorine Chemistry Shanghai Institute of Organic Chemistry,Chinese Academy of Sciences,Shanghai 200032,China | 2011 | Science China Chemistry2011，54，1： | 0 |
| 15 | Enhanced Bioenergy Transformation by Metal-Free Electrozyme-Based Mitochondrion Nanoarchitectonics显示文摘Herein,we couple a synthetic electrozyme in a supramolecule-assembled nanoarchitecture to achieve enhanced bioenergy transformation by mimicking mitochondrial oxidative phosphorylation.Different from the natural counterpart,the metal-free electrozyme is a semiconducting polymer deposited on an electrode.The wellmatched electrocatalytic property of the electrozyme permits oxidization of reduced nicotinamide adenine dinucleotide(NADH)to release protons under a much lower electric potential.As a consequence,the generated proton gradient drives rotary catalysis of adenosine 5′-triphosphate(ATP)synthase reconstituted in a lipid membrane to produce ATP.Remarkably,electrochemical bioenergy conversion of NADH to ATP is accomplished with much higher efficiency in such a bio-like system compared with the natural mitochondria.This work integrates synthetic and natural catalytic chemistry to facilitate enhanced bioenergy transformation,thereby greatly improving prospects in ATP-fueled bioapplications. | Tonghui Wang Jinbo Fei Zhenzhen Dong Xia Xu Weiguang Dong Junbai Li | 2023 | CCS Chemistry2023，5，7： | 0 |
| 16 | Black Phosphorus Nanosheets Enhance Photophosphorylation by Positive Feedback显示文摘We construct a natural-artificial hybrid architecture containing black phosphorus nanosheets(BPNS)to enhance photosynthesis of chloroplast in a positive-feedback manner.In this architecture,oxygen yielded by photosynthesis during water splitting by photosystemⅡpromotes the photoreaction of BPNS to produce proton and inorganic phosphate(Pi).Further,transmembrane proton gradient is increased to drive ATP synthase to synthesize ATP.Meanwhile,additional photogenerated electrons produced by BPNS are transferred to the photosynthesis process.As a consequence,photosynthesis performed by chloroplast is improved.Quantitatively,photophosphorylation efficacy of the hybrid system is increased by 1.89 times in the case of Pi deficiency.This work offers a new path to enhance solar-to-chemical energy conversion,holding promise in boosting natural photosynthesis. | Zhenzhen Dong Jinbo Fei Tonghui Wang Xia Xu Weiguang Dong Junbai Li | 2022 | Chinese Journal of Chemistry2022，40，8： | 0 |
| 17 | Gas-Induced Phase Transition of Dipeptide Supramolecular Assembly显示文摘The manipulation of supramolecular assembly enables single-component architectures to possess diverse structures and functions.Here,we report directed phase transitions of dipeptide supramolecular gel to crystals with excellent selectivity and tunable mechanical properties.To be specific,lamellar-to-orthorhombic rearrangement of dipeptide molecules in the supramolecular assembly was guided by application of ammonia gas,while lamellar-tohexagonal realignment was generated upon water vapor exposure of the assembly.Importantly,this crystal phase control originated from distinct gas-mediated reconstitution of hydrogen-bonding interactions,which endowed the dipeptide materials with remarkably modulated stiffness.The selective phase transformation offers a simple and effective platform for self-assembling peptide crystals with diverse long-range-ordered structures from a single gel-state aggregation.This work opens up new perspectives on peptide-based biomaterials via gas-directed hydrogen-bonding chemistry. | Huimin Xue Jinbo Fei Aoli Wu Xia Xu Junbai Li | 2021 | CCS Chemistry2021，3，11： | 0 |
| 18 | Laser-Derived Interfacial Confinement Enables Planar Growth of 2D SnS_(2) on Graphene for High-Flux Electron/Ion Bridging in Sodium Storage显示文摘Establishing covalent heterointerfaces with face-to-face contact is promising for advanced energy storage,while challenge remains on how to inhibit the anisotropic growth of nucleated crystals on the matrix.Herein,faceto-face covalent bridging in-between the 2 D-nanosheets/graphene heterostructure is constructed by intentionally prebonding of laser-manufactured amorphous and metastable nanoparticles on graphene,where the amorphous nanoparticles were designed via the competitive oxidation of Sn-O and Sn-S bonds,and metastable feature was employed to facilitate the formation of the C-S-Sn covalent bonding in-between the heterostructure.The face-to-face bridging of ultrathin SnS;nanosheets on graphene enables the heterostructure huge covalent coupling area and high loading and thus renders unimpeded electron/ion transfer pathways and indestructible electrode structure,and impressive reversible capacity and rate capability for sodium-ion batteries,which rank among the top in records of the SnS_(2)-based anodes.Present work thus provides an alternative of constructing heterostructures with planar interfaces for electrochemical energy storage and even beyond. | Xiaosa Xu Fei Xu Xiuhai Zhang Changzhen Qu Jinbo Zhang Yuqian Qiu Rong Zhuang Hongqiang Wang | 2022 | Nano-Micro Letters2022，14，6： | 0 |
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