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| 1 | Porphyrin-like Fe-N4 sites with sulfur adjustment on hierarchical porous carbon for different rate-determining steps in oxygen reduction reaction显示文摘We developed a strategy based on coordination polymer to synthesize singleatom site Fe/N and S-codoped hierarchical porous carbon (Fe1/N,S-PC).The as-obtained Fe1/N,S-PC exhibited superior oxygen reduction reaction (ORR) performance with a half-wave potential (Ev2,0.904 V vs.RHE) that was better than that of commercial Pt/C (E1/2,0.86 V vs.RHE),single-atom site Fe/N-doped hierarchical porous carbon (Fe1/N-PC) without S-doped (E1/2,0.85 V vs.RHE),and many other nonprecious metal catalysts in alkaline medium.Moreover,the Fe1/N,S-PC revealed high methanol tolerance and firm stability.The excellent electrocatalytic activity of Fe1/N,S-PC is attributed to the synergistic effects from the atomically dispersed porphyrin-like Fe-N4 active sites,the heteroatom codoping (N and S),and the hierarchical porous structure in the carbon materials.The calculation based on density functional theory further indicates that the catalytic performance of Fe1/N,S-PC is better than that of Fe1/N-PC owing to the sulfur doping that yielded different rate-determining steps. | Konglin Wu Xin Chen Shoujie Liu Yuan Pan Weng-Chon Cheong Wei Zhu Xing Cao Rongan Shen Wenxing Chen Jun LUO Wensheng Yan Lirong Zheng Zheng Chen Dingsheng Wang Qing Peng Chen Chen Yadong Li | 2018 | Nano Research2018，11，12： | 18 |
| 2 | Influence of chronic intermittent hypoxia on growth associated protein 43 expression in the hippocampus of young rats显示文摘This study aimed to explore the pathological change to hippocampal neurons and the expression of growth associated protein 43 in 21-day-old young rats following chronic intermittent hypoxia.Hematoxylin-eosin staining results showed varying degrees of degeneration and necrosis in hippocampal neurons depending on the modeling time.Immunohistochemistry revealed that growth associated protein 43 expression in young rats following chronic intermittent hypoxia decreased,but that levels were still higher than those of normal rats at each time point,especially 4 weeks after modeling.During 1-5 weeks after modeling,a slow growth in rat weight was observed.Experimental findings indicate that chronic intermittent hypoxia may induce growth dysfunction and necrosis of hippocampal neurons,as well as increase the expression of growth associated protein 43 in young rats. | Yan Chen Chunling Zhao Chunlai Zhang Lirong Luo Guang Yu | 2012 | Neural Regeneration Research2012，7，16： | 4 |
| 3 | Responses of biotic interactions of dominant and subordinate species to decadal warming and simulated rotational grazing in Tibetan alpine meadow显示文摘Warming increases competition among plant species in alpine communities by ameliorating harsh environmental conditions,such as low temperatures. Grazing, as the main human activity, may mitigate the effect of warming, as previously reported.However, it is critical to refine the effects of warming on biotic interactions among species, for example, by taking the competitive ability of species into consideration. Based on a 10-year warming and grazing experiment in a Tibetan alpine meadow, we evaluated interspecific biotic interactions of dominant and subordinate species, using the approach of interspecific spatial associations. Warming significantly increased competition between subordinate and dominant species as well as among subordinate species, but not among dominant species. Moreover, facilitation of dominant-subordinate species also increased under warming. Simulated rotational grazing had similar effects to warming, with increasing interspecific competition. Our results show that, when studying the effects of warming on biotic interactions among species, it is necessary to characterize different species pairs relative to their competitive ability, and that simulated rotational grazing does not mitigate the effects of warming in the long term. Our results also provide evidence that the spatial pattern of species is a critical mechanism in species coexistence. | Xin'e Li Xiaoxue Zhu Shiping Wang Shujuan Cui Caiyun LUO Zhenhua Zhang Lirong Zhang Lili Jiang Wangwang Lyu | 2018 | Science China(Life Sciences)2018，61，7： | 4 |
| 4 | Nitrogen-carbon layer coated nickel nanoparticles for efficient electrocatalytic reduction of carbon dioxide显示文摘The application of nickel in electrocatalytic reduction of CO2 has been largely restricted by side reaction (hydrogen evolution reaction) and catalyst poisoning.Here we report a new strategy to improve the electrocatalytic performance of nickel for CO2 reduction by employing a nitrogen-carbon layer for nickel nanoparticles.Such a nickel electrocatalyst exhibits high Faradaic efficiency 97.5% at relatively low potential of-0.61 V for the conversion of CO2 to CO.Density functional theory calculation reveals that it is thermodynamically accomplishable for the reduction product CO to be removed from the catalyst surface,thus avoiding catalyst poisoning.Also,the catalyst renders hydrogen evolution reaction to be suppressed and hence reasonably improves catalytic performance. | Dongxing Tan Chaonan Cui Jinbiao Shi Zhixun Luo Bingxing Zhang Xiuniang Tan Buxing Han Lirong Zheng Jing Zhang Jianling Zhang | 2019 | Nano Research2019，12，5： | 3 |
| 5 | Fluorine emission from combustion of steam coal of North China Plate and Northwest China显示文摘To study the amount of fluorine emission from the combustion of the steam coal (mainly Permo-Carbonif-erous coal) from the North China Plate and Northwest China, the fluorine contents of the coal, the fly ash and the cinder in high-temperature power stations as well as mid-low temperature power stations have been analyzed. This note provides a rough estimate of the total annual amount of fluorine emission as well as emission ratio from steam coal combustion in China. Our results show that by combustion of 1 t of Permo-Carboniferous coal (containing roughly 100 g fluorine), high-temperature power stations emit roughly 90 g fluorine into the atmosphere. The fluorine emission ratio of coal combustion in high-temperature power stations is about 96% and that in mid-low temperature power stations is about 78%. A total of 800 million tons of coal is burnt in China every year, and the coal comes mainly from Permo-Carboniferous deposite in the North China Plate and Northwest China coal mines. Taking the average | LUO Kunli XU Lirong LI Ribang XIANG Lianhua | 2002 | Chinese Science Bulletin2002，47，16： | 2 |
| 6 | 增温和放牧对高寒草甸凋落物分解及其养分释放的影响不依赖于凋落物品质显示文摘在放牧生态系统中,增温、放牧和调落物品质共同决定着凋落物分解和养分释放。然而,在以往的研究中这些因子的效应通常被单独地研究。在本研究中,我们在青藏高原高寒草甸开展了一个昼夜非对称增温和中度放牧两因子的调落物分解试验。从每个处理中收集了调落物样品,这些调落物一部分放在它们的来源处理小区,另一部分放在其他处理小区以此来探究增温、放牧以及调落物品质对调落物分解和养分释放的影响。研究结果表明,增温而不是放牧显著增加了调落物质量的损失、单位面积全碳、全氮以及全磷含量的损失,这主要是因为增温增加了落物生物量和分解速率。然而,尽管同时增温放牧处理也加快了调落物分解速率,但由于降低了调落物生物量,所以增温放牧处理并没有显著影响单位面积的凋落物碳和养分释放量。相比木质素含量和碳氮比而言,季节性土壤平均温度能够更好地预测调落物分解速率。增温和放牧对调落物分解存在交互作用,但它们和调落物品质对调落物的影响均不存在交互作用。单位面积的总氮释放的温度敏感性要高于总磷。因此,我们的结果表明,增温对调落物分解以及养分释放的影响要显著大于调落物品质变化对其分解的影响。在高寒草甸,氮释放的增加可能会间接导致土壤磷有效性的缺乏。 | Bowen Li Wangwang Lv Jianping Sun Lirong Zhang Lili Jiang Yang Zhou Peipei Liu Huan Hong Qi Wang Wang A Suren Zhang Lu Xia Zongsong Wang Tsechoe Dorji Ailing Su Caiyun Luo Zhenhua Zhang Shiping Wang | 2022 | Journal of Plant Ecology2022，15，5： | 1 |
| 7 | Splice Site Prediction with Quadratic Discriminant Analysis Using Diversity Measure显示文摘 | Luo Liaofu | 2003 | Nucleic Acids Research2003，31，： | 1 |
| 8 | Selenium source in the selenosis area of the Daba region,south Qinling mountain,China显示文摘 | Luo Kunli Xu Lirong Tan Jian'an Wang Douhu Xiang Lianhua | 2004 | Environmental Geology2004，45，： | 1 |
| 9 | Improving thin-film crystalline silicon solar cell efficiencies with photonic crystals 显示文摘 | Bermel P Luo Chiyan Zeng Lirong | 2007 | Optics Express2007，15，16： | 1 |
| 10 | Effect of integrated application of gamma irradiation and modified atmosphere packaging on physicochemical and microbiological properties of shiitake mushroom ( Lentinus edodes )显示文摘 | Tianjia Jiang Shasha Luo Qiuping Chen Lirong Shen Tiejin Ying | 2010 | Food Chemistry2010，，3： | 1 |
| 11 | Splice site prediction with quadratic discriminant analysis using diversity measure 显示文摘 | Lirong Zhang Liaofu Luo | 2003 | Nucleic Acids Research2003，31，21： | 1 |
| 12 | Multi-Layer Reconstruction Errors Autoencoding and Density Estimate for Network Anomaly Detection显示文摘Anomaly detection is an important method for intrusion detection.In recent years,unsupervised methods have been widely researched because they do not require labeling.For example,a nonlinear autoencoder can use reconstruction errors to attain the discrimination threshold.This method is not effective when the model complexity is high or the data contains noise.The method for detecting the density of compressed features in a hidden layer can be used to reduce the influence of noise on the selection of the threshold because the density of abnormal data in hidden layers is smaller than normal data.However,compressed features may lose some of the high-dimensional distribution information of the original data.In this paper,we present an efficient anomaly detection framework for unsupervised anomaly detection,which includes network data capturing,processing,feature extraction,and anomaly detection.We employ a deep autoencoder to obtain compressed features and multi-layer reconstruction errors,and feeds them the same to the Gaussian mixture model to estimate the density.The proposed approach is trained and tested on multiple current intrusion detection datasets and real network scenes,and performance indicators,namely accuracy,recall,and F1-score,are better than other autoencoder models. | Ruikun Li Yun Li Wen He Lirong Chen Jianchao Luo | 2021 | Computer Modeling in Engineering & Sciences2021，，7： | 1 |
| 13 | Genetic diversity, linkage disequilibrium, and association mapping analyses of peach ( Prunus persica ) landraces in China显示文摘 | Ke Cao Lirong Wang Gengrui Zhu Weichao Fang Changwen Chen Jing Luo | 2012 | Tree Genetics & Genomes2012，，5： | 1 |
| 14 | Sensors based on galvanic cell generated electrochemilumesence and its application显示文摘 | Luo Lirong Zhang Zhujun | 2006 | Analytica Chimica Acta2006，580，： | 1 |
| 15 | Single-atom nanozymes with axial ligand-induced self-adaptive conformation in alkaline medium boost chemiluminescence显示文摘Mimicking the structure of natural enzymes for designing advanced alternatives provides great opportunities to address the bottleneck of enzyme-involved chemiluminescence(CL). Herein, according to theoretical calculations, we found that an endogenous axial ligand of M-N-C single-atom nanozymes(SAzymes), originating from OH-spontaneously bonding to the metal center in an alkaline medium, can self-adaptively change its strength to facilitate intermediate steps. Furthermore, the lowest energy barrier of the rate-determining step and the strongest affinity and fastest electron transfer with luminol anion endow CoN-C with the highest peroxidase-like activity. Guided by the theoretical calculations, a series of M-N-C SAzymes(M=Fe, Co,Ni) were synthesized to boost CL, where Co-N-C SAzymes with superior catalytic activity and high selective generation of O_(2)·- were validated. As a proof-of-concept, Co-N-C SAzymes were employed for sensitive detection of acetylcholinesterase and organophosphorus pesticide. | Zhen Luo Liliang Tian Hengjia Wang Zhichao Wu Xin Luo Xiaosi Wang Lei Jiao Xiaoqian Wei Ying Qin Lirong Zheng Liuyong Hu Wenling Gu Le Shi Chengzhou Zhu | 2023 | Science China Chemistry2023，66，3： | 0 |
| 16 | Assembly of Two Coordination Polymers Based on 2,2 '-Bipyridyl-4,4'-dicarboxylic Acid Ligand显示文摘 | WANG Jing LUO Xiaolong YUAN Yang ZHANG Lirong | 2015 | Chemical Research in Chinese Universities2015，31，4： | 0 |
| 17 | Screening and Identification of a Bacterial Strain Antagonistic to Vibrio parahaemolyticus显示文摘In the present study,bacterial strains were isolated from the shrimp(Penaeus orientalis)ponds in different regions of Hainan Province,and tested for their antagonistic activity against Vibrio species on 2216E plates,using V.parahaemolyticus,V.harveyi and V.anguillarum as the indicator bacteria.As a result,an antagonistic strain was screened out and numbered 20160522Z-10(referred to as Z-10).Then,the antibacterial activity and minimum inhibitory concentration(MIC)of Z-10 against the indicator bacteria,and its antibacterial effect against other six Vibrio species were determined.The results proved that Z-10 was antagonistic to all the three indicator bacteria,and its MIC against V.parahaemolyticus,V.harveyi and V.anguillarum was 2.5×10~4,2.5×10~5 and 2.5×10~5 CFU/ml.Additionally,Z-10 had a certain antibacterial effect against other Vibrio species.Finally,the strain was identified as a Pseudoalteromonas sp.by 16S rDNA sequence analysis.The bacterium as a new probiotic,is expected to be used in disease prevention and control in marine aquaculture. | Lirong BAI Zhiying ZHAO Dapeng LUO | 2017 | Agricultural Biotechnology2017，6，4： | 0 |
| 18 | Weighted single-step GWAS and RNA sequencing reveals key candidate genes associated with physiological indicators of heat stress in Holstein cattle显示文摘Background: The study of molecular processes regulating heat stress response in dairy cattle is paramount for developing mitigation strategies to improve heat tolerance and animal welfare. Therefore, we aimed to identify quantitative trait loci(QTL) regions associated with three physiological indicators of heat stress response in Holstein cattle, including rectal temperature(RT), respiration rate score(RS), and drooling score(DS). We estimated genetic parameters for all three traits. Subsequently, a weighted single-step genome-wide association study(WssGWAS) was performed based on 3200 genotypes, 151,486 phenotypic records, and 38,101 animals in the pedigree file. The candidate genes located within the identified QTL regions were further investigated through RNA sequencing(RNA-seq) analyses of blood samples for four cows collected in April(non-heat stress group) and four cows collected in July(heat stress group).Results: The heritability estimates for RT, RS, and DS were 0.06, 0.04, and 0.03, respectively. Fourteen, 19, and 20 genomic regions explained 2.94%, 3.74%, and 4.01% of the total additive genetic variance of RT, RS, and DS, respectively. Most of these genomic regions are located in the Bos taurus autosome(BTA) BTA3, BTA6, BTA8, BTA12, BTA14, BTA21, and BTA24. No genomic regions overlapped between the three indicators of heat stress, indicating the polygenic nature of heat tolerance and the complementary mechanisms involved in heat stress response. For the RNA-seq analyses, 2627 genes were significantly upregulated and 369 downregulated in the heat stress group in comparison to the control group. When integrating the WssGWAS, RNA-seq results, and existing literature, the key candidate genes associated with physiological indicators of heat stress in Holstein cattle are: PMAIP1, SBK1, TMEM33, GATB, CHORDC1, RTN4IP1, and BTBD7.Conclusions: Physiological indicators of heat stress are heritable and can be improved through direct selection. Fifty-three QTL regions associated with heat stress indicators confirm the polygenic nature and complex genetic determinism of heat tolerance in dairy cattle. The identified candidate genes will contribute for optimizing genomic evaluation models by assigning higher weights to genetic markers located in these regions as well as to the design of SNP panels containing polymorphisms located within these candidate genes. | Hanpeng Luo Lirong Hu Luiz F.Brito Jinhuan Dou Abdul Sammad Yao Chang Longgang Ma Gang Guo Lin Liu Liwei Zhai Qing Xu Yachun Wang | 2022 | Journal of Animal Science and Biotechnology2022，13，6： | 0 |
| 19 | Association between the Lung Immune Prognostic Index and mortality in patients with idiopathic inflammatory myopathy-associated interstitial lung disease显示文摘Objective:To explore the association between the Lung Immune Prognostic Index(LIPI)and 1-year all-cause mortality in patients with idiopathic inflammatory myopathy related interstitial lung disease(IIM-ILD).Methods:Patients who were diagnosed with IIM-ILD at West China Hospital,Sichuan University from January 2008 to December 2021 were retrospectively included and categorized into three groups based on LIPI.Univariable and multivariable Cox proportional hazards models were conducted to explore potential association between the LIPI and patients'mortality.Results:A total of 1116 patients were screened,and 830 were included in this study.The multivariable Cox analysis showed that,compared with patients with poor LIPI,the hazard ratio(HR)for all-cause 1-year mortality was 0.22(95%CI 0.05-0.93,P=0.04)for patients in the good LIPI group(LDH<250 IU/L and dNLR<3).After excluding patients lost to follow-up within one year,a similar result was found for LIPI(HR 0.20,95%CI 0.05-0.86;P=0.03).Conclusions:Good LIPI was independently associated with decreased risk of all-cause 1-year mortality in patients with IIM-ILD.This easy-to-obtain index might be served as a potential marker for assessing the prognosis of IIM-ILD. | Dan Luo Zhihao Zhao Caizheng Li Wenjun Zhu Wei Zhou Lirong He Huifeng Yan Qiaoli Su | 2023 | Asian Pacific Journal of Tropical Medicine2023，16，11： | 0 |
| 20 | Efficient light-driven reductive amination of furfural to furfurylamine over ruthenium-cluster catalyst显示文摘Selective reductive amination of carbonyl compounds with high activity is very essential for the chemical and pharmaceutical industry,but scarcely successful paradigm was reported via efficient photocatalytic reactions.Herein,the ultrasmall Ru nanoclusters(~0.9 nm)were successfully fabricated over P25 support with positive charged Ru^(δ+)species at the interface.A new route was developed to achieve the furfural(FAL)to furfurylamine(FAM)by coupling the light-driven reductive amination and hydrogen transfer of ethanol over this type catalyst.Strikingly,the photocatalytic activity and selectivity are strongly dependent on the particle size and electronic structure of Ruthenium.The Ru^(δ+)species at the interface promote the formation of active imine intermediates;moreover,the Ru nanoclusters facilitate the separation efficiency of electrons and holes as well as accelerate the further hydrogenation of imine intermediates to product primary amines.In contrast Ru particles in larger nanometer size facilitate the formation of the furfuryl alcohol and excessive hydrogenation products.In addition,the coupling byproducts can be effectively inhibited via the construction of sub-nanocluster.This study offers a new path to produce the primary amines from biomass-derived carbonyl compounds over hybrid semiconductor/metal-clusters photocatalyst via light-driven tandem catalytic process. | Zhen Xue Shasha Wu Yujing Fu Lan Luo Min Li Zhenhua Li Mingfei Shao Lirong Zheng Ming Xu Haohong Duan | 2023 | Journal of Energy Chemistry2023，，1： | 0 |
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