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| 1 | Graphitic carbon nitride/biochar composite synthesized by a facile ball-milling method for the adsorption and photocatalytic degradation of enrofloxacin显示文摘In order to enhance the removal performance of graphitic carbon nitride(g-C_(3)N_(4)) on organic pollutant, a simultaneous process of adsorption and photocatalysis was achieved via the compounding of biochar and g-C_(3)N_(4). In this study, g-C_(3)N_(4) was obtained by a condensation reaction of melamine at 550 °C. Then the g-C_(3)N_(4)/biochar composites were synthesized by ball milling biochar and g-C_(3)N_(4) together, which was considered as a simple, economical, and green strategy. The characterization of resulting g-C_(3)N_(4)/biochar suggested that biochar and g-C_(3)N_(4) achieved effective linkage. The adsorption and photocatalytic performance of the composites were evaluated with enrofloxacin(EFA) as a model pollutant. The result showed that all the g-C_(3)N_(4)/biochar composites displayed higher adsorption and photocatalytic performance to EFA than that of pure g-C_(3)N_(4). The 50% g-C_(3)N_(4)/biochar performed best and removed 45.2% and 81.1% of EFA(10 mg/L) under darkness and light with a dosage of 1 mg/mL, while g-C_(3)N_(4) were 19.0% and 27.3%, respectively. Besides, 50% g-C_(3)N_(4)/biochar showed the highest total organic carbon(TOC) removal efficiency(65.9%). Radical trapping experiments suggested that superoxide radical( ·O_(2)^(-)) and hole(h~+) were the main active species in the photocatalytic process. After 4 cycles, the composite still exhibited activity for catalytic removal of EFA. | Yao Xiao Honghong Lyu Chengliang Yang Beibei Zhao Lan Wang Jingchun Tang | 2021 | Journal of Environmental Sciences2021，33，5： | 8 |
| 2 | Solvent-Free Synthesis of Ultrafine Tungsten Carbide Nanoparticles-Decorated Carbon Nanosheets for Microwave Absorption显示文摘Carbides/carbon composites are emerging as a new kind of binary dielectric systems with good microwave absorption performance.Herein,we obtain a series of tungsten carbide/carbon composites through a simple solvent-free strategy,where the solid mixture of dicyandiamide(DCA)and ammonium metatungstate(AM)is employed as the precursor.Ultrafine cubic WC1-x nanoparticles(3-4 nm)are in situ generated and uniformly dispersed on carbon nanosheets.This configuration overcomes some disadvantages of conventional carbides/carbon composites and is greatly helpful for electromagnetic dissipation.It is found that the weight ratio of DCA to AM can regulate chemical composition of these composites,while less impact on the average size of WC1-x nanoparticles.With the increase in carbon nanosheets,the relative complex permittivity and dielectric loss ability are constantly enhanced through conductive loss and polarization relaxation.The different dielectric properties endow these composites with distinguishable attenuation ability and impedance matching.When DCA/AM weight ratio is 6.0,the optimized composite can produce good microwave absorption performance,whose strongest reflection loss intensity reaches up to-55.6 dB at 17.5 GHz and qualified absorption bandwidth covers 3.6-18.0 GHz by manipulating the thickness from 1.0 to 5.0 mm.Such a performance is superior to many conventional carbides/carbon composites. | Yunlong Lian Binhua Han Dawei Liu Yahui Wang Honghong Zhao Ping Xu Xijiang Han Yunchen Du | 2020 | Nano-Micro Letters2020，12，11： | 7 |
| 3 | Composition Optimization and Microstructure Design in MOFs-Derived Magnetic Carbon-Based Microwave Absorbers:A Review显示文摘Magnetic carbon-based composites are the most attractive candidates for electromagnetic(EM)absorption because they can terminate the propagation of surplus EM waves in space by interacting with both electric and magnetic branches.Metal-organic frameworks(MOFs)have demonstrated their great potential as sacrificing precursors of magnetic metals/carbon composites,because they provide a good platform to achieve high dispersion of magnetic nanoparticles in carbon matrix.Nevertheless,the chemical composition and microstructure of these composites are always highly dependent on their precursors and cannot promise an optimal EM state favorable for EM absorption,which more or less discount the superiority of MOFs-derived strategy.It is hence of great importance to develop some accompanied methods that can regulate EM properties of MOFs-derived magnetic carbon-based composites e ectively.This review comprehensively introduces recent advancements on EM absorption enhancement in MOFs-derived magnetic carbon-based composites and some available strategies therein.In addition,some challenges and prospects are also proposed to indicate the pending issues on performance breakthrough and mechanism exploration in the related field. | Honghong Zhao Fengyuan Wang Liru Cui Xianzhu Xu Xijiang Han Yunchen Du | 2021 | Nano-Micro Letters2021，13，12： | 6 |
| 4 | Advances in core–shell engineering of carbon-based composites for electromagnetic wave absorption显示文摘Electromagnetic(EM)absorption is paving the way to overcome the challenges related to conventional shielding strategy against EM pollution through sustainable energy dissipation.As characteristic functional media that can interact with electric or magnetic field branch,EM wave absorption materials(EWAMs)have received extensive attention and realized considerable development in the past two decades,where carbon-based composites are always considered as promising candidates for high-performance EMAWs due to their synergetic loss mechanism as well as diversified composition and microstructure design.Recent progress indicates that there is more and more interest in the fabrication of carbon-based composites with unique core–shell configuration.On one hand,core–shell configuration usually ensures good chemical homogeneity of final products and provides some positive protections for the components with susceptibility to corrosion,on the other hand,it creates enough heterogeneous interfaces between different EM components,which may bring enhanced polarization effect and intensify the consumption of EM energy.In this review,we firstly introduce EM wave absorption theory,and then highlight the advances of core–shell engineering in carbonbased composites in terms of built-in carbon cores and built-out carbon shells.Moreover,we also show some special core–shell carbon-based composites,including carbon/carbon composites,assembled composites,and decorated composites.After analyzing EM absorption performance of some representative composites,we further propose some challenges and perspectives on the development of core–shell carbon-based composites. | Lixue Gai Honghong Zhao Fengyuan Wang Pan Wang Yonglei Liu Xijiang Han Yunchen Du | 2022 | Nano Research2022，15，10： | 5 |
| 5 | Effects of Ultrasonic Treatment on Residue Properties显示文摘The changes in properties and structural parameters of four vacuum residue samples before and after ultrasonic treatment were analyzed.Ultrasonic treatment could increase the carbon residue value,decrease the average molecular weight and viscosity,which can barely influence the density of vacuum residue.Meanwhile the constitution of residue can be varied including the decrease in the content of saturates,aromatics and asphaltenes,while the increase in the content of resins can lead to an increase in the total content of asphaltenes and resins.Among the four kinds of residue samples,there is a common trend that the more the content of asphaltenes in feedstock is,the more the increase in the content of resins,the more significant decrease in the aromatic content and the less decrease in the saturates content after ultrasonic treatment of residue would be.Changes in the structure and content of asphaltenes caused by ultrasonic treatment have a significant impact on the changes in residue properties.Ultrasonic treatment has changed the structural parameters of residue such as decrease in the total carbon number of average molecule (CTotal),the total number of rings (RT),the aromatic carbon number (CA),the aromatic rings number (RA)and the naphthenic rings number (RN),and increase of characterization factor (KH).The study has indicated that ultrasonic treatment of vacuum residue can change the average structure of residue,and the changes in the content and structure of asphaltenes are the main cause leading to property changes.The results of residue hydrotreating revealed that coke yield decreased,whereas the gas and light oil yield and conversion increased after ultrasonic treatment of vacuum residue. | Sun Yudong Zhang Qiang Shi Honghong Wang Xue Liu Bo | 2013 | China Petroleum Processing & Petrochemical Technology2013，15，4： | 5 |
| 6 | The OsNAC23-Tre6P-SnRK1 a feed-forward loop regulates sugar homeostasis and grain yield in rice显示文摘Tre6P(trehalose-6-phosphate)mediates sensing of carbon availability to maintain sugar homeostasis in plants,which underpins crop yield and resilience.However,how Tre6P responds to fluctuations in sugar levels and regulates the utilization of sugars for growth remains to be addressed.Here,we report that the sugar-inducible rice NAC transcription factor OsNAC23 directly represses the transcription of the Tre6P phosphatase gene TPP1 to simultaneously elevate Tre6P and repress trehalose levels,thus facilitating carbon partitioning from source to sink organs.Meanwhile,OsNAC23 and Tre6P suppress the transcription and enzyme activity of SnRK1a,a low-carbon sensor and antagonist of OsNAC23,to prevent the SnRK1a-mediated phosphorylation and degradation of OsNAC23.Thus,OsNAC23,Tre6P,and SnRK1a form a feed-forward loop to sense sugar and maintain sugar homeostasis by transporting sugars to sink organs.Importantly,plants over-expressing OsNAC23 exhibited an elevated photosynthetic rate,sugar transport,and sink organ size,which consistently increased rice yields by 13%–17%in three elite-variety backgrounds and two locations,suggesting that manipulation of OsNAC23 expression has great potential for rice improvement.Collectively,these findings enhance our understanding of Tre6P-mediated sugar signaling and homeostasis,and provide a new strategy for genetic improvement of rice and possibly also other crops. | Zhiyong Li Xiangjin Wei Xiaohong Tong Juan Zhao Xixi Liu Huimei Wang Liqun Tang Yazhou Shu Guanghao Li Yifeng Wang Jiezheng Ying Guiai Jiao Honghong Hu Peisong Hu Jian Zhang | 2022 | Molecular Plant2022，15，4： | 4 |
| 7 | Co-or Ni-modified Sn-MnO_(x) low-dimensional multi-oxides for high-efficient NH_(3)-SCR De-NO_(x):Performance optimization and reaction mechanism显示文摘NH_(3)-SCR performances were explored to the relationship between structure morphology and physio-chemical properties over low-dimensional ternary Mn-based catalysts prepared by one-step synthesis method.Due to its strong oxidation performance,Sn-MnO_(x) was prone to side reactions between NO,NH_(3)and O_(2),resulting in the generation of more NO_(2)and N_(2)O,here most of N_(2)O was driven from the non-selective oxidation of NH_(3),while a small part generated from the side reaction between NH_(3)and NO_(2).Co or Ni doping into Sn-MnO_(x) as solid solution components obviously stronged the electronic interaction for actively mobilization and weakened the oxidation performance for signally reducing the selective tendency of side reactions to N_(2)O.The optimal modification resulted in improving the surface area and enhancing the strong interaction between polyvalent cations in Co/Ni-Mn-SnO_(2)to provide more surface adsorbed oxygen,active sites of Mn^(3+) and Mn^(4+),high-content Sn^(4+) and plentiful Lewis-acidity for more active intermediates,which significantly broadened the activity window of Sn-MnOx,improved the N^(2) selectivity by inhibiting N_(2)O formation,and also contributed to an acceptable resistances to water and sulfur.At low reaction temperatures,the SCR reactions over three catalysts mainly obeyed the typical Elye-rideal(E-R)routs via the reactions of adsorbed L-NH_(x)(x=3,2,1)and B-NH_(4)^(+) with the gaseous NO to generate N_(2) but also N_(2)O by-products.Except for the above basic E-R reactions,as increasing the reaction temperature,the main adsorbed NO_(x)-species were bidentate nitrates that were also active in the Langmuir-Hinshelwood reactions with adsorbed L-NH_(x) species over Co/Ni modified Mn-SnO_(2) catalyst. | Fengyu Gao Chen Yang Xiaolong Tang Honghong Yi Chengzhi Wang | 2022 | Journal of Environmental Sciences2022，34，3： | 4 |
| 8 | Effects of Cs-substitution and partial reduction on catalytic performance of Keggin-type phosphomolybdic polyoxometalates for selective oxidation of isobutane显示文摘The catalytic performance of Cs-substituted phosphomolybdic salts was studied for selective oxidation of isobutane. The results of activity tests revealed that 360 °C was the optimal reaction temperature. It was demonstrated that oxidizing sites not only took dominating part in the activation of isobutane, but also influenced the product distribution. Besides, appropriate Cs addition led to moderate acidity of catalysts, favoring the selectivity to desired products. Furthermore, to obtain partially reduced catalysts, different calcination atmospheres were investigated and certain proportion of Mo^(5+) produced during calcination was crucial for the redox reaction. The catalyst calcined in N_2 showed the highest yield of MAA(7.0%). Fe-substitution enhanced the activity of catalysts by rapid reoxidation of Mo^(5+). | Shizhe Liu Lu Chen Guowei Wang Jianwei Liu Yanan Gao Chunyi Li Honghong Shan | 2016 | Journal of Energy Chemistry2016，25，1： | 4 |
| 9 | Self reported adherence to antiretroviral treatment and correlates in Hunan province,the Peoples Republic of China显示文摘Aims:This study aimed to describe the adherence level to antiretroviral therapy and its associated factors among people living with HIV in Hunan province,China.Methods:Across-sectional survey study was done at two major HIV treatment sites within Hunan province in China from July 2011 to Oct 2012 through face-to-face interviews.Adherence measures were captured using a 30-day visual analog scale(VAS).Results:A total of 418 participants consented and completed the questionnaires with the mean age being 38 years old.Based on VAS,28%of the participants had lower than 90%ART adherence level.The main reasons for missing drugs were;forgetting,being away from home,being busy and feeling worse after taking drugs.Logistic regression results showed that drug use(B=0.68,OR=2.11),time on ART(B=0.31,OR=0.72)and side effects(B=0.64,OR=1.82)were significantly associated with adherence to ART.Conclusion:Patients on ARVs in Hunan province are faced with adherence challenges notably drug abuse,drug regime scheduling challenges at the initial stages of therapy and drug side effects.It is therefore necessary to institute specific adherence interventions that target those who abuse drugs,ART naïve patients,and those experiencing side effects in order to achieve optimal ART adherence. | John Kipsang Jia Chen Chulei Tang Xianhong Li Honghong Wang | 2018 | International Journal of Nursing Sciences2018，5，2： | 4 |
| 10 | Rare-earth coordination polymer micro/nanomaterials: Preparation, properties and applications显示文摘Rare-earth coordination polymers (RECPs), as a family member ofcoordination polymers (CPs), have been prepared and studied widely. Thanks to their characteristic properties and functions, RECPs have already been used in various application fields ranging from catalysis to drug delivery. In recent years, CPs with tunable morphologies and sizes have drawn increasing interest and attractive attention. This review presents the recent research progress of RECP micro/nanomaterials, and emphasizes the preparation, properties and broad applications of these fascinating materials. | Honghong ZOU Lei WANG Chenghui ZENG Xiaolei GAO Qingqing WANG Shengliang ZHONG | 2018 | Frontiers of Materials Science2018，12，4： | 3 |
| 11 | Novel Mn-Ce bi-oxides loaded on 3D monolithic nickel foam for low-temperature NH_(3)-SCR de-NO_(x):Preparation optimization and reaction mechanism显示文摘This study explored the superior citrate method(CM)to synthesize Mn-Ce bi-oxides on 3 D monolithic Ni-foam(NF)catalysts for the selective catalytic reduction of NO by NH_(3)(NH_(3)-SCR).The 17 wt%Mn(7)Ce(3)O_(x)/NF(CM-17)catalyst shows the NO_(x)conversion of 98.7%at 175℃and 90%in the presence of 10 vol%H2 O.It is revealed that the combination of surface-active oxygen(formed by high-level oxygen vacancies)and strongly oxidized Mn4+species promots the Fast-SCR reactions,in which Mn4+species play a leading role in NH_(3)-SCR reaction,and the unsaturated Ni atoms and also Ce3+species promote electron exchange and thus improve the redox performance.The coexistence mechanisms of Fast-SCR reactions and E-R pathways are observed over Mn-CeO_(x)/NF catalyst,which may be promoted by the Br?nsted sites at low temperature.In addition,the heat resistance,stability,3 D monolithic porous structure and excellent physical properties of foam nickel provide a unique growth substrates for catalysts preparation and reaction sites for NO_(x)purification.Therefore,industrial application of Mn-Ce bioxides loaded on 3 D monolithic is proposed to be achieved through reasonable preparation methods. | Shuquan Ni Xiaolong Tang Honghong Yi Fengyu Gao Chengzhi Wang Yiran Shi Runcao Zhang Wenjuan Zhu | 2022 | Journal of Rare Earths2022，40，2： | 3 |
| 12 | Studies on the preliminary cracking: The reasons why matrix catalytic function is indispensable for the catalytic cracking of feed with large molecular size显示文摘The matrix catalytic function when cracking the feed oil with large molecular size was systematically studied using three different catalyst configurations,including staged bed,partly mixed bed and completely mixed bed.Results showed that molecules in the feed oil with large molecular size indeed preferred to be first precracked on the matrix surface and then entered into the zeolite pores during the practical reaction process.Furthermore,the matrix catalytic function exhibited a great matrix-precracking ability to large feed molecules,which considerably increased the catalyst activity and the light oil selectivity.Besides the much better accessibility,the matrix-precracking ability was also from the similar capability to crack large feed hydrocarbons into the moderate fragments with that of the zeolite component.More interestingly,the interactions between the matrix catalytic function and the zeolite catalytic function made the catalyst not only exhibit much more catalytic advantages of the zeolite component,but also retain the matrix-precracking ability.As a result,the interactions enhanced the catalyst activity and improved the product distribution at the same time.The matrix catalytic function is indispensable for the catalytic cracking of feed with large molecular size,although the matrix component itself presented an inferior catalytic performance than the zeolite component did. | Bin Wang Nan Li Qiang Zhang Chunyi Li Chaohe Yang Honghong Shan | 2016 | Journal of Energy Chemistry2016，25，4： | 2 |
| 13 | Correlation research on psychological health impact on nursing students against stress, coping way and social support显示文摘 | Yang Luo Honghong Wang | 2008 | Nurse Education Today2008，，1： | 2 |
| 14 | The Anti-inflammatory TIPE2 Is an Inhibitor of the Oncogenic Ras显示文摘 | Yael Gus-Brautbar Derek Johnson Li Zhang Honghong Sun Peng Wang Shirley Zhang Lining Zhang Youhai H. Chen | 2012 | Molecular Cell2012，，5： | 2 |
| 15 | Synthesis of sulfur doped C_(3)N_(4) with enhanced photocatalytic activity in molten salt显示文摘In this paper,sulfur doped g-C_(3)N_(4)(S-g-C_(3)N_(4))was successfully prepared at 500℃ for 3 h via a modified molten salt method using dicyandiamide as the main raw material,trithiocyanuric acid as the sulfur source and LiBreKCl as the reaction medium.The as-prepared SeCN5.0% sample(the mass ratio of trithiocyanuric acid to dicyandiamide was 5.0%)composed of irregular flakes showed a band gap of 1.83 eV,which was narrower than that(2.55 eV)of pristine g-C_(3)N_(4).The SeCN5.0% sample also exhibited an outstanding absorption capacity of visible light.Moreover,the photodegradation rate toward methylene blue and tetracycline were respectively 10 and 20 times as high as that of bulk g-C_(3)N_(4) prepared by conventional heating methods,confirming its superior photocatalytic performance.These results can be attributed to that the replacement of lattice nitrogen with sulfur atom tuned the electronic structure of g-C_(3)N_(4),improved the absorption of visible light,optimized the separation of photogenerated electron-hole pairs,and consequently enhanced the photocatalytic activity of g-C_(3)N_(4).Moreover,the trapping experiments implied that hole(ht)and superoxide radical($O2)were the main active species in the process of photodegradation. | Keke Guan Junyi Li Wen Lei Honghong Wang Zhaoming Tong Quanli Jia Haijun Zhang Shaowei Zhang | 2021 | Journal of Materiomics2021，7，5： | 2 |
| 16 | Research progress and debates on gaming disorder显示文摘Gaming disorder has become a significant issue in mental healthcare. While gaming is an important form of entertainment, excessive gaming may cause serious consequences for players. At present, there are still controversies in the academic community concerning the public health problems related to gaming disorder. This article attempts to expound the definition, epidemiology, aetiology, diagnosis, treatment and prevention of gaming disorder, in order to contribute to future conceptualization of gaming disorder. | Qianjin Wang Honghong Ren Jiang Long Yueheng Liu Tieqiao Liu | 2019 | General Psychiatry2019，32，3： | 2 |
| 17 | The biodiversity and composition of the dominant fecal microbiota in patients with inflammatory bowel disease显示文摘 | Sumei Sha Bin Xu Xin Wang Yongguo Zhang Honghong Wang Xiangyun Kong Hongwu Zhu Kaichun Wu | 2012 | Diagnostic Microbiology & Infectious Disease2012，，： | 1 |
| 18 | Nano-sized Ag rather than single-atom Ag determines CO oxidation activity and stability显示文摘Single-atom catalysis recently attracts great attentions,however,whether single atom or their nanoparticle(NP)has the advantage in its intrinsic activity remains under heated debate.Ag/Al_(2)O_(3) is a widely used catalyst for many catalytic reactions,while the effect of Ag particle size on the actity is seldom investigated due to the great difficulty in synthesizing single atom Ag and Ag clusters/particles with different sizes.Herein,we firstly prepared an atomically dispersed Ag/Al_(2)O_(3) catalyst using a nano-sized y-Al_(2)O_(3) as the support,subsequently obtained a series of Ag/Al_(2)O_(3) catalysts with different Ag particle sizes by H_(2) reducing single-atom Ag/Al_(2)O_(3) catalyst at various temperatures.The Ag/Al_(2)O_(3) treated at 600℃demonstrated superior CO oxidation performance over single-atom Ag/Al_(2)O_(3) and the Ag/Al_(2)O_(3) treated at 400 and 800℃.Based on experimental data and dpnsity functional theory(DFT)calculation results,we reveal that the larger Ag°particle is beneficial to oxygen activation and improves the valence stability during oxidation reaction,while the aggregation of Ag°particle also accordingly decreases the concentration of surface active sites,hence,there is an optimum Ag0 particle size.Our findings clearly confirm that Ag0nanoparticle has the advantage over single-atom Ag species in its intrinsic activity for CO oxidation. | Fei Wang Zhao Li Honghong Wang Min Chen Changbin Zhang Ping Ning Hong He | 2022 | Nano Research2022，15，1： | 1 |
| 19 | Polymer-bubbling for one-step synthesis of three-dimensional cobalt/carbon foams against electromagnetic pollution显示文摘Constructing three-dimensional(3D)foam-like structure in magnetic metal/carbon composites is regarded as a promising pathway to reinforce their electromagnetic(EM)functions.Herein,a nitrateassisted polymer-bubbling strategy is reported for the synthesis of Co/carbon foams,which is simply accomplished by direct pyrolyzing the mixture of polyvinylpyrrolidone(PVP)and cobalt nitrate hexahydrate(Co(NO_(3))_(2)·6 H_(2) O).Co(NO_(3))_(2)·6H_(2)O not only plays as the source of Co nanoparticles,but also accounts for the formation of 3D microstructure through releasing gas.By manipulating the weight ratio of Co(NO_(3))_(2)·6H_(2)O to PVP,the chemical composition,microstructure,and EM properties of these composites can be easily regulated.When the weight ratio reaches 1.5,the resultant composite displays good microwave absorption performance,whose reflection loss intensity and effective absorption bandwidth are superior to those of many common Co/C composites.EM analysis reveals that such architecture is greatly helpful to establish cross-linked conductive networks in the wax matrix,resulting in powerful dielectric loss under low absorber loading.Meanwhile,3D microstructure is also beneficial for multiple reflections that equal to extend the transmission path of incident EM waves.Simple synthesis strategy and desirable properties of these magnetic carbon foams may render them as the low-cost substitute of 3D graphene for the application against EM pollution. | Fengyuan Wang Ping Xu Ning Shi Liru Cui Yahui Wang Dawei Liu Honghong Zhao Xijiang Han Yunchen Du | 2021 | Journal of Materials Science & Technology2021，，34： | 1 |
| 20 | Novel functional variants locus in PLCE1 and susceptibility to esophageal squamous cell carcinoma: Based on published genome-wide association studies in a central Chinese population显示文摘 | Fujiao Duan Wei Xie Lihong Cui Peng Wang Chunhua Song Honghong Qu Kaijuan Wang Jianying Zhang Liping Dai | 2013 | Cancer Epidemiology2013，，： | 1 |
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