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| 1 | Ionic liquids produce heteroatom-doped Pt/TiO2 nanocrystals for efficient photocatalytic hydrogen production显示文摘It is of great importance to develop facile strategies to synthesize catalysts with desirable compositions and structures for high-performance photocatalytic hydrogen generation. In this work, we put forward an ionic liquid assisted one-pot route for the synthesis of heteroatom-doped Pt/TiO2 composite material. This route is simple, environmentally benign and adjustable owing to the designable properties of ionic liquids. The as-synthesized Pt/TiO2 nanocrystals exhibit high activity and stability for the photocatalytic hydrogen generation under simulated solar irradiation. This method can be easily applied to the synthesis of various kinds of metal/TiO2 composites doped with desirable heteroatoms (e.g., F, Cl, Br, etc). | Xiuniang Tan Jianling Zhang Dongxing Tan Jinbiao Shi Xiuyan Cheng Fanyu Zhang Lifei Liu Bingxing Zhang Zhuizhui Su Buxing Han | 2019 | Nano Research2019，12，8： | 5 |
| 2 | Supercritical CO2 produces the visible-light-responsive TiO2/COF heterojunction with enhanced electron-hole separation for highperformance hydrogen evolution显示文摘To construct the heterojunctions of TiO2 with other compounds is of great importance for overcoming its inherent shortages and improving the visible-light photocatalytic performance.Here we propose the construction of TiO2/covalent organic framework(COF)heterojunction with tight connection by a supercritical CO2(SC CO2)method,which helps bridging the transformation paths for photo-induced charge between T i02 and COF.The produced T i02/COF heterojunction performs a H2 evolution of 3,962 nmol·g^-1·h^-1 under visible-light irradiation,which is-25 times higher than that of pure TiO2 and 4.5 folds higher than that of TiO2/COF synthesized by the conventional solvothermal method.This study opens up new possibilities for constructing heterojunctions for solar energy utilization. | Lifei Liu Jianling Zhang Xiuniang Tan Bingxing Zhang Jinbiao Shi Xiuyan Cheng Dongxing Tan Buxing Han Lirong Zheng Fanyu Zhang | 2020 | Nano Research2020，13，4： | 4 |
| 3 | Progress in octahedral spherical hohlraum study显示文摘In this paper,we give a review of our theoretical and experimental progress in octahedral spherical hohlraum study.From our theoretical study,the octahedral spherical hohlraums with 6 Laser Entrance Holes(LEHs)of octahedral symmetry have robust high symmetry during the capsule implosion at hohlraum-to-capsule radius ratio larger than 3.7.In addition,the octahedral spherical hohlraums also have potential superiority on low backscattering without supplementary technology.We studied the laser arrangement and constraints of the octahedral spherical hohlraums,and gave a design on the laser arrangement for ignition octahedral hohlraums.As a result,the injection angle of laser beams of 50°-60°was proposed as the optimum candidate range for the octahedral spherical hohlraums.We proposed a novel octahedral spherical hohlraum with cylindrical LEHs and LEH shields,in order to increase the laser coupling efficiency and improve the capsule symmetry and to mitigate the influence of the wall blowoff on laser transport.We studied on the sensitivity of the octahedral spherical hohlraums to random errors and compared the sensitivity among the octahedral spherical hohlraums,the rugby hohlraums and the cylindrical hohlraums,and the results show that the octahedral spherical hohlraums are robust to these random errors while the cylindrical hohlraums are the most sensitive.Up till to now,we have carried out three experiments on the spherical hohlraum with 2 LEHs on Shenguang(SG)laser facilities,including demonstration of improving laser transport by using the cylindrical LEHs in the spherical hohlraums,spherical hohlraum energetics on the SGIII prototype laser facility,and comparisons of laser plasma instabilities between the spherical hohlraums and the cylindrical hohlraums on the SGIII laser facility. | Ke Lan Jie Liu Zhichao Li Xufei Xie Wenyi Huo Yaohua Chen Guoli Ren Chunyang Zheng Dong Yang Sanwei Li Zhiwen Yang Liang Guo Shu Li Mingyu Zhang Xiaoying Han Chuanlei Zhai Lifei Hou Yukun Li Keli Deng Zheng Yuan Xiayu Zhan Feng Wang Guanghui Yuan Haijun Zhang Bobin Jiang Lizhen Huang Wei Zhang Kai Du Runchang Zhao Ping Li Wei Wang Jingqin Su Xuewei Deng Dongxia Hu Wei Zhou Huaiting Jia Yongkun Ding Wanguo Zheng Xiantu He | 2016 | Matter and Radiation at Extremes2016，1，1： | 2 |
| 4 | Improved strength and ductility of AZ31B Mg alloy sheets processed by accumulated extrusion bonding with artificial cooling显示文摘In this study,accumulated extrusion bonding(AEB)process with application of artificial water cooling was successfully performed to fabricate fined-grains AZ31B Mg alloy sheets at 150℃,200℃ and 250℃.The resultant microstructure and mechanical properties are systematically investigated.It reveals that the processing temperature has an important effect on the microstructural evolution during extrusion.During AEB process at 150℃ and 200℃,{10-12}tensile twinning was activated at early stage of extrusion,and subsequently continuous dynamic recrystallization(CDRX)occurred and dominated the further deformation.However,for the sample extruded at 250℃,hardly any twins can be observed,and new fined dynamic recrystallized grains were found along grain boundaries.Artificial cooling was utilized to reduce the rate of grain growth out of the extrusion die,resulting the grains significantly refined from 11μm to 2.5μm.Local high dislocation density region was also observed in the microstructure of sample processed at 150℃ in artificial cooling condition,and the degree decreased with the processing temperature increase.The results summarized from tensile tests indicated that due to the grain refinement the strength and ductility was significantly enhanced(YS of 186 MPa vs.145 MPa,UTS of 391 MPa vs.336 MPa and FE of 31.5%vs.24.5%compared with the as-received sample).Subsequently,annealing treatment at different temperatures was applied to eliminate the high dislocation density.The sample annealed at 200℃ exhibited the best comprehensive mechanical property with YS of 179 MPa,UTS of 390 MPa and FE of 33.0%.As the annealing temperature increasing,the dislocation density was reduced by static recrystallization(SRX)and grain growth,leading to a decreased strength and ductility. | Tingzhuang Han Jingfeng Zou Guangsheng Huang Lifeng Ma Chaojie Che Weitao Jia Lifei Wang Fusheng Pan | 2021 | Journal of Magnesium and Alloys2021，9，5： | 2 |
| 5 | Transport and elec- trochemical properties and spectral features of non-aqueous electrolytes containing LiFSI in linear carbonate solvents显示文摘 | Li Lifei Zhou Sisi Han Hongbo | 2011 | J Electrochem Soc2011，158，2： | 1 |
| 6 | Transport and elec- trochemical properties and spectral features of non - aque- ous electrolytes containing LiFSI in linear carbonate sol- vents 显示文摘 | Li Lifei Zhou Sisi Han Hongbo | 2011 | Journal of The Electrochemical Society2011，158，2： | 1 |
| 7 | The Formation and Evolution of Uvarovite in UHP Serpentinite and Rodingite and its Constraints on Chromium Mobility in the Oceanic Subduction Zone显示文摘The uvarovite-andradite and uvarovite-andradite-grossular solid-solution series are rare in nature.The discovery of uvarovite-andradite in serpentinite and rodingite from the ultra-high pressure(UHP)metamorphic belt in southwestern Tianshan provided an opportunity to investigate its behavior in the subduction zone.Uvarovite(defined as chromiumgarnet)from serpentinite is homogeneous in a single grain,covering compositions in the uvarovite-andradite solid solution series of Adr_(58-66)Uv_(33-41),with few grossular components.Uvarovite from rodingites contain various Cr_(2)O_(3) contents(1.7-17.9 wt%)and mineral compositions being in the range of Adr_(21-31)Uv_(41-50)Grs_(22-37),Adr_(52-90)Uv_(5-25)Grs_(0-21) and Adr_(19-67)Uv_(3-63)Grs_(13-42).Discontinuous chemical variation of uvarovite from core to rim indicates that uvarovite formed by consuming andradite and chromite,which could provide Ca,Cr,Al and Fe.Raman signals of water were identified for uvarovite from both serpentinite and rodingite,with high water content in uvarovite from serpentinite.The high pressure mineral assemblage,as well as the association with perovskite,indicated that the studied uvarovite from serpentinite and rodingite was formed through high pressure metamorphism,during the subduction zone serpentinization and rodingitization.High alkaline and highly reduced fluids released from serpentinization or rodingitization in the oceanic subduction zone promote the mobility of chromium and enable its long-distance migration. | ZHANG Cong SHEN Tingting ZHANG Lifei LIN Congcong ZHANG Zhongwei Qin Xueqing HU Han QIU Tian XIANG Zhenqun ZHANG Jianxin | 2021 | Acta Geologica Sinica(English Edition)2021，95，5： | 1 |
| 8 | Influence of warm pre-stretching on microstructure and properties of AZ31 magnesium alloy显示文摘 | Hua Zhang Guangsheng Huang Jinhan Li Lifei Wang Hans J?rgen Roven | 2013 | Journal of Alloys and Compounds2013，，： | 1 |
| 9 | Correction to:Effect of Extrusion Combination Types on Microstructure and Mechanical Properties of the AZ31/GW103K Bimetallic Composite Plates显示文摘In the original publication,the affliation citation number of the author Boyu Lin has been missed inadvertently in the author group.The afiliation should appear as Boyu Lin'.The original article has been corrected. | Yunpeng Meng Boyu Lin Lifei Wang Jianfeng Fan Shangzhou Zhang Liwei Lu Hans Jorgen Roven Hua Zhang | 2023 | Acta Metallurgica Sinica(English Letters)2023，36，7： | 0 |
| 10 | MoS_(2)core-shell nanoparticles prepared through liquid-phase ablation and light exfoliation of femtosecond laser for chemical sensing显示文摘Molybdenum disulfide(MoS_(2))-based nanostructures are highly desirable for applications such as chemical and biological sensing,photo/electrochemical catalysis,and energy storage due to their unique physical and chemical properties.In this work,MoS_(2)core-shell nanoparticles were first prepared through the liquid-phase processing of bulk MoS2by a femtosecond laser.The core of prepared nanoparticles was incompletely and weakly crystalline MoS_(2);the shell of prepared nanoparticles was highly crystalline MoS_(2),which wrapped around the core layer by layer.The femtosecond laser simultaneously achieved liquid-phase ablation and light exfoliation.The formation mechanism of the core-shell nanoparticles is to prepare the nanonuclei first by laser liquid-phase ablation and then the nanosheets by light exfoliation;the nanosheets will wrap the nanonuclei layer by layer through van der Waals forces to form core-shell nanoparticles.The MoS_(2)core-shell nanoparticles,because of Mo-S bond breakage and recombination,have high chemical activity for chemical catalysis.Afterward,the nanoparticles were used as a reducing agent to directly prepare three-dimensional(3D)Au-MoS_(2)micro/nanostructures,which were applied as surface-enhanced Raman spectroscopy(SERS)substrates to explore chemical sensing activity.The ultrahigh enhancement factor(1.06×10^(11)),ultralow detection limit(10-13M),and good SERS adaptability demonstrate highly sensitive SERS activity,great ability of ultralow concentration detection,and ability to detect diverse analytes,respectively.This work reveals the tremendous potential of 3D Au-MoS_(2)composite structures as excellent SERS substrates for chemical and biological sensing. | ZUO Pei JIANG Lan LI Xin TIAN MengYao YUAN YongJiu HAN WeiNa MA Le HU LiFei HE ZhiCong LI Fang | 2023 | Science China(Technological Sciences)2023，66，3： | 0 |
| 11 | Strength-ductility balance of AZ31 magnesium alloy via accumulated extrusion bonding combined with two-stage artificial cooling Author links open overlay panel显示文摘AZ31 Mg alloy with heterogeneous bimodal grain structure(smaller grain size of 5-20µm and coarser grain size of 100-200µm)was subjected to accumulated extrusion bonding(AEB)at 250℃combined with two-stage artificial cooling in this work,viz.local water cooling and artificial cooling.The microstructure developed consecutively as a result of discontinuous dynamic recrystallization(DDRX)for the AEBed samples.{10-12}tensile twinning also played an important role for the AEB with local water cooling at the initial extrusion stage in the container.Local water cooling could further reduce the DRXed grain size to~2.1µm comparing that without water cooling.And the grain growth rate was reduced by artificial cooling out of extrusion die.Under the combination of two-stage cooling,the fine DRXed grains at sizing band were almost retained with average grain size of~2.3µm after the sheet out of extrusion die,and the unDRXed grains with high residual dislocation density accumulation were also reserved.The tensile tests results indicated that a good strength-ductility balance with a high ultimate tensile strength(319 MPa vs.412 MPa)and fracture elongation(19.9%vs.30.3%)were obtained.The strength enhancement was mainly owing to the grain refinement and local residual plastic strain reserved by the artificial cooling.The excellent ductility originated from fine DRXed microstructure and ED-tilt double peak texture. | Tingzhuang Han Guangsheng Huang Heng Li Lifei Wang Hua Zhang Fusheng Pan | 2023 | Journal of Magnesium and Alloys2023，11，5： | 0 |
| 12 | Early morning off in patients with Parkinson's disease:a Chinese nationwide study and a 7-question screening scale显示文摘Background:Early morning off(EMO)is a common feature of Parkinson's disease(PD).This study aimed to characterize its clinical features and develop a convenient and pragmatic self-assessment instrument in a Chinese nationwide population.Methods:This study was conducted on 942 PD patients admitted to 55 clinic centers for movement disorders between June 2018 and May 2019 in China.Stepwise logistic regression analyses were performed to determine potential risk factors and the most predictive symptoms of EMO,as well as whether EMO was an independent risk factor of functional dependency in daily life.Based on this,a 7-question scale was derived for EMO screening.Diagnostic accuracy of this scale was assessed from the area under the receiver operative characteristic curve(AUROC)and its 95%confidence intervals(CIs).We further calculated sensitivity,specificity,positive predictive value(PPV),and negative predictive value(NPV)for the optimal cutoff point.Results:EMO occurred in 49.2%of PD patients across all disease stages.We identified 7 symptoms most predictive of EMO,including bradykinesia or rigidity,excessive sweating or salivation,ificulty in turning on or getting out of bed,muscle cramp,fatigue or sleepiness,frozen state or freezing gait,and tremor.The resulting 7-item scale was confirmed to be of good discrimination with a relatively large AUROC of 0.83,a relatively high sensitivity of 75.7%,specificity of 77.5%,PPV of 76.5%,and NPV of 76.7%.Nonideal nighttime sleep,long PD duration,advanced H&Y stages,posture instability gait difficulty-dominant or mixed subtypes,and high levodopa dose were independently associated with increased risk of EMO.EMO patients were at 87%higher(OR=1.87,95%C:1.07-3.32)risk of experiencing functional dependency in daily living compared with their counterparts.Conclusions:We demonstrated that EMO is a common feature for PD patients across all disease stages and put forward an EMO-specific screening card of sufficient accuracy and brevity.Meanwhile,we have thrown some light upon potential determinants and negative health effects of EMO.Our findings may exert great impact on improving the awareness,recognition and management of EMO in PD patients. | Chao Han Wei Mao Jing An Lifei Jiao Piu Chan on behalf of the China Early Morning Off(EMO)Study Group | 2020 | Translational Neurodegeneration2020，9，3： | 0 |
| 13 | Effect of Extrusion Combination Types on Microstructure and Mechanical Properties of the AZ31/GW103K Bimetallic Composite Plates显示文摘The AZ31/GW103 K bimetallic composite plates were prepared by co-extrusion of different combination types(sandwich extrusion type and double semicircle extrusion type),and effects of different extrusion combination types on the microstructure and mechanical properties of bimetallic composite plates were systematically investigated.The results show that both the AZ31/GW103 K bimetallic composite plates prepared by different extrusion combination types have good metallurgical bonding,and changing the combination type does not affect the thickness of the interfacial transition layer of composite plates.Compared with the monolithic AZ31 and GW103 K extruded plates,co-extrusion can promote the dynamic recrystallization(DRX)of AZ31 and GW103 K components in composite plates,and double semicircular extrusion type has a better promotion effect on the DRX than sandwich extrusion type.In addition,the texture of AZ31 in both monolithic AZ31 and AZ31/GW103 K/AZ31(A/G/A)plates is a typical(0002)basal texture,while that in the AZ31/GW103 K(A/G)composite plate shifts to the tangent direction(TD)of extruded plate.Compared with the monolithic AZ31 extruded plate,both the yield strength and tensile strength of A/G and A/G/A bimetallic composite plates are significantly improved.The strength of A/G/A composite plate is higher than that of A/G composite plate,but its elongation is worse.Meanwhile,co-extrusion reduces the dislocation density of AZ31 and GW 103 K components in composite plates,and different extrusion combination types also affect the dislocation density. | Yunpeng Meng Boyu Lin Lifei Wang Jianfeng Fan Shangzhou Zhang Liwei Lu Hans Jφrgen Roven Hua Zhang | 2022 | Acta Metallurgica Sinica(English Letters)2022，35，12： | 0 |
| 14 | Biomineralized CO gas-releasing nanoprodrug for endoplasmic reticulum stress mediated cancer therapy显示文摘The anti-tumor effect of therapeutic carbon monoxide(CO)has been considered concerning the electron transport chain on the inner mitochondrial membrane.Herein,a tumor microenvironment and photo-responsive CO nanoplatform Ca-Flav nanoparticles(NPs)were constructed through biomineralizing acryloyl-modified flavonol,which could release CO both in normoxia and hypoxia conditions upon irradiation at tumor lesion.The in vitro experiments demonstrated that the endoplasmic reticulum stress-related signal pathways could be activated through oxidative stress caused by CO mediated mitochondrial biogenesis and calcium ion turbulence induced by Ca_(3)(PO_(4))_(2)acidolysis,resulting in mitochondrial dysfunction and cell apoptosis.In addition,the Ca-Flav NPs exhibited excellent biocompatibility and tumor inhibition effect in vivo.This work provides new insight into the potential characteristics of CO,paving a new way to engineer more efficient treatment based on CO. | Rui Gu Wanlan Yang Lifei Han Chao Liu Yatao Xu Yunlong Liu Weili Si Wenjun Wang Xiaochen Dong | 2023 | Nano Research2023，16，5： | 0 |
| 15 | Amorphous NH_(2)-MIL-68 as an efficient electro-and photo-catalyst for CO_(2)conversion reactions显示文摘To produce metal-organic framework(MOF)catalysts with both high activity and durability is interesting but challenging.We report an amorphous MOF(NH_(2)-MIL-68),which combines the advantages of(1)a large number of open metal sites,(2)the basic building blocks and connectivity of crystalline NH_(2)-MIL-68,and(3)hierarchically meso-and microporous structure.It exhibits high performances in electrocatalytic reduction of CO_(2)and photochemical cycloaddition of CO_(2)under mild conditions.For the former reaction,the maximum Faradaic efficiency for product formic acid(FEHCOOH)reaches 93.3%with a current density of 34.2 mA·cm^(−2)at^(−2).05 V vs.Ag/Ag+catalyzed by amorphous NH_(2)-MIL-68,while the crystalline NH_(2)-MIL-68 shows FEHCOOH of 67.7%with considerable productions of CO and H_(2)at the same experimental conditions.For the photochemical cycloaddition of CO_(2)with styrene oxide,the yield by amorphous NH_(2)-MIL-68 can reach 94.1%at 12 h,which is higher than the reported value under similar conditions.The structure–efficiency relationship of the catalyst for the two reactions was investigated.This work opens up new possibility for designing high-performance MOF and MOF-based catalysts. | Lifei Liu Jianling Zhang Xiuyan Cheng Mingzhao Xu Xinchen Kang Qiang Wan Buxing Han Ningning Wu Lirong Zheng Chenyan Ma | 2023 | Nano Research2023，16，1： | 0 |
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