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| 1 | Human ESC-derived expandable hepatic organoids enable therapeutic liver repopulation and pathophysiological modeling of alcoholic liver injury显示文摘We report the generation of human ESC-derived,expandable hepatic organoids(hEHOs)using our newly established method with wholly defined(serum-free,feeder free)media.The hEHOs stably maintain phenotypic features of bipotential liver stem/progenitor cells that can differentiate into functional hepatocytes or cholangiocytes.The hEHOs can expand for 20 passages enabling large scale expansion to cell numbers requisite for industry or clinical programs.The cells from hEHOs display remarkable repopulation capacity in injured livers of FRG mice following transplantation,and they differentiate in vivo into mature hepatocytes.If implanted into the epididymal fat pads of immune-deficient mice,they do not generate non-hepatic lineages and have no tendency to form teratomas.We further develop a derivative model by incorporating human fetal liver mesenchymal cells(hFLMCs)into the hEHOs,referred to as hFLMC/hEHO,which can model alcoholic liver disease-associated pathophysiologic changes,including oxidative stress generation,steatosis,inflammatory mediators release and fibrosis,under ethanol treatment.Our work demonstrates that the hEHOs have considerable potential to be a novel,ex vivo pathophysiological model for studying alcoholic liver disease as well as a promising cellular source for treating human liver diseases. | Shuyong Wang Xuan Wang Zuolong Tan Yuxin Su Juan Liu Mingyang Chang Fang Yan Jie Chen Tao Chen Chuanjiang Li Jie Hu Yunfang Wang | 2019 | Cell Research2019,29,12: | 20 |
| 2 | Effect of Sanhuangwuji powder,anti-rheumatic drugs,and ginger-partitioned acupoint stimulation on the treatment of rheumatoid arthritis with peptic ulcer:a randomized controlled study显示文摘OBjECTIVE:To observe the efficacy and safety of oral Sanhuangwuji powder,anti-rheumatic drugs(ARDs),and ginger-partitioned acupoint stimulation at Zusanli(ST 36) on the treatment of rheumatoid arthritis(RA) complicated by peptic ulcer.METHODS:This prospective randomized controlled study included 180 eligible inpatients and outpatients randomly assigned to an ARD treatment(n = 60),ginger-partitioned stimulation(n =60),or combination treatment(n = 60).Patients assigned to the ARD group were given oral celecoxib,methotrexate,and esomeprazole.Patients assigned to theginger-partitioned stimulation group were given ginger-partitioned acupoint stimulation at Zusanli(ST 36) in addition to the ARDs.Patients in the combination treatment group were given oral Sanhuangwuji powder,ginger-partitioned acupoint stimulation at Zusanli(ST 36),and ARDs.All patients were followed up for 2 months to evaluate clinical effects and safety.The study was registered in the World Health Organization database at the General Hospital of Chengdu Military Area Command Chinese People's Liberation Army(ChiCTR-TCC12002824).RESULTS:The combination treatment group had significantly greater improvements in RA symptoms,laboratory outcomes,and gastrointestinal symptom scores,compared with the other groups(P < 0.05).The peptic ulcer healing rate in the combination treatment group was significantly greater than that in the ARD treatment group(x^2 = 16.875,P < 0.05) and the ginger-partitioned stimulation group(x^2 = 6.171,P<0.05).CONCLUSION:Combination treatment with ginger-partitioned acupoint stimulation at Zusanli(ST36),oral Sanhuangwuji powder,and ARDs had a better clinical effect for RA with complicated peptic ulcer,compared with ARD treatmentalone or in combination with ginger-partitioned acupoint stimulation. | Liu Defang Guo Mingyang Hu Yonghe Liu Taihua Yan Jiao Luo Yong Yun Mingdong Yang Min Zhang Jun Guo Linglin | 2015 | Journal of Traditional Chinese Medicine2015,35,3: | 9 |
| 3 | Facile electrodeposition of 3D concentration-gradient Ni-Co hydroxide nanostructures on nickel foam as high performance electrodes for asymmetric supercapacitors显示文摘小说三维(3D ) 集中坡度 Ni 公司氢氧化物 nanostructures (3DCGNC ) 被一个灵巧的逐步的电气化学的免职方法直接在镍泡沫上种了并且强烈地为 supercapacitors 调查同样没有文件夹、没有售票员的电极。基于一种三电极的电气化学的描述技术,获得的 3DCGNC 电极表明了 1,760 F 的一个高特定的电容 ???? | Mingyang Yang Hua Cheng Yingying Gu Zhifang Sun Jing Hu Lujie Cao Fucong Lv Minchan Li Wenxi Wang Zhenyu Wang Shaofei Wu Hongtao Liu Zhouguang Lu | 2015 | Nano Research2015,8,8: | 8 |
| 4 | Effect of methotrexate combined with Sanhuang Yilong decoction on serum and synovial fluid aquaporin levels in rheumatoid arthritis dampness-heat blockage syndrome显示文摘OBJECTIVE:To study the effect of methotrexate(MTX) combined with Sanhuang Yilong decoction(SYD) on aquaporin(AQP) expression,and to explore the role of AQPs in the pathogenesis of rheumatoid arthritis(RA).METHODS:A total of 118 dampness-heat blockage type RA patients who were hospitalized in the General Chengdu Military Hospital between January2014 and December 2016 were selected as subjects in this study(30 patient of these patients with knee joint effusion were assigned to the RA synovial fluid group).For the pre-treatment controlgroups,30 healthy volunteers were recruited as the healthy control group and 30 osteoarthritis(OA) patients with knee joint effusion were included as OA synovial fluid control group.The RA dampnessheat blockage syndrome treatment groups were divided into 45 cases in the combined group and 45 cases in the MTX group.The combined group received MTX combined with SYD treatment while the MTX group received MTX alone.AQP1,AQP2 and AQP3 expressions were detected in the serum and synovial fluid.RESULTS:AQP1 had the highest expression,followed by AQP3,and AQP2.The serum levels of AQP1,AQP2 and AQP3 were all significantly lower than those in the healthy volunteers(P < 0.05),while the synovial fluid AQP1,AQP2 and AQP3 expression in the RA group were comparable to these in the OA groups(P > 0.05).After treatment for2 weeks,serum AQP1,AQP2,AQP3 were significantly increased and erythrocyte sedimentation rate,C-reactive protein,disease activity score of 28 joints were decreased in the combined group(P < 0.05).CONCLUSION:Abnormal expression of AQPs inhibits water metabolism in RA dampness-heat blockage syndrome,so liquid is accumulated at the joint,which may play an important role in the pathogenesis of RA.MTX combined with SYD for the treatment of RA can effectively increase AQP expression. | Liu Defang Yan Jiao Guo Mingyang Luo Yong Yang Mei Yang Min Zou Longfu Li Wan Zhong Xiaolong Liu Tao Hu Yonghe | 2018 | Journal of Traditional Chinese Medicine2018,38,4: | 4 |
| 5 | Effect of Sanhuangyilong decoction plus methotrexate on tumor necrosis factor alpha and interferon gamma in serum and synovial fluid in rheumatoid arthritis patients with symptom pattern of damp heat obstruction显示文摘OBJECTIVE: To investigate the effect of Sanhuangyilong decoction plus methotrexate(MTX) on Interferon gamma(IFN-γ) and tumor necrosis factor alpha(TNF-α) in the serum and synovial fluid of rheumatoid arthritis(RA) patients with damp-heat-obstruction symptom pattern, Sanhuangyilong decoction and the role of TNF-α and IFN-γ in the development of RA.METHODS: RA inpatients with damp-heat-obstruction symptom pattern(partly with knee joint effusion) were selected as the research subjects. Before the treatment, healthy subjects and osteoarthritis(OA) patients with knee joint effusion were assigned to the serum control group and the synovial fluid control group, respectively; during the treatment, RA patients with damp-heat-obstruction symptom pattern were divided into two groups:one is combined group that was administered Sanhuangyilong decoction plus MTX; the other group was MTX group that received MTX only. The expression levels of TNF-α and IFN-γ in the serum and synovial fluid were measured with enzyme-linked immunosorbent assay(ELISA) before and after the treatment, and the peripheral blood levels of erythrocyte sedimentation rate(ESR), C-reactive protein(CRP) and disease activity score in 28 joints(DAS28)were determined.RESULTS: Before treatment, the serum levels of TNF-α and IFN-γ in the RA patients with dampheat-obstruction symptom pattern were higher than those in healthy control group(P < 0.05).The expression levels of TNF-α and IFN-γ in the synovial fluid of the RA patients were higher than those in the serum of the RA patients(P < 0.05). The expression levels of TNF-α and IFN-γ in the synovial fluid of the RA patients were higher than those of the sy-novial fluid of the osteoarthritis patients(P < 0.05).The expression of TNF-α and IFN-γ in the serum and synovial fluid of the RA patients had no correlation with the inflammatory activity index ESR, CRP,or DAS28(P > 0.05). After 2 weeks of treatment, the expression level of TNF-α and IFN-γ in the combined group had increased, although the difference was not statistically significant(P > 0.05); in contrast, ESR, CRP, and DAS28 decreased, and the difference was statistically significant(P < 0.01). After 4 weeks of therapy, TNF-alpha and IFN-γ, ESR,CRP, and DAS28 in the combined group decreased compared with the before-treatment levels(P <0.01). After 2 w of treatment, the differences in the TNF-α and IFN-γ expression levels in the combined group were not statistically significant(P > 0.05)compared with that in the MTX group, although there were statistically significant differences in the ESR, CRP, and DAS28(P < 0.05). After 4 weeks of treatment, differences in TNF-α, IFN-γ, ESR, CRP, and DAS28 in the combined group compared with MTX group were statistically significant(P < 0.01).CONCLUSION: TNF-α and IFN-γ might be involved in the development of RA. The RA patients with damp-heat-obstruction symptom pattern show better benefits from the treatment of Sanhuangyilong decoction plus MTX, and the treatment is superior to that of using MTX only. | Liu Defang Yan Jiao Yun Mingdong Yang Ming Luo Yong Zhang Jun Guo Mingyang Yang Mei Yuan Weili Zou Wei Li Hua Hu Yonghe | 2016 | Journal of Traditional Chinese Medicine2016,36,5: | 4 |
| 6 | Knowledge-Domain Semantic Searching and Recommendation Based on Improved Ant Colony Algorithm显示文摘 | Mingyang Liu Shufen Liu Xiaoyan Wang Ming Qu Changhong Hu | 2013 | Journal of Bionic Engineering2013,10,4: | 3 |
| 7 | Effect of hand-ear acupuncture on chronic low-back pain: a randomized controlled trial显示文摘OBJECTIVE: To evaluate the effect of hand-ear acupuncture on chronic low-back pain(cLBP).METHODS: This was an open, randomized and controlled trial in The General Hospital of Western Theater Command, Sichuan Province. The trial was registered with ClinicalTrials.gov, NCT02260284. All the 152 participates with cLBP were randomly assigned to hand-ear acupuncture(n = 54), standard acupuncture(n = 50), or usual care groups(n = 48).Eighteen treatments were provided over 7 weeks.Back-related dysfunction and symptom severity were assessed by the Roland-Morris Disability Questionnaire(RMDQ) and the Visual Analogue Scale(VAS), which were collected at baseline, 2 months and 6 months post to the treatment.RESULTS: At 6 months, the RMDQ scores improved by 7.74 points of hand-ear acupuncture group. Significant improvement of VAS and RMDQ was observed in hand-ear acupuncture group(P < 0.001),but no significant changes of RMDQ were observed in both standard acupuncture group and usual care group. We also observed an overall efficacy rate of 88.89% in hand-ear acupuncture group, as evaluated by Diagnosis and Curative Effect Standard for Symptom pattern of Traditional Chinese Medicine, which was much higher than 45.84% in the usual care group(H = 16.000, P < 0.001).CONCLUSION: Both of the hand-ear acupuncture and standard acupuncture modes have beneficial and persistent effectiveness against cLBP compared with the usual care. Furthermore, hand-ear acupuncture is significantly more effective than the standardized acupuncture, especially in the long term. | Luo Yong Yang Min Liu Tao Zhong Xiaolong Tang Wen Guo Mingyang Hu Yonghe | 2019 | Journal of Traditional Chinese Medicine2019,39,4: | 2 |
| 8 | Association of assisted reproductive technology, germline de novo mutations and congenital heart defects in a prospective birth cohort study显示文摘Emerging evidence suggests that children conceived through assisted reproductive technology(ART)have a higher risk of congenital heart defects(CHDs)even when there is no family history.De novo mutation(DNM)is a well-known cause of sporadic congenital diseases;however,whether ART procedures increase the number of germline DNM(gDNM)has not yet been well studied.Here,we performed whole-genome sequencing of 1137 individuals from 160 families conceived through ART and 205 families conceived spontaneously.Children conceived via ART carried 4.59 more gDNMs than children conceived spontaneously,including 332 paternal and 1.26 maternal DNMs,after correcting for parental age at conception,cigarette smoking,alcohol drinking,and exercise behaviors.Paternal DNMs in offspring conceived via ART are characterized by C>T substitutions at CpG sites,which potentially affect protein-coding genes and are significantly associated with the increased risk of CHD.In addition,the accumulation of non-coding functional mutations was independently associated with CHD and 87.9% of the mutations were originated from the father.Among ART offspring,infertility of the father was associated with elevated paternal DNMs;usage of both recombinant and urinary follicle-stimulating hormone and high-dosage human chorionic gonadotropin trigger was associated with an increase of maternal DNMs.In sum,the increased gDNMs in offspring conceived by ART were primarily originated from fathers,indicating that ART itself may not be a major reason for the accumulation of gDNMs.Our findings emphasize the importance of evaluating the germline status of the fathers in families with the use of ART. | Cheng Wang Hong Lv Xiufeng Ling Hong Li Feiyang Diao Juncheng Dai Jiangbo Du Ting Chen Qi Xi Yang Zhao Kun Zhou Bo Xu Xiumei Han Xiaoyu Liu Meijuan Peng Congcong Chen Shiyao Tao Lei Huang Cong Liu Mingyang Wen Yangqian Jiang Tao Jiang Chuncheng Lu Wei Wu Di Wu Minjian Chen Yuan Lin Xuejiang Guo Ran Huo Jiayin Liu Hongxia Ma Guangfu Jin Yankai Xia Jiahao Sha Hongbing Shen Zhibin Hu | 2021 | Cell Research2021,31,8: | 2 |
| 9 | Colonization and development of the gut microbiome in calves显示文摘Colonization and development of the gut microbiome are crucial for the growth and health of calves.In this review,we summarized the colonization,beneficial nutrition,immune function of gut microbiota,function of the gut barrier,and the evolution of core microbiota in the gut of calves of different ages.Homeostasis of gut microbiome is beneficial for nutritional and immune system development of calves.Disruption of the gut microbiome leads to digestive diseases in calves,such as diarrhea and intestinal inflammation.Microbiota already exists in the gut of calf fetuses,and the colonization of microbiota continues to change dynamically under the influence of various factors,which include probiotics,diet,age,and genotype.Colonization depends on the interaction between the gut microbiota and the immune system of calves.The abundance and diversity of these commensal microbiota stabilize and play a critical role in the health of calves. | Yufeng Du Ya Gao Mingyang Hu Jinxiu Hou Linhai Yang Xianghuang Wang Wenjuan Du Jianxin Liu Qingbiao Xu | 2023 | Journal of Animal Science and Biotechnology2023,14,4: | 1 |
| 10 | Resistivity response of coal under hydraulic fracturing with different injection rates:A laboratory study显示文摘Resistivity will have different response characteristics to the hydraulic fracture propagation process. In this work, a resistivity testing system for hydraulic fracturing specimens was established. Resistivity and acoustic emission(AE) information were jointly analysed to determine the dynamic response characteristics of resistivity during hydraulic fracture propagation. The results show that the water and fracture exert a competitive influence on the connection structure of the circuit, and there are two significant peak resistivity points in the curve, presenting a double peak therein. The peak resistivity data of the specimen with a larger fracture area are much different from the initial value. With the increase of the rate of injection, the range of variation of the highest value that can be reached with the specimen resistivity decreases. High resistivity rates or high resistivity fluctuations exhibit rapid a release of fracture energy. The fracture failure mode dominated by shear fractures makes the formation produce a “series+parallel” electrical connection structure;a calculation model of formation resistivity based on shear and tensile failure was proposed to characterize the proportion of different types of hydraulic fractures and elucidate the control effect of matrix resistivity on the electrical performance of the overall circuit structure. | Mingyang Song Quangui Li Qianting Hu Yanqing Wu Guanhua Ni Yangcheng Xu Yuebing Zhang Liangping Hu Jialin Shi Jichuan Liu Yize Deng | 2022 | International Journal of Mining Science and Technology2022,32,4: | 1 |
| 11 | Seroprevalence of Toxoplasma gondii Infection in Pet Dogs in Shenyang, Northeastern China显示文摘 | Yang Na Mu Mingyang Li Hongkui Hu Jianmin Gao Weifan Yang Shuhua He Jianbin | 2013 | The Journal of Parasitology2013,,1: | 1 |
| 12 | Prof. Lü Shuxiang’s Theoretical Contributions to Grammar——In Honour of the Ninetieth Anniversary of Prof. Lü’s Birthday显示文摘In China, studies of grammar as a humanistic discipline in the sense as generallyunderstood in western countries began by the end of the nineteenth century when the pi-oneer in this field Ma Jianzhong published in 1898 his Ma Shi Wentong(Ma’s Grammarof Classic Chinese), modelled on traditional grammar in the West. Later Chinese gram-marians continued to draw on what were new in western linguistics and worked withnewer frameworks and methodology elaborated by different linguistic schools. Howev-er, works on Chinese grammar, though apparently marked with western influence, arenot mere imitations. Description of a language greatly different from the Indo-Europeanlanguages, on the basis of which evolved the various schools of grammar, traditional | Hu Mingyang | 1993 | 世界汉语教学1993,7,4: | 0 |
| 13 | Decision-making Method of Sharing Mode for Multi-microgrid System Considering Risk and Coordination Cost显示文摘Power sharing can improve the benefit of the multi-microgrid(MMG)system.However,the information disclosure may appear during the sharing process,which would bring privacy risk to a local microgrid.Actually,the risk and coordination cost are different in different sharing modes.Therefore,this paper develops a decision-making method to decide the most suitable one of three mostly used sharing modes(i.e.,cooperative game with complete information,cooperative game with incomplete information,and noncooperative game).Firstly,power sharing paradigms and coordination mechanisms in the three modes are formulated in detail.Particularly,different economic operation models of MMG system are included to analyze the economic benefit from different sharing modes.Based on the different disclosed information,the risk cost is evaluated by using the simplified fuzzy analytic hierarchy process(FAHP).And the coordination cost for different sharing modes is expressed in different functions.In addition,a hierarchical evaluation system including three decision-making factors(e.g.,economics,risk,and coordination)is set up.Meanwhile,a combination weighting method(e.g.,the simplified FAHP combined with the anti-entropy weight method)is applied to obtain the weight of each factor for comprehensive evaluation.Finally,the optimal sharing solution of MMG system is decided by comparing and analyzing the difference among the three sharing modes.Numerical results validate that the proposed method can provide a reference to deciding a suitable sharing mode. | Hongjun Gao Jingxi Yang Shuaijia He Jianglin Zhang Junyong Liu Mingyang Hu | 2022 | Journal of Modern Power Systems and Clean Energy2022,10,6: | 0 |
| 14 | Taxonomic bias in occurrence information of angiosperm species in China显示文摘Taxonomic bias is a well-known shortcoming of species occurrence databases.Understanding the causes of taxonomic bias facilitates future biological surveys and addresses current knowledge gaps.Here,we investigate the main drivers of taxonomic bias in occurrence data of angiosperm species in China.We used a database including 5,936,768 records for 28,968 angiosperm species derived from herbarium specimens and literature sources.Generalized additive models(GAMs)were applied to investigate explanatory powers of 17 variables on the variation in record numbers of species.Five explanatory variables were selected for a multi-predictor GAM that explained 69%of the variation in record numbers:plant height,range size,elevational range,numbers of scientific publications and web pages.Range size was the most important predictor in the model and positively correlated with number of records.Morphological and phenological traits and social-economic factors including economic values and conservation status had weak explanatory powers on record numbers of plant species,which differs from the findings in animals,suggesting that causes of taxonomic bias in occurrence databases may vary between taxonomic groups.Our results suggest that future floristic surveys in China should more focus on range-restricted and socially or scientifically less'interesting'species. | Wenjing Yang Dandan Liu Qinghui You Bin Chen Minfei Jian Qiwu Hu Mingyang Cong Keping Ma | 2021 | Science China(Life Sciences)2021,64,4: | 0 |
| 15 | An integrated machine learning model for accurate and robust prediction of superconducting critical temperature显示文摘Discovering new superconductors via traditional trial-and-error experimental approaches is apparently a time-consuming process,and the correlations between the critical temperature(Tc) and material features are still obscure.The rise of machine learning(ML) technology provides new opportunities to speed up inefficient exploration processes,and could potentially uncover new hints on the unclear correlations.In this work,we utilize open-source materials data,ML models,and data mining methods to explore the correlation between the chemical features and Tcvalues of superconducting materials.To further improve the prediction accuracy,a new model is created by integrating three basic algorithms,showing an enhanced accuracy with the coefficient of determination(R2) score of 95.9 % and root mean square error(RMSE) of 6.3 K.The average marginal contributions of material features towards Tcvalues are estimated to determine the importance of various features during prediction processes.The results suggest that the range thermal conductivity plays a critical role in Tcprediction among all element features.Furthermore,the integrated ML model is utilized to screen out potential twenty superconducting materials with Tcvalues beyond 50.0 K.This study provides insights towards Tcprediction to accelerate the exploration of potential high-Tcsuperconductors. | Jingzi Zhang Ke Zhang Shaomeng Xu Yi Li Chengquan Zhong Mengkun Zhao Hua-Jun Qiu Mingyang Qin X.-D.Xiang Kailong Hu Xi Lin | 2023 | Journal of Energy Chemistry2023,,3: | 0 |
| 16 | PUTONGHUA, THE CHINESE STANDARD NATIONAL COMMON SPEECH, AND THE BEIJING VERNACULAR显示文摘1.What is Putonghua? Putonghua is the official term for the Chinese standard national common speech since1955.Before 1949 it was Guoyü(the national language),which is still in use in Taiwanand in some other regions.Mandarin,from Portuguese mandarin,introduced by Por-tuguese missionaries in late Ming Dynasty to mean both Chinese officials and the partic- | Hu Mingyang, People’s University of China | 1992 | 世界汉语教学1992,6,1: | 0 |
| 17 | A low-floor bit-mapping scheme for LDPC coded BICM for 5G and beyond systems显示文摘This paper proposes a low-floor bit-mapping(LFBM)scheme for bit-interleaved coded modulation(BICM)systems to meet more stringent quality of service requirements of 5G and beyond.For highefficiency transmissions,we consider the 5G low-density parity-check codes with high-order 2m-quadrature amplitude modulations(QAMs).The proposed LFBM scheme overcomes plenty of trapping sets induced by the bit interleaver,which focuses on the waterfall performance too aggressively.When the high-order QAM is used,the row-column interleaver specified by the 5G standard is such a bit interleaver.The LFBM scheme only optimizes the rule of mapping an m-bit tuple output by the row-column interleaver to a modulation symbol,rather than the entire bit interleaver.Therefore,the optimized bit mapper is actually an m-bit permutation module concatenated with the original bit interleaver employed in the current 5G BICM systems.The simulation results confirm that the LFBM scheme can lower the error floor of the 5G BICM system by approximately two orders of magnitude,while with negligible performance loss in the waterfall region. | Mingyang ZHU Ming JIANG Chunming ZHAO Lijie HU Xiaodong XU | 2023 | Science China(Information Sciences)2023,66,10: | 0 |
| 18 | Strain tuned efficient heterostructure photoelectrodes显示文摘van der Waals (vdWs) heterostructures based on two-dimensional (2D) materials have become a promising candidate for photoelectrochemical (PEC) catalyst not only because of the freedom in materials design that enable the band-offset construction and facilitate the charge separation. They also provide a platform for the study of various of interface effect in PEC. Here, we report a new kind of mixed-dimensional vdWs heterostructure photoelectrode and investigate the strain enhanced PEC performance at vdWs interfaces. Our heterostructures are composed of 2D n-type MoS_(2) nanosheets and three-dimensional (3D) p-type Cu_(2)O nanorod arrays (NRAs), where Cu_(2)O NRAs introduce periodically strain in the p-n junction interface. We find a promotion of the HER catalytic activities in heterostructure based PEC photoelectrodes using in-situ measurement techniques including the scanning electrochemical cell microscopy and various local spectrum probe measurements. This is attributed to the efficient charge separation at the strained heterointerface. Our results demonstrate an interesting venue for understanding the local interface effects with high spatial resolution, and shed light on design and developing high-efficiency photoelectrodes. 1L MoS_(2)/Cu_(2)O vdWs heterostructure photocathodes were prepared by nanoindentation technology. The effects of strain on promoting charge separation at the heterointerface were verified by the enhanced performances in PEC hydrogen evolution reaction of vdWs heterostructure through scanning electrochemical cell microscopy technique and various local spectrum probe measurements. | Haihong Zheng Mingyang Li Jinsong Chen Anchang Quan Kaihang Ye Hang Ren Sheng Hu Yang Cao | 2022 | Chinese Chemical Letters2022,33,3: | 0 |
| 19 | Visible-Light-Driven Methane Conversion with Oxygen Enabled by Atomically Precise Nickel Catalyst显示文摘It remains an extreme challenge to activate thermodynamically unfavorable,chemically inert methane molecules under mild conditions.Herein,we report a molecular-like nickel-thiolate hexameric cluster[Ni_(6)(PET)_(12);PET=SC_(2)H_(4)Ph]catalyst that resembles a double crown,comprising of a hexagonal Ni6 kernel encapsulated by an exterior shell of 12 thiolates capable of efficient conversion of methane plus O_(2) to methanol and formic acid under visible light irradiation. | Weigang Hu Yongnan Sun Shuohao Li Xinglian Cheng Xiao Cai Mingyang Chen Yan Zhu | 2021 | CCS Chemistry2021,3,9: | 0 |
| 20 | Defect electrons accelerate iron cycle of novel Fe-based Fenton:Long-term effective quinoline degradation显示文摘Heterogeneous Fenton has been widely used in the disposal of organic pollutants,however,slow regeneration of≡Fe(II)remains limitation for its practical application of long-term treatment.Herein,we come up with a novel Fe-based heterogeneous Fenton catalyst named as FeS_(x)O_(y)-X(X is the ratio of ethylene glycol to N,N-dimethylformamide).With the help of the abundant defect electrons in Sulfur vacancies,≡Fe(Ⅱ)regeneration on the surface of FeS_(x)O_(y)-1:1 was accelerated,resulting in a stable proportion of≡Fe(Ⅱ)on the surface,which maintained continuously stable generation of hydroxyl radical(·OH)and singlet oxygen(^(1)O_(2)).Thus,without any organic reagents or cocatalysts,FeS_(x)O_(y)-1:1 based Fenton system achieved effective long-term degradation of 560 mg/L quinoline within only 7 days,which was evidently better than reported Fe S and SV-Fe S_(2)(SV:Sulfur vacancy).The system had excellent adaptability to water quality and the COD removal rate of biochemical wastewater was as high as 79.8%. | Weikang Hu Ming Yang Qingyun Yan Jiahui Ji Yan Bao Jinlong Zhang Mingyang Xing | 2023 | Chinese Chemical Letters2023,34,6: | 0 |