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| 1 | gt-C3N4 coordinated single atom as an efficient electrocatalyst for nitrogen reduction reaction显示文摘The electrochemical reduction of nitrogen to ammonia is a promising way to produce ammonia at mild condition.The design and preparation of an efficient catalyst with high ammonia selectivity is critical for the real applications.In this work,a series of transition metal (TM =Sc,Ti,V,Cr,Mn,Fe,Co,Ni,Cu,Zn,Y,Zr,Nb,Mo,Tc,Ru,Rh,Pd,Ag,and Cd) atoms supported by gt-C3N4 (TM/gt-C3N4) are investigated as electrocatalysts for the nitrogen reduction reaction (NRR) based on density functional calculations.It is found that Mo/gt-C3N4 with a limiting potential of-0.82 V is the best catalyst for standing-on adsorbed N2 cases.While for lying-on adsorbed N2 cases,V/gt-C3N4 with a limiting potential of-0.79 V is berer than other materials.It is believed that this work provides several promising candidates for the non-noble metal electrocatalysts for NRR at mild condition. | Lifu Zhang Wanghui Zhao Wenhua Zhang Jing Chen Zhenpeng Hu | 2019 | Nano Research2019，12，5： | 11 |
| 2 | A New Species of the Genus Rhacophorus (Anura: Rhacophoridae) from Dabie Mountains in East China显示文摘A new species of rhacophorid of the genus Rhacophorus is described from the Dabie Mountains of west Anhui,east China.The new species,Rhacophorus zhoukaiyae sp.nov.is distinguished from its congeners by a combination of the following characters: 1) the ventral surface and front-and-rear of the femur is paler yellowish and decorated with irregular grayish blotching,and without obvious spots on the dorsum of the hand and foot webbing; 2) the outer metatarsal tubercle is small; 3) outer fingers are half-webbed and outer toes two third webbed; 4) the skin on the dorsum is smooth and without compressed warts; 5) the throat,chest and belly are pure paler yellowish; 6) the dorsal part of the fingers and toes are grayish-white; 7) the iris is golden-yellow.In addition,the phylogenetic tree showed that all the individuals of R.zhoukaiyae sp.nov.clustered into one distinct clade which suggested the validity of this species.This results could also be used to the support of species delimitation.Currently,this species is known only from mid-elevation montane evergreen forest in the Dabie Mountains of west Anhui,China. | Tao PAN Yanan ZHANG Hui WANG Jun WU Xing KANG Lifu QIAN Kai LI Yu ZHANG Jinyun CHEN Dingqi RAO Jianping JIANG Baowei ZHANG | 2017 | Asian Herpetological Research2017，18，1： | 5 |
| 3 | An artificial chromosome for data storage显示文摘DNA digital storage provides an alternative for information storage with high density and long-term stability.Here,we report the de novo design and synthesis of an artificial chromosome that encodes two pictures and a video clip.The encoding paradigm utilizing the superposition of sparsified error correction codewords and pseudo-random sequences tolerates base insertions/deletions and is well suited to error-prone nanopore sequencing for data retrieval.The entire 254 kb sequence was 95.27%occupied by encoded data.The Transformation-Associated Recombination method was used in the construction of this chromosome from DNA fragments and necessary autonomous replication sequences.The stability was demonstrated by transmitting the data-carrying chromosome to the 100 th generation.This study demonstrates a data storage method using encoded artificial chromosomes via in vivo assembly for write-once and stable replication for multiple retrievals,similar to a compact disc,with potential in economically massive data distribution. | Weigang Chen Mingzhe Han Jianting Zhou Qi Ge Panpan Wang Xinchen Zhang Siyu Zhu Lifu Song Yingjin Yuan | 2021 | National Science Review2021，8，5： | 3 |
| 4 | Significant difference between sirolimus and paclitaxel nanoparticles in antiproliferation effect in normoxia and hypoxia: The basis of better selection of atherosclerosis treatment显示文摘Compared with paclitaxel,sirolimus has been more used in the treatment of vascular restenosis gradually as an anti-proliferative drug,but few basic studies have elucidated its mechanism.The anti-proliferative effects of sirolimus or paclitaxel have been demonstrated by numerous studies under normoxia,but few studies have been achieved focusing hypoxia.In this study,porcine carotid artery injury model and classical cobalt chloride hypoxia cell model were established.Sirolimus nanoparticles(SRM-NPs),paclitaxel nanoparticles(PTX-NPs)and blank nanoparticles(Blank-NPs)were prepared respectively.The effect of RPM-NPs on the degree of stenosis,proliferative index and the expression of PCNA after 28 days of porcine carotid artery injury model was evaluated.Compared with saline group and SRM groups,SRM-NPs group suppressed vascular stenosis,proliferative index and the expression of PCNA(P<0.01 and P<0.05).Endothelial cell(EC)and smooth muscle cell(SMC)were pre-treated with cobaltous chloride,followed by SRM-NPs,PTX-NPs,Blank-NPs or PBS control treating,the effects on cell proliferation,HIF-1 expression and glycolysis were detected.SRM-NPs could inhibit EC and SMC proliferation under hypoxia,while PTX-NPs couldn't(P<0.001).Significant differences between sirolimus and paclitaxel NPs in anti-proliferation effect under normoxia and hypoxia may due to the different inhibitory effects on HIF-1αexpression and glycolysis.In conclusion,these results suggest that sirolimus can inhibit the proliferation of hypoxic cells more effectively than paclitaxel.These observations may provide a basis for understanding clinical vascular stenosis therapeutic differences between rapamycin and paclitaxel. | Youlu Chen Yong Zeng Xiaowei Zhu Lifu Miao Xiaoyu Liang Jianwei Duan Huiyang Li Xinxin Tian Liyun Pang Yongxiang Wei Jing Yang | 2021 | Bioactive Materials2021，6，3： | 2 |
| 5 | Dual role of MdSND1 in the biosynthesis of lignin and in signal transduction in response to salt and osmotic stress in apple显示文摘Clarifying the stress signal transduction pathway would be helpful for understanding the abiotic stress resistance mechanism in apple(Malus×domestica Borkh.)and could assist in the development of new varieties with high stress tolerance by genetic engineering.The key NAC transcription factor SND1,which is involved in the lignin biosynthesis process in apple,was functionally analyzed.The results of the stress treatments indicated that MdSND1 could be induced by salt,mannitol and ABA.Compared with wild-type GL-3 plants,MdSND1-overexpressing apple plants with greater antioxidant capacity and lignin were more resistant to salt and simulated osmotic stress,while RNAi plants were more vulnerable.Additionally,molecular experiments confirmed that MdSND1 could regulate the biosynthesis of lignin by activating the transcription of MdMYB46/83.Moreover,genes known to be involved in the stress signal transduction pathway(MdAREB1A,MdAREB1B,MdDREB2A,MdRD29A,and MdRD22)were screened for their close correlations with the expression of MdSND1 and the response to salt and osmotic stress.Multiple verification tests further demonstrated that MdSND1 could directly bind to these gene promoters and activate their transcription.The above results revealed that MdSND1 is directly involved in the regulation of lignin biosynthesis and the signal transduction pathway involved in the response to both salt and osmotic stress in apple. | Keqin Chen Yunna Guo Mengru Song Lifu Liu Hao Xue Hongyan Dai Zhihong Zhang | 2020 | Horticulture Research2020，7，1： | 2 |
| 6 | Reduction of phonon thermal conduction in isotopic graphene nanoribbon superlattices显示文摘Graphene nanoribbons(GNR_s)recently have drawn much interest because of their novel electronic properties such as well-controlled electronic structures[1],high Seebeck coefficient[2],and intriguing electronic transport[3].For the thermoelectric energy conversion,GNR_s are thought to be rather poor candidates because of too high phonon | ZhongXiang Xie XueKun Chen Xia Yu Yong Zhang HaiBin Wang LiFu Zhang | 2017 | Science China(Physics,Mechanics & Astronomy)2017，60，10： | 2 |
| 7 | Antimicrobial effect of pressurized carbon dioxide on Listeria monocytogenes显示文摘 | Lin homu Cao Ningjun Chen Lifu | 1994 | Journal of Food Science1994，59，3： | 1 |
| 8 | Thermal Stress in Free-standing Diamond Films with Cr Interlayer Destroyed显示文摘Thermal stress in large area free-standing diamond films was remarkable during the post-deposition cooling of direct current (DC) arc plasma jet chemical vapor deposition (CVD) process.In this research,the stress release caused by delamination of Cr interlayer was of great importance to ensure the integrity of free-standing diamond film.The effects of Cr interlayer on Mo substrate,namely composite substrate,on thermal stress were investigated.Thermo-mechanical coupling analysis of the thermal stress was applied by finite element analysis (FEA) using ANSYS code.It was found that the interlayer could be destroyed first by the large thermal stress,and then the stress could be released and the probability of diamond film crack initiation would be reduced.The stress concentration at the bent edge of diamond film was also discussed.In addition,diamond films deposited on Mo substrates with and without Cr interlayer were prepared by DC arc plasma jet CVD system and experimental measurements were used to characterize these films.It was found that composite substrate could be an effective method of growing free-standing crack-free diamond films by DC arc plasma jet CVD system when there is no special requirement to the film strength. | Zheng Liu,Liangxian Chen,Chengming Li,Lifu Hei,Jianhua Song,Guangchao Chen,Weizhong Tang and Fanxiu Lv School of Materials Science and Engineering,University of Science and Technology Beijing,Beijing 100083,China | 2010 | Journal of Materials Science & Technology2010，26，11： | 1 |
| 9 | Danhong Injection Inhibits the Development of Atherosclerosis in Both Apoe?/? and Ldlr?/? Mice显示文摘 | Yuanli Chen Mengyang Liu Tao Zhao Buchang Zhao Lifu Jia Yan Zhu Boli Zhang Xiumei Gao Guangliang Li Xiaoju Li Rong Xiang Jihong Han Yajun Duan | 2014 | Journal of Cardiovascular Pharmacology2014，，5： | 1 |
| 10 | Salt stress-induced changes in soil metabolites promote cadmium transport into wheat tissues显示文摘Soil salinity is known to improve cadmium(Cd)mobility,especially in arid soils.However,the mechanisms involved in how salt stress-associated metabolic profiles participate in mediating Cd transport in the soil-plant system remain poorly understood.This study was designed to investigate the effects of salinity-induced changes in soil metabolites on Cd bioavailability.Sodium salts in different combinations according to molar ratio(NaCl:Na_(2)SO_(4)=1:1;NaCl:Na_(2)SO_(4):NaHCO_(3)=1:2:1;NaCl:Na_(2)SO_(4):NaHCO_(3):Na_(2)CO_(3)=1:9:9:1;NaCl:Na_(2)SO_(4):NaHCO_(3):Na_(2)CO_(3)=1:1:1:1)were applied to the Cd-contaminated soils,which increased soil Cd availability by 22.36%and the Cd content in wheat grains by 36.61%,compared to the control.Salt stress resulted in soil metabolic reprogramming,which might explain the decreased growth of wheat plants and increased Cd transport from the soil into wheat tissues.For example,down-regulation of starch and sucrose metabolism reduced the production of sugars,which adversely affected growth;up-regulation of fatty acid metabolism allowed wheat plants to maintain a normal intracellular environment under saline conditions;up-regulation of the tricarboxylic acid(TCA)cycle was triggered,causing an increase in organic acid synthesis and the accumulation of organic acids,which facilitated the migration of soil Cd into wheat tissues.In summary,salt stress can facilitate Cd transport into wheat tissues by the direct effect of salt-based ions and the combined effect of altered soil physicochemical properties and soil metabolic profiles in Cd-contaminated soils. | Lifu Wang Luyao Qin Xiaoyi Sun Shuwen Zhao Lei Yu Shibao Chen Meng Wang | 2023 | Journal of Environmental Sciences2023，，5： | 1 |
| 11 | D-Xylose fermentation to ethanol bySchizosaccharomyces pombe cloned with xylose isomerase gene显示文摘 | Err-Cheng Chan P. P. Ueng Lifu Chen | 1986 | Biotechnology Letters1986，，4： | 1 |
| 12 | D-Xylose fermentation to ethanol bySchizosaccharomyces pombe cloned with xylose isomerase gene显示文摘 | Err-Cheng Chan P. P. Ueng Lifu Chen | 1986 | Biotechnology Letters1986，，4： | 1 |
| 13 | Determina- tion of oxymatrine and its metabolite matrine in rat blood and dermal microdialysates by high throughput liquid chromatogra- phy/tandem mass spectrometry显示文摘 | Zheng Hong Chen GuangChun Shi LiFu | 2009 | J Pharm Biomed Anal2009，49，2： | 1 |
| 14 | Electro-oxidation of hydrazine shows marcusian electron transfer kinetics显示文摘Although hydrazine(N2 H4) oxidation in an electrochemical environment has been of great interest for years,its intrinsic electron transfer kinetics remain uncertain.We report that the phenomenological Butler-Volmer(BV) theory is not appropriate for interpreting the process of hydrazine oxidation for which an astonishingly wide range of transfer coefficients,Tafel slopes and diffusion coefficient have been previously reported.Rather Tafel analysis for voltammetry recorded at Glassy Carbon(GC)electrodes reveals a strong potential dependence of the anodic transfer coefficient,consistent with the symmetric Marcus-Hush(sMH) theory.According to the relationship β=λ+FEf^0/2λ-F/2λ E,the reorganization energy(0.35±0.07 eV) and an approximate formal potential of the rate-determining first electron transfer were successfully extracted from the voltammetric responses. | Ruiyang Miao Lifu Chen Richard G Compton | 2021 | Science China Chemistry2021，64，2： | 1 |
| 15 | Combining Explicit and Symbolic Representation in Incremental Model Checking显示文摘 | TAO Zhihong CHEN Zhenyu CHEN Zhong WANG Lifu | 2007 | Chinese Journal of Electronics2007，16，1： | 0 |
| 16 | Quality influencing factors of dispersion curves from short period dense arrays based on a convolutional neural network across the north section of the Xiaojiang fault area显示文摘The number of dispersion curves increases significantly when the scale of a short-period dense array increases.Owing to a substantial increase in data volume,it is important to quickly evaluate dispersion curve quality as well as select the available dispersion curve.Accordingly,this study quantitatively evaluated dispersion curve quality by training a convolutional neural network model for ambient noise tomography using a short-period dense array.The model can select high-quality dispersion curves that exhibit a≤10%difference between the results of manual screening and the proposed model.In addition,this study established a dispersion curve loss function by analyzing the quality of the dispersion curve and the corresponding influencing factors,thereby estimating the number of available dispersion curves for the existing observation systems.Furthermore,a Monte Carlo simulation experiment is used to illustrates the station-pair interval distance probability density function,which is independent of station number in the observational system with randomly deployed stations.The results suggested that the straight-line length should exceed 15 km to ensure that loss rate of dispersion curves remains<0.5,while maintaining the threshold ambient noise tomography accuracy within the study area. | Si Chen Rui Gao Zhanwu Lu Yao Liang Wei Cai Lifu Cao Zilong Chen Guangwen Wang | 2023 | Earthquake Science2023，36，3： | 0 |
| 17 | Preparation and Electromechanical Properties of PVDF Matrix Piezoelectric Composites Containing Highly Oriented BaTiO_3 Whiskers显示文摘The piezoelectric composites containing highly oriented BaTiO3 whiskers as active phase and PVDF as matrix have been prepared by micro-hole extrusion and orientation in carried fibers. The morphology of oriented BaTiO3 whiskers and microstructure of the composites were observed by SEM. As for its electromechanical properties, it is found that the dielectric constant, piezoelectric constant and remnant of polarization in the BaTiO3 whisker-PVDF composite are considerably higher than that in the BaTiO3 powders-PVDF composite, while the loss factors follow the opposite trend. For the BaTiO3 whisker-PVDF composite, the values of ε, d33 and Pr parallel to the whisker orientation (normal specimen) are much higher than that perpendicular to the whisker orientation (parallel specimen). The significant effects of the connective passages of active phase on electromechanical properties of the piezoelectric composites has also been investigated. | Xuetao LUO, Lifu CHEN, Xiaojun CHEN and Qianjun HUANGDepartment of Materials Science and Engineering, Xiamen University, Xiamen 361005, China | 2004 | Journal of Materials Science & Technology2004，20，4： | 0 |
| 18 | DanHong Injection inhibits the development of primary abdominal aortic aneurysms in apoE knockout mice显示文摘Clinical observations indicate that DanHong Injection(DHI)can increase blood flow and reduce various syndromes in patients with cardiovascular disease.However,it still needs to define the function of DHI and the involved mechanisms in details,such as the protective effect on the development of primary abdominal aortic aneurysms(AAAs).In this study,we determined whether DHI is able to inhibit AAA in apoE knockout(apoE-/-)mice.Thirty apoE-/-male mice on high-fat diet(0.5%cholesterol,21%fat)were randomly divided into two groups and received i.p.injection of saline(100 lL/day)and DHI(100 lL/day),respectively,for 16 weeks.At the end of experiment,we determined the development of atherosclerosis in en face aorta and aneurysms,pathological morphology of arterial wall,and serum lipid levels.We also determined the expression of monocyte chemoattractant protein-1(MCP-1),MMP-2,and MMP-9mRNA in aortic wall using real-time RT-PCR.Our results indicated that high-fat diet induced the development of AAAs in apoE-/-mice,but the induction was totally blocked by DHI(P\0.01).The result of staining of abdominal aortic cross sections showed that DHI maintained the collagen content in arterial wall,thereby preventing the animals from the development of AAA.Although DHI had little effect on serum total-and LDLcholesterol levels,it reduced the expression of MCP-1,MMP-2,and MMP-9 mRNA in aortic wall(P\0.01).Taken together,our study suggests that DHI can inhibit the high-fat diet-induced AAA formation.The inhibitory effects may be related to the maintenance of the collagen content and inhibition of expression of AAA-related genes.Our study may suggest a new application of DHI in clinics. | Mengyang Liu Yuanli Chen Xiaoxiao Yang Ling Zhang Tao Zhao Buchang Zhao Lifu Jia Yan Zhu Xiumei Gao Boli Zhang Xiaoju Li Rong Xiang Jihong Han Yajun Duan | 2014 | Chinese Science Bulletin2014，59，13： | 0 |
| 19 | Biological basis of “depression with liver-qi stagnation and spleen deficiency syndrome”: A digital gene expression profiling study显示文摘Objective:To investigate the biological basis of“depression with liver-qi stagnation and spleen deficiency syndrome”.Methods:A digital gene expression profiling method was conducted to explore global changes in the mRNA transcriptome in a rat model of depression with liver-qi stagnation and spleen deficiency syndrome.Real-time quantitative polymerase chain reaction(q-PCR)was performed to verify the five genes most interest based on the Kyoto Encyclopedia of Genes and Genome(KEGG)analysis.Sini San,which disperses stagnated liver qi and strengthens the spleen,was administered to the model rats to observe whether it could reverse these genetic changes in the liver.Results:Forty-six differentially expressed genes were identified.Three of the five genes of most interestdHnf4a,Hnf4g and Cyp1a1dbased on KEGG analysis,were confirmed by realtime q-PCR.Sini San reduced the gene expression changes of Hnf4a,Hnf4g and Cyp1a1 in the rat model.Conclusions:Hnf4a,Hnf4g and Cyp1a1 are involved in“depression with liver-qi stagnation and spleen deficiency syndrome”.These findings indicate that depressed rats with liver-qi stagnation and spleen deficiency syndrome are at risk of liver diseases.Furthermore,our results will inform exploration of the etiology of depression and help in the development of effective therapeutic strategies. | Junling Li Lifu Bi Kai Xia Kuo Gao Jianxin Chen Shuzhen Guo Tian Wang Xueling Ma Weiming Wang Huihui Zhao Yubo Li Wei Wang | 2015 | Journal of Traditional Chinese Medical Sciences2015，2，3： | 0 |
| 20 | Achieving improved stability and minimal non-radiative recombination loss for over 18%binary organic photovoltaics via versatile interfacial regulation strategy显示文摘Interfacial regulation,serving multiple roles,is critical for the fabrication of stable and efficient organic photovoltaics(OPVs).Herein,a multifunctional cathode interlayer PDINO(15 nm)is prepared by regulating film thickness,which is inserted between active components and stable silver electrode to align work function,and maintain good interfacial contact and device stability.The thick film can help to reduce interfacial surface defects,keep stable surface morphology,and block the silver diffusion into the active layer.Consequently,the optimal PM6:Y6 device records an impressive power conversion efficiency(PCE)of 17.48%with minimized non-radiative recombination loss of 0.239 V.More importantly,the unencapsulated device maintains 91%of the original PCE after aging for over 60 days at 25℃ and 10%relative humidity in dark conditions.Meanwhile,the PM6:eC9 device achieves a remarkable PCE of 18.22%with the enhancement of open-circuit voltage(V_(oc)).Furthermore,the 1 cm^(2) device-based PDINO(15 nm)/Ag shows a high PCE of 15.2%while only 12.6%for PDINO(9 nm)/Al,indicating the good compatibility of PDINO(15 nm)interlayer with the R2R coating processes used in large-area OPVs fabrication.This work highlights the promise of interfacial regulation to simultaneously stabilize and enhance the efficiency of organic photovoltaics. | Lifu Zhang Houdong Mao Liqiang Huang Lei Hu Xinkang Wang Licheng Tan Yiwang Chen | 2022 | Science China Chemistry2022，65，8： | 0 |
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