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| 1 | Comprehensive reform of community health service in east,middle and west regions of China:from patients’perspective显示文摘Objectives:To analyze the satisfaction of patients with community health service(CHS)and the changes of the CHS delivered before and after the new health reform in different regions of China,and to put forward relevant policy recommendations for CHS development.Methods:Twelve community health centers were selected by random sampling in each of the eight typical cities in the east,middle and west regions of China.Questionnaire survey was conducted among patients visiting these institutions during daily work hours.Results:The proportions of the participants who stated that the medical environment,service attitude and medical skills of the doctors were improved were higher in the west region than those of the east and middle regions;but the percentage of patients who held that the drug price had lowered was higher in the east region than those of the middle and west region,the differences were of statistical significance(P<0.0125).The patients’satisfaction rates with medical environment,service attitude,and technical skills of the medical staff in the west region were 88.9%,91.5%and 81.6%respectively,which were higher than those in the east and middle regions.In the east region,the satisfaction rate with the reimbursement for this visit was 58.5%,which was highest among the three regions;in the west region,patients’satisfaction rates with drug types and preventive care were 51.5%and 65.9%,respectively,which was significantly higher than those in the east and middle regions(P<0.0125).As recommended by the participants,the top three aspects of health services that need to be improved were drug type and quality(25.3%),drug prices(21.8%)and technical skills(18.2%)in the east region;infrastructure(28.2%),drug prices(21.8%)and drug types and quality(21.2%)in the middle region;infrastructure(30.8%),drug types and quality(28.1%)and reimbursement(27.9%)in the west region.Conclusions:The comprehensive CHS reform should take the opinions of patients into account;essential drug system should be consolidated continually;and the reform of the payment system should be promoted by actively cooperating with the health insurance organizations. | JIANGMEI QIN YANCHUN ZHANG LIFANG ZHANG LIQUN LIU WEI ZHOU CAILING LIU LIKUN WANG JING LI | 2013 | Family Medicine and Community Health2013，1，2： | 6 |
| 2 | Efficient photo-assisted Fenton oxidation treatment of multi-walled carbon nanotubes显示文摘In this paper,a new and efficient way to oxidize and functionalize the multi-walled carbon nanotubes (MWNTs) has been developed by using a combination of ultraviolet (UV) irradiation and Fenton oxida-tion process,namely UV/Fenton oxidation treatment. Comparing with conventionally individual Fenton oxidation treatment of MWNTs,UV/Fenton combined treatment improved the etching rates and effi-ciencies and hence reduced the time for surface modification of MWNTs,which was proved to be an effective method in etching and functionalizing CNTs. The formation of new functional groups,struc-tural changes and thermal stability during oxidation period were characterized by Fourier transform infrared spectroscopy (FTIR),Raman spectroscopy and could be clarified by thermogravimetric analy-sis (TGA),which showed that it was under UV irradiation conditions that MWNTs could be rapidly functionalized with hydroxyl,carbonyl and carboxyl groups in the presence of Fenton reagents,origi-nating from the increase in the gross HO· concentration and the existent synergetic effect when using UV irradiation combing with Fenton oxidation process. Introduction of such new oxygen-containing functional groups was attributed to attacks of HO· on defect sites and unsaturated bonds of C=C in the MWNTs sample,which should play an important role in accounting for the FTIR and Raman spectral changes. | FAN CaiLing LI Wei LI Xin ZHAO ShiJu ZHANG Ling MO YuJun CHENG RongMing | 2007 | Chinese Science Bulletin2007，52，15： | 4 |
| 3 | N-doped carbon supported Pd catalysts for N-formylation of amines with CO2/H2显示文摘Using mesoporous N-doped carbons(NCs)derived from glucose and melamine as the supports,a series of Pd/NC catalysts were prepared,in which Pd nanoparticles with average size<2.0 nm were uniformly distributed on the supports.It was indicated that the resultant Pd/NC catalysts were effective for N-formylation of amines with CO_2and H_2in ethanol without any additives.Especially,the catalyst Pd/NC-800-6.9%containing quaternary N showed the best performance,affording a series of formylamides in good or even excellent yields.Further investigation reveals that the interaction between the Pd nanoparticles and quaternary nitrogen in the NC support was responsible for the good performance of the catalyst. | Xiaoying Luo Hongye Zhang Zhengang Ke Cailing Wu Shien Guo Yunyan Wu Bo Yu Zhimin Liu | 2018 | Science China Chemistry2018，61，6： | 4 |
| 4 | Template-directed Synthesis of Three Metal Oxalates via 4-Connected Building Units显示文摘 | TIAN Ruijing WANG Fuxiang DU Chunyu FENG Lijuan LIU Ying ZHANG Cailing PAN Qinhe | 2014 | Chemical Research in Chinese Universities2014，30，6： | 3 |
| 5 | Impacts of Land-Use Data on the Simulation of Surface Air Temperature in Northwest China显示文摘This study examines the impacts of land-use data on the simulation of surface air temperature in Northwest China by the Weather Research and Forecasting(WRF) model. International Geosphere–Biosphere Program(IGBP) landuse data with 500-m spatial resolution are generated from Moderate Resolution Imaging Spectroradiometer(MODIS)satellite products. These data are used to replace the default U.S. Geological Survey(USGS) land-use data in the WRF model. Based on the data recorded by national basic meteorological observing stations in Northwest China, results are compared and evaluated. It is found that replacing the default USGS land-use data in the WRF model with the IGBP data improves the ability of the model to simulate surface air temperature in Northwest China in July and December 2015. Errors in the simulated daytime surface air temperature are reduced, while the results vary between seasons. There is some variation in the degree and range of impacts of land-use data on surface air temperature among seasons. Using the IGBP data, the simulated daytime surface air temperature in July 2015 improves at a relatively small number of stations, but to a relatively large degree; whereas the simulation of daytime surface air temperature in December 2015 improves at almost all stations, but only to a relatively small degree(within 1°C). Mitigation of daytime surface air temperature overestimation in July 2015 is influenced mainly by the change in ground heat flux. The modification of underestimated temperature comes mainly from the improvement of simulated net radiation in December 2015. | Yaohui LI Cailing ZHAO Tiejun ZHANG Wei WANG Haixia DUAN Yuanpu LIU Yulong REN Zhaoxia PU | 2018 | Journal of Meteorological Research2018，32，6： | 2 |
| 6 | Evaluation of the Forecast Accuracy of Near-Surface Temperature and Wind in Northwest China Based on the WRF Model显示文摘This study investigated the performance of the mesoscale Weather Research and Forecasting(WRF) model in predicting near-surface atmospheric temperature and wind for a complex underlying surface in Northwest China in June and December 2015. The spatial distribution of the monthly average bias errors in the forecasts of 2-m temperature and 10-m wind speed is analyzed first. It is found that the forecast errors for 2-m temperature and 10-m wind speed in June are strongly correlated with the terrain distribution. However, this type of correlation is not apparent in December, perhaps due to the inaccurate specification of the surface albedo and freezing-thawing process of frozen soil in winter in Northwest China in the WRF model. In addition, the WRF model is able to reproduce the diurnal variation in 2-m temperature and 10-m wind speed, although with weakened magnitude. Elevations and land-use types have strong influences on the forecast of near-surface variables with seasonal variations. The overall results imply that accurate specification of the complex underlying surface and seasonal changes in land cover is necessary for improving near-surface forecasts over Northwest China. | Haixia DUAN Yaohui LI Tiejun ZHANG Zhaoxia PU Cailing ZHAO Yuanpu LIU | 2018 | Journal of Meteorological Research2018，32，3： | 2 |
| 7 | Different expression of alternative lengthening of telomere (ALT)-associated proteins/ mRNAs in osteosarcoma cell lines显示文摘 | ZHANG Y CAIL L WEIR X | 2011 | Oncology Letter2011，2，6： | 1 |
| 8 | The eli;err of cation content of some raw an ion-exchanged Victoria lignites on their equilibrium moisture content and surface area 显示文摘 | Yi Fei Cailing Zhang Marc Marshall | 2007 | Fuel2007，86，： | 1 |
| 9 | Freeze-drying and hot-pressing strategy to embed two-dimensional Ti_(0.87)O_(2) monolayers in commercial polypropylene films with enhanced dielectric properties显示文摘The dielectric capacitor has been widely used in advanced electronic and electrical power systems due to its capability of ultrafast charging–discharging and ultrahigh power density.Nevertheless,its energy density is still limited by the low dielectric constant(≈2.2)of the commercial dielectric polypropylene(PP).The conventional enhancement strategy by embedding inorganic fillers in PP matrix is still difficult and challenging due to that PP hardly dissolves in any inorganic/organic solvent.In this work,we develop a new strategy including freeze-drying,surface functionalization,and hot-pressing to incorporate Ti_(0.87)O_(2) monolayers in PP film.A series of uniform composited Ti_(0.87)O_(2)@PP film has been successfully fabricated with Ti0.87O2 content range of 0–15 wt%.The maximum dielectric constant of the as-prepared Ti_(0.87)O_(2)@PP film is 3.27 when the Ti_(0.87)O_(2) content is 9 wt%,which is about 1.5 times higher than that of pure PP.Our study provides a feasible strategy to embed two-dimensional material into commercial PP thin-film with superior dielectric performance for practical application. | Wenchao Tian Fei Yan Cailing Cai Zeyi Wu Chenchen Zhang Ting Yin Sijia Lao Linfeng Hu | 2021 | Journal of Advanced Ceramics2021，10，2： | 1 |
| 10 | Electron transfer in protein modifications:from detection to imaging显示文摘Signal pathways participate in vital biological processes and regulate complex life activities through protein modifications.Protein modifications in signal pathways are accompanied by electron transfer.The study of electronic behavior helps to explore the physical and chemical processes in signal pathways,receiving extensive attention.There are some excellent reviews that have summarized methods for signal pathway detection,while few discussions are from an electron transfer perspective.This review describes the relationship between signal pathways and electron transfer in protein modification.Subsequently,we summarize the electron transfer-based detection methods,such as electrochemical,photoelectrochemical and electrochemiluminescence methods.Additionally,the applications of signal pathway detection in mechanism study and imaging are also reviewed.Finally,a comprehensive discussion of the summary and outlooks in this field is presented,aiming to provide valuable guidance for the molecular mechanism of life processes and the development of new analytical techniques. | Lei Zhang Mengge Chu Cailing Ji Wenjie Wang Jie Tan Quan Yuan | 2023 | Science China Chemistry2023，66，2： | 1 |
| 11 | Synthesis and Characterization of a PVA/LiCl Blend Membrane for Air Dehumidification显示文摘 | Zhang Lizhi Wang Yuanyuan Wang Cailing | 2008 | Journal of Membrane Science2008，308，12： | 1 |
| 12 | Ionic liquids-SBA-15 hybrid catalysts for highly efficient and solvent-free synthesis of diphenyl carbonate显示文摘Diphenyl carbonate(DPC)is one of the versatile carbonates,and is often used for the production of polycarbonates.In recent years,the catalytic synthesis of DPC has become an important topic but the development of a highly active metal-free catalyst is a great challenge.Herein,a series of ionic liquids-SBA-15 hybrid catalysts with different functional groups have been developed for the synthesis of DPC under solventfree condition,which are effective and clean instead of the metal-containing catalysts.It is found that in the presence of[SBA-15-IL-OH]Br catalyst,methyl phenyl carbonate(MPC)conversion of 80.5%along with 99.6%DPC selectivity is achieved,the TOF value is thrice higher than the best value reported by using transition metal-based catalysts.Moreover,the catalyst displays remarkable stability and recyclability.This work provides a new idea to design and prepare eco-friendly catalysts in a broad range of applications for the green synthesis of carbonates. | Songlin Wang Qiying Zhang Chengxing Cui Hongying Niu Cailing Wu Jianji Wang | 2023 | Green Energy & Environment2023，8，1： | 1 |
| 13 | The effects of different vegetation restoration patterns on soil bacterial diversity for sandy land in Hulunbeier显示文摘 | Haifang Zhang Xiaolong Song Cailing Wang Hongmei Liu Jingni Zhang Yujie Li Gang Li Dianlin Yang Shulan Zhao | 2013 | Acta Ecologica Sinica2013，，4： | 1 |
| 14 | Preparation,applications,and challenges of functional DNA nanomaterials显示文摘As a carrier of genetic information,DNA is a versatile module for fabricating nanostructures and nanodevices.Functional molecules could be integrated into DNA by precise base complementary pairing,greatly expanding the functions of DNA nanomaterials.These functions endow DNA nanomaterials with great potential in the application of biomedical field.In recent years,functional DNA nanomaterials have been rapidly investigated and perfected.There have been reviews that classified DNA nanomaterials from the perspective of functions,while this review primarily focuses on the preparation methods of functional DNA nanomaterials.This review comprehensively introduces the preparation methods of DNA nanomaterials with functions such as molecular recognition,nanozyme catalysis,drug delivery,and biomedical material templates.Then,the latest application progress of functional DNA nanomaterials is systematically reviewed.Finally,current challenges and future prospects for functional DNA nanomaterials are discussed. | Lei Zhang Mengge Chu Cailing Ji Jie Tan Quan Yuan | 2023 | Nano Research2023，16，3： | 0 |
| 15 | Oxidized Nb_(2)C MXene as catalysts for lithium-sulfur batteries:Mitigating the shuttle phenomenon by facilitating catalytic conversion of lithium polysulfides显示文摘Extensive research has been devoted to lithium-sulfur(Li-S)batteries due to their overwhelming promises and advantages such as high theoretical capacity(1675 m Ah g^(-1)),extremely cost effectiveness and abundance and availability of sulfur.Nevertheless,a sluggish electrochemical kinetics of the battery limited by a slow conversion of lithium polysulfide(LiPSs)intermediates and Li PSs shuttle effect severely hinder its development towards industrial application.Herein,we designed the oxidized Nb2_(C)MXene with amorphous carbon(Nb_(2)O_(5)/C)composites as sulfur host using CO_(2)treatment to address the above issues.The Nb_(2)O_(5)/C composites with high conductivity are directly employed as sulfur hosts for Li-S battery capable to remarkably mitigate the shuttle phenomenon due to a combined effect of their Li PSs trapping ability and catalytic activity towards their accelerated conversion.Meanwhile,the unique layered structure of the composite facilitates ion transfer and accommodates the volume changes of the cathode during cycling.With this rational design,the resultant Li-S batteries exhibit superior electrochemical performance with a high initial specific capacity of 745 m Ah g^(-1)at 1.0 C and a reversible capacity of 620 m Ah g^(-1)at a high rate cycling at 3.0 C. | Cailing Song Wen Zhang Qianwen Jin Yan Zhao Yongguang Zhang Xin Wang Zhumabay Bakenov | 2022 | Journal of Materials Science & Technology2022，，24： | 0 |
| 16 | Metal-atom-doped W_(18)O_(49) nanowires for electrocatalytic oxygen evolution reaction in alkaline medium显示文摘Non-noble transition metal oxides(TMOs)are promising catalysts with improved catalytic activity and stability in oxygen evolution reaction(OER).However,the structural complexity of TMO-based electrocatalysts renders the determination of the active sites and OER mechanisms challenging.Here,we demonstrate that the OER activity of Co-doped one-dimensional W_(18)O_(49)(Co-W_(18)O_(49))is intrinsically dominated by the surface structure and electronic properties of the octahedral sites and Co-O-W bonds.Compared with RuO_(2) and W_(18)O_(49) heterogeneous electrocatalysts,Co-W_(18)O_(49) exhibits higher turnover frequency,attaining 1.97 s−1 at 500 mV overpotential.The results indicate that Co substitution contributes to the localized charge distribution of the active octahedral sites constructed by the Co-O-W bonds under OER conditions.Here,we determine the mechanism of TMOs for the OER,which may be applied to various other TMOs for OER electrocatalyst design. | Liangbo Xie Long Hai Yuan Meng Wenwen Zheng Huapu Hu Denghui Shang Ke Shao Cailing Zhang Yi Li | 2023 | ChemPhysMater2023，2，2： | 0 |
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