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| 1 | Recent advances in bifunctional catalysts for zinc-air batteries:Synthesis and potential mechanisms显示文摘Zinc-air batteries(ZABs) are considered promising candidates for next-generation clean and sustainable energy storage devices because of their low cost, safety, environment-friendliness, and high specific energy density. However, owing to its poor chargedischarge capacity and low efficiency, its practical application remains challenging. The main obstacles are the intrinsic slow reaction kinetics on the air cathode, including the oxygen reduction reaction(ORR) during discharging and oxygen evolution reaction(OER) during recharging. Therefore, a reasonable design of bifunctional ORR/OER electrocatalysts with high activity and stability is the key to the development of ZABs. In this review, the recent advances in bifunctional ORR/OER electrocatalysts as air cathodes in ZABs are discussed from three perspectives: metal-organic framework-based catalysts, metal-free carbon catalysts, and metal-based catalysts. In particular, the synthesis, electrocatalytic activity, and potential mechanism of bifunctional catalysts in ZABs are discussed. In recent years, research on bifunctional catalysts has intensified, and the performance of these catalysts has significantly improved. However, most of the experimental products have complex preparation processes and high costs;therefore, the industrialization of these experimental products remains difficult. This review offers prospects for the optimal design of high-activity rechargeable ZAB bifunctional air cathodes. | ZHAO LinWei GU TengTeng LIANG ZiWei LIU Jun | 2022 | Science China(Technological Sciences)2022，65，10： | 3 |
| 2 | Mineralogical and compositional characteristics of Late Permian coals from an area of high lung cancer rate in Xuan Wei, Yunnan, China: Occurrence and origin of quartz and chamosite显示文摘 | Shifeng Dai Linwei Tian Chen-Lin Chou Yiping Zhou Mingquan Zhang Lei Zhao Jumin Wang Zong Yang Hongzhi Cao Deyi Ren | 2008 | International Journal of Coal Geology2008，，4： | 1 |
| 3 | Regional Variations in Trabecular Morphological Features of Femoral Head of Patients with Proximal Femoral Fractures显示文摘 | Linwei Lv Guangwei Meng He Gong Dong Zhu Jiazi Gao Meisheng Zhao | 2015 | Journal of Bionic Engineering2015，12，2： | 1 |
| 4 | An improved buck PFC converter with high power factor 显示文摘 | XIE Xiagao ZHAO Chen ZHENG Linwei | 2012 | IEEE Trans Power Elec2012，28，22： | 1 |
| 5 | Global DEMs vary from one to another:an evaluation of newly released Copernicus,NASA and AW3D30 DEM on selected terrains of China using ICESat-2 altimetry data显示文摘A good understanding of the quality of digital elevation model(DEM)is a perquisite for various applications.This study investigates the accuracy of three most recently released 1-arcsec global DEMs(GDEMs,Copernicus,NASA and AW3D30)in five selected terrains of China,using more than 240,000 high-quality ICESat-2(Ice,Cloud and land Elevation Satellite)ALT08 points.The results indicate the three GDEMs have similar overall vertical accuracy,with RMSE of 6.73(Copernicus),6.59(NASA)and 6.63 m(AW3D30).While the accuracy varies considerably over study areas and among GDEMs.The results show a clear correlation between the accuracy and terrain slopes,and some relationship between the accuracy and land covers.Our analysis reveals the land cover exerts a greater impact on the accuracy than that of the terrain slope for the study area.Visual inspections of terrain representation indicate Copernicus DEM exhibits the greatest detail of terrain,followed by AW3D30,and then by NASADEM.This study has demonstrated that ICESat-2 altimetry offers an important tool for DEM assessment.The findings provide a timely and comprehensive understanding of the quality of newly released GDEMs,which are informative for the selection of suitable DEMs,and for the improvement of GDEM in future studies. | Hui Li Jiayang Zhao Bingqi Yan Linwei Yue Lunche Wang | 2022 | International Journal of Digital Earth2022，15，1： | 1 |
| 6 | Engineering in-plane silicon nanowire springs for highly stretchable electronics显示文摘Crystalline silicon(c-Si) is unambiguously the most important semiconductor that underpins the development of modern microelectronics and optoelectronics, though the rigid and brittle nature of bulk c-Si makes it difficult to implement directly for stretchable applications. Fortunately, the one-dimensional(1 D) geometry, or the line-shape, of Si nanowire(SiNW) can be engineered into elastic springs, which indicates an exciting opportunity to fabricate highly stretchable 1 D c-Si channels. The implementation of such line-shape-engineering strategy demands both a tiny diameter of the SiNWs, in order to accommodate the strains under large stretching, and a precise growth location, orientation and path control to facilitate device integration. In this review, we will first introduce the recent progresses of an in-plane self-assembly growth of SiNW springs, via a new in-plane solid-liquidsolid(IPSLS) mechanism, where mono-like but elastic SiNW springs are produced by surface-running metal droplets that absorb amorphous Si thin film as precursor. Then, the critical growth control and engineering parameters, the mechanical properties of the SiNW springs and the prospects of developing c-Si based stretchable electronics, will be addressed. This efficient line-shape-engineering strategy of SiNW springs, accomplished via a low temperature batch-manufacturing, holds a strong promise to extend the legend of modern Si technology into the emerging stretchable electronic applications, where the high carrier mobility, excellent stability and established doping and passivation controls of c-Si can be well inherited. | Zhaoguo Xue Taige Dong Zhimin Zhu Yaolong Zhao Ying Sun Linwei Yu | 2018 | Journal of Semiconductors2018，39，1： | 1 |
| 7 | Short-term Effects of Nitrogen Deposition on Soil Enzyme Activities in Tibet Grasslands显示文摘[Objective] The paper was to study the effects of nitrogen deposition on enzyme activity in different layers of soil. [Method] With grassland located in Zhuqudeng Village, Bujiu Township, Linzhi City, the Tibet Autonomous Region, as the object, nitrogen deposition was simulated from July 2014 to August 2015. Four N addition treatments were established: control(0 kg·hm2/a), low N(LN, 25 kg·hm2/a), medium N(MN, 50 kg·hm2/a) and High N(HN, 150 kg·hm2/a), aiming at measuring enzyme activity(invertase, catalase, urease, amylase, cellulase, polyphenol oxidase and β-glucosidase) in different layers of grassland soil(0-20 cm and 20-40 cm). [Result](1) Different levels of simulated nitrogen deposition had significant impact on invertase and β-glucosidase at the soil depth of 0-20 cm(P<0.05), but no significant impact on catalase, urease, amylase, cellulase and polyphenol oxidase(P>0.05); invertase, polyphenol oxidase and β-glucosidase had significant response to nitrogen deposition at the soil depth of 20-40 cm(P<0.05), while catalase, urease, amylase and cellulose had no significant response( P>0.05).(2) The activities of invertase and polyphenol oxidase were enhanced at the soil depth of 0-20 cm, and that of β-glucosidase was inhibited.(3) With the deepening of nitrogen deposition, the ac-tivities of invertase and cellulose were enhanced at the soil depth of 20-40 cm; the activity of polyphenol oxidase was reduced in LN treatment, but increased in HN treatment; the activity of β-glucosidase was increased in LN treatment, but decreased in MN treatment.(4) With the deepening of soil layers, invertase and polyphenol oxidase responded similarly to simulated nitrogen deposition. [Conclusion] The results provide certain scientific basis and fundamental data for better understanding and evaluating the effects of nitrogen deposition on enzyme activity in grassland soil. | Han Yanying Gao Yi Ye Yanhui Liu Yunlong Da Buqiong Zhao Yalei Li Linwei | 2018 | Animal Husbandry and Feed Science2018，10，3： | 0 |
| 8 | Radiation-induced one-pot synthesis of grafted covalent organic frameworks显示文摘Post-synthetic functionalization of covalent organic frameworks(COFs)is an alternative way to enhance and broaden their properties and potential applications.However,the chemical functionalization of COFs is a great challenge because traditional procedures are often time-and energy-consuming,while the crystallinity of COFs can be damaged under harsh conditions.Here we report the in-situ introduction of functional graft chains onto the skeleton of COFs during the synthesis process through the combination of radiation-induced synthesis and graft polymerization techniques under ^(60)Co gamma-ray radiation.The synthesis and functionalization of COFs are simultaneously accomplished in a chemical system under ambient conditions yielding a large number of different functionalized COFs.The obtained carboxyl-functionalized COFs exhibit excellent radioactive uranium removal capabilities from aqueous solution with fast uptake dynamics,high adsorption capacity,and excellent selectivity over other competing metal ions. | Mingxing Zhang Mengjia Yuan Xiaofang Zhao Junchang Chen Linwei He Qianhong Gao Jiangtao Hu Guozhong Wu Zhifang Chai Shuao Wang | 2023 | Science China Chemistry2023，66，6： | 0 |
| 9 | Synergy of first-and second-sphere interactions in a covalent organic framework boosts highly selective platinum uptake显示文摘Platinum recovery from waste electrical and electronic equipment(WEEE) in highly acidic solutions is significant to the electronics industry and environmental remediation. However, the lack of ingenious design and synergetic coordination gives rise to unsatisfied PtCl_(4)^(2-)extraction capacities and selectivities in most previously reported adsorbents(e.g., polymeric and inorganic materials). Herein, we proposed a synergistic strategy that realizes highly selective PtCl_(4)^(2-)uptake through first-and second-sphere coordinations. The proof-of-concept imine-linked covalent organic framework(SCU-COF-3) was found to chelate Pt Cl42-via the direct N…Pt coordination and the synergistically interlaminar N–H…Cl hydrogen bonds, which was disclosed by the comprehensive analysis of extended X-ray adsorption fine structure(EXAFS) characterizations and density functional theory(DFT) calculations. The unique adsorption mechanism imparts a superior adsorption capacity(168.4 mg g-1)and extraordinary Pt(II) selectivity to SCU-COF-3 under static conditions. In addition, SCU-COF-3 exhibits an upgraded distribution coefficient of 1.62 × 10^(5)mL· g^(-1), one order of magnitude higher than those of reported natural adsorbents. Specifically, SCU-COF-3 can extract PtCl_(4)^(2- )quantitatively from a simulated acidic waste solution coexisting with other 12 competitive ions, suggesting its promising application in practical scenarios. | Linwei He Baoyu Li Zhonglin Ma Lixi Chen Shicheng Gong Mingxing Zhang Yaoyao Bai Qi Guo Fuqi Wu Fuqiang Zhao Jie Li Duo Zhang Daopeng Sheng Xing Dai Long Chen Jie Shu Zhifang Chai Shuao Wang | 2023 | Science China Chemistry2023，66，3： | 0 |
| 10 | Temporal trend of mortality from major cancers in Xuanwei, China显示文摘尽管很多研究在 Xuanwei 县检验了肺癌症的病原学,中国,在这个县的癌症的另外的类型没系统地被报导。这研究试图从三死亡调查(19731975, 19901992,和 20042005 ) 用数据在 Xuanwei 县调查八主要癌症的时间的趋势。在 1990 的中国人口被用作一张标准人口计算 agestandardized 死亡率。肺,肝,胸,大脑,食管,白血病,直肠,和胃的癌症以死亡率在这个县作为领先的癌症被识别。在三次经期期间,肺癌症作为癌症的最普通的类型留下了。为癌症的所有另外的类型的死亡率是比国家一般水准的那些低的,但是一个增加的趋势为所有癌症被观察,特别地从 19901992 ~ 20042005。时间的趋势能被变化部分在风险因素解释,但是它可能也由于在癌症诊断的改进并且屏蔽。进一步流行病学的研究被保证系统地在 Xuanwei 县为主要癌症的时间的趋势检验内在的原因。 | Hualiang Lin Bofu Ning Jihua Li Guangqiang Zhao Yunchao Huang Linwei Tian | 2015 | Frontiers of Medicine2015，9，4： | 0 |
| 11 | Land use and cover change and influencing factor analysis in the Shiyang River Basin,China显示文摘Land use and cover change(LUCC)is the most direct manifestation of the interaction between anthropological activities and the natural environment on Earth's surface,with significant impacts on the environment and social economy.Rapid economic development and climate change have resulted in significant changes in land use and cover.The Shiyang River Basin,located in the eastern part of the Hexi Corridor in China,has undergone significant climate change and LUCC over the past few decades.In this study,we used the random forest classification to obtain the land use and cover datasets of the Shiyang River Basin in 1991,1995,2000,2005,2010,2015,and 2020 based on Landsat images.We validated the land use and cover data in 2015 from the random forest classification results(this study),the high-resolution dataset of annual global land cover from 2000 to 2015(AGLC-2000-2015),the global 30 m land cover classification with a fine classification system(GLC_FCS30),and the first Landsat-derived annual China Land Cover Dataset(CLCD)against ground-truth classification results to evaluate the accuracy of the classification results in this study.Furthermore,we explored and compared the spatiotemporal patterns of LUCC in the upper,middle,and lower reaches of the Shiyang River Basin over the past 30 years,and employed the random forest importance ranking method to analyze the influencing factors of LUCC based on natural(evapotranspiration,precipitation,temperature,and surface soil moisture)and anthropogenic(nighttime light,gross domestic product(GDP),and population)factors.The results indicated that the random forest classification results for land use and cover in the Shiyang River Basin in 2015 outperformed the AGLC-2000-2015,GLC_FCS30,and CLCD datasets in both overall and partial validations.Moreover,the classification results in this study exhibited a high level of agreement with the ground truth features.From 1991 to 2020,the area of bare land exhibited a decreasing trend,with changes primarily occurring in the middle and lower reaches of the basin.The area of grassland initially decreased and then increased,with changes occurring mainly in the upper and middle reaches of the basin.In contrast,the area of cropland initially increased and then decreased,with changes occurring in the middle and lower reaches.The LUCC was influenced by both natural and anthropogenic factors.Climatic factors and population contributed significantly to LUCC,and the importance values of evapotranspiration,precipitation,temperature,and population were 22.12%,32.41%,21.89%,and 19.65%,respectively.Moreover,policy interventions also played an important role.Land use and cover in the Shiyang River Basin exhibited fluctuating changes over the past 30 years,with the ecological environment improving in the last 10 years.This suggests that governance efforts in the study area have had some effects,and the government can continue to move in this direction in the future.The findings can provide crucial insights for related research and regional sustainable development in the Shiyang River Basin and other similar arid and semi-arid areas. | ZHAO Yaxuan CAO Bo SHA Linwei CHENG Jinquan ZHAO Xuanru GUAN Weijin PAN Baotian | 2024 | Journal of Arid Land2024，16，2： | 0 |
| 12 | The Effect of Nitrogen Deposition on Soil Enzyme Activity in the Forest Grassland Landscape Boundary of Tibet显示文摘The simulated nitrogen deposition [control check(CK), 0 kg·hm^2/a; low nitrogen(LN),25 kg·hm^2/a; medium nitrogen(MN), 50 kg·hm^2/a; high nitrogen(HN), 150 kg·hm^2/a] was performed from July 2014 to August 2015 in the forest-grassland boundary in Zhuqudeng Village, Bujiu Township,Linzhi City, Tibet Autonomous Region to analyze the activity of enzymes(invertase, catalase, urease,amylase, cellulase, polyphenol oxidase, and β-glucosidase) in soil layers of 0-20 cm and 20-40 cm and explore the effect of different levels of nitrogen deposition on enzyme activity different layers of soil.The results showed that: ① different levels of simulated nitrogen deposition had remarkable effects on sucrase, amylase, cellulase, polyphenol oxidase and β-glucosidase in the soil layer of 0-20 cm(p < 0.05) and unremarkable effects on catalase and urease(p > 0.05); in the soil layer of 20-40 cm, the response made by sucrase, catalase, urease, amylase, cellulase, polyphenol oxidase and β-glucosidase to nitrogen deposition reached a significant level(p < 0.05). ② In the soil layer of 0-20 cm, the activity of urease and poyphenol oxidase reduced under LN treatment and enhanced under HN treatment, and the activity of invertase,catalase, amylase, cellulose, and β-glucosidase was inhibited by nitrogen deposition. ③ In the soil layer of20-40 cm, the activity of polyphenol oxidase and β-glucosidase reduced under under LN treatment and enhanced under HN treatment, and the activity of invertase, catalase, urease, amylase, and cellulase was inhibited by nitrogen deposition. ④ With the deepening of the boundary soil layer(from 0-20 cm to20-40 cm), urease and β-glucosidase made different responses to the different levels of nitrogen deposition,while invertase, catalase, amylase, cellulose, and polyphenol oxidase showed the same response to nitrogen deposition. | HAN Yanying LIU Yunlong YE Yanhui DA Buqiong GAO Yi ZHAO Yalei LI Linwei LIU Shuanghao | 2018 | Journal of Landscape Research2018，10，4： | 0 |
| 13 | Kidney-Qi deficiency diagnosed by Deng's diagnosis standard was not correlated with aging based on clinical observation of 90 participants显示文摘OBJECTIVE: To verify the Traditional Chinese Medicine(TCM) theory that kidney-Qi deficiency(KQD)is considered to be the main cause of aging using cross-sectional study.METHODS: Demographic and lifestyle characteristics of 90 healthy participants were collected with a self-administered questionnaire. KQD syndrome was diagnosed according to Deng's diagnosis standard. Creatinine-adjusted urinary 8-hydroxy-2'-deoxyguanosine(8-OH-dG) and 8-isomeric-prostaglandin2α(8-iso-PGF2α), salivary advanced oxidation protein products(AOPPs), malondialdehyde(MDA) and dehydroepiandrosterone-sulfate(DHEA-S) were selected as aging markers and measured using enzyme-linked immunosorbent assay.RESULTS: No significant differences were observed in participant characteristics between the KQD group and non-KQD(NKQD) group(P > 0.05). Levels of 8-OH-dG, 8-iso-PGF2α, AOPPs, and MDA increased with age, except for a slight decrease in8-OH-dG in the older group. The increase in8-iso-PGF2α was significant(P < 0.05). DHEA-S significantly decreased with increasing age(P < 0.01).8-OH-dG levels were higher in the KQD group compared with the NKQD group. Levels of urinary8-iso-PGF2α, salivary AOPPs, and MDA in the KQD group were lower than in the NKQD group. Salivary DHEA-S was higher in the KQD group compared with the NKQD group. However, differences between KQD group and NKQD group were not significant.CONCLUSION: The current results suggested that KQD syndrome, as diagnosed by Deng's standard,does not underlie the aging phenotype. | Zhao Zhengxiao Liu Lumei Tang Zihui Mohammadtursun Nabijan Lu Linwei Li Mihui Lü Yibao Mo Shuming Ma Wenjuan Wang Meng Wei Ying Gong Weiyi Dong Jingcheng | 2019 | Journal of Traditional Chinese Medicine2019，39，2： | 0 |
| 14 | Graph attention network for global search of atomic clusters:A case study of Ag_(n)(n=14-26)clusters显示文摘Due to coexistence of huge number of structural isomers,global search for the ground-state structures of atomic clusters is a challenging issue.The difficulty also originates from the computational cost of ab initio methods for describing the potential energy surface.Recently,machine learning techniques have been widely utilized to accelerate materials discovery and molecular simulation.Compared to the commonly used artificial neural network,graph network is naturally suitable for clusters with flexible geometric environment of each atom.Herein we develop a cluster graph attention network(CGANet)by aggregating information of neighboring vertices and edges using attention mechanism,which can precisely predict the binding energy and force of silver clusters with root mean square error of 5.4 meV/atom and mean absolute error of 42.3 meV/Å,respectively.As a proof-of-concept,we have performed global optimization of mediumsized Agn clusters(n=14–26)by combining CGANet and genetic algorithm.The reported ground-state structures for n=14–21,have been successfully reproduced,while entirely new lowest-energy structures are obtained for n=22–26.In addition to the description of potential energy surface,the CGANet is also applied to predict the electronic properties of clusters,such as HOMO energy and HOMO-LUMO gap.With accuracy comparable to ab initio methods and acceleration by at least two orders of magnitude,CGANet holds great promise in global search of lowest-energy structures of large clusters and inverse design of functional clusters. | Linwei Sai Li Fu Qiuying Du Jijun Zhao | 2023 | Frontiers of physics2023，18，1： | 0 |
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