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| 1 | Ultraflexible,highly efficient electromagnetic interference shielding,and self-healable triboelectric nanogenerator based on Ti_(3)C_(2)T_(x) MXene for self-powered wearable electronics显示文摘Integrating smart functions into one flexible electronic is vastly valuable in improving their working performances and broadening applications.Here,this work reports a ultraflexible,highly efficient electromagnetic interference(EMI)shielding,and self-healable triboelectric nanogenerator(TENG)that is assembled by modified Ti_(3)C_(2)T_(x) MXene(m-MXene)-based nanocomposite elastomers.Benefitting from the excellent electronegativity of m-MXene,the single-electrode mode-based TENG can generate high open-circuit voltage(V_(oc))oscillating between-65 and 245 V,high short-circuit current(I_(sc))of 29 μA,and an instantaneously maximum peak power density of 1150 mW m^(-2) that can power twenty light-emitting diodes(LEDs).Moreover,the resultant TENG possesses outstanding EMI shielding performance with the maximum shielding effectiveness of 48.1 dB in the X-band.The enhanced shielding capability is dominated by the electromagnetic absorption owning to high conduction loss in m-MXene network,multiple reflections between m-MXene sheets,and polarization effect on the surface of m-MXene sheets.Additionally,a self-powered wearable sensor is fabricated based on the as-prepared TENG.The sensor shows an intrinsic healing ability with healing efficiency of 98.2% and can accurately detect the human large-scale motions and delicate physical signal.This work provides an enhanced way to fabricate the wearable electronics integrated with smart functions,and the reported MXene-based TENG may have a broad prospect in the fields of aerospace,artificial intelligence,and healthcare systems. | Yuzhang Du Xudong Wang Xingyi Dai Wenxuan Lu Yusheng Tang Jie Kong | 2022 | Journal of Materials Science & Technology2022，，5： | 2 |
| 2 | Factors affecting poplar wetwood characteristics显示文摘Wet wood is an abnormal phenomenon in growing trees,which adversely affects growth,subsequent wood processing and economic values of wood products.In this study,the influences of factors such as clones,afforestation methods,site conditions and climate conditions on the characteristics of poplar wetwood were studied through field investigations in 27 clones from 48 sample plots in 28 counties.Results showed that the incidences of wetwood were almost 100%in all plots.Ratios of wetwood area among the48 plots differed from 15.1 to 90.2%.Wetwood area ratios,moisture contents and pH differed significantly between the 27 clones.Wetwood area ratios of the clones ranged from18.7 to 62.3%.Ratios of wetwood areas were positively correlated with wet wood moisture content and pH,tree age,and negatively correlated with pH of sap wood.The repeatability of wet wood area ratios was 0.52,moderately controlled by genetics.Wetwood moisture content and pH were highly controlled by genetics,indicated by the repeatability of 0.91 and 0.89,respectively.There were significant differences in wetwood area ratios,moisture content and pH between different site conditions,afforestation methods,and geographical regions.Sloping land had the lowest wetwood area ratios and moisture content among four types of sites.Afforestation by direct seeding and rooted cuttings had the lowest wetwood area ratios and moisture content,respectively.In the three geographical regions,the Yellow River Basin had the lowest wetwood values of all three factors. | Qilin Zhang Xingyi Hu Qian Hu Jiawei Yang Tianyu Zhao Kebing Du | 2023 | Journal of Forestry Research2023，34，5： | 1 |
| 3 | Enzymatic formation of curcumin in vitro and in vivo显示文摘 | Jiaqing wang Taotao Xiong Jie Zhou Hongjian He Dongdong Wu Xuewen Du Xingyi Li Bing Xu | 2018 | Nano Research2018，11，6： | 1 |
| 4 | Drug-peptide supramolecular hydrogel boosting transcorneal permeability and pharmacological activity via ligand-receptor interaction显示文摘Boosting transcorneal permeability and pharmacological activity of drug poses a great challenge in the field of ocular drug delivery.In the present study,we propose a drug-peptide supramolecular hydrogel based on anti-inflammatory drug,dexamethasone(Dex),and Arg-Gly-Asp(RGD)motif for boosting transcorneal permeability and pharmacological activity via the ligand-receptor interaction.The drug-peptide(Dex-SA-RGD/RGE)supramolecular hydrogel comprised of uniform nanotube architecture formed spontaneously in phosphate buffered saline(PBS,pH=7.4)without external stimuli.Upon storage at 4℃,25℃,and 37℃ for 70 days,Dex-SA-RGD in hydrogel did not undergo significant hydrolysis,suggesting great long-term stability.In comparison to Dex-SA-RGE,Dex-SA-RGD exhibited a more potent in vitro anti-inflammatory efficacy in lipopolysaccharide(LPS)-activated RAW 264.7 macrophages via the inhibition of nuclear factorкB(NF-κB)signal pathway.More importantly,using drug-peptide supramolecular hydrogel labeled with 7-nitro-2,1,3-benzoxadiazole(NBD),the Dex-SA-K(NBD)RGD showed increased performance in terms of integrin targeting and cellular uptake compared to Dex-SA-K(NBD)RGE,as revealed by cellular uptake assay.On topical instillation in rabbit’s eye,the proposed Dex-SA-K(NBD)RGD could effectively enhance the transcorneal distribution and permeability with respect to the Dex-SA-K(NBD)RGE.Overall,our findings demonstrate the performance of the ligand-receptor interaction for boosting transcorneal permeability and pharmacological activity of drug. | Lin Chen Jie Deng Ailing Yu Yuhan Hu Bo Jin Pengyuan Du Jianhong Zhou Lei Lei Yuan Wang Serhii Vakal Xingyi Li | 2022 | Bioactive Materials2022，7，4： | 0 |
| 5 | A concise total synthesis of natural flavonols显示文摘In this study,we designed a convenient method,to total synthesis of fl avonols especially for C-5 substituted ones and derivatives on a large scale.Beginning from the inexpensively available 2,4,6-trihydroxyacetophenone through Aldol condensation reaction,I2/DMSO cyclization reaction,Oxone“one pot”oxidation,kaempferol(1)and derivative(2)was obtained in an overall yield of 35%.The structures of the target compound and key intermediates were verifi ed by MS,IR,1H-NMR and 13C-NMR techniques,and the structure of 5a was further confi rmed by X-ray diff raction analysis. | Gaigai Liu Shunqiang Gong Zhan Li Xingyi Du Xiaolou Miao Xuhong Ren | 2020 | Journal of Polyphenols2020，2，1： | 0 |
| 6 | Autocatalytic strategy for tuning drug release from peptide-drug supramolecular hydrogel显示文摘Peptide-drug conjugates(PDCs) composed of peptide, spacer and drug have gained extensive attention in the field of drug delivery owing to its precise control over the drug payload and architecture. However,the achievement of controllable and rapid drug release at targeted site by PDCs is still a great challenge for pharmaceutist. Herein, we introduced the histidine residue into PDCs to generate a supramolecular hydrogel via a p H-trigger strategy, which exhibited an autocatalytic effect to precisely tune drug release from PDCs hydrogel. Using indomethacin(Idm) as model drug, various PDCs(Y(Idm)EEH, Y(Idm)EEK and Y(Idm)EER) were synthesized and their self-assembling properties were investigated in terms of critical aggregation concentration(CAC), transmission electron microscopy(TEM) and rheometer. Introduction of histidine residue into PDCs presented a robust catalytic activity on the ester hydrolysis of p-nitrophenyl acetate in aqueous solution, as well conferred the autocatalytic capacity to hydrolyze the PDCs into active parent drug(Idm). Overall, we reported an autocatalytic activity of histidine residue to precisely tune drug release from PDCs hydrogels. | Yuqin Wu Tian Xia Xiaohui Ma Lei Lei Lulu Du Xiaoning Xu Xiangyi Liu Yueting Shi Xingyi Li Deqing Lin | 2023 | Chinese Chemical Letters2023，34，10： | 0 |
| 7 | Damage mechanism and evaluation model of compressor impeller remanufacturing blanks:A review显示文摘The theoretical and technological achievements in the damage mechanism and evaluation model obtained through the national basic research program“Key Fundamental Scientific Problems on Mechanical Equipment Remanufacturing”are reviewed in this work.Large centrifugal compressor impeller blanks were used as the study object.The materials of the blanks were FV520B and KMN.The mechanism and evaluation model of ultra-high cycle fatigue,erosion wear,and corrosion damage were studied via theoretical calculation,finite element simulation,and experimentation.For ultra-high cycle fatigue damage,the characteristics of ultra-high cycle fatigue of the impeller material were clarified,and prediction models of ultra-high cycle fatigue strength were established.A residual life evaluation technique based on the“b-HV-N”(where b was the nonlinear parameter,HV was the Vickers hardness,and N was the fatigue life)double criterion method was proposed.For erosion wear,the flow field of gas-solid two-phase flow inside the impeller was simulated,and the erosion wear law was clarified.Two models for erosion rate and erosion depth calculation were established.For corrosion damage,the electrochemical and stress corrosion behaviors of the impeller material and welded joints in H2S/CO2 environment were investigated.KISCC(critical stress intensity factor)and da/dt(crack growth rate,where a is the total crack length and t is time)varied with H2S concentration and temperature,and their variation laws were revealed.Through this research,the key scientific problems of the damage behavior and mechanism of remanufacturing objects in the multi-strength field and cross-scale were solved.The findings provide theoretical and evaluation model support for the analysis and evaluation of large centrifugal compressor impellers before remanufacturing. | Haiyang LU Yanle LI Fangyi LI Xingyi ZHANG Chuanwei ZHANG Jiyu DU Zhen LI Xueju RAN Jianfeng LI Weiqiang WANG | 2019 | Frontiers of Mechanical Engineering2019，14，4： | 0 |
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