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| 1 | Low-dose real-time X-ray imaging with nontoxic double perovskite scintillators显示文摘X-rays are widely used in probing inside information nondestructively,enabling broad applications in the medical radiography and electronic industries.X-ray imaging based on emerging lead halide perovskite scintillators has received extensive attention recently.However,the strong self-absorption,relatively low light yield and lead toxicity of these perovskites restrict their practical applications.Here,we report a series of nontoxic double-perovskite scintillators of Cs_(2)Ag_(0.6)Na_(0.4)In_(1-y)Bi_(y)Cl_(6).By controlling the content of the heavy atom Bi^(3+),the X-ray absorption coefficient,radiative emission efficiency,light yield and light decay were manipulated to maximise the scintillator performance.A light yield of up to 39,000±7000 photons/MeV for Cs_(2)Ag_(0.6)Na_(0.4)In_(0.85)Bi_(0.15)Cl_(6) was obtained,which is much higher than that for the previously reported lead halide perovskite colloidal CsPbBr_(3)(21,000 photons/MeV).The large Stokes shift between the radioluminescence(RL)and absorption spectra benefiting from self-trapped excitons(STEs)led to a negligible selfabsorption effect.Given the high light output and fast light decay of this scintillator,static X-ray imaging was attained under an extremely low dose of ∼1μGy_(air),and dynamic X-ray imaging of finger bending without a ghosting effect was demonstrated under a low-dose rate of 47.2μGy_(air) s^(−1).After thermal treatment at 85℃ for 50 h followed by X-ray irradiation for 50 h in ambient air,the scintillator performance in terms of the RL intensity and X-ray image quality remained almost unchanged.Our results shed light on exploring highly competitive scintillators beyond the scope of lead halide perovskites,not only for avoiding toxicity but also for better performance. | Wenjuan Zhu Wenbo Ma Yirong Su Zeng Chen Xinya Chen Yaoguang Ma Lizhong Bai Wenge Xiao Tianyu Liu Haiming Zhu Xiaofeng Liu Huafeng Liu Xu Liu Yang(Michael)Yang | 2020 | Light(Science & Applications)2020，9，1： | 9 |
| 2 | Perovskite semiconductors for direct X-ray detection and imaging显示文摘Halide perovskites have emerged as the next generation of optoelectronic materials and their remarkable performances have been attractive in the fields of solar cells,light-emitting diodes,photodetectors,etc.In addition,halide perovskites have been reported as an attractive new class of X-ray direct detecting materials recently,owning to the strong X-ray stopping capacity,excellent carrier transport,high sensitivity,and cost-effective manufacturing.Meanwhile,perovskite based direct Xray imagers have been successfully demonstrated as well.In this review article,we firstly introduced some fundamental principles of direct X-ray detection and imaging,and summarized the advances of perovskite materials for these purposes and finally put forward some needful and feasible directions. | Yirong Su Wenbo Ma Yang(Michael)Yang | 2020 | Journal of Semiconductors2020，41，5： | 6 |
| 3 | Characterizing noise correlation and enhancing coherence via qubit motion显示文摘The identification of spacial noise correlation is of critical importance in developing error-corrected quantum devices,but it has barely been studied so far.In this work,we utilize an effective method called qubit motion,to efficiently determine the noise correlations between any pair of qubits in a 7-qubit superconducting quantum system.The noise correlations between the same pairs of qubits are also investigated when the qubits are at distinct operating frequencies.What’s more,in this multi-qubit system with the presence of noise correlations,we demonstrate the enhancing effect of qubit motion on the coherence of logic qubits,and we propose a Motion-CPMG operation sequence to more efficiently protect the logic state from decoherence,which is experimentally demonstrated to extend the coherence time of logic qubits by nearly one order of magnitude. | Jiaxiu Han Zhiyuan Li Jingning Zhang Huikai Xu Kehuan Linghu Yongchao Li Chengyao Li Mo Chen Zhen Yang Junhua Wang Teng Ma Guangming Xue Yirong Jin Haifeng Yu | 2021 | Fundamental Research2021，1，1： | 1 |
| 4 | Design,synthesis,and evaluation of PD-L1 degraders to enhance T cell killing activity against melanoma显示文摘Inhibitor targeting immune checkpoint is a promising new anticancer therapy.Blocking the interaction between PD-1 and PD-L1 can reverse the immunosuppression state and improve the lethality of immune cells to tumor cells.Here,we report PROTAC-based PD-L1 degraders to enhance T cell killing activity against melanoma.Four series of PD-L1 degraders were designed and synthesized to VHL,CRBN,MDM2 or c IAP E3 ligase system,in which CRBN-ligand-based compound BMS-37-C3 was identified as the most active PROTAC molecule.BMS-37-C3 also significantly enhanced the killing ability of T cells in a co-culture model of A375 and T cells.Furthermore,western blot data and flow cytometry demonstrated that BMS-37-C3 could reduce the protein levels of PD-L1 in dose and time dependent manner,which may provide a new therapeutic method for tumor immunotherapy. | Yang Liu Mengzhu Zheng Zhilu Ma Yirong Zhou Junfeng Huo Wenbo Zhang Yu Liu Yuanyuan Guo Xuechen Zhou Hua Li Lixia Chen | 2023 | Chinese Chemical Letters2023，34，5： | 0 |
| 5 | Statement on Establishment of Public Health Protection Guideline for Cold Spells—China显示文摘Cold spells are extreme weather events characterized by the invasion of cold air from high latitudes into the middle and low latitudes,resulting in significant cooling.Cold spells have various adverse health effects,including epidermal damage,respiratory tract spasms,respiratory immune abnormalities,acute cardiopulmonary diseases,and exacerbation of urinary and endocrine disorders.In response to the frequent cold spells in recent years. | Tiantian Li Qinghua Sun Chen Chen Qing Wang Jie Ban Runmei Ma Yi Zhang Lijun Pan Yuanyuan Liu Qiutong Li Leyao Chang Hanshuo Zhang Yirong Liu Miaoyou Niu Xiangxiang Wei Lin Wang | 2024 | China CDC weekly2024，6，5： | 0 |
| 6 | Transition metal embedded in nonmetal-doped T-carbon [110]: A superior synergistic trifunctional electrocatalyst for HER, OER and ORR显示文摘The design of efficient and low-cost multifunctional electrocatalysts for hydrogen evolution reaction(HER), oxygen evolution reaction(OER) and oxygen reduction reaction(ORR) is critical for the development of clean energy. Two-dimensional(2D) carbon-based nano-materials are becoming more and more popular in heterogeneous catalysis due to their cost-effective and multi-scale tunability as single-atom catalysis(SACs) substrates. In this paper, by using first-principles calculation, we designed and demonstrated a novel macropore T-carbon [110](TC) monolayer as 2D electrocatalyst substrate for HER/OER/ORR, and the synergistic modification of the transition metal and nonmetal atoms(TM-X) were investigated to enhance the multifunctional electrocatalytic performance. We screened out the Co embedded in N-doped TC(Co3@N-TC) from 30 TM@X-TC monolayers as a trifunctional electrocatalysts, which exhibits superior performance for HER/ORR/OER on both thermodynamic and kinetic scales, and with excellent thermal and electrochemical stability. Then, the TC monolayer is naturally macropore with a diameter of 5.36 A and exhibits excellent adsorption capacity for the intermediates and products of the redox reactions. Moreover, we revealed the origin of the electrocatalytic activity using the crystal orbital Hamilton population(COHP) and the molecular orbitals(MOs). The d orbital of Co3@N-TC is significantly hybridized with the p orbital of the intermediates, so that the lone electrons initially occupied in the antibonding state pair up and occupy the downward bonding state, allowing *OH to be appropriately adsorbed onto the TC monolayer. This work not only demonstrates that the TM@X-TC monolayer is a superior synergistic trifunctional electrocatalyst, but also reveals a macropore monolayer material with potential applications in electrocatalysis. | Zhengqin Zhao Jinbo Hao Baonan Jia Xinhui Zhang Ge Wu Chunling Zhang Long Li Shuli Gao Yirong Ma Yuanzi Li Pengfei Lu | 2023 | Journal of Energy Chemistry2023，，8： | 0 |
| 7 | Solution-processed halide perovskite microcavity exciton-polariton light-emitting diodes working at room temperature显示文摘Exciton-polaritons offer the potential to achieve electrically pumped perovskite polariton lasers with much lower current thresholds than conventional photonic lasers. While optically pumped exciton-polaritons have been widely studied in halide perovskites, electrically-pumped polaritons remain limited. In this study, we demonstrate the use of a solution-processing strategy to develop halide perovskite polariton light-emitting diodes(LEDs) that operate at room temperature. The strong coupling of excitons and cavity photons is confirmed through the dispersion relation from angle-resolved reflectivity, with a Rabi splitting energy of 64 meV. Our devices exhibit angle-resolved electroluminescence following the low polariton branch and achieve external quantum efficiencies of 1.7%, 3.85%, and 3.7% for detunings of 1.1,-77, and-128 meV, respectively. We also explore devices with higher efficiency of 5.37% and a narrower spectral bandwidth of 6.5 nm through the optimization of a top emitting electrode. Our work demonstrates, to our knowledge, the first room-temperature perovskite polariton LED with a typical vertical geometry and represents a significant step towards realizing electrically pumped perovskite polariton lasers. | TIANYU LIU PENG RAN YIRONG SU ZENG CHEN RENCHEN LAI WEIDONG SHEN YAOGUANG MA HAIMING ZHU YANG(MICHAEL)YANG | 2023 | Photonics Research2023，11，10： | 0 |
| 8 | Reaching for the Stars显示文摘I paid great attention to the Alibaba program that nurtures entrepreneurs.We must conduct dialogue with African governments,so that they support young entrepreneurs and cultivate e-commerce systems.'These are the words of Dr.Mukhissa Kituyi,secretary general of the United Nations Conference on Trade and | LIU ZHUORAN NI YIRONG MA LI | 2018 | China Today2018，67，9： | 0 |
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