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| 1 | Ionic liquid mediated CO_2 activation for DMC synthesis显示文摘Promoted catalytic reaction between methanol and CO2 for dimethyl carbonate(DMC) synthesis is conducted over K2CO3/CH3 I catalyst in the presence of ionic liquid under microwave irradiation.The effect of ionic liquids incorporated with microwave irradiation on the yield of DMC is investigated.DMC was found to form at lower temperature in a relative short time,which indicated an enhanced catalytic process by ionic liquid.Among the ionic liquids used,1-butyl-3-methylimidazolium chloride is the most effective promoter.Density functional theory calculations indicate that CO2 bond lengths and angles changed due to the molecular interaction of ionic liquid and CO2,resulting in the activation of CO2 molecules and consequently the acceleration of reaction rate. | Jun Du Jing Shi Zhengfei Li Zuohua Liu Xing Fan Changyuan Tao | 2012 | Journal of Natural Gas Chemistry2012，21，4： | 7 |
| 2 | Direct observation of Pt nanocrystal coalescence induced by electron-excitation-enhanced van der Waals interactions显示文摘 | Ying Jiang Yong Wang Yu Yang Zhang Zhengfei Zhang Wentao Yuan Chenghua Sun Xiao Wei Casey N. Brodsky Chia-Kuang Tsung Jixue Li Xiaofeng Zhang Scott X. Mao Shengbai Zhang Ze Zhang | 2014 | Nano Research2014，7，3： | 4 |
| 3 | Integrated treatment for lower-limb stage Ⅱ thromboangiitis obliterans by interventional therapy and oral administration of Chinese medicine: a randomized controlled clinical trial显示文摘OBJECTIVE: To observe if integrated treatment is better than other therapies for lower-limb stage thromboangiitis obliterans(TAO).ⅡMETHODS: Ninety lower-limb stage randomly dividedⅡ i or worse TAO patients werento three groups: group A(30 cases) treated by intervention and oral administration of Chinese medicine; groupB(30 cases) treated by intervention alone; and group C(30 cases) treated only with oral administration of Chinese medicine. Therapeutic effects were observed, including the cure rate; the recurrence rate after one month, three months, six months, nine months, and one year; the ankle brachial indexes; the incidence of complications; and the level of C-reactive protein and erythrocyte sedimentation rate.RESULTS: Group A had significantly better clinically curative effects, related indexes, and outcomes during the long-term follow-up survey, than that of groups B and C.CONCLUSION: Integrated treatment is more effective for treating lower-limb stage Ⅱ or worse TAO. | Chang Yaowen Li Fenqiang Wang Wenhui Song Laichang Li Li Li Zhengfei Su Dongjun Fu Zhaoliang | 2015 | Journal of Traditional Chinese Medicine2015，35，1： | 3 |
| 4 | CuAlCl4 doped MIL-101 as a high capacity CO adsorbent with selectivity over N2显示文摘 | Yixiu WANG Chao LI Fanchao MENG Shuling LV Jintao GUO Xiaoqin LIU Chongqing WANG Zhengfei MA | 2014 | Frontiers of Chemical Science and Engineering2014，8，3： | 3 |
| 5 | Lamellar hafnium ditelluride as an ultrasensitive surface-enhanced Raman scattering platform for label-free detection of uric acid显示文摘The development of two-dimensional(2D)transition metal dichalcogenides has been in a rapid growth phase for the utilization in surface-enhanced Raman scattering(SERS)analysis.Here,we report a promising 2D transition metal tellurides(TMTs)material,hafnium ditelluride(HfTe2),as an ultrasensitive platform for Raman identification of trace molecules,which demonstrates extraordinary SERS activity in sensitivity,uniformity,and reproducibility.The highest Raman enhancement factor of 2.32×10^(6)is attained for a rhodamine 6G molecule through the highly efficient charge transfer process at the interface between the HfTe2 layered structure and the adsorbed molecules.At the same time,we provide an effective route for large-scale preparation of SERS substrates in practical applications via a facile stripping strategy.Further application of the nanosheets for reliable,rapid,and label-free SERS fingerprint analysis of uric acid molecules,one of the biomarkers associated with gout disease,is performed,which indicates arresting SERS signals with the limits of detection as low as 0.1 mmol/L.The study based on this type of 2D SERS substrate not only reveals the feasibility of applying TMTs to SERS analysis,but also paves the way for nanodiagnostics,especially early marker detection. | YANG LI HAOLIN CHEN YANXIAN GUO KANGKANG WANG YUE ZHANG PEILIN LAN JINHAO GUO WEN ZHANG HUIQING ZHONG ZHOUYI GUO ZHENGFEI ZHUANG ZHIMING LIU | 2021 | Photonics Research2021，9，6： | 2 |
| 6 | MicroRNA 23b Regulates Autophagy Associated With Radioresistance of Pancreatic Cancer Cells显示文摘 | Peng Wang Juan Zhang Li Zhang Zhengfei Zhu Jie Fan Lianyu Chen Liping Zhuang Jianmin Luo Hao Chen Luming Liu Zhen Chen Zhiqiang Meng | 2013 | Gastroenterology2013，，5： | 1 |
| 7 | miR-92a is a critical regulator of the apoptosis pathway in glioblastomawith inverse expression of BCL2L11显示文摘 | Huanjiang Niu Kun Wang Anling Zhang Shuxu Yang Zhengfei Song Wei Wang Cong Qian Xinwei Li Yinxin Zhu Yirong Wang | 2012 | Oncology Reports2012，，5： | 1 |
| 8 | Observation of Pt-{100}-p(2×2)-O reconstruction by an environmental TEM显示文摘The surface structure of noble metal nanoparticles usually plays a crucial role during the catalytic process in the fields of energy and environment. It has been studied extensively by surface analytic methods, such as scanning tunneling microscopy. However, it is still challenging to secure a direct observation of the structural evolution of surfaces of nanocatalysts in reaction(gas and heating) conditions at the atomic scale. Here we report an in-situ observation of atomic reconstruction on Pt {100} surfaces exposed to oxygen in an environmental transmission electron microscope(TEM). Our high-resolution TEM images revealed that Pt-{100}-p(2×2)-O reconstruction occurs during the reaction between oxygen atoms and{100} facets. A reconstruction model was proposed, and TEM images simulated according to this model with different defocus values match the experimental results well. | Hengbo Li Wentao Yuan Ying Jiang Zhengfei Zhang Ze Zhang Yong Wang | 2016 | Progress in Natural Science:Materials International2016，26，3： | 1 |
| 9 | Magnetecaloric Effect of GdCo2-x Alx Compounds 显示文摘 | Gu Zhengfei Zhou Bo Li Junqin | 2007 | Solid State Communications2007，141，： | 1 |
| 10 | Number of Negative Lymph Nodes is Associated with Survival in Thoracic Esophageal Squamous Cell Carcinoma Patients Undergoing Three-Field Lymphadenectomy显示文摘 | Zhengfei Zhu Haiquan Chen Weiwei Yu Xiaolong Fu Jiaqing Xiang Hecheng Li Yawei Zhang Menghong Sun Qiao Wei Weixin Zhao Kuaile Zhao | 2014 | Annals of Surgical Oncology2014，，9： | 1 |
| 11 | Transcriptional landscapes of de novo root regeneration from detached Arabidopsis leaves revealed by time-lapse and single-cell RNA sequencing analyses显示文摘Detached Arabidopsis thaliana leaves can regenerate adventitious roots,providing a platformfor studying de novo root regeneration(DNRR).However,the comprehensive transcriptional framework of DNRR remains elusive.Here,we provide a high-resolution landscape of transcriptome reprogramming from wound response to root organogenesis in DNRR and show key factors involved in DNRR.Time-lapse RNA sequencing(RNA-seq)of the entire leaf within 12 h of leaf detachment revealed rapid activation of jasmonate,ethylene,and reactive oxygen species(ROS)pathways in response towounding.Genetic analyses confirmed that ethylene andROSmay serve as wound signals to promoteDNRR.Next,time-lapse RNA-seq within 5 d of leaf detachment revealed the activation of genes involved in organogenesis,wound-induced regeneration,and resource allocation in the wounded region of detached leaves during adventitious rooting.Genetic studies showed that BLADE-ON-PETIOLE1/2,which control aboveground organs,PLETHORA3/5/7,which control root organogenesis,and ETHYLENE RESPONSE FACTOR115,which controlswound-induced regeneration,are involved in DNRR.Furthermore,single-cell RNA-seq data revealed gene expression patterns in thewounded region of detached leaves during adventitious rooting.Overall,our study not only provides transcriptome tools but also reveals key factors involved in DNRR from detached Arabidopsis leaves. | Wu Liu Yuyun Zhang Xing Fang Sorrel Tran Ning Zhai Zhengfei Yang Fu Guo Lyuqin Chen Jie Yu Madalene SIson Teng Zhang Lijun Sun Hongwu Bian Yijing Zhang Li Yang Lin Xu | 2022 | Plant Communications2022，3，4： | 0 |
| 12 | Evolutionary changes of Hox genes and relevant regulatory factors provide novel insights into mammalian morphological modifications显示文摘The diversity of body plans of mammals accelerates the innovation of lifestyles and the extensive adaptation to different habitats,including terrestrial,aerial and aquatic habitats.However,the genetic basis of those phenotypic modifications,which have occurred during mammalian evolution,remains poorly explored.In the present study,we synthetically surveyed the evolutionary pattern of Hox clusters that played a powerful role in the morphogenesis along the head-tail axis of animal embryos and the main regulatory factors(Mll,Bmi1 and E2f6)that control the expression of Hox genes.A deflected density of repetitive elements and lineage-specific radical mutations of Mll have been determined in marine mammals with morphological changes,suggesting that evolutionary changes may alter Hox gene expression in these lineages,leading to the morphological modification of these lineages.Although no positive selection was detected at certain ancestor nodes of lineages,the increasedωvalues of Hox genes implied the relaxation of functional constraints of these genes during the mammalian evolutionary process.More importantly,49 positively-selected sites were identified in mammalian lineages with phenotypic modifications,indicating adaptive evolution acting on Hox genes and regulatory factors.In addition,3 parallel amino acid substitutions in some Hox genes were examined in marine mammals,which might be responsible for their streamlined body. | Kui LI Xiaohui SUN Meixiu CHEN Yingying SUN Ran TIAN Zhengfei WANG Shixia XU Guang YANG | 2018 | Integrative Zoology2018，13，1： | 0 |
| 13 | Smart Management Information Systems(Smis):Concept,Evolution,Research Hotspots and Applications显示文摘Management information system(MiS),a human-computer system that deeply integrates next-generation information technology and management services,has become the nerve center of society and organizations.With the development of next-generation information technology,Mis has gradually entered the smart period.However,research on smart managementinformation systems(SMIS)is still limited,lacking systematic summarization of its conceptual definition,evolution,research hotspots,and typical applications.Therefore,this paper defines the conceptual characteristics of SMIS,provides an overview of the evolution of SMIS,examines research focus areas using bibliometric methods,and elaborates on typical application practices of sMis in fields such as health care,elderly care,manufacturing,and transportation.Furthermore,we discuss the future development directions of SMIS in four key areas:smart interaction,smart decisionmaking,efficient resource allocation,and flexible system architecture.These discussions provide guidance and a foundation for the theoretical development and practical application of SMIS. | Changyong Liang Xiaoxiao Wang Dongxiao Gu Pengyu Li Hui Chen Zhengfei Xu | 2023 | Data Intelligence2023，5，4： | 0 |
| 14 | Dual-sized hollow particle incorporated fibroin thermal insulating coatings on catheter for cerebral therapeutic hypothermia显示文摘Selective endovascular hypothermia has been used to provide cooling-induced cerebral neuroprotection,but current catheters do not support thermally-insulated transfer of cold infusate,which results in an increased exit temperature,causes hemodilution,and limits its cooling efficiency.Herein,air-sprayed fibroin/silica-based coatings combined with chemical vapor deposited parylene-C capping film was prepared on catheter.This coating features in dual-sized-hollow-microparticle incorporated structures with low thermal conductivity.The infusate exit temperature is tunable by adjusting the coating thickness and infusion rate.No peeling or cracking was observed on the coatings under bending and rotational scenarios in the vascular models.Its efficiency was verified in a swine model,and the outlet temperature of coated catheter(75μm thickness)was 1.8-2.0◦C lower than that of the uncoated one.This pioneering work on catheter thermal insulation coatings may facilitate the clinical translation of selective endovascular hypothermia for neuroprotection in patients with acute ischemic stroke. | Ming Li Yuan Gao Miaowen Jiang Hongkang Zhang Yang Zhang Yan Wu Wenhao Zhou Di Wu Chuanjie Wu Longfei Wu Luzi Bao Xiaoxiao Ge Zhengfei Qi Ming Wei Ang Li Yuchuan Ding Jicheng Zhang Guangzhen Pan Yu Wu Yan Cheng Yufeng Zheng Xunming Ji | 2023 | Bioactive Materials2023，，8： | 0 |
| 15 | Responses of diff erent biodiversity indices to subsampling efforts in lotic macroinvertebrate assemblages显示文摘As a less time-consuming procedure, subsampling technology has been widely used in biological monitoring and assessment programs. It is clear that subsampling counts af fect the value of traditional biodiversity indices, but its ef fect on taxonomic distinctness(TD) indices is less well studied. Here, we examined the responses of traditional(species richness, Shannon-Wiener diversity) and TD(average taxonomic distinctness: Δ +, and variation in taxonomic distinctness: Λ +) indices to subsample counts using a random subsampling procedure from 50 to 400 individuals, based on macroinvertebrate datasets from three dif ferent river systems in China. At regional scale, taxa richness asymptotically increased with ?xed-count size; ≥250–300 individuals to express 95% information of the raw data. In contrast, TD indices were less sensitive to the subsampling procedure. At local scale, TD indices were more stable and had less deviation than species richness and Shannon-Wiener index, even at low subsample counts, with ≥100 individuals needed to estimate 95% of the information of the actual Δ + and Λ + in the three river basins. We also found that abundance had a certain ef fect on diversity indices during the subsampling procedure, with dif ferent subsampling counts for species richness and TD indices varying by regions. Therefore, we suggest that TD indices are suitable for biodiversity assessment and environment monitoring. Meanwhile, pilot analyses are necessary when to determine the appropriate subsample counts for bioassessment in a new region or habitat type. | WANG Jun LI Zhengfei SONG Zhuoyan ZHANG Yun JIANG Xiaoming XIE Zhicai | 2019 | Journal of Oceanology and Limnology2019，37，1： | 0 |
| 16 | Preparation and characterization of SO_(4)^(2−)−/TiO_(2)and S_(2)O_(8)^(2)−/TiO_(2) catalysts显示文摘Nanosized solid superacids SO_(4)^(2−)/TiO_(2)and S_(2)O_(8)^(2)−/TiO_(2),as well as MCM-41-supported SO_(4)^(2−)/ZrO_(2),were prepared.Their structures,acidities,and catalytic activities were investigated and compared using XRD,N2 adsorption-desorption,and in situ FTIR-pyridine adsorption,as well as an evaluation reaction with pseudoionone cyclization.The results showed that SO_(4)^(2−)/TiO_(2)and S_(2)O_(8)^(2)−/TiO_(2)possess not only nanosized particles with diameters<7.0 nm,a BET sur-face greater than 140 cm2/g and relatively regular mesostruc-tures with pores around 4.0 nm,but also a pure anatase phase and strong acidity.Different from the Lewis acid nature of SO_(4)^(2−)/ZrO_(2)/MCM-41,SO_(4)^(2−)/TiO_(2)and S_(2)O_(8)^(2)−/TiO_(2)exhibit mainly Brønsted acidities.The strongest Brønsted acid sites were produced on SO_(4)^(2−)/TiO_(2)promoted with H2SO4,while Lewis acid sites on S_(2)O_(8)^(2)−/TiO_(2)even stronger than those on SO_(4)^(2−)/ZrO_(2)/MCM-41 were generated when persulfate solu-tion was used as sulfating agent.Because of their distinct acid natures,SO_(4)^(2−)/TiO_(2)and S_(2)O_(8)^(2)−/TiO_(2)exhibited catalytic activities for the cyclization of pseudoionone that were much higher than that of SO_(4)^(2−)/ZrO_(2)/MCM-41.It can be concluded that the existence of more Brønsted acid sites was favorable for proton participation in the cyclization reaction. | MA Xuedan GUO Daishi JIANG Qizhong MA Zifeng MA Zhengfei YE Weidong LI Chunbo | 2007 | Frontiers of Chemical Science and Engineering2007，1，1： | 0 |
| 17 | Environmental filtering and spatial processes equally contributed to macroinvertebrate metacommunity dynamics in the highly urbanized river networks in Shenzhen, South China显示文摘Background:Disentangling the relative roles of environmental filtering and spatial processes in structuring ecological communities is a central topic in metacommunity ecology.Metacommunity ecology in the temperate river ecosystems has been well developed,while less attention has been paid to subtropical urban river networks.Here,we examined the ecological factors and seasonal difference in structuring macroinvertebrates metacommunity assembly in the subtropical urban river networks in Shenzhen,South China.Results:Our results revealed that there was no significant distinction of macroinvertebrate community composition among seasons,with only the relative abundance of Mollusca and Odonata significantly differed in both wet and dry seasons.One possible explanation was that most macroinvertebrates are generally pollution-tolerant taxa characterized with nonseasonal life cycle.In addition,distance-based redundancy analysis and variation partitioning approach revealed that metacommunity was determined equally by the environmental and dispersal-related factors.Further,our results showed that,although a slight temporal variation of relative contribution,the identity and explanation power of ecological factors were different among seasons.Specifically,stronger environmental filtering structuring community dynamics was observed in the dry than wet seasons,which might be owing to higher environmental heterogeneity under a low water-flow condition.Moreover,we detected that the influence of spatial processes was stronger in the wet than dry seasons,indicating an obvious dispersal processes due to high connectivity among sites.Conclusion:Overall,our results revealed that environmental and spatial factors equally explained variations of macroinvertebrate metacommunity,implying the necessity of considering dispersal-related processes structuring ecological communities in river bioassessment programs.Moreover,degraded habitat conditions and water quality were the predominant factors that affected macroinvertebrate communities,indicating the significance and feasibility of improving local abiotic conditions to sustain local biodiversity.Further,our findings revealed the importance of seasonal dynamics of these urban river networks in structuring macroinvertebrate metacommunity.Thereby,our study improves the understanding of ecological processes governing macroinvertebrate metacommunity and underlines the idea that community ecology studies should go beyond the single snapshot survey in river networks. | Zhenyuan Liu Tingting Zhou Yongde Cui Zhengfei Li Weimin Wang Yushun Chen Zhicai Xie | 2021 | Ecological Processes2021，10，1： | 0 |
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