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| 1 | An novel identification method of the environmental risk sources for surfacewater pollution accidents in chemical industrial parks显示文摘The chemical industry is a major source of various pollution accidents. Improving the management level of risk sources for pollution accidents has become an urgentdemand for most industrialized countries. In pollution accidents, the released chemicals harm the receptors to some extentdepending on their sensitivity or susceptibility. Therefore, identifying the potential risk sources from such a large number of chemical enterprises has become pressingly urgent. Based on the simulation of thewhole accident process, a novel and expandable identification method for risk sources causingwater pollution accidents is presented. The newlydeveloped approach, by analyzing and stimulating thewhole process of a pollution accident between sources and receptors, can be applied to identify risk sources, especially on the nationwide scale. Three major types of losses, such as social, economic and ecological losses,were normalized, analyzed and used for overall consequence modeling. A specific case study area, located in a chemical industry park (CIP) along the Yangtze River in Jiangsu Province, China,was selected to test the potential of the identification method. The results showed that therewere four risk sources for pollution accidents in this CIP. Aniline leakage in the HS Chemical Plantwould lead to the most serious impact on the surroundingwater environment. This potential accidentwould severelydamage the ecosystem up to3.8 kmdownstream of Yangtze River, and lead to pollution over adistance stretching to 73.7 kmdownstream. The proposed method is easily extended to the nationwide identification of potential risk sources. | Jianfeng Peng Yonghui Song Peng Yuan Shuhu Xiao Lu Han | 2013 | Journal of Environmental Sciences2013，25，7： | 9 |
| 2 | Enhanced photoelectrocatalytic degradation of ammonia by in situ photoelectrogenerated active chlorine on TiO_2 nanotube electrodes显示文摘TiO_2 nanotube(Ti NT) electrodes anodized in fluorinated organic solutions were successfully prepared on Ti sheets. Field-emission scanning electron microscopy(FE-SEM) and X-ray diffraction(XRD) were performed to characterize the TiNT electrodes. The linear voltammetry results under irradiation showed that the TiNT electrode annealed at 450°C presented the highest photoelectrochemical activity. By combining photocatalytic with electrochemical process, a significantly synergetic effect on ammonia degradation was observed with Na_2SO_4 as supporting electrolyte at pH 10.7. Furthermore, the photoelectrocatalytic efficiency on the ammonia degradation was greatly enhanced in presence of chloride ions without the limitation of pH. The degradation rate was improved by 14.8 times reaching 4.98 × 10^(-2) min^(-1) at pH 10.7 and a faster degradation rate of 6.34 × 10^(-2) min^(-1)was obtained at pH 3.01. The in situ photoelectrocatalytic generated active chlorine was proposed to be responsible for the improved efficiency. On the other hand, an enhanced degradation of ammonia using TiNT electrode fabricated in fluorinated organic solution was also confirmed compared to TiNT electrode anodized in fluorinated water solution and TiO_2 film electrode fabricated by sol–gel method. Finally, the effect of chloride concentration was also discussed. | Shuhu Xiao Dongjin Wan Kun Zhang Hongbin Qu Jianfeng Peng | 2016 | Journal of Environmental Sciences2016，28，12： | 2 |
| 3 | 显示文摘 | Zhu Hua Zhong Lian Xiao Shuhu | 2004 | Electrochimica Acta2004，49，： | 1 |
| 4 | Application ofPolyaniline to Galvanic Anodic Protection on Stainless Steel in H2SO4 Solutions显示文摘 | Zhong Lian Xiao Shuhu Hu Jie | 2006 | Corrosion Science2006，48，12： | 1 |
| 5 | Degradation of biologically treated landfill leachate by using electrochemical process combined with UV irradiation显示文摘 | Shuhu Xiao Jianfeng Peng Yonghui Song Dongsheng Zhang Ruixia Liu Ping Zeng | 2013 | Separation and Purification Technology2013，，： | 1 |
| 6 | Analytical magnetic field analysis and prediction of cogging force and torque of a linear and rotary permanent magnet actuator显示文摘 | Jin Ping Fang Shuhu~ Lin Heyun | 2011 | IEEE Transactions on Magnetics2011，47，10： | 1 |
| 7 | Integrated UV-based photo microreactor-distillation technology toward process intensification of continuous ultra-high-purity electronic-grade silicon tetrachloride manufacture显示文摘Ultra-high-purity silicon tetrachloride(SiCl4)is demanded as an electronic-grade chemical to meet the stringent requirements of the rapidly developing semiconductor industry.The high requirement for ultra-high-purity SiCl4 has created the need for a high-efficient process for reducing energy consumption as well as satisfying product quality.In this paper,a mass of production technology of ultra-high-purity SiCl4 was successfully developed through chlorination reaction in the ultraviolet(UV)-based photo microreactor coupled with the distillation process.The influences of key operational parameters,including temperature,pressure,UV wavelength and light intensity on the product quality,especially for hydrogen-containing impurities,were quantified by the infrared transmittance of Fourier transform infrared spectroscopy(FT-IR)at 2185 cm^-1and 2160 cm^-1indicating that chara cteristic vib rational modes of Si-H bonds,as well as the operating conditions of distillation were also investigated as key factors for metal impurities removing.The advanced intensification of SiCl4 manufactured by the integration of photo microreactor and distillation achieves the products with superior specifications higher than the standard commercial products. | Ye Wan Wenhui Guo Jin Xiao Dazhou Yan Xiong Zhao Shuhu Guo Jianhua Liu Qifan Zhong Tao Yang Yu Zhao Xin Chang Xin Gao | 2020 | Chinese Journal of Chemical Engineering2020，28，9： | 1 |
| 8 | Accelerating effect and mechanism of passivation of polyaniline on ferrous metals显示文摘 | Hua Z Lian Z Shuhu X | 2004 | Electrochemical Acta2004，49，： | 1 |
| 9 | Ultra-uniform Sn Ox/carbon nanohybrids toward advanced lithium-ion battery anodes显示文摘 | ZHOU Xiaosi DAI Zhihui LIU Shuhu | 2014 | Advanced Materials2014，26，23： | 1 |
| 10 | Treatment of berberine hydrochloride wastewater by using pulse electro-coagulation process with Fe electrode显示文摘 | Meijie Ren Yonghui Song Shuhu Xiao Ping Zeng Jianfeng Peng | 2011 | Chemical Engineering Journal2011，，1： | 1 |
| 11 | Application of polyaniline to galvanic anodie protection on stainless steel in H2SO4 solutions显示文摘 | Lian Zhong Shuhu Xiao Jie Hu | 2006 | Corrosion science2006，48，12： | 1 |
| 12 | Isolation, identification and antioxidative capacity of water-soluble phenylpropanoid compounds from Rhodiola crenulata显示文摘 | Danjun Chen Junting Fan Peng Wang Lanying Zhu Yang Jin Yan Peng Shuhu Du | 2012 | Food Chemistry2012，，4： | 1 |
| 13 | Microwave electrodeless lamp assisted catalytic degradation of X-GRL with manganese dioxides: Adsorption and manganese(IV) reductive dissolution effects显示文摘 | Ruiping Liu Hongjie Wang Xu Zhao Shuhu Xiao Jiuhui Qu | 2008 | Catalysis Today2008，，1： | 1 |
| 14 | Stability comprehensive analysis model of iron deposit retained goaf显示文摘 | Lu Hongjian Yan Shuhu Pan Guihao | 2013 | Applied Mechanics and Materials2013，256，1： | 1 |
| 15 | miR-124 Represses ROCK1 Expression to Promote Neurite Elongation Through Activation of the PI3K/Akt Signal Pathway显示文摘 | Xi Gu Siying Meng Shuhu Liu Chunhong Jia Yingying Fang Shuji Li Congcong Fu Qiancheng Song Lifang Lin Xuemin Wang | 2014 | Journal of Molecular Neuroscience2014，，1： | 1 |
| 16 | Asymmetrically coordinated single-atom iron nanozymes with Fe-N_(1)C_(2)structure:A peroxidase mimetic for melatonin detection显示文摘Owing to the unique coordination environment and high atom utilization efficiency,single atom catalysts have been considered as an ideal artificial enzyme to mimic natural enzymes.Herein,single-atom Fe nanozyme anchored on N-doped Ti_(3)C_(2)Tx(Fe SA/N-Ti_(3)C_(2)Tx)with asymmetrically coordinated Fe-N_(1)C_(2)configuration is synthesized by vacancy capture and heteroatom doping strategy,which exhibits excellent peroxidase-like activity.Based on the results of peroxidase catalytic kinetics and X-ray adsorption fine spectroscopy,the Fe-N_(1)C_(2)active sites in Fe SA/N-Ti_(3)C_(2)Tx are responsible for the excellent performance.Furthermore,the developed Fe SA/N-Ti_(3)C_(2)Tx can be employed to quantitative detection of melatonin(MT),which shows a wide linear detection range(0.01-100μM)and an excellent detection limit(7.3 nM)in buffer,0.01-100μM and 7.8 nM in serum samples.Our work proves that MXene-based single atoms can be promising nanozyme in the field of bioassays. | Lihong Lin Heng Li Hongfei Gu Zhiyi Sun Juan Huang Zhenni Qian Hang Li Juzhe Liu Hongyan Xi Pengfei Wu Qingqing Liu Shuhu Liu Lirong Zheng Zhuo Chen Zhengbo Chen Juanjuan Qi | 2023 | Nano Research2023，16，4： | 1 |
| 17 | Accelerating Effect and Mechanism of Passivation of Polyaniline on Ferrous Metals显示文摘 | Zhu Hua Zhong Lian Xiao Shuhu | 2004 | Electrochimica Acta2004，49，： | 1 |
| 18 | Optical design and optimization study of metrology sector at high energy photon source显示文摘Introduction X-ray metrology,including the metrological calibration of X-ray detectors,optical elements and sources,is important for many frontier science,such as X-ray astronomy,EUV-lithography,plasma physics.Among many types of X-ray sources,synchrotron-radiation is considered perfect for X-ray metrology,mainly due to that arbitrarily X-rays specifications can be tailored to meet the demands of metrological calibration of X-ray detectors and optical elements.As a consequence,many metrology beamlines around the world are built,upgrading or to be constructed,including the metrology sector to be constructed at High Energy Photon Source(HEPS).Method One reasonable way to access good metrological data is using a stable X-ray beam,which means that beam position as well as flux should be as constant as possible and the beamline configuration should be simple and robust to reduce the uncertainty from beamline itself.In addition,the spectral purity of monochromatic X-rays is another crucial factor for X-ray metrology,which means stray X-rays and harmonic X-rays must be as low as possible.Many measures are taken to satisfy these requirements.Conclusion An optical design of the metrology sector optimized for synchrotron-radiation-based-metrology is described here.The metrology sector,ranging from 50 eV to 20 keV,will be set up to meet the growing needs of X-ray metrology in China.All beamlines’configurations are simple and easy to use,with an acceptable ratio of high-order harmonics and stray X-rays,which can be under 1%in the entire energy range. | Xiaojuan Zhao Yidong Zhao Lei Zheng Kun Tang Shuhu Liu Fan Li Jianmin Li | 2021 | Radiation Detection Technology and Methods2021，5，2： | 0 |
| 19 | A soft X-ray cryogenic radiometer built on BSRF显示文摘Introduction In the field of the high injection rate X-ray meterage,currently there are no national standards in China,which are urgently needed in areas such as inertial confinement fusion diagnosis and aerospace observation.Globally,many metrology laboratories have developed their own meterage standards based on Cryogenic radiometers.And one soft X-ray cryogenic radiometer has been installed at 4B7B experiment station on Beijing Synchrotron Radiation Facility to measure the X-ray power from 50 nW to 1μW.Purpose The purpose is to verify the accuracy of the X-ray power measurement and the performance of the cryogenic radiometer.Experimental The spectral responsivity of a Si photodiode detector calibrated in the Physikalisch-Technische Bundesanstalt of Germany is calibrated at 750eV again with the cryogenic radiometer based on synchrotron light source.Results Some important performance parameters(e.g.,time constant,responsivity,and nonequivalence error)of the cryogenic radiometer were measured and were in agreement with the design indexes.Calibration results show that total relative uncertainties of X-ray power measurement were below 1%(k=1),and that good consistency was received compared with the calibrations done by the PTB.Conclusion The cryogenic radiometer built at 4B7B is reliable and accurate for soft X-ray power measurement.And the performance of the cryogenic radiometer is also very good. | Xiaoliang Zhao Yidong Zhao Kun Tang Yashuai Zhao Fan Li Lei Zheng Shuhu Liu | 2018 | Radiation Detection Technology and Methods2018，2，2： | 0 |
| 20 | On the construction of the mechanism for the smooth operation of the internal power of the universities显示文摘 | He Shuhu | 2014 | International English Education Research2014，，4： | 0 |
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