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| 1 | Fluorescence regional integration and differential fluorescence spectroscopy for analysis of structural characteristics and proton binding properties of fulvic acid sub-fractions显示文摘Structural characteristics and proton binding properties of sub-fractions(FA3–FA13) of fulvic acid(FA), eluted stepwise by pyrophosphate buffer were examined by use of fluorescence titration combined with fluorescence regional integration(FRI) and differential fluorescence spectroscopy(DFS). Humic-like(H-L) and fulvic-like(F-L) materials, which accounted for more than 80% of fluorescence response, were dominant in five sub-fractions of FA. Based on FRI analysis, except the response of F-L materials in FA9 and FA13, maximum changes in percent fluorescence response were less than 10% as pH was increased from 2.5 to 11.5.Contents of carboxylic and phenolic groups were compared for fluorescence peaks of FA sub-fractions based on pH-dependent fluorescence derived from DFS. Static quenching was the dominant mechanism for binding of protons by FA sub-fractions. Dissociation constants(p Ka) were calculated by use of results of DFS and the modified Stern-Volmer relationship. The p Kaof H-L, F-L, tryptophan-like and tyrosine-like materials of FA subfractions exhibited ranges of 3.17–4.06, 3.12–3.97, 4.14–4.45 and 4.25–4.76, respectively, for acidic pHs. At basic pHs, values of p Ka for corresponding materials were in ranges of 9.71–10.24, 9.62–10.99, 9.67–10.31 and 9.33–10.28, respectively. At acidic pH, protein-like(P-L)materials had greater affinities for protons than did either H-L or F-L materials. The dicarboxylic and phenolic groups were likely predominant sites of protonation for both H-L and F-L materials at both acidic and basic pHs. Amino acid groups were significant factors during proton binding to protein-like materials of FA sub-fractions at basic pH. | Fanhao Song Fengchang Wu Weiying Feng Zhi Tang John P.Giesy Fei Guo Di Shi Xiaofei Liu Ning Qin Baoshan Xing Yingchen Bai | 2018 | Journal of Environmental Sciences2018，30，12： | 9 |
| 2 | Spatiotemporal variation in snow cover and its effects on grassland phenology on the Mongolian Plateau显示文摘Snow cover is an important water source for vegetation growth in arid and semi-arid areas,and grassland phenology provides valuable information on the response of terrestrial ecosystems to climate change.The Mongolian Plateau features both abundant snow cover resources and typical grassland ecosystems.In recent years,with the intensification of global climate change,the snow cover on the Mongolian Plateau has changed correspondingly,with resulting effects on vegetation growth.In this study,using MOD10A1 snow cover data and MOD13A1 Normalized Difference Vegetation Index(NDVI)data combined with remote sensing(RS)and geographic information system(GIS)techniques,we analyzed the spatiotemporal changes in snow cover and grassland phenology on the Mongolian Plateau from 2001 to 2018.The correlation analysis and grey relation analysis were used to determine the influence of snow cover parameters(snow cover fraction(SCF),snow cover duration(SCD),snow cover onset date(SCOD),and snow cover end date(SCED))on different types of grassland vegetation.The results showed wide snow cover areas,an early start time,a late end time,and a long duration of snow cover over the northern Mongolian Plateau.Additionally,a late start,an early end,and a short duration were observed for grassland phenology,but the southern area showed the opposite trend.The SCF decreased at an annual rate of 0.33%.The SCD was shortened at an annual rate of 0.57 d.The SCOD and SCED in more than half of the study area advanced at annual rates of 5.33 and 5.74 DOY(day of year),respectively.For grassland phenology,the start of the growing season(SOS)advanced at an annual rate of 0.03 DOY,the end of the growing season(EOS)was delayed at an annual rate of 0.14 DOY,and the length of the growing season(LOS)was prolonged at an annual rate of 0.17 d.The SCF,SCD,and SCED in the snow season were significantly positively correlated with the SOS and negatively correlated with the EOS and LOS.The SCOD was significantly negatively correlated with the SOS and positively correlated with the EOS and LOS.The SCD and SCF can directly affect the SOS of grassland vegetation,while the EOS and LOS were obviously influenced by the SCOD and SCED.This study provides a scientific basis for exploring the response trends of alpine vegetation to global climate change. | SA Chula MENG Fanhao LUO Min LI Chenhao WANG Mulan ADIYA Saruulzaya BAO Yuhai | 2021 | Journal of Arid Land2021，13，4： | 5 |
| 3 | Simulated photo-degradation of dissolved organic matter in lakes revealed by three-dimensional excitation-emission matrix with regional integration and parallel factor analysis显示文摘Simulated photo-degradation of fluorescent dissolved organic matter(FDOM) in Lake Baihua(BH) and Lake Hongfeng(HF) was investigated with three-dimensional excitationemission matrix(3 DEEM) fluorescence combined with the fluorescence regional integration(FRI),parallel factor(PARAFAC) analysis,and multi-order kinetic models.In the FRI analysis,fulvic-like and humic-like materials were the main constituents for both BH-FDOM and HF-FDOM.Four individual components were identified by use of PARAFAC analysis as humic-like components(C1),fulvic-like components(C2),protein-like components(C3) and unidentified components(C4).The maximum 3 DEEM fluorescence intensity of PARAFAC components C1-C3 decreased by about 60%,70% and 90%,respectively after photo-degradation.The multi-order kinetic model was acceptable to represent the photo-degradation of FDOM with correlation coefficient(Radj2)(0.963-0.998).The photo-degradation rate constants(kn) showed differences of three orders of magnitude,from 1.09 × 10-6 to 4.02 × 10-4 min-1,and half-life of multi-order model(T1/2n)ranged from 5.26 to 64.01 min.The decreased values of fluorescence index(FI) and biogenic index(BI),the fact that of percent fluorescence response parameter of Region I(PⅠ,n) showed the greatest change ratio,followed by percent fluorescence response parameter of Region II(PⅡ,n,while the largest decrease ratio was found for C3 components,and the lowest T1/2n was observed for C3,indicated preferential degradation of protein-like materials/components derived from biological sources during photodegradation.This research on the degradation of FDOM by 3 DEEM/FRI-PARAFAC would be beneficial to understanding the photo-degradation of FD OM in natural environments and accurately predicting the environmental behaviors of contaminants in the presence of FDOM. | Jin Zhang Fanhao Song Tingting Li Kefu Xie Huiying Yao Baoshan Xing Zhongyu Li Yingchen Bai | 2020 | Journal of Environmental Sciences2020，32，4： | 3 |
| 4 | Three decades of changes in water environment of a large freshwater Lake and its relationship with socio-economic indicators显示文摘Tai Lake(Ch: Taihu) has attracted international attention forcyanobacteria blooms.However, the drivers of cultural eutrophication, especially long-term socio-economic indicators have been little researched. The results of research demonstrate how socioeconomic development affected quality of water and how it has been improved by anthropogenic activities. This study described variability in indicators of water quality in Tai Lakeand investigated thedrivers. Significant relationships existed between concentrations of annual mean total nitrogen(TN), total phosphorous(TP), chemical oxygen demand(COD) and biological oxygen demand(BOD), and population, per capital gross domestic production(GDP) and sewage discharge(p < 0.05). However, mechanisms causing change varied among TN, TP, COD and BOD. Before 2000, the main contributors to increases in concentrations of TN were human population, GDP and volumes of domestic sewage discharges. After 2000, discharges of industrial sewage become the primary contributor. After 1998, the regressions of annual mean TN, TP and COD on per capital GDP, population and domestic sewage discharge were reversed compared to the former period. Since 1999, an apparent inverted U-shaped relationship between environmental pollution and economic development has developed, which indicated that actions taken by governments have markedly improved quality of water in Tai Lake. The statistical relationship between BOD and per capital GDP didn't conform to the Kuznet curve. The Ushaped Kuznet curve may offer hope for the future that with significant environmental investments a high GDP can be reached and maintained without degradation of the environment, especially through appropriate management of industrial sewage discharge. | Cuicui Li Weiying Feng Fanhao Song Zhongqi He Fengchang Wu Yuanrong Zhu John P.Giesy Yingchen Bai | 2019 | Journal of Environmental Sciences2019，31，3： | 3 |
| 5 | Assessing remotely sensed and reanalysis products in characterizing surface soil moisture in the Mongolian Plateau显示文摘Soil moisture(SM)plays a crucial role in the dynamics of coupled atmosphere,water,energy,and carbon cycles.In this study,the spatiotemporal distribution and variations of SM in the Mongolian Plateau were investigated for the period of 1982-2018 based on four gridded SM datasets.Taking the observed SM from 33 monitoring stations as a reference,the reliability of these four gridded products was validated,and the three-cornered hat(TCH)method was also applied to evaluate their uncertainties.Major results indicated that all these four products underestimated the SM in this region at different levels.The ERA-Interim SM performed much better than other three products,with a higher R of 0.53 and lower ubRMSE of 0.0378 m^(3)·m^(−3).Except for ECV,the surface SM exhibited a decreasing trend at−0.0004 to−0.0008 m^(3)·m^(−3)/decade in the warm season(from April to October)over the past 37 years.The greatest decreases in SM occurred in the summer season.Precipitation change plays a more important role in explaining the variations of SM than temperature reported by partial correlation analysis.The results of this study will benefit our understanding of the climate change effects and the protection of the ecological systems in this region. | Min Luo Chula Sa Fanhao Meng Yongchao Duan Tie Liu Yuhai Bao | 2021 | International Journal of Digital Earth2021，14，10： | 2 |
| 6 | 显示文摘 | Cheng Jie Bo Dong Wang Fanhao | 2003 | Electronic Journals2003，18，7： | 1 |
| 7 | Proliferation and gene expression of osteoblasts cultured in DMEM containing the ionic products of dicalcium silicate coating显示文摘 | Junying Sun Jianyou Li Xuanyong Liu Li Wei Guocheng Wang Fanhao Meng | 2009 | Biomedicine & Pharmacotherapy2009，，9： | 1 |
| 8 | Tensile creep behavior of heat-treated TC11 titanium alloy at 450–550<ce:hsp sp='0.25'/>°C显示文摘 | Yi Gu Fanhao Zeng Yanling Qi Changqing Xia Xiang Xiong | 2013 | Materials Science & Engineering A2013，，： | 1 |
| 9 | Preparation and antibacterial prope nano-titania/silver coatings 显示文摘 | BAOE L XUANYONG L FANHAO M | 2009 | Materials Chemistry and Physics2009，118，： | 1 |
| 10 | LC determination of luteolin-7-O-β-D-glucoside and apigenin-7-O-β-D-glucoside in rat plasma after administration of Humulus scandens extract and its application to pharmacokinetic studies显示文摘 | Zaixing Chen Xixiang Ying Shu Meng Xu Zhu Hong Jiang Qishen Cao Lin Wang Fanhao Meng | 2012 | Natural Product Research2012，，6： | 1 |
| 11 | The isothermal section of the Al-4Mg-Sc-Zr quaternary system in Al-rich range显示文摘 | Zeng Fanhao Xia Changqing Gu Yi | 2004 | Journal of Alloys and Compounds2004，363，： | 1 |
| 12 | Large-scale growth of In2O3 nanowires and their optical properties显示文摘 | Zeng Fanhao Zhang X Wang Jin | 2004 | Nanotechnology2004，15，5： | 1 |
| 13 | Prediction of protected band edge states and dielectric tunable quasiparticle and excitonic properties of monolayer MoSi_(2)N_(4)显示文摘The electronic structure of two-dimensional(2D)materials are inherently prone to environmental perturbations,which may pose significant challenges to their applications in electronic or optoelectronic devices.A 2D material couples with its environment through two mechanisms:local chemical coupling and nonlocal dielectric screening effects.The local chemical coupling is often difficult to predict or control experimentally.Nonlocal dielectric screening,on the other hand,can be tuned by choosing the substrates or layer thickness in a controllable manner.Therefore,a compelling 2D electronic material should offer band edge states that are robust against local chemical coupling effects.Here it is demonstrated that the recently synthesized MoSi_(2)N_(4)is an ideal 2D semiconductor with robust band edge states protected from capricious environmental chemical coupling effects.Detailed many-body perturbation theory calculations are carried out to illustrate how the band edge states of MoSi_(2)N_(4)are shielded from the direct chemical coupling effects,but its quasiparticle and excitonic properties can be modulated through the nonlocal dielectric screening effects.This unique property,together with the moderate band gap and the thermodynamic and mechanical stability of this material,paves the way for a range of applications of MoSi_(2)N_(4)in areas including energy,2D electronics,and optoelectronics. | Yabei Wu Zhao Tang Weiyi Xia Weiwei Gao Fanhao Jia Yubo Zhang Wenguang Zhu Wenqing Zhang Peihong Zhang | 2022 | npj Computational Materials2022，，1： | 0 |
| 14 | Digital Simulation of Projective Non-Abelian Anyons with 68 Superconducting Qubits显示文摘Non-Abelian anyons are exotic quasiparticle excitations hosted by certain topological phases of matter.They break the fermion-boson dichotomy and obey non-Abelian braiding statistics:their interchanges yield unitary operations,rather than merely a phase factor,in a space spanned by topologically degenerate wavefunctions.They are the building blocks of topological quantum computing.However,experimental observation of non-Abelian anyons and their characterizing braiding statistics is notoriously challenging and has remained elusive hitherto,in spite of various theoretical proposals.Here,we report an experimental quantum digital simulation of projective non-Abelian anyons and their braiding statistics with up to 68 programmable superconducting qubits arranged on a two-dimensional lattice.By implementing the ground states of the toric-code model with twists through quantum circuits,we demonstrate that twists exchange electric and magnetic charges and behave as a particular type of non-Abelian anyons,i.e.,the Ising anyons.In particular,we show experimentally that these twists follow the fusion rules and non-Abelian braiding statistics of the Ising type,and can be explored to encode topological logical qubits.Furthermore,we demonstrate how to implement both single-and two-qubit logic gates through applying a sequence of elementary Pauli gates on the underlying physical qubits.Our results demonstrate a versatile quantum digital approach for simulating non-Abelian anyons,offering a new lens into the study of such peculiar quasiparticles. | Shibo Xu Zheng-Zhi Sun Ke Wang Liang Xiang Zehang Bao Zitian Zhu Fanhao Shen Zixuan Song Pengfei Zhang Wenhui Ren Xu Zhang Hang Dong Jinfeng Deng Jiachen Chen Yaozu Wu Ziqi Tan Yu Gao Feitong Jin Xuhao Zhu Chuanyu Zhang Ning Wang Yiren Zou Jiarun Zhong Aosai Zhang Weikang Li Wenjie Jiang Li-Wei Yu Yunyan Yao Zhen Wang Hekang Li Qiujiang Guo Chao Song H.Wang Dong-Ling Deng | 2023 | Chinese Physics Letters2023，40，6： | 0 |
| 15 | Spatiotemporal changes of gross primary productivity and its response to drought in the Mongolian Plateau under climate change显示文摘Gross primary productivity(GPP)of vegetation is an important constituent of the terrestrial carbon sinks and is significantly influenced by drought.Understanding the impact of droughts on different types of vegetation GPP provides insight into the spatiotemporal variation of terrestrial carbon sinks,aiding efforts to mitigate the detrimental effects of climate change.In this study,we utilized the precipitation and temperature data from the Climatic Research Unit,the standardized precipitation evapotranspiration index(SPEI),the standardized precipitation index(SPI),and the simulated vegetation GPP using the eddy covariance-light use efficiency(EC-LUE)model to analyze the spatiotemporal change of GPP and its response to different drought indices in the Mongolian Plateau during 1982-2018.The main findings indicated that vegetation GPP decreased in 50.53% of the plateau,mainly in its northern and northeastern parts,while it increased in the remaining 49.47%area.Specifically,meadow steppe(78.92%)and deciduous forest(79.46%)witnessed a significant decrease in vegetation GPP,while alpine steppe(75.08%),cropland(76.27%),and sandy vegetation(87.88%)recovered well.Warming aridification areas accounted for 71.39% of the affected areas,while 28.53% of the areas underwent severe aridification,mainly located in the south and central regions.Notably,the warming aridification areas of desert steppe(92.68%)and sandy vegetation(90.24%)were significant.Climate warming was found to amplify the sensitivity of coniferous forest,deciduous forest,meadow steppe,and alpine steppe GPP to drought.Additionally,the drought sensitivity of vegetation GPP in the Mongolian Plateau gradually decreased as altitude increased.The cumulative effect of drought on vegetation GPP persisted for 3.00-8.00 months.The findings of this study will improve the understanding of how drought influences vegetation in arid and semi-arid areas. | ZHAO Xuqin LUO Min MENG Fanhao SA Chula BAO Shanhu BAO Yuhai | 2024 | Journal of Arid Land2024，16，1： | 0 |
| 16 | Spatiotemporal changes of typical glaciers and their responses to climate change in Xinjiang,Northwest China显示文摘Glaciers are highly sensitive to climate change and are undergoing significant changes in mid-latitudes.In this study,we analyzed the spatiotemporal changes of typical glaciers and their responses to climate change in the period of 1990-2015 in 4 different mountainous sub-regions in Xinjiang Uygur Autonomous Region of Northwest China:the Bogda Peak and Karlik Mountain sub-regions in the Tianshan Mountains;the Yinsugaiti Glacier sub-region in the Karakorum Mountains;and the Youyi Peak sub-region in the Altay Mountains.The standardized snow cover index(NDSI)and correlation analysis were used to reveal the glacier area changes in the 4 sub-regions from 1990 to 2015.Glacial areas in the Bogda Peak,Karlik Mountain,Yinsugaiti Glacier,and Youyi Peak sub-regions in the period of 1990-2015 decreased by 57.7,369.1,369.1,and 170.4 km^(2),respectively.Analysis of glacier area center of gravity showed that quadrant changes of glacier areas in the 4 sub-regions moved towards the origin.Glacier area on the south aspect of the Karlik Mountain sub-region was larger than that on the north aspect,while glacier areas on the north aspect of the other 3 sub-regions were larger than those on the south aspect.Increased precipitation in the Karlik Mountain sub-region inhibited the retreat of glaciers to a certain extent.However,glacier area changes in the Bogda Peak and Youyi Peak sub-regions were not sensitive to the increased precipitation.On a seasonal time scale,glacier area changes in the Bogda Peak,Karlik Mountain,Yinsugaiti Glacier,and Youyi Peak sub-regions were mainly caused by accumulated temperature in the wet season;on an annual time scale,the correlation coefficient between glacier area and annual average temperature was-0.72 and passed the significance test at P<0.05 level in the Karlik Mountain sub-region.The findings of this study can provide a scientific basis for water resources management in the arid and semi-arid regions of Northwest China in the context of global warming. | HUANG Xiaoran BAO Anming GUO Hao MENG Fanhao ZHANG Pengfei ZHENG Guoxiong YU Tao QI Peng Vincent NZABARINDA DU Weibing | 2022 | Journal of Arid Land2022，14，5： | 0 |
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