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| 1 | 2020 Roadmap on two-dimensional nanomaterials for environmental catalysis显示文摘Environmental catalysis has drawn a great deal ofattention due to its clean ways to produce useful chemicals or carry out some chemical processes.Photocatalysis and electrocatalysis play important roles in these fields.They can decompose and remove organic pollutants from the aqueous environment,and prepare some fine chemicals.Moreover,they also can carry out some important reactions,such as 02 reduction reaction(ORR),O2 evolution reaction(OER),H2 evolution reaction(HER),CO2 reduction reaction(C02 RR),and N2 fixation(NRR).For catalytic reactions,it is the key to develop high-performance catalysts to meet the demand fortargeted reactions.In recentyears,two-dimensional(2 D) materials have attracted great interest in environmental catalysis due to their unique layered structures,which offer us to make use of their electronic and structural characteristics.Great progress has been made so far,including graphene,black phosphorus,oxides,layered double hydroxides(LDHs),chalcogenides,bismuth-based layered compounds,MXenes,metal organic frameworks(MOFs),covalent organic frameworks(COFs),and others.This content drives us to invite many famous groups in these fields to write the roadmap on two-dimensional nanomaterials for environmental catalysis.We hope that this roadmap can give the useful guidance to researchers in future researches,and provide the research directions. | Yulu Yang Mingguang Wu Xingwang Zhu Hui Xu Si Ma Yongfeng Zhi Hong Xia Xiaoming Liu Jun Pan Jie-Yinn Tang Siang-Piao Chai Leonardo Palmisano Francesco Parrino Junli Liu Jianzhong Ma Ze-Lin Wang Ling Tan Yu-Fei Zhao Yu-Fei Song Pardeep Singh Pankaj Raizada Deli Jiang Di Li R.A.Geioushy Jizhen Ma Jintao Zhang Song Hu Rongjuan Feng Gang Liu Minghua Liu Zhenhua Li Mingfei Shao Neng Li Jiahe Peng Wee-Jun Ong Nikolay Kornienko Zhenyu Xing Xiujun Fan Jianmin Ma | 2019 | Chinese Chemical Letters2019，30，12： | 2 |
| 2 | LiMn_2O_4 thin films derived by rapid thermal annealing and their performance as cathode materials for Li ion battery显示文摘The LiMn2O4 thin film as a cathode material was prepared through solution deposition followed by rapid thermal annealing (RTA). The phase identification and the study of surface morphology were carried out by X-ray diffraction and scanning electron microscopy. Electrochemical properties were examined by cyclic voltammetry, galvanostatic charge-discharge experiments, and electrochemical impedance spectroscopy. The results show that the film prepared by this method is homogeneous, dense, and crack-free. The thin film has a capacity of 38 μAh/(cm2?μm) with the capacity loss of 0.037% per cycle after being cycled for 100 times. The average diffusion coefficient for lithium ions in the RTA-derived LiMn2O4 thin film is 1 × 10?10 cm2?s?1. | WU Xianming HE Zeqiang MA Mingyou XIAO Zhuobing XU Mingfei | 2006 | Rare Metals2006，25，6： | 2 |
| 3 | Characterization and electrochemical properties of LiMn2O4 thin films prepared by solution deposition显示文摘 | Wu Xianming Ph D He Zeqiang Xu Mingfei Li Xinhai Xiao Zhuobing | 2006 | Journal of Wuhan University of Technology - Mater Sci Ed2006，，3： | 1 |
| 4 | A thermochemical study of K2M (IO3)4 · 2H2O (M =Mg2+, Ni2+,Zn2+) 显示文摘 | Hu Tuncheng Wan Hongwen Xu Mingfei Wang Tianzhi | 2000 | Thermochimica Acta2000，345，： | 1 |
| 5 | Transa-ction management of database in mobile computing environment显示文摘 | Xu Lizhen Jiang Mingfei Dong Yisheng | 2002 | Journal of Southeast University2002，32，6： | 1 |
| 6 | Cold sodium hydroxide/urea based pretreatment of bamboo for bioethanol production: characterization of the cellulose rich fraction显示文摘 | Li Mingfei Fan Yongming Xu Feng | 2010 | Ind Crops Prod2010，32，： | 1 |
| 7 | An organic sensitizer with a fused dithienothiophene unit for efficient and stable dye - sensitized solar cells 显示文摘 | Qin Hao Wenger Sophie Xu Mingfei | 2008 | Journal of the American Chemical Society2008，130，29： | 1 |
| 8 | Cold sodium hydroxide/urea based pretreatment of bamboo for bioethanol production:characterization of the cellulose rich fraction显示文摘 | Li Mingfei Fan Yongming Xu Feng | | 0，，03： | 1 |
| 9 | Engineering of Push‐Pull Thiophene Dyes to Enhance Light Absorption and Modulate Charge Recombination in Mesoscopic Solar Cells显示文摘 | Ning Cai Yinglin Wang Mingfei Xu Ye Fan Renzhi Li Min Zhang Peng Wang | 2012 | Adv Funct Mater2012，，14： | 1 |
| 10 | Preparation, properties and application of polypropylene micro/nanofiber membranes显示文摘 | Mengjun Zhu Guanbiao Xu Mingfei Yu | 2012 | Polymers for Advanced Technologies2012，，23： | 1 |
| 11 | Simplified transient isotachophoresis/capillary gel electrophoresis method for highly sensitive analysis of polymerase chain reaction samples on a microchip with laserinduced fluorescence detection显示文摘 | Liu Dayu Ou Ziyou Xu Mingfei | 2008 | Journal of Chromatography A2008，1214，12： | 1 |
| 12 | QTL analysis reveals reduction of fruit water loss by NAC042 through regulation of cuticular wax synthesis in citrus fruit显示文摘Postharvest water loss is a critical factor that determines the quality and shelf life of fresh fruit.Cuticular wax constitutes a key barrier to reduce fruit water loss.Our previous study has shown that HJ(Citrus reticulata)has a significantly higher postharvest water loss rate than ZK(Poncirus trifoliata).Here,we investigated the fruit water loss rate of the HJ×ZK F1pseudo-testcross population in 2016 and 2019.QTL mapping for fruit water loss rate was performed by high-density genetic map and bulk segregant analysis,and QTL9 was identified to be associated with fruit water loss.The expression of NAC042 from QTL9 in ZK was 170-fold that in HJ.Heterologous expression in Arabidopsis showed that NAC042could reduce the water loss of leaves by increasing the cuticular wax content(especially alkanes).Further expression analysis revealed that NAC042 could enhance the expression of many wax-related genes in Arabidopsis leaves,including AtKCS1,AtKCS2,AtKCS9,AtKCS20,At CER1 and At CER3.Therefore,NAC042 might be involved in fruit cuticular wax synthesis to reduce fruit water loss.The findings provide new insights into the regulation of cuticular wax and fruit water loss as well as valuable information for breeding of citrus with better storability. | Hongbin Yang Zhifeng Zhu Mingfei Zhang Xin Li Rangwei Xu Feng Zhu Juan Xu Xiuxin Deng Yunjiang Cheng | 2022 | Horticultural Plant Journal2022，8，6： | 1 |
| 13 | Single-atom Catalysts Based on Layered Double Hydroxides显示文摘Single-atom catalysts(SACs)have attracted much attention for their superior catalytic performance in various fields.It has been widely accepted that the selection of appropriate substrates is crucial to the fabrication and application of SACs.Layered double hydroxides(LDHs)have been developed as one of the promising substrates for single-atoms due to their unique adjustable supramolecular structures.In this review,we comprehensively sort out the research of SACs based on LDHs.By analyzing the characteristics of LDHs and the single-atoms,respectively,the preparation strategies of SACs by using LDHs are summarized.Their applications as efficient catalysts in electrocatalysis,photocatalysis and thermal catalysis are then discussed.Finally,we summarize the opportunities and challenges for the rational design and application expansion of SACs based on LDHs in the future. | FAN Kui SUN Yining XU Pengcheng GUO Jian LI Zhenhua SHAO Mingfei | 2022 | Chemical Research in Chinese Universities2022，38，5： | 0 |
| 14 | Co-thermal in-situ reduction of inorganic carbonates to reduce carbon-dioxide emission显示文摘Thermal decomposition of inorganic metal carbonates is the main path to prepare metal oxides;nonetheless,it is always accompanied by the emission of large amounts of CO_(2) as one of the gas products.This study reports a concept of co-thermal insitu reduction of inorganic carbonates by using the energy released by carbonate decomposition under pure hydrogen atmosphere,which reduces the decarboxylation temperature and significantly inhibits the CO_(2) emissions.A combination of hydrogen–deuterium exchange,isotope experiment,and density functional theory calculations demonstrates that the CO results from the selective cleavage of Ca–O bonds at the surface of CaCO_(3) via the direct hydrogenation mechanism at relatively low temperature.However,it undergoes the reverse water–gas shift reaction path at high temperature,i.e.,CO being produced by the reduction of CO_(2) released by the decomposition of carbonates.This study sheds light on the potential of green hydrogen technology for inorganic carbonate valorization toward high value-added products,which can facilitate the large-scale industrial applications. | Zhen Xue Jingyi Guo Shasha Wu Wenfu Xie Yujing Fu Xiaojie Zhao Kui Fan Ming Xu Hong Yan Mingfei Shao Xue Duan | 2023 | Science China Chemistry2023，66，4： | 0 |
| 15 | Refining acceptor aggregation in nonfullerene organic solar cells to achieve high efficiency and superior thermal stability显示文摘With the rapid increase in photoelectric conversion efficiency of organic photovoltaics(OPVs),prolonging the operational lifetime of devices becomes one of the critical prerequisites for commercial applications.Guided by the theoretical calculations of molecular stacking and miscibility,we proposed an effective approach to simultaneously improve device performance and thermal stability of high-efficiency OPVs by refining the aggregation of Y-series acceptors.The key to this approach is deliberately designing an asymmetric Y-series acceptor,named Y6-CNO,which acts as a third component regulator to finely tune the degree of acceptor aggregation and crystallization in the benchmark PM6:Y6-BO system.Strikingly,a champion photovoltaic efficiency of 18.0%was achieved by introducing 15 wt%Y6-CNO into the PM6:Y6-BO system,significantly higher than the control binary cell(16.7%).Moreover,annealing at 100°C for over 1,200 h does not markedly affect the photovoltaic performance of the optimal ternary devices,maintaining above 95%of the initial performance and exhibiting an exceptionally high T_(80)lifetime of 9,000 h under continuous thermal annealing.By contrast,binary devices suffer from excessive crystallization of acceptors with long-term annealing.Additionally,mixing thermodynamics combined with morphological characterizations were employed to elucidate the microstructure-thermal stability relationships.The ternary OPVs consisting of symmetric and asymmetric homologous acceptors form better charge transport channels and can effectively suppress excessive aggregation of acceptors under long-term annealing.This work demonstrates the effectiveness of refining acceptor aggregation via molecular design for highly efficient and stable nonfullerene-based OPVs. | Kaihu Xian Shengnan Zhang Ye Xu Junwei Liu Kangkang Zhou Zhongxiang Peng Mingfei Li Wenchao Zhao Yu Chen Zhuping Fei Jianhui Hou Yanhou Geng Long Ye | 2023 | Science China Chemistry2023，66，1： | 0 |
| 16 | Efficient light-driven reductive amination of furfural to furfurylamine over ruthenium-cluster catalyst显示文摘Selective reductive amination of carbonyl compounds with high activity is very essential for the chemical and pharmaceutical industry,but scarcely successful paradigm was reported via efficient photocatalytic reactions.Herein,the ultrasmall Ru nanoclusters(~0.9 nm)were successfully fabricated over P25 support with positive charged Ru^(δ+)species at the interface.A new route was developed to achieve the furfural(FAL)to furfurylamine(FAM)by coupling the light-driven reductive amination and hydrogen transfer of ethanol over this type catalyst.Strikingly,the photocatalytic activity and selectivity are strongly dependent on the particle size and electronic structure of Ruthenium.The Ru^(δ+)species at the interface promote the formation of active imine intermediates;moreover,the Ru nanoclusters facilitate the separation efficiency of electrons and holes as well as accelerate the further hydrogenation of imine intermediates to product primary amines.In contrast Ru particles in larger nanometer size facilitate the formation of the furfuryl alcohol and excessive hydrogenation products.In addition,the coupling byproducts can be effectively inhibited via the construction of sub-nanocluster.This study offers a new path to produce the primary amines from biomass-derived carbonyl compounds over hybrid semiconductor/metal-clusters photocatalyst via light-driven tandem catalytic process. | Zhen Xue Shasha Wu Yujing Fu Lan Luo Min Li Zhenhua Li Mingfei Shao Lirong Zheng Ming Xu Haohong Duan | 2023 | Journal of Energy Chemistry2023，，1： | 0 |
| 17 | Comparative Study of LiMn2O4 Thin Films Heat-treated by Conventional and Rapid Thermal Annealing显示文摘阴极材料 LiMn_2O_4 薄电影被常规热退火跟随的答案免职(CTA )(RTA ) 并且快速的热退火作为开始材料用醋酸锂和乙酸锰准备。阶段和表面形态学鉴定被 X 光检查衍射和扫描电子显微镜学做。薄电影的电气化学的性质被循环伏安法,费用分泌物实验,电气化学的阻抗光谱学和潜在的步骤技术执行。结果证明两部薄电影同类、没有裂缝。与 CTA 相比导出薄电影,有更小的谷物的导出的缩放的 RTA 更光滑、稠密。CTA 和 RTA 导出 LiMn_2O_4 薄电影交付 34.5 muAh/(cm^2 中心点妈妈) 和 38 muAh/(cm^2 中心点妈妈) 的能力并且在分别地被骑车 100 次以后每周期显示出 0.050% 和 0.037% 的能力损失。在 CTA 的锂离子的散开系数导出 LiMn_2O_4 thin-filmelectrode 是 4.59 X 10 ^(-11) cm^2/s,和在 RTA 的锂离子的导出一个是 3.86 X10^(-11) cm^2/s。 | Xianming WU Mingyou MA Zhuobing XIAO Zeqiang HE Jianben LIU Mingfei XU | 2006 | Journal of Materials Science & Technology2006，22，3： | 0 |
| 18 | A CBL4-CIPK6 module confers salt tolerance in cucumber显示文摘Soil salinization is a major threat to cucumbers grown under protected cultivation.Under stressful environments,calcineurin B-like proteins(CBLs)can sense and bind Ca2+signals and regulate CBL-interacting protein kinases(CIPKs)to transmit signals and induce cellular responses.Although CBL-CIPK modules play central roles in plant development and response to various abiotic stresses in Arabidopsis,little is known about their functions in cucumber.In this study,we demonstrate that CsCBL4 interacts with CsCIPK6,which exhibited similar responses to salt stress in cucumber.Furthermore,salt stress resulted in greater accumulation of CsCBL4 and CsCIPK6.Comprehensive phenotype analysis demonstrated that silencing CsCBL4 or CsCIPK6 reduced the salt tolerance of cucumber,and overexpression of CsCBL4 increased the salt tolerance of Arabidopsis.Collectively,these results indicate that the CsCBL4-CsCIPK6 module plays an important role in the resistance of cucumber to salt stress.The information provides insights for the genetic breeding of salt tolerance in cucumber in the future. | Mingfei Wang Songlin Yang Lei Sun Zhongxuan Feng Yiming Gao Xuling Zhai Yuming Dong Haoying Wu Yuanyuan Cui Sen Li Shuo Xu Ezra S.Bartholomew Huazhong Ren Xingwang Liu | 2022 | Vegetable Research2022，2，1： | 0 |
| 19 | Hierarchical carbon nanosheet confined defective MoS_(x) cathode towards long-cycling zinc-ion-battery显示文摘Aqueous zinc-ion batteries(ZIBs)have attracted increasing attention due to their low cost and high safety.MoS_(2) is a promising cathode material for aqueous ZIBs due to its favorable Zn^(2+)accommodation ability.However,the structural strain and large volume changes during intercalation/deintercalation lead to exfoliation of active materials from substrate and cause irreversible capacity fading.In this work,a highly stable cathode was developed by designing a hierarchical carbon nanosheet-confined defective MoS_(x)material(CNS@MoS_(x)).This cathode material exhibits an excellent cycling stability with high capacity retention of 88.3%and~100%Coulombic efficiency after 400 cycles at 1.2 A·g^(-1),much superior compared to bare MoS_(2).Density functional theory(DFT)calculations combined with experiments illustrate that the promising electrochemical properties of CNS@MoS_(x)are due to the unique porous conductive structure of CNS with abundant active sites to anchor MoS_(x)via strong chemical bonding,enabling MoS_(x)to be firmly confined on the substrate.Moreover,this unique hierarchical complex structure ensures the fast migration of Zn^(2+)within MoS_(x)interlayer. | Xiaoqi Wang Shimeng Zhang Rui Yang Shengchi Bai Jianbo Li Yu Wu Bowen Jin Xu Jin Mingfei Shao Bo Wang | 2023 | Nano Research2023，16，7： | 0 |
| 20 | ARoad Segmentation Model Based on Mixture of the Convolutional Neural Network and the Transformer Network显示文摘Convolutional neural networks(CNN)based on U-shaped structures and skip connections play a pivotal role in various image segmentation tasks.Recently,Transformer starts to lead new trends in the image segmentation task.Transformer layer can construct the relationship between all pixels,and the two parties can complement each other well.On the basis of these characteristics,we try to combine Transformer pipeline and convolutional neural network pipeline to gain the advantages of both.The image is put into the U-shaped encoder-decoder architecture based on empirical combination of self-attention and convolution,in which skip connections are utilized for localglobal semantic feature learning.At the same time,the image is also put into the convolutional neural network architecture.The final segmentation result will be formed by Mix block which combines both.The mixture model of the convolutional neural network and the Transformer network for road segmentation(MCTNet)can achieve effective segmentation results on KITTI dataset and Unstructured Road Scene(URS)dataset built by ourselves.Codes,self-built datasets and trainable models will be available on http://gffzz188fe103f8f1460asvk9n6npxwo9v6k0x.ffgz.tsg.suse.edu.cn/xflxfl1992/MCTNet. | Fenglei Xu Haokai Zhao Fuyuan Hu Mingfei Shen Yifei Wu | 2023 | Computer Modeling in Engineering & Sciences2023，，5： | 0 |
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