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| 1 | The Notch signaling pathway in retinal dysplasia and retina vascular homeostasis显示文摘The retina is one of the most essential elements of vision pathway in vertebrate. The dysplasia of retina cause congenital blindness or vision disability in individuals, and the misbalance in adult retinal vascular homeostasis leads to neovascularization-associated diseases in adults, such as diabetic retinopathy or age-related macular degeneration. Many developmental signaling pathways are involved in the process of retinal development and vascular homeostasis. Among them, Notch signaling pathway has long been studied, and Notch signaling-interfered mouse models show both neural retina dysplasia and vascular abnormality. In this review, we discuss the roles of Notch signaling in the maintenance of retinal progenitor cells, specification of retinal neurons and glial cells, and the sustaining of retina vascular homeostasis, especially from the aspects of conditional knockout mouse models. The potential of Notch signal manipulation may provide a powerful cell fate- and neovascularization-controlling tool that could have important applications in treatment of retinal diseases. | Minhua Zheng Zifeng Zhang Xingcheng Zhao Yuqiang Ding Hua Han | 2010 | Journal of Genetics and Genomics2010，37，9： | 13 |
| 2 | Oncogenic AURKA-enhanced N6-methyladenosine modification increases DROSHA mRNA stability to transactivate STC1 in breast cancer stem-like cells显示文摘RNase III DROSHA is upregulated in multiple cancers and contributes to tumor progression by hitherto unclear mechanisms.Here,we demonstrate that DROSHA interacts withβ-Catenin to transactivate STC1 in an RNA cleavage-independent manner,contributing to breast cancer stem-like cell(BCSC)properties.DROSHA mRNA stability is enhanced by N6-methyladenosine(m^(6)A)modification which is activated by AURKA in BCSCs.AURKA stabilizes METTL14 by inhibiting its ubiquitylation and degradation to promote DROSHA mRNA methylation.Moreover,binding of AURKA to DROSHA transcript further strengthens the binding of the m^(6)A reader IGF2BP2 to stabilize m^(6)A-modified DROSHA.In addition,wild-type DROSHA,but not an m^(6)A methylation-deficient mutant,enhances BCSC stemness maintenance,while inhibition of DROSHA m^(6)A modification attenuates BCSC traits.Our study unveils the AURKA-induced oncogenic m^(6)A modification as a key regulator of DROSHA in breast cancer and identifies a novel DROSHA transcriptional function in promoting the BCSC phenotype. | Fei Peng Jie Xu Bai Cui Qilan Liang Sai Zeng Bin He Hong Zou Manman Li Huan Zhao Yuting Meng Jin Chen Bing Liu Shasha Lv Peng Chu Fan An Zifeng Wang Junxiu Huang Yajing Zhan Yuwei Liao Jinxin Lu Lingzhi Xu Jin Zhang Zhaolin Su Zhiguang Li Fangjun Wang Eric W-FLam Quentin Liu | 2021 | Cell Research2021，31，3： | 9 |
| 3 | Wheat genomic study for genetic improvement of traits in China显示文摘Bread wheat(Triticum aestivum L.)is a major crop that feeds 40%of the world’s population.Over the past several decades,advances in genomics have led to tremendous achievements in understanding the origin and domestication of wheat,and the genetic basis of agronomically important traits,which promote the breeding of elite varieties.In this review,we focus on progress that has been made in genomic research and genetic improvement of traits such as grain yield,end-use traits,flowering regulation,nutrient use efficiency,and biotic and abiotic stress responses,and various breeding strategies that contributed mainly by Chinese scientists.Functional genomic research in wheat is entering a new era with the availability of multiple reference wheat genome assemblies and the development of cutting-edge technologies such as precise genome editing tools,highthroughput phenotyping platforms,sequencing-based cloning strategies,high-efficiency genetic transformation systems,and speed-breeding facilities.These insights will further extend our understanding of the molecular mechanisms and regulatory networks underlying agronomic traits and facilitate the breeding process,ultimately contributing to more sustainable agriculture in China and throughout the world. | Jun Xiao Bao Liu Yingyin Yao Zifeng Guo Haiyan Jia Lingrang Kong Aimin Zhang Wujun Ma Zhongfu Ni Shengbao Xu Fei Lu Yuannian Jiao Wuyun Yang Xuelei Lin Silong Sun Zefu Lu Lifeng Gao Guangyao Zhao Shuanghe Cao Qian Chen Kunpu Zhang Mengcheng Wang Meng Wang Zhaorong Hu Weilong Guo Guoqiang Li Xin Ma Junming Li Fangpu Han Xiangdong Fu Zhengqiang Ma Daowen Wang Xueyong Zhang Hong-Qing Ling Guangmin Xia Yiping Tong Zhiyong Liu Zhonghu He Jizeng Jia Kang Chong | 2022 | Science China(Life Sciences)2022，65，9： | 9 |
| 4 | Increased mitochondrial fission drives the reprogramming of fatty acid metabolism in hepatocellular carcinoma cells through suppression of Sirtuin 1显示文摘Background:Mitochondria are dynamic organelles that constantly change their morphology through fission and fusion processes.Recently,abnormally increased mitochondrial fission has been observed in several types of can-cer.However,the functional roles of increased mitochondrial fission in lipid metabolism reprogramming in cancer cells remain unclear.This study aimed to explore the role of increased mitochondrial fission in lipid metabolism in hepa-tocellular carcinoma(HCC)cells.Methods:Lipid metabolism was determined by evaluating the changes in the expressions of core lipid metabolic enzymes and intracellular lipid content.The rate of fatty acid oxidation was evaluated by[PH]-labelled oleic acid.The mito-chondrial morphology in HCC cells was evaluated by fluorescent staining.The expression of protein was determined by real-time PCR,imnmunohistochemistry and Western blotting.Results:Activation of mitochondrial fission significantly promoted de novo fatty acid synthesis in HCC cells through upregulating the expression of lipogenic genes fatty acid synthase(FASN),acetyl-CoA carboxylasel(ACCI),and elonga-tion of very long chain fatty acid protein 6(ELOVL6),while suppressed fatty acid oxidation by downregulating carnitine palmitoyl transferase 1A(CPTIA)and acyl-CoA oxidase 1(ACOX1).Consistently,suppressed mitochondrial fission exhibited the opposite effects.Moreover,in vitro and in vivo studies revealed that mitochondrial fission-induced lipid metabolism reprogramming significantly promoted the proliferation and metastasis of HCC cells.Mechanistically,mito-chondrial fission increased the acetylation level of sterol regulatory element-binding protein 1(SREBPI)and peroxisome proliferator-activated receptor coaC-tivator 1 alpha(PGC-1a)by suppressing nicotinamide adenine dinucleotide(NAD+)/Sirtuin 1(SIRTI)signaling.The elevated SREBP1 then upregulated the expression of FASN,ACC1 and ELOVL6 in HCC cells,while PGC-1c/PPARa sup-pressed the expression of CPTIA and ACOXL Conclusions:Increased mitochondrial fission plays a crucial role in the repro-gramming of lipid metabolism in HCC cells,which provides strong evidence for the use of this process as a drug target in the treatment of this malignancy. | Dan Wu Yi Yang Yiran Hou Zifeng Zhao Ning Liang Peng Yuan Tao Yang Jinliang Xing Jibin Li | 2022 | Cancer Communications2022，42，1： | 4 |
| 5 | Deep-blue organic light-emitting diodes based on a doublet d-f transition cerium(Ⅲ) complex with 100% exciton utilization efficiency显示文摘Compared to red and green organic light-emitting diodes(OLEDs),blue OLEDs are still the bottleneck due to the lack of efficient emitters with simultaneous high exciton utilization efficiency(EUE)and short excited-state lifetime.Different from the fluorescence,phosphorescence,thermally activated delayed fluorescence(TADF),and organic radical materials traditionally used in OLEDs,we demonstrate herein a new type of emitter,cerium(Ⅲ)complex Ce-1 with spin-allowed and parity-allowed d-f transition of the centre Ce^(3+) ion.The compound exhibits a high EUE up to 100% in OLEDs and a short excited-state lifetime of 42 ns,which is considerably faster than that achieved in efficient phosphorescence and TADF emitters.The optimized OLEDs show an average maximum external quantum efficiency(EQE)of 12.4% and Commission Internationale de L’Eclairage(CIE)coordinates of(0.146,0.078). | Liding Wang Zifeng Zhao Ge Zhan Huayi Fang Hannan Yang Tianyu Huang Yuewei Zhang Nan Jiang Lian Duan Zhiwei Liu Zuqiang Bian Zhenghong Lu Chunhui Huang | 2020 | Light(Science & Applications)2020，9，1： | 3 |
| 6 | Efficient rare earth cerium(Ⅲ)complex with nanosecond d-f emission for blue organic light-emitting diodes显示文摘In the field of RGB diodes,development of a blue organic light-emitting diode(OLED)is a challenge because of the lack of an emitter which simultaneously has a short excited state lifetime and a high theoretical external quantum efficiency(EQE).We demonstrate herein a blue emissive rare earth cerium(III)complex Ce-2 showing a high photoluminescence quantum yield of 95%and a short excited state lifetime of 52.0 ns in doped film,which is considerably faster than that achieved in typical efficient phosphorescence or thermally activated delayed fluorescence emitters(typical lifetimes>1μs).The corresponding OLED shows a maximum EQE up to 20.8%and a still high EQE of 18.2%at 1000 cd m^(-2),as well as an operation lifetime 70 times longer than that of a classic phosphorescence OLED.The excellent performance indicates that cerium(III)complex could be a candidate for efficient and stable blue OLEDs because of its spin-and parity-allowed d-f transition from the Ce^(3+)ion. | Zifeng Zhao Liding Wang Ge Zhan Zhiwei Liu Zuqiang Bian Chunhui Huang | 2021 | National Science Review2021，8，2： | 3 |
| 7 | Epitaxial growth of hyperbranched Cu/Cu2O/CuO coreshell nanowire heterostructures for lithium-ion batteries显示文摘nano 建筑学的小心的设计和期望的活跃材料的聪明的杂交能导致更先进的性质。这里,我们设计了新奇层次分叉 Cu/Cu 2 由联合一个灵巧的热水的方法和随后的控制氧化过程的 O/CuO heteronanostructure。在分支和脊梁之间的好结构和取向附生的关系被高分辨率的传播电子显微镜学调查。而且,分支生长的进化也在 Cu nanowire 表面的渐渐的氧化期间被观察了。试验性的结果建议经由二拍子的圆舞暴露进程要表现到改变湿度以便完成的表面氧化需要优化了核心壳的形成结构化的分叉的建筑学。最后,象在锂离子电池的阳极材料的如此的一个层次框架的功能的 proof-of-concept 被表明。分叉的核心壳 heterostructure 由几个工具改进电池性能:取向附生地成年的分支提供的(i) 为到卷变化的提高的电解质可接近性和高抵抗的一个高表面区域由 Li+ 置闰 / 抽取导致了;(ii ) 有它的明确的异质接面的核心壳结构增加在 lithiation 期间便于有效费用运输的接触区域;(iii ) 铜核心象提供结构的加强一样充当一个当前的收集者。 | Yuxin Zhao Ying Zhang Hu Zhao Xuejin Li Yanpeng Li Ling wen Zifeng Yan Ziyang Huo | 2015 | Nano Research2015，8，8： | 2 |
| 8 | Hydrogen-induced Modification in the Deformation and Fracture of a Precipitation-hardened Fe-Ni Based Austenitic Alloy显示文摘Hydrogen-induced modification in the deformation and fracture of a precipitation-hardened Fe e Ni based austenitic alloy has been investigated in the present study by means of thermal hydrogen charging experiment, tensile tests, scanning electron microscopy(SEM) and transmission electron microscopy(TEM). It is found that the g0 particles are subjected to the multiple shearing by dislocations during plastic deformation,which promotes the occurrence of the dislocation planar slip. Moreover, the alloy will be enhanced by hydrogen resulting in the formation of strain localization at macroscale. So, the mechanisms of deformation and fracture in the alloy have been proposed in terms of serious hydrogen-induced planar slip at microscale which can lead to macroscopic strain localization. | Mingjiu Zhao Zifeng Guo Shenghu Chen Hao Liang Lijian Rong | 2014 | Journal of Materials Science & Technology2014，30，11： | 1 |
| 9 | Trace determination and characterization of ginsenosides in rat plasma through magnetic dispersive solid-phase extraction based on core-shell polydopamine-coated magnetic nanoparticles显示文摘Enrichment of trace bioactive constituents and metabolites from complex biological samples is challenging.This study presented a one-pot synthesis of magnetic polydopamine nanoparticles(Fe3O4@-SiO2@PDA NPs)with multiple recognition sites for the magnetic dispersive solid-phase extraction(MDSPE)of ginsenosides from rat plasma treated with white ginseng.The extracted ginsenosides were characterized by combining an ultra-high-performance liquid chromatography coupled to a highresolution mass spectrometry with supplemental UNIFI libraries.Response surface methodology was statistically used to optimize the extraction procedure of the ginsenosides.The reusability of Fe3O4@-SiO2@PDA NPs was also examined and the results showed that the recovery rate exceeded 80%after recycling 6 times.Furthermore,the proposed method showed greater enrichment efficiency and could rapidly determine and characterize 23 ginsenoside prototypes and metabolites from plasma.In comparison,conventional methanol method can only detect 8 ginsenosides from the same plasma samples.The proposed approach can provide methodological reference for the trace determination and characterization of different bioactive ingredients and metabolites of traditional Chinese medicines and food. | Ningning Zhao Shu Liu Junpeng Xing Zifeng Pi Fengrui Song Zhiqiang Liu | 2020 | Journal of Pharmaceutical Analysis2020，10，1： | 1 |
| 10 | Effect of the number of layers on the bond strength for multi-layer brittle coating-substrate system显示文摘Finite element method(FEM) was used to investigate the effect of the number of layers on the bond strength for the brittle coating/substrate materials at contact load condition,which has not been addressed previously.The maximum shear stress was used to act as the criterion of the bonded strength.This paper discussed the relationship between the number of coating layers and the maximum shear stress of the layer/substrate interface.Firstly,the results of the FEM and the Hertz analytical method were compared to verify the accuracy of the FEM model.It was found that with the increase in the number of coating layers,the position of the suddenly changed stress along the z axis is transformed from the interface to the external surface of the coating.Finally,the increase in the number of layers contributes to the decrement of the stress along the x axis. | WANG YongGuang NI ZiFeng CHEN GuoZhong CHEN AnQi SU YongShuai ZHAO YongWu | 2012 | Science China(Technological Sciences)2012，55，10： | 1 |
| 11 | Synthesis and luminescence properties of Mn^(4+)-dopant Ca_(14)Zn_6Ga_(10-x)Al_xO_(35)solid solution显示文摘Mn^(4+)-activated oxide phosphors,owing to their desirable spectral features,eco-friendly and low cost,are emerging as a new class of non-rare-earth red phosphors for warm white LEDs.However,these phosphors possess low photoluminescence quantum efficiency excited by blue chip currently.Herein we report an isostructural solid solution of Ca_(14)Zn_6Ga_(10-x)Al_xO_(35):0.15Mn^(4+)(0≤x≤10)synthesized by a traditional solidstate reaction route.The microstructure and luminescent performance of this red-emitting phosphor are investigated in detail with the aids of X-ray diffraction,diffuse reflection spectra,photoluminescence spectra/decay/QE,and temperature-dependent PL/QE measurements.Blue shift of energy peaks of^4A_2→~4T_1and^4A_2→~4T_2transition is illustrated by the Tanabe–Sugano diagram and the configurational coordinate diagram.The crystal field strength(Dq)and the Racah parameters(B and C)are carefully calculated to estimate the nephelauxetic effectβrespectively.Particularly we achieve external and internal quantum efficiencies as high as26.1%and 40.3%for Ca_(14)Zn_6Ga_6Al_4O_(35):0.15Mn^(4+)excited by 466 nm,the highest one ever reported in Mn^(4+)activated oxide phosphors under the similar condition. | Yiyang Zhou Weiren Zhao Chongrui Lu Zifeng Liao | 2018 | Progress in Natural Science:Materials International2018，28，3： | 1 |
| 12 | Laser-induced porous graphene on Polyimide/PDMS composites andits kirigami-inspired strain sensor显示文摘The laser-induced porous graphene(LIG)prepared in a straightforward fabrication method is presented,and its applications in stretchable strain sensors to detect the applied strain are also explored.The LIGformed on the polyimide/polydimethylsiloxane(PI/PDMS)composite exhibits a naturally high stretchabil-ity(over 30%),bypassing the transfer printing process compared to the one prepared by laser scribing onPI films.The PI/PDMS composite with LIG shows tunable mechanical and electronic performances withdifferent PI particle concentrations in PDMS.The good cyclic stability and almost linear response of theprepared LIG’s resistance with respect to tensile strain provide its access to wearable electronics.To im-prove the PDMS/PI composite stretchability,we designed and optimized a kirigami-inspired strain sensorwith LIG on the top surface,dramatically increasing the maximum strain value that in linear response toapplied strain from 3%to 79%. | Hao Wang Zifeng Zhao Panpan Liu Xiaogang Guo | 2021 | Theoretical & Applied Mechanics Letters2021，11，2： | 0 |
| 13 | Engineering Sodium Metal Anode with Sodiophilic Bismuthide Penetration for Dendrite-Free and High-Rate Sodium-Ion Battery显示文摘Sodium(Na)metal batteries with a high volumetric energy density that can be operated at high rates are highly desirable.However,an uneven Na-ion migration in bulk Na anodes leads to localized deposition/dissolution of sodium during high-rate plating/stripping behaviors,followed by severe dendrite growth and loose stacking.Herein,we engineer the Na hybrid anode with sodiophilic Na_(3)Bi-penetration to develop the abundant phase-boundary ionic transport channels.Compared to intrinsic Na,the reduced adsorption energy and ion-diffusion barrier on Na_(3)Bi ensure even Na^(+)nucleation and rapid Na^(+)migration within the hybrid electrode,leading to uniform deposition and dissolution at high current densities.Furthermore,the bismuthide enables compact Na deposition within the sodiophilic framework during cycling,thus favoring a high volumetric capacity.Consequently,the obtained anode was endowed with a high current density(up to 5 mA∙cm^(−2)),high areal capacity(up to 5 mA∙h∙cm^(−2)),and long-term cycling stability(up to 2800 h at 2 mA∙cm^(−2)). | Wanyu Zhao Min Guo Zhijun Zuo Xiaoli Zhao Huanglin Dou Yijie Zhang Shiying Li Zichen Wu Yayun Shi Zifeng Ma Xiaowei Yang | 2022 | Engineering2022，8，4： | 0 |
| 14 | Luminescent d-f transition Yb(Ⅱ)-containing azacryptates with high photoluminescence quantum yields显示文摘Emission tunable d-f transition lanthanide complexes have wide applications in many fields such as lighting and photoredox catalysis.Compared with Ce(Ⅲ)and Eu(Ⅱ)complexes,which have achieved near-unity photoluminescence quantum yields(PLQYs),Yb(Ⅱ)complexes still suffer from low reported PLQYs not exceeding 10%.In this work,two luminescent Yb(Ⅱ)-containing azacryptates YbI_(2)-N8M6(N8M6=4,7,13,16,21,24-hexamethyl-1,4,7,10,13,16,21,24-octaazabicyclo[8.8.8]hexacosane)and YbI2-N8E6(N8E6=4,7,13,16,21,24-hexaethyl-1,4,7,10,13,16,21,24-octaazabicyclo[8.8.8]hexacosane)were synthesized and characterized.YbI2-N8M6 in solid powder exhibits blue emission with a maximum emission wavelength(λm)of 464 nm and a PLQY of 76%,while YbI_(2)-N8E6 in solid powder exhibits green emission with a λ_(m) of 537 nm and a PLQY up to93%.Moreover,YbI_(2)-N8M6 exhibits mechanochromic property,showing an emission color change from deep-blue to cyan under mechanical grinding.These results will inspire the studies about luminescent Yb(Ⅱ)complexes and their further applications. | Wenchao Yan Zifeng Zhao Gang Yu Hao Qi Ruoyao Guo Nanlong Zheng Zuqiang Bian Zhiwei Liu | 2023 | Science China Chemistry2023，66，6： | 0 |
| 15 | Highly efficient green organic light-emitting devices based on terbium complex by employing hole block material as host显示文摘In this work,efficient green electroluminescent(EL)devices with simplified device structure were prepared by doping trivalent terbium complex Tb(PMIP)_3into hole block material Tm Py PB.The high triplet energy of Tm Py PB helps to confine excitons within light-emitting layer,while the electron transport characteristic of Tm Py PB facilitates the balance of carriers on Tb(PMIP)_3molecules.By optimizing the doping concentration of Tb(PMIP)_3and the thickness of each functional layer,highly efficient green EL device with the structure of ITO/Mo O_3(3 nm)/TAPC(50 nm)/Tb(PMIP)_3(30 wt%):Tm Py PB(25 nm)/Tm Py PB(60 nm)/Li F(1 nm)/Al(100 nm)displayed pure Tb^(3+)characteristic emission with maximum current efficiency,power efficiency and brightness up to 47.24 cd/A(external quantum efficiency(EQE)of 14.4%),43.63 lm/W and 1694 cd/m^2,respectively.At certain brightness of 100 cd/m^2,the device still maintained a current efficiency of 19.96 cd/A(EQE=6.1%).Such a device design strategy helps to improve the EL performances of Tb(PMIP)_3and to simplify device fabrication processes,thus reduce the fabrication cost. | ZHAO XueSen ZHAO ZiFeng ZHOU Liang ZHU Qi LIU ZhiWei BIAN ZuQiang HUANG ChunHui ZHANG HongJie | 2018 | Science China(Technological Sciences)2018，61，9： | 0 |
| 16 | Electrolyte and interphase engineering through solvation structure regulation for stable lithium metal batteries显示文摘Lithium metal batteries(LMBs)are considered to be one of the most promising high-energy-density battery systems.However,their practical application in carbonate electrolytes is hampered by lithium dendrite growth,resulting in short cycle life.Herein,an electrolyte regulation strategy is developed to improve the cyclability of LMBs in carbonate electrolytes by introducing LiNO3 using trimethyl phosphate with a slightly higher donor number compared to NO_(3)^(-)as a solubilizer.This not only allows the formaion of Li^(+)-coordinated NO3 but also achieves the regulation of electrolyte solvation structures,leading to the formation of robust and ion-conductive solid-electrolyte interphase films with inorganic-rich inner and organic-rich outer layers on the Li metal anodes.As a result,high Coulombic efficiency of 99.1%and stable plating/stripping cycling of Li metal anode in LilCu cells were realized.Furthermore,excellent performance was also demonstrated in Li||LiNi_(0.83)Co_(0.11)Mn_(0.06)O_(2)(NCM83)full cells and Cul/NCM83 anodefree cells using high mass-loading cathodes.This work provides a simple interphase engineering strategy through regulating the electrolyte solvation structures for high-energy-density LMBs. | Hai Su Haikuo Zhang Zifeng Chen Mengjie Li Jiwei Zhao Haiyan Xun Jie Sun Yunhua Xu | 2023 | Chinese Chemical Letters2023，34，12： | 0 |
| 17 | The wheat sucrose synthase gene TaSus1 is a determinant of grain number per spike显示文摘Some haplotypes of the sucrose synthase gene TaSus1 are associated with thousand-grain weight(TGW)in wheat(Triticum aestivum L.).However,no mutations have been identified within the gene to test this association.The effects of TaSus1 on grain number per spike(GNS)also are largely unknown.Our previous genome-wide association study identified TaSus-A1 as a candidate gene controlling fertile spikelet number per spike(FSN).In the present study,we generated two independent mutants for the three TaSus1 homoeologs by CRISPR/Cas9-mediated genome editing.The triple mutants displayed lower FSN,GNS,grain number per spikelet(GNST),and TGW than wild-type plants.In 306 hexaploid wheat accessions,two single-nucleotide polymorphisms in TaSus-A1 contributed differently to GNS.Introgression of the two alleles into a wheat genetic background confirmed their effects.The alleles differed in geographical distribution among the accessions. | Liping Shen Lili Zhang Changbin Yin Xiaowan Xu Yangyang Liu Kuocheng Shen He Wu Zhiwen Sun Ke Wang Zhonghu He Xueyong Zhang Chenyang Hao Jian Hou Aoyue Bi Xuebo Zhao Daxing Xu Botao Ye Xuchang Yu Ziying Wang Danni Liu Yuanfeng Hao Fei Lu Zifeng Guo | 2024 | The Crop Journal2024，12，1： | 0 |
| 18 | Lanthanide complexes with d-f transition:new emitters for single-emitting-layer white organic light-emitting diodes显示文摘White organic light-emitting diodes(WOLEDs)is a new generation of lighting technology and has stimulated wide-ranging studies.Despite the advantage of simple device structure,single-emitting-layer WOLEDs(SEL-WOLEDs)still face the challenges of difficult material screening and fine energy level regulation.Herein,we report efficient SEL-WOLEDs with a sky-blue emitting cerium(Ⅲ)complex Ce-TBO2Et and an orange-red emitting europium(Ⅱ)complex Eu(Tp2Et)2 as the emitters,showing a maximum external quantum efficiency of 15.9%and Commission Internationale de l'Eclairage coordinates of(0.33,0.39)at various luminances.Most importantly,the electroluminescence mechanism of direct hole capture and hindered energy transfer between the two emitters facilitate a manageable weight doping concentration of 5%for Eu(Tp2Et)2,avoiding the low concentration(<1%)of the low-energy emitter in typical SEL-WOLEDs.Our results indicate that d-f transition emitters may circumvent fine energy level regulation and provide development potential for SEL-WOLEDs. | Peiyu Fang Peihao Huo Liding Wang Zifeng Zhao Gang Yu Yanyi Huang Zuqiang Bian Zhiwei Liu | 2023 | Light(Science & Applications)2023，12，8： | 0 |
| 19 | Efficient green OLEDs achieved by a terbium(Ⅲ)complex with photoluminescent quantum yield close to 100%显示文摘Electroluminescence of f-f transition lanthanide complex is a traditional topic for display over decades.Here we report highly efficient organic light-emitting diodes based on a new terbium(III)complex with novel ligand CPMIP(1-(4-cyanophenyl)-3-methyl-4-isobutyryl-pyrazoline-5-one).The high triplet energy level of CPMIP(3.0 e V)and inhibited quenching effects in the solid-state lead to a nearly 100%photoluminescent quantum efficiency of Tb(CPMIP)3.The best Tb(CPMIP)3 device exhibited maximum external quantum efficiency up to 19.7%,setting a new record of OLEDs based on f-f transition lanthanide complexes. | Zifeng Zhao Mengying Bian Chenjian Lin Xuzheng Fu Gang Yu Huibo Wei Zhiwei Liu Zuqiang Bian Chunhui Huang | 2021 | Science China Chemistry2021，64，9： | 0 |
| 20 | Construction of Frame-Structured Flexible MXene Film Electrode to Achieve High Areal Capacitance Micro-Supercapacitor显示文摘Two-dimensional MXene-based film materials as flexible electrodes have been widely studied in wearable microsupercapacitors(MSCs).However,the existence of strong van derWaals interactions leads to serious self-stacking ofMXene layers,resulting in poor ionic dynamics and loss of active sites,which causes MXene film electrodes to exhibit low capacitance and poor rate performance in practical studies.To solve this,a frame-structured hybrid film(labeled as CN-MX hybrid film)is constructed by introducing intercalating agents(nanometer g-C_(3)N_(4))into MXene layers.In this unique hybrid film,the g-C_(3)N_(4)nanoparticles rationally occupy the interspace between MXene layers so as to alleviate layer stacking,thus effectively expanding the electrochemically active surface and promoting proton transfer.Synergistic pseudocapacitance inducted by g-C_(3)N_(4)surface groups,consequently,the CN-MX hybrid film electrode achieves an enhanced capacitive capability.In the three-electrode system,this frame-structured film electrode exhibits an ultra-high areal capacitance of 1932.8 mF cm^(−2).The assembled symmetry flexible MSC device based on CN-MX hybrid film can achieve an energy density of 2.28μWh cm^(−2)at 0.075 mW cm^(−2),as well as a superior cyclic stability with 90.4%retention after 700 cycles in alternating 90o bending and releasing states,revealing its potential in practical applications. | Yesheng Wang Yongpeng Cui Dongqing Kong Xiaoning Wang Wenting Feng Pengyun Liu Tonghui Cai Xuejin Li Lianming Zhao Debin Kong Linjie Zhi Qingzhong Xue Zifeng Yan Wei Xing | 2023 | Renewables2023，1，2： | 0 |
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